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RESEARCH PAPER · Chemical Science · 2019

Frontiers and progress in cation-uptake and exchange chemistry of polyoxometalate-based compounds

Sayaka Uchida

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Frontiers and progress in cation-uptake and exchange chemistry of polyoxometalate-based compoundsOriginal{Mo72Fe30} Nanoclusters for the Visible-Light-Driven Photocatalytic Degradation of Organic Dyes31Application of polyoxometalate derivatives in rechargeable batteries133Isostructural mesoporous ionic crystals as a tunable platform for acid catalysis7Sustained release of Ag + confined inside polyoxometalates for long-lasting bacterial resistance43Self-Assembly and Properties of a Discrete Water-Soluble Prussian Blue Analogue FeII/CoIIICube: Confinement of a Water Molecule in Aqueous Solution12The Uptake of Hazardous Metal Ions into a High-Nuclearity Cluster-Based Compound with Structural Transformation and Proton Conduction19Amorphous High-Surface-Area Aluminum Hydroxide–Bicarbonates for Highly Efficient Methyl Orange Removal from Water16Two-Dimensional Supramolecular Ionic Frameworks for Precise Membrane Separation of Small Nanoparticles26Diaryl‐λ 3 ‐iodane Woven Supramolecular Architecture of Polyoxometalate3An Ultrastable, Small {Ag7}5+ Nanocluster within a Triangular Hollow Polyoxometalate Framework91An Ultrastable, Small {Ag7}5+ Nanocluster within a Triangular Hollow Polyoxometalate Framework23Cyclodextrin-Assisted Hierarchical Aggregation of Dawson-type Polyoxometalate in the Presence of {Re6Se8} Based Clusters25Cesium doped H3PW12O40 nanocrystalline thin films using single step hydrothermal route and its photoelectrochemical properties6Structure-function Relationships of Porous Ionic Crystals (PICs) Based on Polyoxometalate Anions and Oxo-centered Trinuclear Metal Carboxylates as Counter Cations25Polyoxometalate-Based Ionic Frameworks for Highly Selective CO 2 Capture and Separation42An octahedral polyoxomolybdate–organic molecular cage16A trapped hexaaqua Co II complex between the polyanionic sheets of decavanadate reveals high axial anisotropy and field induced SIM behaviour27Incorporating highly basic polyoxometalate anions comprising Nb or Ta into nanoscale reaction fields of porous ionic crystals24Integrating molecular design and crystal engineering approaches in non-humidified intermediate-temperature proton conductors based on a Dawson-type polyoxometalate and poly(ethylene glycol) derivatives30Minerals in biology and medicine25Preyssler-type polyoxometalate-based crystalline materials for the electrochemical detection of H 2 O 221Reductive silylation of polyoxovanadate surfaces using Mashima's reagent12Regulating the catalytic activity of multi-Ru-bridged polyoxometalates based on differential active site environments with six-coordinate geometry and five-coordinate geometry transitions34Formation of Mixed‐Valence Luminescent Silver Clusters via Cation‐Coupled Electron‐Transfer in a Redox‐Active Ionic Crystal Based on a Dawson‐type Polyoxometalate with Closed Pores7Ultrahigh Proton Conduction via Extended Hydrogen-Bonding Network in a Preyssler-Type Polyoxometalate-Based Framework Functionalized with a Lanthanide Ion58A Molecular Hybrid of an Atomically Precise Silver Nanocluster and Polyoxometalates for H 2 Cleavage into Protons and Electrons97A Molecular Hybrid of an Atomically Precise Silver Nanocluster and Polyoxometalates for H2 Cleavage into Protons and Electrons9Polyelectrolytes of Inorganic Polyoxometalates: Acids, Salts, and Complexes13Exploration of the Cs Trapping Phenomenon by Combining Graphene Oxide with α-K6P2W18O62 as Nanocomposite7A new route to polyoxometalates via mechanochemistry15Recent Advances on Polyoxometalate‐Based Ion‐Conducting Electrolytes for Energy‐Related Devices76All-Inorganic Zeolitic Octahedral Metal Oxides0Surface ligands influence the selectivity of cation uptake in polyoxovanadate–alkoxide clusters7Variable control of the electronic states of a silver nanocluster via protonation/deprotonation of polyoxometalate ligands36Crown‐Ether‐Based Cryptands with Rarely Strong Affinities for Binding Neutral Organic Molecules1Polyoxomolybdate Layered Crystals Constructed from a Heterocyclic Surfactant: Syntheses, Pseudopolymorphism and Introduction of Metal Cations4Proton conduction in ionic crystals based on polyoxometalates167High-capacity recovery of Cs+ ions by facilely synthesized layered vanadyl oxalatophosphates with the clear insight into remediation mechanism25Oxidation Catalysis over Solid-State Keggin-Type Phosphomolybdic Acid with Oxygen Defects72Proton-Conductive Crystals Based on Polyoxometalates0Removal of trace radioactive Cs+ by zirconium titanium phosphate: From bench-scale to pilot-scale24Polyoxocationic antimony oxide cluster with acidic protons12Giant Polyoxoniobate‐Based Inorganic Molecular Tweezers: Metal Recognitions, Ion‐Exchange Interactions and Mechanism Studies24Giant Polyoxoniobate‐Based Inorganic Molecular Tweezers: Metal Recognitions, Ion‐Exchange Interactions and Mechanism Studies4A redox-active inorganic crown ether based on a polyoxometalate capsule12Preparation of Zinc Ferrous Hydride on Diatomite Surface for Adsorption of Cs + From Solution0Research progress of POMs constructed by 1,3,5-benzene-tricarboxylic acid: From synthesis to application56Size‐Controlled Synthesis of Luminescent Few‐Atom Silver Clusters via Electron Transfer in Isostructural Redox‐Active Porous Ionic Crystals12New insight into polystyrene ion exchange resin for efficient cesium sequestration: The synergistic role of confined zirconium phosphate nanocrystalline36Metal–oxo-cluster-based crystals as solid catalysts30Photochromic Polyoxoniobates with Photoinduced “D‐f‐A” Electron Transfer Mechanism58Photochromic Polyoxoniobates with Photoinduced “D‐f‐A” Electron Transfer Mechanism5H8[PV5Mo7O40] – A Unique Polyoxometalate for Acid and RedOx Catalysis: Synthesis, Characterization, and Modern Applications in Green Chemical Processes37Investigating the Antiviral Properties of Copper- and Silver-containing Polyoxometalates Using a High-throughput Screening Method1Four New Terpyridine Complexes Based Polyoxometalates with [ W10O32 ]4– Anions as High‐Efficiency Dual‐Site Catalysis for Thioether Oxidation Reaction†7Reduction‐Induced Uptake of Cs+ in Metal–Organic Frameworks Loaded with Polyoxometalates11A Chromium-Incorporated All-Inorganic Polyoxoniobate Framework Material: Good Chemical Stability and Selective Ion Exchange Capability0Controlling the structural and adsorption features of polyoxovanadate-based metal–organic clusters by adjustable template effect15Keplerate polyoxometalate compounds: a multifunctional nano-platform for advanced materials9Small luminescent silver clusters stabilized in porous crystalline solids9Synthesis of polyoxothiometalates through site-selective post-editing sulfurization of polyoxometalates8Microstructure, adsorption site energetics, and formation enthalpy control for FAU-Zeolite Cs+ exchange10Preyssler-type polyoxometalates, smallest POM with internal cavity: Synthesis, structure and function18Inorganic‐Organic Hybrid Crystals Derived from Polyoxovanadate and Ionic‐Liquid toward Promising Conductive Materials4A chromium-incorporated all-inorganic polyoxoniobate framework material: Good chemical stability and selective ion exchange capability1Enhanced Electrical Conductivity of Polyoxometalates by Bridging with Mixed‐Valent Multinuclear Platinum Complexes0Enhanced Electrical Conductivity of Polyoxometalates by Bridging with Mixed‐Valent Multinuclear Platinum Complexes8Synthesis of a Gold–Silver Alloy Nanocluster within a Ring‐Shaped Polyoxometalate and Its Photocatalytic Property2Synthesis of a Gold–Silver Alloy Nanocluster within a Ring‐Shaped Polyoxometalate and Its Photocatalytic Property60Tuning Proton Conduction by Staggered Arrays of Polar Preyssler-Type Oxoclusters47Metastable layered lithium-rich niobium and tantalum oxides via nearly instantaneous cation exchange1Site differentiation strategy for selective strontium uptake and elution within an all-inorganic polyoxoniobate framework20Heteroatom Effect on Site-Selective Oxygen–Sulfur Substitution Reactions of Keggin-Type Polyoxotungstates5Enhanced Proton Conduction via Proton-Coupled Electron Transfer Reaction by a Keplerate-Type Polyoxometalate Capsule10Giant {Mo 132 } polyoxometalate isolated with diverse organic cations: a systematic proton conductivity study5Tailorable Ionic Frameworks for Selective Gas Adsorption and Separation: Bridging Experimental Insights with Mechanistic Understanding7Engineering cofacial porphyrin dimers using lacunary polyoxotungstates10High-performance Co 4 S 3 -MnS-MoS 2 @CC catalysts for the hydrogen evolution reaction9Ligand-directed top-down synthesis of trivacant lacunary polyoxomolybdates from plenary Keggin-type [α-XMo 12 O 40 ] 3− (X = P, As, V) in organic media3Synthesis of a Keggin-type polyoxoselenidotungstate via site-selective oxygen-to-selenium substitution6Emerging Functionalized Lindqvist‐Type Polyoxometalate‐Based Compounds: Design, Synthesis, and Applications12Ligand-directed bottom-up synthesis of trivacant lacunary polyoxomolybdates in organic media1Recent Advances in Polyoxometalate‒Metal Nanocluster Hybrids11A nickel-antimony cluster-substituted polyoxotungstate-based all-inorganic two-dimensional layered material: synthesis, structure, and properties0Efficient and selective adsorption of strategic metal In(III) from discarded waste leaching solution based on nanoconfinement-mediated zirconium phosphate10Elucidating ion capture and transport mechanisms of Preyssler anions in aqueous solutions using biased MACE-accelerated MD simulations1Properties of Polyoxometalates0Mechanistic Insights into Selective Cs + Adsorption and Exchange by Mo 72 Fe 30 Keplerate Capsules from Aqueous Solution0Solid-phase-based separation of transuranium elements: Current status and insights into the synergistic separation mechanism6In situ X-ray absorption and emission spectroscopy to understand the electron transfer–oxygen transfer reaction of vanadium polyoxomolybdate in a homogeneous medium0Polyoxometalates in environmental remediation and energy storage7Tungsten-Substituted α-Keggin Ammonium Phosphomolybdate [(NH4)3PWxMo12-xO40·nH2O]: A Multifunctional Adsorbent, Photocatalyst, and Cation Exchanger0Two “X”-shaped {Eu 6 }-embedded water-soluble heterometallic polyoxotungstates based on {Eu 6 M 4 WSe 4 (GeW 10 ) 4 } (M = Cr, Al) clusters with resistance-switching0α-Keggin-type Tungsten (W) Substituted Ammonium Phosphomolybdate [(NH4)3PWxMo12-xO40·nH2O]: A Multifunctional Adsorbent, Photocatalyst, and Cation Exchanger0Programming Structural Flexibility for Tunable Gas Sorption via Hydrogen Bonding in Polyoxometalate-Based Porous Ionic Crystals1Beyond Intrinsic Oxidation Activity: Charge-Distributed Reaction Fields in Polyoxometalate-Based Porous Ionic Crystals0Quantitative cation exchange in Anderson-type polyoxometalate hybrid polyelectrolytes: Structural evolution and ion-transport mechanism transition0

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  1. {Mo72Fe30} Nanoclusters for the Visible-Light-Driven Photocatalytic Degradation of Organic Dyes

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  2. Application of polyoxometalate derivatives in rechargeable batteries

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  3. Isostructural mesoporous ionic crystals as a tunable platform for acid catalysis

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  4. Sustained release of Ag + confined inside polyoxometalates for long-lasting bacterial resistance

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  5. Self-Assembly and Properties of a Discrete Water-Soluble Prussian Blue Analogue FeII/CoIIICube: Confinement of a Water Molecule in Aqueous Solution

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  7. Amorphous High-Surface-Area Aluminum Hydroxide–Bicarbonates for Highly Efficient Methyl Orange Removal from Water

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  9. Diaryl‐λ 3 ‐iodane Woven Supramolecular Architecture of Polyoxometalate

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  10. An Ultrastable, Small {Ag7}5+ Nanocluster within a Triangular Hollow Polyoxometalate Framework

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  11. An Ultrastable, Small {Ag7}5+ Nanocluster within a Triangular Hollow Polyoxometalate Framework

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  12. Cyclodextrin-Assisted Hierarchical Aggregation of Dawson-type Polyoxometalate in the Presence of {Re6Se8} Based Clusters

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  13. Cesium doped H3PW12O40 nanocrystalline thin films using single step hydrothermal route and its photoelectrochemical properties

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  14. Structure-function Relationships of Porous Ionic Crystals (PICs) Based on Polyoxometalate Anions and Oxo-centered Trinuclear Metal Carboxylates as Counter Cations

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  15. Polyoxometalate-Based Ionic Frameworks for Highly Selective CO 2 Capture and Separation

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  16. An octahedral polyoxomolybdate–organic molecular cage

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  17. A trapped hexaaqua Co II complex between the polyanionic sheets of decavanadate reveals high axial anisotropy and field induced SIM behaviour

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  18. Incorporating highly basic polyoxometalate anions comprising Nb or Ta into nanoscale reaction fields of porous ionic crystals

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  19. Integrating molecular design and crystal engineering approaches in non-humidified intermediate-temperature proton conductors based on a Dawson-type polyoxometalate and poly(ethylene glycol) derivatives

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  22. Reductive silylation of polyoxovanadate surfaces using Mashima's reagent

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  24. Formation of Mixed‐Valence Luminescent Silver Clusters via Cation‐Coupled Electron‐Transfer in a Redox‐Active Ionic Crystal Based on a Dawson‐type Polyoxometalate with Closed Pores

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  26. A Molecular Hybrid of an Atomically Precise Silver Nanocluster and Polyoxometalates for H 2 Cleavage into Protons and Electrons

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  29. Exploration of the Cs Trapping Phenomenon by Combining Graphene Oxide with α-K6P2W18O62 as Nanocomposite

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  30. A new route to polyoxometalates via mechanochemistry

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  31. Recent Advances on Polyoxometalate‐Based Ion‐Conducting Electrolytes for Energy‐Related Devices

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  32. All-Inorganic Zeolitic Octahedral Metal Oxides

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  33. Surface ligands influence the selectivity of cation uptake in polyoxovanadate–alkoxide clusters

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  34. Variable control of the electronic states of a silver nanocluster via protonation/deprotonation of polyoxometalate ligands

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  35. Crown‐Ether‐Based Cryptands with Rarely Strong Affinities for Binding Neutral Organic Molecules

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  36. Polyoxomolybdate Layered Crystals Constructed from a Heterocyclic Surfactant: Syntheses, Pseudopolymorphism and Introduction of Metal Cations

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  37. Proton conduction in ionic crystals based on polyoxometalates

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  38. High-capacity recovery of Cs+ ions by facilely synthesized layered vanadyl oxalatophosphates with the clear insight into remediation mechanism

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  39. Oxidation Catalysis over Solid-State Keggin-Type Phosphomolybdic Acid with Oxygen Defects

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  40. Proton-Conductive Crystals Based on Polyoxometalates

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  41. Removal of trace radioactive Cs+ by zirconium titanium phosphate: From bench-scale to pilot-scale

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  42. Polyoxocationic antimony oxide cluster with acidic protons

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  43. Giant Polyoxoniobate‐Based Inorganic Molecular Tweezers: Metal Recognitions, Ion‐Exchange Interactions and Mechanism Studies

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  45. A redox-active inorganic crown ether based on a polyoxometalate capsule

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  46. Preparation of Zinc Ferrous Hydride on Diatomite Surface for Adsorption of Cs + From Solution

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  47. Research progress of POMs constructed by 1,3,5-benzene-tricarboxylic acid: From synthesis to application

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  48. Size‐Controlled Synthesis of Luminescent Few‐Atom Silver Clusters via Electron Transfer in Isostructural Redox‐Active Porous Ionic Crystals

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  49. New insight into polystyrene ion exchange resin for efficient cesium sequestration: The synergistic role of confined zirconium phosphate nanocrystalline

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  50. Metal–oxo-cluster-based crystals as solid catalysts

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