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RESEARCH PAPER · Journal of the American Chemical Society · 2019

Lewis Acid Dominant Windmill-Shaped V8 Clusters: A Bifunctional Heterogeneous Catalyst for CO2 Cycloaddition and Oxidation of Sulfides

Jia‐Peng Cao, Yun‐Shan Xue, Ning-Fang Li, Jun-Jie Gong, Run‐Kun Kang, Yan Xu

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Lewis Acid Dominant Windmill-Shaped V8 Clusters: A Bifunctional Heterogeneous Catalyst for CO2 Cycloaddition and Oxidation of SulfidesOriginalNew pronounced progress in the synthesis of group 5 polyoxometalates29Efficient CO2 enrichment and fixation by engineering micropores of multifunctional hypercrosslinked ionic polymers165A Bicadmium-Substituted Polyoxometalate Network Based on a Vanadosilicate Cluster for the Selective Oxidation of Styrene to Benzaldehyde24Exploring the influence of metal ions/ligands ratio for the structure of polyoxometalate-based host-guest compounds, exhibiting different magnetic phenomena5Engineering donor-acceptor conjugated organic polymers with boron nitride to enhance photocatalytic performance towards visible-light-driven metal-free selective oxidation of sulfides66Progress in polyoxometalate catalysis102D Hybrid Architectures Constructed from Two Kinds of Polyoxovanadates as Efficient Heterogeneous Catalysts for Cyanosilylation and Knoevenagel Condensation63Equi–size nesting of Platonic and Archimedean metal–organic polyhedra into a twin capsid42Scalable, Durable, and Recyclable Metal‐Free Catalysts for Highly Efficient Conversion of CO2 to Cyclic Carbonates147Scalable, Durable, and Recyclable Metal‐Free Catalysts for Highly Efficient Conversion of CO2 to Cyclic Carbonates43An Unprecedented Bird Nest Molybdenum(V) Cobalto‐Phosphate Nanosized Wheel Constructed from the [H55(Mo24O48)(Co4O)2Co16(PO4)42(py)6(EtOH)2(H2O)11]3− Anion6Two new Schiff-base modified vanadium complexes with third-order NLO properties3Sustainable Carbons and Fuels: Recent Advances of CO2 Conversion in Molten Salts50One-step multiple-site integration strategy for CO2 capture and conversion into cyclic carbonates under atmospheric and cocatalyst/metal/solvent-free conditions128The crystal structure of hexakis(2-(pyridin-2-ylamino)pyridin-1-ium) decavanadate(V) dihydrate, C60H64N18O30V101In Situ Ligand-Transformation-Involved Synthesis of Inorganic–Organic Hybrid Polyoxovanadates as Efficient Heterogeneous Catalysts for the Selective Oxidation of Sulfides53Integrating hydrogen production with anodic selective oxidation of sulfides over a CoFe layered double hydroxide electrode69Polyoxometalate-Based Metal–Organic Frameworks with Unique High-Nuclearity Water Clusters40Eight-membered ring petal-shaped V8 cluster: An efficient heterogeneous catalyst for selective sulfur oxidation6Synthesis, structure and catalytic study of a new sandwiched-type vanadoselenite4Polyoxometalate-Based Organic–Inorganic Hybrids as Heterogeneous Catalysts for Cycloaddition of CO2 with Epoxides and Oxidative Desulfurization Reactions25Air atmospheric photocatalytic oxidation by ultrathin C,N-TiO 2 nanosheets18Organo-functionalized polyoxovanadates: crystal architecture and property aspects64Selective synthesis of sulfoxides and sulfones via controllable oxidation of sulfides with N -fluorobenzenesulfonimide28Tandem-like vanadium cluster chains in a polyoxovanadate-based metal–organic framework for efficient catalytic oxidation of sulfides65Two Polyoxometalate‐Based Hybrid Compounds Modified by Iron Schiff Base Complexes: Syntheses, Crystal structures, Cyclic Voltametric Studies and Nonlinear Optical Properties11Two three-dimensional polyanionic clusters [M(P 4 Mo 6 ) 2 ] (M = Co, Zn) exhibiting excellent photocatalytic CO 2 reduction performance19Self-Assembled Polyoxometalate-Based Metal-Organic Polyhedra as an Effective Heterogeneous Catalyst for Oxidation of Sulfide26Decavanadate-based clusters as bifunctional catalysts for efficient treatment of carbon dioxide and simulant sulfur mustard32One-step preparation of ammonium-specified pyrazolium ionic liquids unveil the more popular pathway for the CO2 fixation: Integrated experimental and theoretical studies15Lacunary {Se4V10} Heteropolyoxovanadate Precursor with Monometal, Metal-Richer-Sandwiched Derivatives {Se8V20M} and {Se8V20M3}: Correlations between the Synthesis, Structure, and Catalytic Property6Accelerated Oxidation of Organic Sulfides by Microdroplet Chemistry32Incorporating Photochromic Triphenylamine into a Zirconium–Organic Framework for Highly Effective Photocatalytic Aerobic Oxidation of Sulfides102Two Co(II)-Based MOFs Constructed from Resorcin[4]Arene Ligand: Syntheses, Structures, and Heterogeneous Catalyst for Conversion of CO24Decavanadate‐based Transition Metal Hybrids as Bifunctional Catalysts for Sulfide Oxidation and C—C Bond Construction29Extractive desulfurization of diesel fuel by amide-based type IV deep eutectic solvents71Adjusting accommodation microenvironment for Cu+ to enhance oxidation inhibition for thiophene capture24Three Polyoxovanadates-Based Organic–Inorganic Hybrids: Structural Variation, Bifunctional Electrocatalytic Activities, and Computational Studies24Synergistic Catalysis of Ionic Liquid-Decorated Covalent Organic Frameworks with Polyoxometalates for CO2 Cycloaddition Reaction under Mild Conditions79Self-assembly of three Ag-polyoxovanadates frameworks for their efficient construction of C N bond and detoxification of simulant sulfur mustard24Atomically Dispersed High‐Density Al–N4 Sites in Porous Carbon for Efficient Photodriven CO2 Cycloaddition169Four novel Z-shaped hexanuclear vanadium oxide clusters as efficient heterogeneous catalysts for cycloaddition of CO2 and oxidative desulfurization reactions18Defected MoS2 Modified by Vanadium-Substituted Keggin-Type Polyoxometalates as Electrocatalysts for Triiodide Reduction in Dye-Sensitized Solar Cells18A POM-based porous supramolecular framework for efficient sulfide–sulfoxide transformations with a low molar O/S ratio33Amino induced high-loading atomically dispersed Co sites on N-doped hollow carbon for efficient CO 2 transformation15An anthracene-9-carboxylic acid-based [Cu 20 ] cluster templated by a bromine anion for heterogeneous catalytic chemical fixation of carbon dioxide5High-nuclear polyoxovanadates assembled from pentagonal building blocks27Highly efficient multi-site synergistic catalysis of a polyoxovanadate-based metal–organic framework for benzylic C–H bond oxidation40Oxidative Desulfurization and Magnetic Properties of a Mixed-Valence Cobalt Vanadate6Serendipitous synthesis of 2-alkenyl- and 2-aryl-4-thiazolidinones using dithiodiglycolic anhydride2Single Walled Carbon Nanotubes with Encapsulated Pt(Ii) Photocatalyst for the Oxidation of Sulfides in Water11Three Si-substituted polyoxovanadates as efficient catalysts for Knoevenagel condensation and selective oxidation of styrene to benzaldehyde17Imidazole-Dependent Assembly of Copper Polymolybdate Frameworks for One-Pot Sulfide Oxidation and C–H Activation3Near-Infrared Photothermal Catalysis for Enhanced Conversion of Carbon Dioxide under Mild Conditions48Highly Crystalline Ag‐based Coordination Polymers for Efficient Photocatalytic Oxidation of Sulfides4Electrochemically Assisted Cycloaddition of Carbon Dioxide to Styrene Oxide on Copper/Carbon Hybrid Electrodes: Active Species and Reaction Mechanism10Exceptional structure flexibility and adaptive catalytic desulfurization of a cyclic decanuclear polyoxoalkoxyvanadate (Ⅲ)2S-Scheme Bi-oxide/Ti-oxide Molecular Hybrid for Photocatalytic Cycloaddition of Carbon Dioxide to Epoxides96Two 1D Anderson-Type Polyoxometalate-Based Metal–Organic Complexes as Bifunctional Heterogeneous Catalysts for CO2 Photoreduction and Sulfur Oxidation27Supported TiO 2 /silica gel as an efficient and inexpensive catalyst for nonsolvent liquid‐phase oxidation of cyclohexylamine to cyclohexanone oxime2Catalytic application of polyoxovanadates in the selective oxidation of organic molecules110Nonredox CO2 Fixation in Solvent-Free Conditions Using a Lewis Acid Metal–Organic Framework Constructed from a Sustainably Sourced Ligand18Four unprecedented V14 clusters as highly efficient heterogeneous catalyst for CO2 fixation with epoxides and oxidation of sulfides26Vacancy-cluster-mediated surface activation for boosting CO 2 chemical fixation25Fabrication of dianthracene-based hyper-cross-linked polymers for selective photocatalytic oxidation of organic sulfides25Polyoxovanadate-based metal–organic frameworks consisted of open vanadium sites for selective catalytic oxidation of sulfides17{V6} Ring Sandwiched Polyoxoniobate as Molecular Electrocatalyst for Oxidant‐Free Synthesis of Sulfoxides7Transition Metal Single Atoms Constructed by Using Inherent Confined Space60Photoexcited Single-Electron Transfer for Efficient Green Synthesis of Cyclic Carbonate from CO 256Precise design of nickel phthalocyanine molecular structure: Optimizing electronic and spatial effects for remarkable electrocatalytic CO2 reduction19A Nonionic Octanuclear Vanadium(V) Oxide Cluster Complex as a Precatalyst for Visible-light Photooxidation of Alcohols under O2 Atmosphere0Supramolecular Chemistry of Windmill-like Al10 Clusters: Adjustable Guests and Hydrogen-Bonding Networks for Enhanced Optical Limiting1CO 2 Cycloaddition under Ambient Conditions over Cu–Fe Bimetallic Metal–Organic Frameworks62Multifunctional Aryl Sulfonium Decavanadates: Tuning the Photochromic and Heterogeneous Oxidative Desulfurization Catalytic Properties Using Salicylaldehyde-type Functional Moieties on Counterions6Experimental and Theoretical Studies on Two Dual-Functional Organic–Inorganic Hybrids Based on [V4O12]4– Clusters2C2-phenyl-substituted benzimidazolium-based covalent organic framework as efficient catalyst for CO2 conversion without solvents, metals, and cocatalysts17Synthesis and Structure of High-Nuclearity Carboxylate-Modified Heteropolyoxovanadate Serving as a Heterogeneous Catalyst for Selective Oxidation of Alkylbenzenes8Constructing Two Cu-Modified Organophosphomolybdates from a Nanocluster to a One-Dimensional Chain for Boosted Visible-Light-Driven Hydrogen Production10Sustainable Production of Cyclic Carbonates from CO 2 and Epoxides Using Transition Metal Substituted Polyoxometalate-TBA Hybrid Catalysts0Ligation of Titanium-oxide and {Mo2} Units for Solar CO2 Storage11Designed synergetic bifunctional catalyst based on diverse nucleophilic-functionalized sites for high-efficient CO2 cycloaddition under co-catalyst and solvent-free conditions11Metal cluster/ruthenium photosensitizer/cobalt phthalocyanine synergistic photocatalytic cycloaddition of carbon dioxide and propylene oxide12Rational fabrication of three imidazole-functionalized ionic-type Pd-Polyoxovanadates for aerobic oxidation of 5-Hydroxymethulfurfural to 2,5-Diformylfuran22De novo assembly of frustrated Lewis pair bearing metal‐organic frameworks for atmospheric CO 2 cycloaddition8Ionic liquids bonded in mesoporous HAP serve as efficient catalysts for CO2 fixation40Duality of Semiconductor Photocatalysts for Sulfides Oxidation in Supercritical CO2 Medium: Graphitic Carbon Nitride (gC3N4) vs Nano Titania (TiO2)0Green synthesis of hypercrosslinked polymers for CO 2 capture and conversion: recent advances, opportunities, and challenges108Self-assembled novel Co/Ni-based ε-Keggin crystal materials as highly efficient photocatalysts for diluted CO 2 photoreduction14Revealing the roles of the dual active-sites on a polyoxometalate-based metal–organic framework in catalyzing Knoevenagel condensations24Molten Salt Electrolytic CO 2 -Derived Carbon-Based Nanomaterials for Energy Storage and Electrocatalysis: A Review10Photoredox‐Catalyzed Transition‐Metal‐Free C( sp 2 )−H Phosphorylation Using 9‐Mesityl‐10‐Methylacridinium Perchlorate Photocatalyst1Desulfurization and Denitrogenation Using Betaine-Based Deep Eutectic Solvents14Single-atom-mediated electron islands boost photocatalytic CO2 chemical fixation11Highly efficient C16-PW9/SiO2 designed based on trivacant tungstophosphate ([A-PW9O34]9−) for rapid oxidative desulfurization under mild conditions15Vanadium-Silsesquioxane Nanocages as Heterogeneous Catalysts for Synthesis of Quinazolinones19Insight into the Mechanism of CO 2 Chemical Fixation into Epoxides by Windmill-Shaped Polyoxovanadate and n -Bu 4 NX (X = Br, I)8Discovery of a new family member of arsenic–vanadium polyoxometalates with high catalytic performance for one-pot coupling of CO2, epoxides and amines7Self-assembly of organoarsonic acid functionalized polyoxovanadate cage from cap-like building block0Swift Proton Release Enhancing Proton Conductivity in Anderson-Polyoxometalates-Based Metal–Organic Frameworks39Unlocking versatile capabilities: Mixed-valence decavanadate aerogels for boosting radar, infrared, and thermal stealth3Rational fabrication of two polyoxovanadate-based frameworks for efficient detoxifying mustard gas simulant10A resorcin[4]arene-based MOF as a Lewis acid catalyst for the CO2 coupling reaction3Homogeneous and heterogeneous selective oxidation of ethyl lactate regulated by a novel vanadium complex4Dual-antenna@reactor with active “hot spots” for full-spectrum driven CO2 cycloaddition studied at single-particle level19A theoretical study on the formation mechanism of peroxovanadate and the origin of its high activity for oxidation of sulfide2Amine functionalized quinolinium polyoxometalates as highly active heterogeneous catalysts for solvent-free CO 2 cycloaddition and Knoevenagel condensation reactions3Construction of V 2 O 3 /VN@GO heterojunction cathodes derived from polyoxovanadates for high-performance aqueous zinc ion batteries8Modulating the catalytic properties of decavanadate hybrids using a mixed counterion strategy for selective oxidation of thiophene-based sulfides and detoxification of mustard gas simulant0The stepwise construction of polyoxovanadate-based Zn-MOF nanoparticles with Lewis acid sites for the one-pot synthesis of N-heterocycles in air2Two new isopolyoxovanadates based on V 10 and V 6 : structural assembly and dual catalytic applications2Catalytic Conversion of Carbon Dioxide to Propylene Carbonate: Catalyst Design and Industrialization Progress38Experimental and Theoretical Study of Two 3D Difunctional Electrocatalytic Hybrid Vanadate-Containing Metal–Organic Motifs0Engineering Nitrogen‐Coordinated Single‐Atom Catalysts for Efficient CO 2 Cycloaddition29The first chiral polyoxometalate-based photocatalyst for highly efficient carbon dioxide reduction13Catalytic Oxidative Valorization of Biobased 5-Hydroxymethylfurfural over Multi-ligand Functionalized Polyoxovanadates2NH2-MIL-101(Fe) Nanocrystals Synthesized by the Ionic Liquid–Ethanol Interface for Efficient CO2 Fixation at Mild Conditions7Electronic State Modulation of a Single‐Cu Site on a Bimetallically Doped Titanium‐Oxo Cluster to Enhance CO 2 Storage0Electronic State Modulation of a Single‐Cu Site on a Bimetallically Doped Titanium‐Oxo Cluster to Enhance CO 2 Storage10Synthesis of cyclic carbonates by CO2 cycloaddition with epoxides: recent advances, challenges, and perspectives20Construction and shaping of polyoxometalate‐based covalent organic framework for boosting one‐pot CO2 conversion6Duality of Semiconductor Photocatalysts for Sulfide Oxidation in a Supercritical CO2 Medium: Graphitic Carbon Nitride (gC3N4) versus Nano Titania (TiO2)3Disordered Ru–O 6 Octahedrons for Efficient and Selective Electro-oxidation of Sulfide to Sulfoxide via Boosted Surface Oxygen Kinetics18The synergistic effects between light and Lewis acid sites in MIL-MOFs for promoting highly efficient CO2 cycloaddition reactions5Mass transfer and kinetic behavior studies on cycloaddition of carbon dioxide with propylene oxide catalyzed by ionic liquid in microchannel reactor2Two Imidazole-Functionalized Mixed-Valence Oxidovanadium Clusters for Catalytic Oxidation of Sulfides2Elucidating the boosted performance of Ni 3 ZnC 0.7 alloy catalyst fabricated by MOFs templated strategy for CO 2 cycloaddition reaction2Polyoxometalate-based catalysts for visible-light-driven hydrolytic hydrogen production: coordinatively unsaturated Cu-based active sites enhance performance1Fivefold-symmetry-induced reverse template effect: self-assembly of a high-nuclear core–shell polyoxophosphovanadate0Layered vanadium oxides with expanded interlayer spacing for rapid degradation of mustard gas simulants0Recent advances in single-crystal polyoxometalate-based metal–organic complex catalytic systems for sulfide–sulfoxide selective transformations2Tartrate-bridged ring-shaped polyoxometalates comprising mixed lacunary Keggin and Lindqvist fragments0Multifunctional Cd(II)-Viologen-Sensitized coordination polymers synthesized via carboxylic acid regulation: photochromism and selective photocatalytic sulfoxidation4Polyoxovanadate Building Units in Metal–Organic Frameworks: Coordination Connectivity and Selective Oxidation of Aromatic Thioether7Copper‐Bonded Polyoxovanadates‐Based Hybrids as Efficient Catalysts for Azide−Alkyne Cycloaddition1Application of computational tools for experimental data analysis of homogeneous catalytic systems in the synthesis of cyclic carbonates1Directional Charge Transfer in V–P–Ni 1D Chain for CO 2 Photoreduction and Mustard-Gas Simulant Detoxification1An Imidazole-Functionalized Polyoxovanadate with a Classical {V 18 O 42 } Core and Its Photothermal Conversion Behavior0Hollow Tubular Engineering and Electronic Structure Modulation of Vanadium-Incorporated MoP for Boosting Alkaline Hydrogen Evolution0Terminal Oxygen as a Proton Acceptor: S–H Activation via Proton-Coupled Electron Transfer in Decavanadate-Catalyzed P(O)–S Coupling0

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  40. Self-assembly of three Ag-polyoxovanadates frameworks for their efficient construction of C N bond and detoxification of simulant sulfur mustard

    Chinese Chemical Letters · 2021-09-16

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  41. Atomically Dispersed High‐Density Al–N4 Sites in Porous Carbon for Efficient Photodriven CO2 Cycloaddition

    Advanced Materials · 2021-09-18

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  42. Four novel Z-shaped hexanuclear vanadium oxide clusters as efficient heterogeneous catalysts for cycloaddition of CO2 and oxidative desulfurization reactions

    Chinese Chemical Letters · 2021-11-07

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  43. Defected MoS2 Modified by Vanadium-Substituted Keggin-Type Polyoxometalates as Electrocatalysts for Triiodide Reduction in Dye-Sensitized Solar Cells

    Inorganic Chemistry · 2021-12-13

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  44. A POM-based porous supramolecular framework for efficient sulfide–sulfoxide transformations with a low molar O/S ratio

    Inorganic Chemistry Frontiers · 2022-01-01

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  45. Amino induced high-loading atomically dispersed Co sites on N-doped hollow carbon for efficient CO 2 transformation

    Chemical Communications · 2022-01-01

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  46. An anthracene-9-carboxylic acid-based [Cu 20 ] cluster templated by a bromine anion for heterogeneous catalytic chemical fixation of carbon dioxide

    Journal of Materials Chemistry A · 2022-01-01

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  47. High-nuclear polyoxovanadates assembled from pentagonal building blocks

    Chemical Communications · 2022-01-01

    Ting Zhang, Yu-Han Hou, Baoshan Hou, Liang Zhao, Xinlong Wang, Chao Qin, Zhong‐Min Su

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  48. Highly efficient multi-site synergistic catalysis of a polyoxovanadate-based metal–organic framework for benzylic C–H bond oxidation

    Journal of Materials Chemistry A · 2022-01-01

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  49. Oxidative Desulfurization and Magnetic Properties of a Mixed-Valence Cobalt Vanadate

    Polyhedron · 2022-01-01

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  50. Serendipitous synthesis of 2-alkenyl- and 2-aryl-4-thiazolidinones using dithiodiglycolic anhydride

    New Journal of Chemistry · 2022-01-01

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