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RESEARCH PAPER · Chemical Science · 2019

Metal-free perovskites for non linear optical materials

Thomas W. Kasel, Zeyu Deng, Austin M. Mroz, Christopher H. Hendon, Keith T. Butler, Pieremanuele Canepa

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Metal-free perovskites for non linear optical materialsOriginalExtraordinarily Large Electrocaloric Strength of Metal‐Free Perovskites68Understanding the Structural and Electronic Properties of Bismuth Trihalides and Related Compounds12Study on new quinacridone derivatives with enhanced third-order nonlinear optical properties8Harmonic generation at the nanoscale95Metal‐Free Halide Perovskite Single Crystals with Very Long Charge Lifetimes for Efficient X‐ray Imaging129Nonlinear optical properties of halide perovskites and their applications202Potassium L-ascorbate monohydrate: a new metal–organic nonlinear optical crystal6Metal‐Free Organic Halide Perovskite: A New Class for Next Optoelectronic Generation Devices64Strongly Coupled Systems for Nonlinear Optics57The structural phase transition of a metal-free perovskite (C4N2H12)(NH4I3)∙H2O0Photovoltaic properties of metal-free semiconductor DMEDA·I6: A first-principles investigation1Halide-modulated self-assembly of metal-free perovskite single crystals for bio-friendly X-ray detection92Advances in Lead-Free Perovskite Single Crystals: Fundamentals and Applications124Designed Giant Room‐Temperature Electrocaloric Effects in Metal‐Free Organic Perovskite [MDABCO](NH4)I3 by Phase–Field Simulations49Wide-Band-Gap Metal-Free Perovskite for Third-Order Nonlinear Optics26Highly Luminescent Metal‐Free Perovskite Single Crystal for Biocompatible X‐Ray Detector to Attain Highest Sensitivity102Multiple‐Ring Aromatic Spacer Cation Tailored Interlayer Interaction for Efficient and Air‐Stable Ruddlesden–Popper Perovskite Solar Cells8Giant room temperature elastocaloric effect in metal-free thin-film perovskites17Layered Metal‐Halide Perovskite Single‐Crystalline Microwire Arrays for Anisotropic Nonlinear Optics62Solid phase synthesis of metal-free perovskite crystalline materials15Synthetic Approaches Targeting Metal-Free Perovskite [HMDABCO](NH4)I3 Thin Films5Engineering hydrogen bonding to align molecular dipoles in organic solids for efficient second harmonic generation31Materials discovery and design limits in MDABCO perovskites5Toward Eco‐Friendly Lead‐Free Low‐Dimensional Perovskites13Structural and Functional Insights into Metal-Free Perovskites25Metal-free ferroelectric halide perovskite exhibits visible photoluminescence correlated with local ferroelectricity39A Review of Metal-Free Organic Halide Perovskite: Future Directions for the Next Generation of Solar Cells33Hybrid Germanium Bromide Perovskites with Tunable Second Harmonic Generation122Hybrid Germanium Bromide Perovskites with Tunable Second Harmonic Generation8Application of perovskites in bioimaging: the state-of-the-art and future developments12First-Principles Calculations to Investigate the Effect of Van der Waals Interactions on the Crystal and Electronic Structures of Tin-Based 0D Hybrid Perovskites65Piezocatalytic Techniques in Environmental Remediation58Piezocatalytic Techniques in Environmental Remediation227Lead-Free MDABCO-NH4I3 Perovskite Crystals Embedded in Electrospun Nanofibers13Phase diagrams, dielectric, and piezoelectric properties of metal-free perovskite thin films: Phase-field simulations6Introduction to perovskites4Hydrogen Bonds Strengthened Metal‐Free Perovskite for Degradable X‐ray Detector with Enhanced Stability, Flexibility and Sensitivity72Hydrogen Bonds Strengthened Metal‐Free Perovskite for Degradable X‐ray Detector with Enhanced Stability, Flexibility and Sensitivity1Recent Development of Halide Perovskite Materials and Devices for Ionizing Radiation Detection237Large Piezoelectric Response in a Metal-Free Three-Dimensional Perovskite Ferroelectric78Two-Dimensional Hybrid Dion–Jacobson Germanium Halide Perovskites58Large Enhancements in Optical and Piezoelectric Properties in Ferroelectric Zn1‐xMgxO Thin Films through Engineering Electronic and Ionic Anharmonicities18Metal‐Free Perovskites for X‐Ray Detection11A review on solution- and vapor-responsive sensors for the detection of phthalates10Terahertz Emission via Optical Rectification in a Metal-Free Perovskite Crystal3B-site substitution effects on the mechanical properties of halide perovskites [C 4 H 12 N 2 ][BCl 3 ]·H 2 O (B = NH 4 + ; K + )1First principles study on polarization and piezoelectric properties of group substitution regulated lead-free organic perovskite ferroelectrics0Strategically designed metal-free deep-ultraviolet birefringent crystals with superior optical properties18The past 10 years of molecular ferroelectrics: structures, design, and properties173Few-mode metal-free perovskite optical fiber with second-order optical nonlinearity7Molecularly thin, two-dimensional all-organic perovskites50Aminoazanium of A-site Cations in Metal-Free Halide Perovskite Single Crystals to Reduce Thermal Expansion for Efficient X-ray Detection11Metal-Free Perovskite Ferroelectrics with the Most Equivalent Polarization Axes40Advanced Materials for Energy Harvesting and Soft Robotics: Emerging Frontiers to Enhance Piezoelectric Performance and Functionality107Lead-free alternatives and toxicity mitigation strategies for sustainable perovskite solar cells: a critical review122The emergence of metal-free molecular perovskites: challenges and opportunities5Reversible colossal barocaloric effect in methylphosphonium tin bromide for room-temperature refrigeration7Femtosecond Laser Breaks the Lattice Symmetry and Induces Broadband Second Harmonic Generation in 3D Halide Perovskites6Polarization‐Selective Switchable Mode‐Locked Pulses in Fiber Lasers Based on Anisotropic Quasi‐2D Perovskites4Metal‐Free Perovskites for X‐Ray Detection and Imaging: Progress and Prospects5Diverse Perovskite Solar Cells: Progress, Challenges, and Perspectives74Femtosecond laser processing for the perovskite quantum dots: Mechanism, fabrication, and nanophotonic applications1Lead‐Free Perovskites for Piezoelectric–Triboelectric Energy Harvesting and Sensing Applications: A Comprehensive Review7无金属钙钛矿及其非线性光学特性与器件研究进展（特邀）1Dimensionality Engineering: A Pathway to Ferroelectric Halide Perovskites3Confinement of Organic–Inorganic Hybrid Perovskites within MOF Cavities for Synergistic Regulation of Third-Order Nonlinear Optics0Temperature-dependent evolution of electronic, optical, and surface electrical properties with phase transition mechanism in (C 4 H 9 NH 3 ) 2 (C 2 H 5 NH 3 ) 2 Pb 3 Br 100Improving the performance of lead-free perovskite solar cells2Synergistic Effect of Chirality and Symmetry Reduction Enables Metal‐Free Perovskite Single Crystal With Stable Self‐Driven X‐ray Detection0Synergistic Effect of Chirality and Symmetry Reduction Enables Metal‐Free Perovskite Single Crystal With Stable Self‐Driven X‐ray Detection0

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  1. Extraordinarily Large Electrocaloric Strength of Metal‐Free Perovskites

    Advanced Materials · 2019-12-27

    Jianjun Wang, Daniel Fortino, Bo Wang, Xinye Zhao, Long‐Qing Chen

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  2. Understanding the Structural and Electronic Properties of Bismuth Trihalides and Related Compounds

    Inorganic Chemistry · 2020-01-28

    Zeyu Deng, Fengxia Wei, Yue Wu, Ram Seshadri, Anthony Kevin Cheetham, Pieremanuele Canepa

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  3. Study on new quinacridone derivatives with enhanced third-order nonlinear optical properties

    Tetrahedron · 2020-04-10

    Yanhong Cui, Guanqiu Liang, Jianhong Jia, Guoyi Yu, Yangcheng Sha, Chunsong Zhou, Yuanbin She

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  4. Harmonic generation at the nanoscale

    Journal of Applied Physics · 2020-06-15

    Luigi Bonacina, Pierre‐François Brevet, Marco Finazzi, Michele Celebrano

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  5. Metal‐Free Halide Perovskite Single Crystals with Very Long Charge Lifetimes for Efficient X‐ray Imaging

    Advanced Materials · 2020-09-15

    Xin Li Song, Qingyue Cui, Yucheng Liu, Zhuo Xu, Hagai Cohen, Chuang Ma, Yuanyuan Fan, Yunxia Zhang, Haochen Ye, Zhanhui Peng, Ruipeng Li, Yonghua Chen, Jianpu Wang, Huaming Sun, Zhou Yang, Zhike Liu, Zupei Yang, Wei Huang, Gary Hodes, Shengzhong Frank Liu, Kui Zhao

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  6. Nonlinear optical properties of halide perovskites and their applications

    Applied Physics Reviews · 2020-12-01

    Yixuan Zhou, Yuanyuan Huang, Xinlong Xu, Zeyu Fan, Jacob B. Khurgin, Qihua Xiong

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  7. Potassium L-ascorbate monohydrate: a new metal–organic nonlinear optical crystal

    Applied Physics B · 2021-01-01

    Dhanpal Bairwa, K. Raghavendra Rao, Diptikanta Swain, Tayur N. Guru Row, H. L. Bhat, Suja Elizabeth

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  8. Metal‐Free Organic Halide Perovskite: A New Class for Next Optoelectronic Generation Devices

    Advanced Energy Materials · 2021-01-29

    Xin Li Song, Gary Hodes, Kui Zhao, Shengzhong Frank Liu

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  9. Strongly Coupled Systems for Nonlinear Optics

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  10. The structural phase transition of a metal-free perovskite (C4N2H12)(NH4I3)∙H2O

    Inorganic Chemistry Communications · 2021-03-07

    Lin-Sui Li, Hongqiang Gao, Shisi Liu, Liting Shi, Wen‐Juan Wei, Yu‐Hui Tan

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  11. Photovoltaic properties of metal-free semiconductor DMEDA·I6: A first-principles investigation

    Materials Research Express · 2021-03-22

    Fuxiang Liu, Peng Xu

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  12. Halide-modulated self-assembly of metal-free perovskite single crystals for bio-friendly X-ray detection

    Matter · 2021-06-14

    Qingyue Cui, Xin Li Song, Yucheng Liu, Zhuo Xu, Haochen Ye, Zhou Yang, Kui Zhao, Shengzhong Frank Liu

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  13. Advances in Lead-Free Perovskite Single Crystals: Fundamentals and Applications

    ACS Materials Letters · 2021-06-21

    Naveen Kumar Tailor, Shaoni Kar, Pranjal Mishra, Albert These, Christian Kupfer, Hanlin Hu, Muhammad Awais, Makhsud I. Saidaminov, M. Ibrahim Dar, Christoph Josef Brabec, Soumitra Satapathi

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  14. Designed Giant Room‐Temperature Electrocaloric Effects in Metal‐Free Organic Perovskite [MDABCO](NH4)I3 by Phase–Field Simulations

    Advanced Functional Materials · 2021-06-29

    Rongzhen Gao, Xiaoming Shi, Jing Wang, Guangzu Zhang, Houbing Huang

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  15. Wide-Band-Gap Metal-Free Perovskite for Third-Order Nonlinear Optics

    ACS Photonics · 2021-07-14

    Dumitru Sirbu, Hei Chit Leo Tsui, Naseem Alsaif, Susana Iglesias-Porras, Yifeng Zhang, Ming Wang, Mingzhen Liu, Anna C. Peacock, Pablo Docampo, N. Healy

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  16. Highly Luminescent Metal‐Free Perovskite Single Crystal for Biocompatible X‐Ray Detector to Attain Highest Sensitivity

    Advanced Materials · 2021-07-26

    Xin Li Song, Qian Li, Han Jiang, Chuang Ma, Zhuo Xu, Haojin Li, Peijun Wang, Zhou Yang, Qingyue Cui, Lili Gao, Zewei Quan, Shengzhong Frank Liu, Kui Zhao

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  17. Multiple‐Ring Aromatic Spacer Cation Tailored Interlayer Interaction for Efficient and Air‐Stable Ruddlesden–Popper Perovskite Solar Cells

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    Chang Liu, Rui Liu, Zhuoneng Bi, Yue Yu, Gang Xu, Hongming Hou, Qiaofeng Wu, Hua Yu, Xueqing Xu

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  18. Giant room temperature elastocaloric effect in metal-free thin-film perovskites

    npj Computational Materials · 2021-08-16

    Cheng Li, Yu Huang, Jianjun Wang, Bo Wang, Yong Jun Wu, He Tian, Long‐Qing Chen, Zijian Hong

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  19. Layered Metal‐Halide Perovskite Single‐Crystalline Microwire Arrays for Anisotropic Nonlinear Optics

    Advanced Functional Materials · 2021-08-28

    Jinjin Zhao, Yingjie Zhao, Yangwu Guo, Xiuqin Zhan, Jiangang Feng, Yue Geng, Meng Yuan, Xin Hui Fan, Hanfei Gao, Lei Jiang, Yongli Yan, Yuchen Wu

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  20. Solid phase synthesis of metal-free perovskite crystalline materials

    Journal of Solid State Chemistry · 2021-08-28

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  21. Synthetic Approaches Targeting Metal-Free Perovskite [HMDABCO](NH4)I3 Thin Films

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  22. Engineering hydrogen bonding to align molecular dipoles in organic solids for efficient second harmonic generation

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  23. Materials discovery and design limits in MDABCO perovskites

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  24. Toward Eco‐Friendly Lead‐Free Low‐Dimensional Perovskites

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  25. Structural and Functional Insights into Metal-Free Perovskites

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  26. Metal-free ferroelectric halide perovskite exhibits visible photoluminescence correlated with local ferroelectricity

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  27. A Review of Metal-Free Organic Halide Perovskite: Future Directions for the Next Generation of Solar Cells

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  28. Hybrid Germanium Bromide Perovskites with Tunable Second Harmonic Generation

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  29. Hybrid Germanium Bromide Perovskites with Tunable Second Harmonic Generation

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  30. Application of perovskites in bioimaging: the state-of-the-art and future developments

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  31. First-Principles Calculations to Investigate the Effect of Van der Waals Interactions on the Crystal and Electronic Structures of Tin-Based 0D Hybrid Perovskites

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  32. Piezocatalytic Techniques in Environmental Remediation

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  34. Lead-Free MDABCO-NH4I3 Perovskite Crystals Embedded in Electrospun Nanofibers

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  35. Phase diagrams, dielectric, and piezoelectric properties of metal-free perovskite thin films: Phase-field simulations

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  36. Introduction to perovskites

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  37. Hydrogen Bonds Strengthened Metal‐Free Perovskite for Degradable X‐ray Detector with Enhanced Stability, Flexibility and Sensitivity

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  38. Hydrogen Bonds Strengthened Metal‐Free Perovskite for Degradable X‐ray Detector with Enhanced Stability, Flexibility and Sensitivity

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  39. Recent Development of Halide Perovskite Materials and Devices for Ionizing Radiation Detection

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  40. Large Piezoelectric Response in a Metal-Free Three-Dimensional Perovskite Ferroelectric

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  41. Two-Dimensional Hybrid Dion–Jacobson Germanium Halide Perovskites

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  42. Large Enhancements in Optical and Piezoelectric Properties in Ferroelectric Zn1‐xMgxO Thin Films through Engineering Electronic and Ionic Anharmonicities

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  43. Metal‐Free Perovskites for X‐Ray Detection

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  44. A review on solution- and vapor-responsive sensors for the detection of phthalates

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  45. Terahertz Emission via Optical Rectification in a Metal-Free Perovskite Crystal

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  46. B-site substitution effects on the mechanical properties of halide perovskites [C 4 H 12 N 2 ][BCl 3 ]·H 2 O (B = NH 4 + ; K + )

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  47. First principles study on polarization and piezoelectric properties of group substitution regulated lead-free organic perovskite ferroelectrics

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  48. Strategically designed metal-free deep-ultraviolet birefringent crystals with superior optical properties

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  49. The past 10 years of molecular ferroelectrics: structures, design, and properties

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  50. Few-mode metal-free perovskite optical fiber with second-order optical nonlinearity

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