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RESEARCH PAPER · Advanced Energy Materials · 2019

Tin Halide Perovskites: Progress and Challenges

Wenfan Yang, Femi O. Igbari, Yanhui Lou, Zhao‐Kui Wang, Liang‐Sheng Liao

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Tin Halide Perovskites: Progress and ChallengesOriginalLead Oxalate-Induced Nucleation Retardation for High-Performance Indoor and Outdoor Perovskite Photovoltaics27Progress and Perspective of Tin Perovskite Solar Cells5Searching for stable perovskite solar cell materials using materials genome techniques and high-throughput calculations40Two-dimensional organic–inorganic hybrid Ruddlesden–Popper perovskite materials: preparation, enhanced stability, and applications in photodetection61Ultraviolet‐Protective Transparent Photovoltaics Based on Lead‐Free Double Perovskites41Enriched Photophysical Properties and Thermal Stability of Tin(II) Substituted Lead-Based Perovskite Nanocrystals with Mixed Organic–Inorganic Cations27Simultaneous Power Conversion Efficiency and Stability Enhancement of Cs 2 AgBiBr 6 Lead‐Free Inorganic Perovskite Solar Cell through Adopting a Multifunctional Dye Interlayer235First-Principles Study on the Oxygen–Light-Induced Iodide Vacancy Formation in FASnI3 Perovskite28Computational determination of the physical-thermoelectric parameters of tin-based organomatallic halide perovskites (CH3NH3SnX3, X = Br and I): Emerging materials for optoelectronic devices32Ligand Orientation-Induced Lattice Robustness for Highly Efficient and Stable Tin-Based Perovskite Solar Cells125Dealing with Lead in Hybrid Perovskite: A Challenge to Tackle for a Bright Future of This Technology?70Femtosecond Transient Absorption Spectra and Dynamics of Carrier Relaxation of Tin Perovskites in the Absence and Presence of Additives80Recent Advances in Cs2AgBiBr6‑Based Halide Double Perovskites as Lead-Free and Inorganic Light Absorbers for Perovskite Solar Cells241Efficient Nonlead Double Perovskite Solar Cell with Multiple Hole Transport Layers26Lead-free halide perovskite photovoltaics: Challenges, open questions, and opportunities110Recent progress, fabrication challenges and stability issues of lead-free tin-based perovskite thin films in the field of photovoltaics103Crystallization Kinetics Modulation of FASnI 3 Films with Pre‐nucleation Clusters for Efficient Lead‐Free Perovskite Solar Cells142Crystallization Kinetics Modulation of FASnI3 Films with Pre‐nucleation Clusters for Efficient Lead‐Free Perovskite Solar Cells38Tin-Based Defects and Passivation Strategies in Tin-Related Perovskite Solar Cells258Boosting triplet self-trapped exciton emission in Te(IV)-doped Cs2SnCl6 perovskite variants239Solution-processed NiO x nanoparticles with a wide pH window as an efficient hole transport material for high performance tin-based perovskite solar cells13Additive engineering for Sn-based PSCs: Enhancement of open-circuit voltage and fill factor19Alkylamine screening and zinc doping of highly luminescent 2D tin-halide perovskites for LED lighting27Impact of noncovalent interactions on structural and photophysical properties of zero-dimensional tellurium( iv ) perovskites17Photon management to reduce energy loss in perovskite solar cells197Rational strategies toward efficient and stable lead-free tin halide perovskite solar cells15Recent progress of tin-based perovskites and their applications in light-emitting diodes3Structural evolution, optical gap and thermoelectric properties of CH 3 NH 3 SnBr 3 hybrid perovskite, prepared by mechanochemistry21Suppressed oxidation of tin perovskite by Catechin for eco-friendly indoor photovoltaics53Efficient Passivation Strategy on Sn Related Defects for High Performance All‐Inorganic CsSnI3 Perovskite Solar Cells220Photoferroelectric perovskite solar cells: Principles, advances and insights108Recent progress toward highly efficient tin‐based perovskite (ASnX3) solar cells33Revealing the Local Sn and Pb Arrangements in CsSnxPb1–xBr3 Perovskites with Solid-State NMR Spectroscopy45Synthèse de matrices vitreuses en conditions extrêmes dopées en iode : application au stockage sous pression des radioisotopes produits de l’industrie nucléaire0Close-loop recycling of perovskite solar cells through dissolution-recrystallization of perovskite by butylamine83Organic Cation Engineering for Vertical Charge Transport in Lead‐Free Perovskite Quantum Wells11Lead‐free halide perovskite photodetectors spanning from near‐infrared to X‐ray range: a review53Tunable electronic properties and large optical anisotropy in the CsPbXnY3-n (X, Y = Cl, Br, I) perovskite5In-Situ Nano-Auger Probe of Chloride-Ions during CH3NH3PbI3−xClx Perovskite Formation72D Nanomaterials for Effective Energy Scavenging84Additive Engineering toward High‐Performance Tin Perovskite Solar Cells582D WSe2 Flakes for Synergistic Modulation of Grain Growth and Charge Transfer in Tin‐Based Perovskite Solar Cells73Making Room for Growing Oriented FASnI3 with Large Grains via Cold Precursor Solution91Controlled Structural Transformation in Sb‐Doped Indium Halides A3InCl6 and A2InCl5∙H2O Yields Reversible Green‐to‐Yellow Emission Switch86Metal‐Halide Perovskite Crystallization Kinetics: A Review of Experimental and Theoretical Studies87Real-Time Investigation of Sn(II) Oxidation in Pb-Free Halide Perovskites by X-ray Absorption and Mössbauer Spectroscopy13Property Modulation of Two-Dimensional Lead-Free Perovskite Thin Films by Aromatic Polymer Additives for Performance Enhancement of Field-Effect Transistors36High efficient and stable Tin-based perovskite solar cells via short-chain ligand modification8Biocompatible and Biodegradable Light‐Emitting Materials and Devices48Benzylammonium‐Mediated Formamidinium Lead Iodide Perovskite Phase Stabilization for Photovoltaics45Designing hole conductor free tin–lead halide based all-perovskite heterojunction solar cell by numerical simulation68Cation Dynamics in Hybrid Halide Perovskites40Optoelectronic property refinement of FASnI3 films for photovoltaic application5Insights into the impact of metal tin substitution on methylammonium lead bromide perovskite performance for photovoltaic application23Stability of Sn-Pb mixed organic–inorganic halide perovskite solar cells: Progress, challenges, and perspectives83Stability Improvement of Tin‐Based Halide Perovskite by Precursor‐Solution Regulation with Dual‐Functional Reagents72Efficient and stable Ruddlesden-Popper layered tin-based perovskite solar cells enabled by ionic liquid-bulky spacers50Heterogeneous 2D/3D Tin‐Halides Perovskite Solar Cells with Certified Conversion Efficiency Breaking 14%579Architecture of p-i-n Sn-Based Perovskite Solar Cells: Characteristics, Advances, and Perspectives138Lead-Free Cesium-Containing Halide Perovskite and Its Application in Solar Cells23Dopants for Enhanced Performance of Tin-Based Perovskite Solar Cells—A Short Review10The Evolution of Photoluminescence Properties of PEA2SnI4 Upon Oxygen Exposure: Insight into Concentration Effects41Controlling Quantum-Well Width Distribution and Crystal Orientation in Two-Dimensional Tin Halide Perovskites via a Strong Interlayer Electrostatic Interaction21Improving efficiency of perovskite solar cell using optimized front surface nanospheres grating17Recent Advances in Blue Perovskite Quantum Dots for Light‐Emitting Diodes105The Voltage Loss in Tin Halide Perovskite Solar Cells: Origins and Perspectives91Electronic defect passivation of FASnI3 films by simultaneous Hydrogen-bonding and chlorine co-ordination for highly efficient and stable perovskite solar cells40Crystallization Dynamics of Sn‐Based Perovskite Thin Films: Toward Efficient and Stable Photovoltaic Devices197Microampere-level piezoelectric energy generation in Pb-free inorganic halide thin-film multilayers with Cu interlayers16Acetic Acid‐Assisted Synergistic Modulation of Crystallization Kinetics and Inhibition of Sn2+ Oxidation in Tin‐Based Perovskite Solar Cells190Optical Properties of Mixed-Halide Double Perovskites Cs2AgBi(Br1-xIx)6: First-Principle Study5Plasmon-coupled Au-nanochain functionalized PEDOT:PSS for efficient mixed tin–lead iodide perovskite solar cells12Micro‐Light‐Emitting Diodes Based on InGaN Materials with Quantum Dots42Density functional theory investigation of the mechanical, electronic and optical properties of Pb-free vacancy-ordered double perovskites K 2 PdCl 6 and K 2 PdBr 613Insight on noncovalent interactions and orbital constructs in low-dimensional antimony halide perovskites6Lead-free hybrid perovskite photocatalysts: surface engineering, charge-carrier behaviors, and solar-driven applications61Metal Halide Perovskite-Based Phosphors and Their Applications in LEDs3One-pot synthesis of novel ligand-free tin( ii )-based hybrid metal halide perovskite quantum dots with high anti-water stability for solution-processed UVC photodetectors12Research progress of ABX 3 -type lead-free perovskites for optoelectronic applications: materials and devices49Synergistic effect of two hydrochlorides resulting in significantly enhanced performance of tin-based perovskite solar cells with 3D to quasi-2D structural transition20Tin-based halide perovskite materials: properties and applications132Use of anti-solvent to enhance thermoelectric response of hybrid halide perovskite thin films60D/2D Mixed Dimensional Lead-Free Caesium Bismuth Iodide Perovskite for Solar Cell Application22Computational chemistry advances on benzodithiophene-based organic photovoltaic materials12Toward Eco‐Friendly Lead‐Free Low‐Dimensional Perovskites13An efficient and stable lead-free organic–inorganic tin iodide perovskite for photovoltaic device: Progress and challenges34Directional and Polarized Lasing Action on Pb‐free FASnI3 Integrated in Flexible Optical Waveguides21Performance improvement of dye-sensitized double perovskite solar cells by adding Ti3C2T MXene79Recent progress of rare earth conversion material in perovskite solar cells: A mini review24The effects of organic cation rotation in hybrid Organic-Inorganic Perovskites: A critical review48Improved charge extraction and atmospheric stability of all-inorganic Cs2AgBiBr6 perovskite solar cells by MoS2 nanoflakes30Frist principle study of double perovskites Cs2AgSbX6 (X = Cl, Br, I) for solar cell and renewable energy applications46Organic‐Free and Lead‐Free Perovskite Solar Cells with Efficiency over 11%75Trapped-Hydrogen-Induced Energy Loss in Tin-Based Hybrid Perovskite Solar Cells3Highly Efficient and Stable FASnI3 Perovskite Solar Cell via Modification with Tetrapotassium Hexacyanoferrate4Progress and challenges in the fabrication of lead-free all-inorganic perovskites solar cells using solvent and compositional engineering Techniques-A review13Flexible perovskite light-emitting diodes: Progress, challenges and perspective32Study of new double perovskites Tl2PtX6 (X = Cl, Br, I) for solar cells and thermoelectric applications15Efficient and Stable Mesoporous CsSnI3 Perovskite Solar Cells via Imidazolium‐Based Ionic Liquid Additive17Thermodynamically regulated preparation of high performance for carbon-based Cs2AgBiBr6 perovskite solar cells8Red Perovskite Light‐Emitting Diodes: Recent Advances and Perspectives72Emerging Chalcohalide Materials for Energy Applications163Phase-Controlled Strategy for High-Quality Single-Source Vapor-Deposited Cs2AgBiBr6 Thin Films14Pure Tin Halide Perovskite Solar Cells: Focusing on Preparation and Strategies76Resolving Oxidation States and X –site Composition of Sn Perovskites through Auger Parameter Analysis in XPS35Lead acetate as a superior lead source enables highly efficient and stable all-inorganic lead-tin perovskite solar cells25[(CH 3 ) 2 NH 2 ] 2 PdBr 4 , a layered hybrid halide perovskite semiconductor with improved optical and electrical properties14Efficient Tin-Based Perovskite Solar Cell with Cesium Acetate Pre-Buried Pedot:Pss Hole Transport Layer0Efficient Tin-Based Perovskite Solar Cell with Cesium Acetate Pre-Buried Pedot:Pss Hole Transport Layer0Pernicious effects and management of lead leakage from perovskite solar cells14X-ray absorption spectroscopy as a technique to study environmentally sustainable materials0High-member low-dimensional Sn-based perovskite solar cells64Study of lead free double perovskites Na2XAgCl6 (X = Ga, In Tl) for solar cells and transport applications8Sn‐Based Self‐Powered Ultrafast Perovskite Photodetectors with Highly Crystalline Order for Flexible Imaging Applications76Ammonium Salt Assisted Crystallization for High Performance Two-Dimensional Lead-Free Perovskite Photodetector4Structure stabilized with robust molecular cation N(CH3)4+ in high efficiency perovskite solar cells2Origins, Impacts, and Mitigation Strategies of Strain in Efficient and Stable Perovskite Solar Cells36Vibrational, mechanical, electronic and thermodynamic properties of rhenium-based perovskites XReO3(X = Li, Be) by an ab-initio computation30Study on the performance of CuBr2 doped Cs2AgBiBr6 perovskite solar cells with carbon electrode and without a hole-transporting layer7Study of optoelectronic, thermoelectric, mechanical, and thermodynamic properties of Cs2NaTlX6 (X = Cl, Br, I) for energy harvesting24The Effect of Different Precursor Solutions on the Structural, Morphological, and Optical Properties of Nickel Oxide as an Efficient Hole Transport Layer for Perovskite Solar Cells6The narrow band bap double perovskites X2CuInCl6 (X = K, Rb, Cs) for optoelectronics, and thermoelectric applications37Functional 2D Phases in Mixed Dimensional Perovskite Photovoltaics13Study of inorganic double perovskites Cs2RbZI6 (Z = Ga, In) as energy harvesting aspirant: a DFT approach21Efficient and stable Sn based perovskite solar cells by the modulation of crystallization with bulky organic cation for large nucleation cluster0DeePKS Model for Halide Perovskites with the Accuracy of a Hybrid Functional5Inhibition of Sn 2+ Oxidation in FASnI 3 Perovskite Precursor Solution and Enhanced Stability of Perovskite Solar Cells by Reductive Additive47Improved Air Stability of Tin Halide Perovskite Solar Cells by an N‐Type Active Moisture Barrier34Propylamine hydrobromide passivated tin-based perovskites to efficient solar cells5Lead-Free Perovskite Solar Cells1Composition Dependent Strain Engineering of Lead-Free Halide Double Perovskite: Computational Insights17Environmentally Friendly Perovskite‐Based Photovoltaics and Luminescence: Lead Less or Lead Free15Mitigating Environmental Effects in Halide Perovskites through Hybrid Perovskite-Polymer Nanocomposites: A Short Review8Temperature-induced gradient tin–lead-mixed halide perovskite photodetector10DFT Insights into Layer-Dependent Superhigh Piezoelectricity and Carrier Mobility in 2D Hexagonal SnNBr7Investigation of highly efficient self-powered photo-detector performance of all inorganic lead-free halide perovskites (CsSnCl3) nanocrystals (NCs) decorated Er: ZnO nanowires (NWs)/Si heterojunctions8Seeking environmentally friendly halide perovskite photocatalysts: synthesis, structure and photocatalytic performance exploration2Fundamental understanding in the performance-limiting factors of Cs2AgBiBr6-based perovskite photovoltaics43Bi‐Functional Phosphine Oxide Passivator for Efficient Near‐Infrared Sn‐Based Perovskite Light‐Emitting Diodes with Ultra‐Low Efficiency Roll‐Off56All Inorganic Perovskite Solar Cells1Dynamic synergy of tin in the electron-transfer layer and absorber layer for advancing perovskite solar cells: a comprehensive review28Multi-functional molecule advancing the efficiency of pure 3D FASnI 3 perovskite solar cells based on the tin tetraiodide reduction method14Recent progress in all-inorganic tin-based perovskite solar cells: a review28Constructing Charge Bridge Path for High‐Performance Tin Perovskite Photovoltaics29Selective oxidative coupling of amines through light‐activated bismuth halide perovskites14Efficient Tin-Based Perovskite Solar Cell with a Cesium Acetate Pre-buried PEDOT:PSS Hole Transport Layer17Structural, electronic, and optical study of lead-free perovskite CH3NH3SnBr3 under compressive strain using DFT and DFT+U17Tailoring Single‐Mode Random Lasing of Tin Halide Perovskites Integrated in a Vertical Cavity28Cross‐Linkable Fullerene Enables Elastic and Conductive Grain Boundaries for Efficient and Wearable Tin‐Based Perovskite Solar Cells35Cross‐Linkable Fullerene Enables Elastic and Conductive Grain Boundaries for Efficient and Wearable Tin‐Based Perovskite Solar Cells8

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  1. Lead Oxalate-Induced Nucleation Retardation for High-Performance Indoor and Outdoor Perovskite Photovoltaics

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  10. Ligand Orientation-Induced Lattice Robustness for Highly Efficient and Stable Tin-Based Perovskite Solar Cells

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  11. Dealing with Lead in Hybrid Perovskite: A Challenge to Tackle for a Bright Future of This Technology?

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  12. Femtosecond Transient Absorption Spectra and Dynamics of Carrier Relaxation of Tin Perovskites in the Absence and Presence of Additives

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  13. Recent Advances in Cs2AgBiBr6‑Based Halide Double Perovskites as Lead-Free and Inorganic Light Absorbers for Perovskite Solar Cells

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  14. Efficient Nonlead Double Perovskite Solar Cell with Multiple Hole Transport Layers

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  16. Recent progress, fabrication challenges and stability issues of lead-free tin-based perovskite thin films in the field of photovoltaics

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  19. Tin-Based Defects and Passivation Strategies in Tin-Related Perovskite Solar Cells

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  21. Solution-processed NiO x nanoparticles with a wide pH window as an efficient hole transport material for high performance tin-based perovskite solar cells

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  33. Revealing the Local Sn and Pb Arrangements in CsSnxPb1–xBr3 Perovskites with Solid-State NMR Spectroscopy

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  34. Synthèse de matrices vitreuses en conditions extrêmes dopées en iode : application au stockage sous pression des radioisotopes produits de l’industrie nucléaire

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  35. Close-loop recycling of perovskite solar cells through dissolution-recrystallization of perovskite by butylamine

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  36. Organic Cation Engineering for Vertical Charge Transport in Lead‐Free Perovskite Quantum Wells

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  37. Lead‐free halide perovskite photodetectors spanning from near‐infrared to X‐ray range: a review

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  38. Tunable electronic properties and large optical anisotropy in the CsPbXnY3-n (X, Y = Cl, Br, I) perovskite

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  39. In-Situ Nano-Auger Probe of Chloride-Ions during CH3NH3PbI3−xClx Perovskite Formation

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  40. 2D Nanomaterials for Effective Energy Scavenging

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  41. Additive Engineering toward High‐Performance Tin Perovskite Solar Cells

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  42. 2D WSe2 Flakes for Synergistic Modulation of Grain Growth and Charge Transfer in Tin‐Based Perovskite Solar Cells

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  43. Making Room for Growing Oriented FASnI3 with Large Grains via Cold Precursor Solution

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