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RESEARCH PAPER · Advanced Functional Materials · 2019

Versatile and Highly Efficient Controls of Reversible Topotactic Metal–Insulator Transitions through Proton Intercalation

Shanquan Chen, Haiping Zhou, Xing Ye, Zuhuang Chen, Jin-Zhu Zhao, Sujit Das, Christoph Klewe, Lei Zhang, Eduardo Lupi, Padraic Shafer, Elke Arenholz, Dun Jin, Haoliang Huang, Yalin Lu, Xiaowen Li, Meng Qiang Wu, Shanming Ke, Hu Xu, Xierong Zeng, Chuanwei Huang, Lane W. Martin, Lang Chen

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Versatile and Highly Efficient Controls of Reversible Topotactic Metal–Insulator Transitions through Proton IntercalationOriginalTopotactic fluorination induced stable structure and tunable electronic transport in perovskite barium ferrite thin films10Defects in complex oxide thin films for electronics and energy applications: challenges and opportunities190Nanoscale Phase Mixture and Multifield-Induced Topotactic Phase Transformation in SrFeOx24Hydrogen Control of Double Exchange Interaction in La0.67Sr0.33MnO3 for Ionic–Electric–Magnetic Coupled Applications33Hydrogenation driven structural transformation and adjustable electronic properties of epitaxial La0.3Sr0.7MnO3− δ films6Doping-Enabled Reconfigurable Strongly Correlated Phase in a Quasi-2D Perovskite1Metal–Insulator Transition via Ion Irradiation in Epitaxial La0.7Sr0.3MnO3−δ Thin Films6Surface De-Fluorination and Bond Modification of CFx by High-Density Hydrogen Plasma Processing31High‐Conductive Protonated Layered Oxides from H2O Vapor‐Annealed Brownmillerites14Symmetry-aware recursive image similarity exploration for materials microscopy8Migration Kinetics of Surface Ions in Oxygen‐Deficient Perovskite During Topotactic Transitions11Exploring the Spatial Control of Topotactic Phase Transitions Using Vertically Oriented Epitaxial Interfaces12Epitaxial growth of metastable La0.67Sr0.33MnO3−δ films by using Sr3Al2O6 as multifunctional buffer layers4Comparison of topotactic and magnetic structures for manganite oxide films2Reversible Hydrogen-Induced Phase Transformations in La0.7Sr0.3MnO3 Thin Films Characterized by In Situ Neutron Reflectometry23Morphologically and chemically regulated 3D carbon for Dendrite-free lithium metal anodes by a plasma processing8Converting Brownmillerite to Alternate Layers of Oxygen‐Deficient and Conductive Nano‐Sheets with Enhanced Thermoelectric Properties14Plasma-enhanced fluorination of multi-walled carbon nanotubes for CFx cathode materials with ultrahigh electrochemical performance16Highly-conductive Cu-substituted brownmillerite with emergent 3-dimensional oxygen vacancy channels3Orbital polarization change and magnetic enhancement in rutile MnO2-δ epitaxial films0Synthesis of freestanding perovskite oxide thin films by using brownmillerite SrCoO2.5 as a sacrificial layer16Coordination Tailoring of Epitaxial Perovskite-Derived Iron Oxide Films for Efficient Water Oxidation Electrocatalysis23Topotactic Transition: A Promising Opportunity for Creating New Oxides44Modulation of Exchange Bias in La0.35Sr0.65MnO3/La0.7Sr0.3MnO3 through Volatile Polarization of P(VDF‐TrFE) Gate Dielectric3Protonation-Induced Colossal Lattice Expansion in La2/3Sr1/3MnO34Highly efficient and fast modulation of magnetic coupling interaction in the SrCoO 2.5 /La 0.7 Ca 0.3 MnO 3 heterostructure0Topotactic transformation of perovskite-based manganite film triggered via simple oxygen getter layer0Strain-Induced Uphill Hydrogen Distribution in Perovskite Oxide Films12Intercalation of functional materials with phase transitions for neuromorphic applications6Recent advances in multi-field manipulations of the metal–insulator transition in correlated vanadium oxides enabling interdisciplinary applications6Above 400 K robust ferromagnetic insulating phase in hydrogenated brownmillerite iron oxide films with distinct coordinate2Topotactic Reduction‐Driven Crystal Field Excitations in Brownmillerite Manganite Thin Films2Quasi–two-dimensional ferroelectricity with multiple switchable polarization states in N-H coinjected perovskite manganites5Reversible topotactic reduction induced metal–insulator transformations in La2/3Sr1/3MnO3 thin films0Topotactic Phase Transition in Epitaxial La 0.7 Sr 0.3 MnO 3‐δ Films Induced by Oxygen Getter Assisted Thermal Annealing0Interface-engineered oxygen vacancy channels in epitaxial brownmillerite manganite films0Asymmetric oxygen displacement-induced contrast modulation and multi-state ferroelectricity in distorted perovskite oxides1Reduction-mediated oxidation and new topotactic phase transition in SrCoOx0Reversible On–Off Switching of Chirality via Electrochemical Intercalation Control of Enantiopure Molecular Cations in a Layered van der Waals Material0Electrochemical Proton Injection Induced Phase Transitions in Hydrothermally Synthesized A-Site Multi-doped Manganate Perovskites1

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  1. Topotactic fluorination induced stable structure and tunable electronic transport in perovskite barium ferrite thin films

    Ceramics International · 2019-12-16

    Junjie Li, Haoliang Huang, Peiqi Qiu, Zhaolong Liao, Xierong Zeng, Yalin Lu, Chuanwei Huang

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  2. Defects in complex oxide thin films for electronics and energy applications: challenges and opportunities

    Materials Horizons · 2020-01-01

    Weiwei Li, Jueli Shi, Kelvin H. L. Zhang, Judith L. MacManus‐Driscoll

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  3. Nanoscale Phase Mixture and Multifield-Induced Topotactic Phase Transformation in SrFeOx

    ACS Applied Materials & Interfaces · 2020-04-21

    Junjiang Tian, Yang Zhang, Zhen Hong Fan, Haijun Wu, Lei Zhao, Jingjing Rao, Zuhuang Chen, Haizhong Guo, Xubing Lu, Guofu Zhou, Stephen John Pennycook, Xingsen Gao, Jun‐Ming Liu

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  4. Hydrogen Control of Double Exchange Interaction in La0.67Sr0.33MnO3 for Ionic–Electric–Magnetic Coupled Applications

    Advanced Materials · 2021-02-12

    Jae‐Hyun Lee, Youngkyoung Ha, Shinbuhm Lee

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  5. Hydrogenation driven structural transformation and adjustable electronic properties of epitaxial La0.3Sr0.7MnO3− δ films

    Applied Physics Letters · 2021-03-01

    Dun Jin, Sixia Hu, Haoliang Huang, Peiqi Qiu, Yalin Lu, Xierong Zeng, Haiping Zhou, Xiaohua Li, Chuanwei Huang

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  6. Doping-Enabled Reconfigurable Strongly Correlated Phase in a Quasi-2D Perovskite

    The Journal of Physical Chemistry Letters · 2021-05-24

    Lifu Zhang, Jie Jiang, Yao Cai, Shukai Yao, Bilal Azhar, Zhizhong Chen, Yang Hu, Saloni Pendse, Yuwei Guo, Ru Jia, Zhiting Tian, Chengliang Sun, Peilin Liao, Jian Zhong Shi

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  7. Metal–Insulator Transition via Ion Irradiation in Epitaxial La0.7Sr0.3MnO3−δ Thin Films

    physica status solidi (RRL) - Rapid Research Letters · 2021-07-27

    Lei Cao, Andreas Herklotz, Diana Rata, Chenyang Yin, O. Petracic, Ulrich Kentsch, M. Helm, Shengqiang Zhou

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  8. Surface De-Fluorination and Bond Modification of CFx by High-Density Hydrogen Plasma Processing

    ACS Applied Energy Materials · 2021-08-11

    Guotao Chen, Haiping Zhou, Shu Zhang, Zidong Zhang, Tingting Feng, Ziqiang Xu, Mengqiang Wu

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  9. High‐Conductive Protonated Layered Oxides from H2O Vapor‐Annealed Brownmillerites

    Advanced Materials · 2021-09-29

    Songbai Hu, Yuanmin Zhu, Wenqiao Han, Xiaowen Li, Yanjiang Ji, Mao Ye, Jin Hui Cai, Qi Liu, Sixia Hu, Jiaou Wang, Junling Wang, Jiaqing He, Claudio Cazorla, Lang Chen

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  10. Symmetry-aware recursive image similarity exploration for materials microscopy

    npj Computational Materials · 2021-10-08

    Tri Nguyen, Yichen Guo, Shuyu Qin, Kylie S. Frew, Ruijuan Xu, Joshua Agar

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  11. Migration Kinetics of Surface Ions in Oxygen‐Deficient Perovskite During Topotactic Transitions

    Small · 2021-11-17

    Lei Cao, O. Petracic, Xian‐Kui Wei, Hengbo Zhang, Tomáš Duchoň, Felix Gunkel, Alexandros G. Koutsioubas, Kirill Zhernenkov, Konstantin Z. Rushchanskii, Heinrich Hartmann, Marek Wilhelm, Zichao Li, Yufang Xie, Suqin He, Moritz Lukas Weber, Kateřina Veltruská, Annika Stellhorn, Joachim Mayer, Shengqiang Zhou, Thomas Brückel

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  12. Exploring the Spatial Control of Topotactic Phase Transitions Using Vertically Oriented Epitaxial Interfaces

    Nano-Micro Letters · 2021-12-02

    Wenrui Zhang, Jie Zhang, Shaobo Cheng, Christopher M. Rouleau, Kim Kisslinger, Lihua Zhang, Yimei Zhu, Thomas Zac Ward, Gyula Eres

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  13. Epitaxial growth of metastable La0.67Sr0.33MnO3−δ films by using Sr3Al2O6 as multifunctional buffer layers

    Journal of Vacuum Science & Technology A Vacuum Surfaces and Films · 2021-12-28

    Yanhan Fang, Wenjie Sun, Lu Han, Zeya Li, Haoying Sun, Hongtao Yuan, Zhengbin Gu, Yuefeng Nie

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  14. Comparison of topotactic and magnetic structures for manganite oxide films

    Ceramics International · 2022-01-17

    Yukuai Liu, Sixia Hu, Boyang Zhao, Xinrong Shi, Xiezong Zeng, Chi Wah Leung, Chuanwei Huang

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  15. Reversible Hydrogen-Induced Phase Transformations in La0.7Sr0.3MnO3 Thin Films Characterized by In Situ Neutron Reflectometry

    ACS Applied Materials & Interfaces · 2022-02-16

    Alessandro R. Mazza, Qiyang Lu, Guoxiang Hu, Haoxiang Li, James F. Browning, Timothy Randall Charlton, Matthew Brahlek, Panchapakesan Ganesh, Thomas Zac Ward, Ho Nyung Lee, Gyula Eres

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  16. Morphologically and chemically regulated 3D carbon for Dendrite-free lithium metal anodes by a plasma processing

    Journal of Colloid and Interface Science · 2022-03-29

    Haiping Zhou, Hao Zhang, Zidong Zhang, Jian Wei Yang, Shu Zhang, Tingting Feng, Ziqiang Xu, Mengqiang Wu

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  17. Converting Brownmillerite to Alternate Layers of Oxygen‐Deficient and Conductive Nano‐Sheets with Enhanced Thermoelectric Properties

    Advanced Energy Materials · 2022-06-11

    Songbai Hu, Wenqiao Han, Xiaowen Li, Mao Ye, Yao Lu, Jin Hui Cai, Qi Liu, Junling Wang, Jiaqing He, Claudio Cazorla, Yuanmin Zhu, Lang Chen

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  18. Plasma-enhanced fluorination of multi-walled carbon nanotubes for CFx cathode materials with ultrahigh electrochemical performance

    Applied Physics Letters · 2022-07-11

    Haiping Zhou, L.S. Yao, G.T. Chen, S. Zhang, Tingting Feng, Ziqiang Xu, Mengqiang Wu

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  19. Highly-conductive Cu-substituted brownmillerite with emergent 3-dimensional oxygen vacancy channels

    Journal of Materials Chemistry C · 2023-01-01

    Wenqiao Han, Songbai Hu, Xiaowen Li, Qi Liu, Mao Ye, Zedong Xu, Sixia Hu, Yuanmin Zhu, Lang Chen

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  20. Orbital polarization change and magnetic enhancement in rutile MnO2-δ epitaxial films

    Applied Surface Science · 2023-02-04

    Wenyi Liu, Haoliang Huang, Shuming Zeng, Haiping Zhou, Liang Xi Xie, Zhongyuan Jiang, Jian Zhang, Lenan Wang, Jianlin Wang, Qiuping Huang, Zhengping Fu, Yusong Tu, Yalin Lu

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  21. Synthesis of freestanding perovskite oxide thin films by using brownmillerite SrCoO2.5 as a sacrificial layer

    Applied Physics Letters · 2023-02-06

    Weikun Zhou, Wenqiao Han, Yihao Yang, Liang Shu, Qinggui Luo, Yanjiang Ji, Jin Hui Cai, Yingli Zhang, Jiahao Song, Mao Ye, Qi Liu, Songbai Hu, Lang Chen

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  22. Coordination Tailoring of Epitaxial Perovskite-Derived Iron Oxide Films for Efficient Water Oxidation Electrocatalysis

    ACS Catalysis · 2023-02-08

    Zhuanglin Weng, Haoliang Huang, Xiaowen Li, Yihao Zhang, Ruiwen Shao, Yazhuo Yi, Yalin Lu, Xierong Zeng, Jizhao Zou, Lang Chen, Wei Li, Yuying Meng, Tewodros Asefa, Chuanwei Huang

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  23. Topotactic Transition: A Promising Opportunity for Creating New Oxides

    Advanced Functional Materials · 2023-06-15

    Ziang Meng, Han Yan, Peixin Qin, Xiaorong Zhou, Xiaoning Wang, Hongyu Chen, Li Liu, Zhiqi Liu

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  24. Modulation of Exchange Bias in La0.35Sr0.65MnO3/La0.7Sr0.3MnO3 through Volatile Polarization of P(VDF‐TrFE) Gate Dielectric

    Advanced Materials Interfaces · 2023-07-20

    Xu Zhao, Hon Fai Wong, Yukuai Liu, Sheung Mei Ng, Min Gan, Lok Wing Wong, Jiong Xin Zhao, Zongrong Wang, Wang Fai Cheng, Chuanwei Huang, Linfeng Fei, Chee Leung Mak, Chi Wah Leung

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  25. Protonation-Induced Colossal Lattice Expansion in La2/3Sr1/3MnO3

    ACS Applied Materials & Interfaces · 2023-11-28

    Muhammad Umer Fayaz, Qian Wang, Shixuan Liang, Lei Han, Feng Pan, Cheng Song

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  26. Highly efficient and fast modulation of magnetic coupling interaction in the SrCoO 2.5 /La 0.7 Ca 0.3 MnO 3 heterostructure

    Physical Chemistry Chemical Physics · 2024-01-01

    Huihui Ji, Siqi Wang, Guowei Zhou, Xuanchi Zhou, Jiarui Dou, Penghua Kang, Jingsheng Chen, Xiaohong Xu

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  27. Topotactic transformation of perovskite-based manganite film triggered via simple oxygen getter layer

    Ceramics International · 2024-01-09

    Qiaoqi Cen, Xi Zhang, Jiazhi Peng, Xierong Zeng, Chuanwei Huang

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  28. Strain-Induced Uphill Hydrogen Distribution in Perovskite Oxide Films

    ACS Applied Materials & Interfaces · 2024-01-10

    Qian Wang, Youdi Gu, Chong Chen, Lei Han, Muhammad Umer Fayaz, Feng Pan, Cheng Song

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  29. Intercalation of functional materials with phase transitions for neuromorphic applications

    Matter · 2025-01-01

    Xin He, Hua Wang, Jian Dong Sun, Xixiang Zhang, Kai Chang, Fei Xue

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  30. Recent advances in multi-field manipulations of the metal–insulator transition in correlated vanadium oxides enabling interdisciplinary applications

    Journal of Materials Chemistry C · 2025-01-01

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  31. Above 400 K robust ferromagnetic insulating phase in hydrogenated brownmillerite iron oxide films with distinct coordinate

    Applied Physics Reviews · 2025-02-13

    Jiahui Ou, Haiping Zhou, Haoliang Huang, Feng Rao, Xierong Zeng, Lang Chen, Ruiwen Shao, Man-Yi Duan, Chuanwei Huang

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  32. Topotactic Reduction‐Driven Crystal Field Excitations in Brownmillerite Manganite Thin Films

    Advanced Functional Materials · 2025-02-19

    Feng Jin, Shiyu Fan, Mingqiang Gu, Qiming Lv, Min Ge, Zixun Zhang, Jinfeng Zhang, Jingdi Lu, Taehun Kim, Vivek Kumar Bhartiya, Zhen Huang, Lingfei Wang, Valentina Bisogni, Jonathan Pelliciari, Wenbin Wu

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  33. Quasi–two-dimensional ferroelectricity with multiple switchable polarization states in N-H coinjected perovskite manganites

    Science Advances · 2025-10-01

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  34. Reversible topotactic reduction induced metal–insulator transformations in La2/3Sr1/3MnO3 thin films

    Journal of Applied Physics · 2025-12-04

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  35. Topotactic Phase Transition in Epitaxial La 0.7 Sr 0.3 MnO 3‐δ Films Induced by Oxygen Getter Assisted Thermal Annealing

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  36. Interface-engineered oxygen vacancy channels in epitaxial brownmillerite manganite films

    Physical Review Materials · 2025-12-10

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  37. Asymmetric oxygen displacement-induced contrast modulation and multi-state ferroelectricity in distorted perovskite oxides

    Applied Physics Reviews · 2026-02-02

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  38. Reduction-mediated oxidation and new topotactic phase transition in SrCoOx

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  39. Reversible On–Off Switching of Chirality via Electrochemical Intercalation Control of Enantiopure Molecular Cations in a Layered van der Waals Material

    ACS Nano · 2026-05-18

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  40. Electrochemical Proton Injection Induced Phase Transitions in Hydrothermally Synthesized A-Site Multi-doped Manganate Perovskites

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