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RESEARCH PAPER · Nature Communications · 2019

Harnessing liquid-in-liquid printing and micropatterned substrates to fabricate 3-dimensional all-liquid fluidic devices

Wenqian Feng, Yu Chai, Joe Forth, Paul D. Ashby, Thomas P. Russell, Brett A. Helms

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Harnessing liquid-in-liquid printing and micropatterned substrates to fabricate 3-dimensional all-liquid fluidic devicesOriginalProgrammable unidirectional liquid transport on peristome-mimetic surfaces under liquid environments31Microfluidic chip and its application in autophagy detection32Controllable Liquid-Liquid Printing with Defect-free, Corrosion-Resistance, Unrestricted Wetting Condition14Quantification of the binding preference of selected dyes at a solid-liquid interface in organized media0Self‐Assembly of Nanoparticles in 2D and 3D: Recent Advances and Future Trends63Compartmentalized, All-Aqueous Flow-Through-Coordinated Reaction Systems75Sculpting Liquids with Two-Dimensional Materials: The Assembly of Ti3C2Tx MXene Sheets at Liquid–Liquid Interfaces74Self‐Assembly of MXene‐Surfactants at Liquid–Liquid Interfaces: From Structured Liquids to 3D Aerogels234Self‐Assembly of MXene‐Surfactants at Liquid–Liquid Interfaces: From Structured Liquids to 3D Aerogels15Inner Surface Design of Functional Microchannels for Microscale Flow Control72Interfacial Assembly and Jamming of Polyelectrolyte Surfactants: A Simple Route To Print Liquids in Low-Viscosity Solution67Bijels the Easy Way0Under oil open-channel microfluidics empowered by exclusive liquid repellency52Photoresponsive Structured Liquids Enabled by Molecular Recognition at Liquid–Liquid Interfaces111Integrating self-assembly and biofabrication for the development of structures with enhanced complexity and hierarchical control58Rapid Multilevel Compartmentalization of Stable All-Aqueous Blastosomes by Interfacial Aqueous-Phase Separation37Perspective: Ferromagnetic Liquids10Bioinspired Robust All‐Aqueous Droplet via Diffusion‐Controlled Interfacial Coacervation27Nanoparticle surfactants and structured liquids37Freezing of axisymmetric liquid bridges14The future of sustainable chemistry and process: Convergence of artificial intelligence, data and hardware34Stabilizing Aqueous Three-Dimensional Printed Constructs Using Chitosan-Cellulose Nanocrystal Assemblies26Direct observation of nanoparticle-surfactant assembly and jamming at the water-oil interface87Nanoarchitectonics for Coordination Asymmetry and Related Chemistry100Under-Oil Autonomously Regulated Oxygen Microenvironments: A Goldilocks Principle-Based Approach For Microscale Cell Culture2Stabilizing liquid drops in nonequilibrium shapes by the interfacial crosslinking of nanoparticles21Growth Mechanism of Polymer Membranes Obtained by H-Bonding Across Immiscible Liquid Interfaces10Molding and Encoding Carbon Nitride-Containing Edible Oil Liquid Objects via Interfacial Toughening in Waterborne Systems10Visualizing Interfacial Jamming Using an Aggregation‐Induced‐Emission Molecular Reporter30Visualizing Interfacial Jamming Using an Aggregation‐Induced‐Emission Molecular Reporter5An interfacial self-assembling bioink for the manufacturing of capillary-like structures with tuneable and anisotropic permeability28Ferromagnetic liquid droplets with adjustable magnetic properties30Redox-Responsive, Reconfigurable All-Liquid Constructs76Host–Guest Molecular Recognition at Liquid–Liquid Interfaces404D Printing of Multi‐Stimuli Responsive Protein‐Based Hydrogels for Autonomous Shape Transformations158Interfacial Synthesis: Morphology, Structure, and Properties of Interfacial Formations in Liquid–Liquid Systems14Liquid‐Based Adaptive Structural Materials52Gated Molecular Diffusion at Liquid–Liquid Interfaces39Gated Molecular Diffusion at Liquid–Liquid Interfaces9Molecular Brush Surfactants: Versatile Emulsifiers for Stabilizing and Structuring Liquids14Molecular Brush Surfactants: Versatile Emulsifiers for Stabilizing and Structuring Liquids56The Buckling Spectra of Nanoparticle Surfactant Assemblies16Microfluidics on Standard Petri Dishes for Bioscientists8Responsive Interfacial Assemblies Based on Charge‐Transfer Interactions31Responsive Interfacial Assemblies Based on Charge‐Transfer Interactions11Layer‐by‐Layer Engineered All‐Liquid Microfluidic Chips for Enzyme Immobilization52Visualizing Assembly Dynamics of All‐Liquid 3D Architectures9Interfacial Assembly of Graphene Oxide: From Super Elastic Interfaces to Liquid‐in‐Liquid Printing27Microfluidics-Enabled Soft Manufacture of Materials with Tailorable Wettability120The Assembly and Jamming of Nanoparticle Surfactants at Liquid–Liquid Interfaces24The Assembly and Jamming of Nanoparticle Surfactants at Liquid–Liquid Interfaces41The advantages of nanoparticle surfactants over Janus nanoparticles on structuring liquids14Structuring of a Liquid in a Water–Lanthanide (or Nickel) Salt–D2EHPA–Diluent System0Under‐Oil Autonomously Regulated Oxygen Microenvironments: A Goldilocks Principle‐Based Approach for Microscale Cell Culture23Structured-Liquid Batteries30Thermocapillary convection in liquid-in-liquid capillary bridges due to a heating/cooling ring9Structured Ultra‐Flyweight Aerogels by Interfacial Complexation: Self‐Assembly Enabling Multiscale Designs31Dynamic Reconfiguration of Compressed 2D Nanoparticle Monolayers15Polyoxometalate‐Surfactant Assemblies: Responsiveness to Orthogonal Stimuli4Polyoxometalate‐Surfactant Assemblies: Responsiveness to Orthogonal Stimuli59Reconfigurable structured liquids21Rational Design and Construction of Monolithic Ordered Mesoporous Co 3 O 4 @SiO 2 Catalyst by a Novel 3D Printed Technology for Catalytic Oxidation of Toluene53Overflow Control for Sustainable Development by Superwetting Surface with Biomimetic Structure73Divide, Conquer, and Stabilize: Engineering Strong Fluid–Fluid Interfaces13Scaling Laws for Block Copolymer Surface Micelles6Spontaneous water-on-water spreading of polyelectrolyte membranes inspired by skin formation60All‐Aqueous Freeform Fabrication of Perfusable Self‐Standing Soft Compartments30Reconfigurable Liquids Constructed by Pillar[6]arene‐Based Nanoparticle Surfactants23Reconfigurable Liquids Constructed by Pillar[6]arene‐Based Nanoparticle Surfactants2Application of under-oil open microfluidic systems for rapid phenotypic antimicrobial susceptibility testing0Anisotropic Compartmentalization of the Liquid–Liquid Interface using Dynamic Imine Chemistry10Investigating water/oil interfaces with opto-thermophoresis21Shape-Reconfigurable Ferrofluids31Suppression of Filament Defects in Embedded 3D Printing48A Reactive Superhydrophobic Platform for Living Photolithography44Spongy all-in-liquid materials by in-situ formation of emulsions at oil-water interfaces31Aquabots26Simulated stress mitigation strategies in embedded bioprinting16All‐Liquid Reconfigurable Electronics Using Jammed MXene Interfaces25Stabilizing and structuring oil–oil interfaces by molecular brush surfactants16Interfacial Assembly and Jamming of Soft Nanoparticle Surfactants into Colloidosomes and Structured Liquids21Under-oil open microfluidic systems for rapid phenotypic antimicrobial susceptibility testing20Experimental investigation of the sedimentation behavior of metal droplets in liquid–liquid systems3Associative Liquid‐In‐Liquid 3D Printing Techniques for Freeform Fabrication of Soft Matter39Probing the Mechanism of Targeted Delivery of Molecular Surfactants Loaded into Nanoparticles after Their Assembly at Oil–Water Interfaces14Liquid-embedded (bio)printing of alginate-free, standalone, ultrafine, and ultrathin-walled cannular structures61Interfacial Polyelectrolyte Complexation-Inspired Bioprinting of Vascular Constructs12Reactive Superhydrophobic Surfaces for Interlayer Electrical Connectivity in Three‐dimensional Electronics12Reactive Superhydrophobic Surfaces for Interlayer Electrical Connectivity in Three‐dimensional Electronics0Bioinspired Superwetting Open Microfluidics: From Concepts, Phenomena to Applications61Liquid sculpture and curing of bio-inspired polyelectrolyte aqueous two-phase systems29A multimaterial 3D printing-assisted micropatterning for heat dissipation applications33Stabilizing Liquids Using Interfacial Supramolecular Assemblies26Stabilizing Liquids Using Interfacial Supramolecular Assemblies3Open millifluidics based on powder-encased channels27Structuring liquids through solvent-assisted interfacial association of oppositely charged polyelectrolytes and amphiphiles4Recent advances in organic solar cells: materials, design, and performance35Liquid-in-liquid printing of 3D and mechanically tunable conductive hydrogels154Bottlebrush Polymers at Liquid Interfaces: Assembly Dynamics, Mechanical Properties, and All-Liquid Printed Constructs48Liquid‐Templating Aerogels53Jamming of Miscible Liquids via Electrostatic Repulsion Between Polystyrene‐Modified Gold Nanorods and Toluene1Rapid plasma membrane isolation via intracellular polymerization-mediated biomolecular confinement12Functional Janus structured liquids and aerogels56Self-assembly of nanoparticles with stimulated responses at liquid interfaces30In Situ 4D Printing of Polyelectrolyte/Magnetic Composites for Sutureless Gastric Perforation Sealing18AIE‐Switching and Enantioselective Reactivity at Jammed Liquid‐Liquid Interface3Self-Assembly of Polyoxometalate-Based Nanoparticle Surfactants in Solutions6Rod‐Shaped Liquid Plasticine as Cuttable Minireactor for Photodynamic Therapy of Tumors9Transient structuring of liquids using dissipative interfacial assemblies3Interfacial jamming of surface-alkylated synthetic nanocelluloses for structuring liquids10Reconfigurable liquid devices from liquid building blocks27Visualization-enhanced under-oil open microfluidic system for in situ characterization of multi-phase chemical reactions15Reconfiguring liquid devices0Vascular network-inspired fluidic system (VasFluidics) with spatially functionalizable membranous walls22Highly Interfacial Active Gemini Surfactants as Simple and Versatile Emulsifiers for Stabilizing, Lubricating and Structuring Liquids0Highly Interfacial Active Gemini Surfactants as Simple and Versatile Emulsifiers for Stabilizing, Lubricating and Structuring Liquids37Thermal Welding of Liquids15Nano-enabled smart and functional materials toward human well-being and sustainable developments15Building Functional Liquid‐Based Interfaces: From Mechanism to Application14Building Functional Liquid‐Based Interfaces: From Mechanism to Application1Optical Actuation of Nanoparticle-Loaded Liquid–Liquid Interfaces for Active Photonics3Reconfigurable liquids enabled by dynamic covalent chemistry10Responsive‐Hydrogel Aquabots9Reconfigurable All‐Oil Microfluidic Devices by 3D Printing5Chaperone solvent-assisted assembly of polymers at the interface of two immiscible liquids14A review on the rapid liquid printing (RLP): future 3D printing technology5All‐Aqueous Embedded 3D Printing for Freeform Fabrication of Biomimetic 3D Constructs21A Simple Route for Open Fluidic Devices with Particle Walls26Recent Advances of Stimuli-Responsive Liquid–Liquid Interfaces Stabilized by Nanoparticles22Droplet-templating soft materials into structured bead-based aerogels with compartmentalized or welded configurations3Multifunctional all-liquid microfluidic devices stabilized with molecular brush surfactants1Confinement by Liquid‐Liquid Interface Replicates In Vivo Neutrophil Deformations and Elicits Bleb‐Based Migration9Shape-recovering liquids5Immobilization strategies for heterogeneous catalysts in micro flow chemistry: Key techniques for efficient and sustainable chemical transformations13Capillary-assisted printing of droplets at a solid-like liquid-liquid interface7Engineering Morphologies of Metal‐Based Colloidal Assemblies via Colloid Jamming at Liquid–Liquid Interfaces0Surfactant Assemblies Directing Chemical Transfer Cascades in Convective Marangoni Flow Pumps2Nanopatterning of Liquid–Liquid Interfaces by Mikto-Grafted Molecular Brush Polymers9Fast and High‐Angle‐Climbing Capable Self‐Driven Surface Directional Liquid Transport via Bio‐Inspired Eccentric Channels2Processing soft thin films on liquid surface for seamless creation of on-liquid walkable devices2Emerging Selective Ion Transport via 2D Confined Space for the Innovations in Separation and Energy Technologies14Modeling for nanoparticle-stabilized, robust small-domain bicontinuous emulsions1Liquid-in-liquid printing and machine learning assisting the achievement of omni-directional, self-encapsulated flexible strain sensors0Hierarchical assembly of mixed 2D surfactants in polyHIPEs: tuning conductive networks through multi-scale structuring2Solvent-Controlled Formation of Arrested Polyelectrolyte–Surfactant Interfacial Assemblies and Their Impact on Emulsion Stability0Reconfiguring Liquid Shapes Using Lignin Nanoparticles2In Situ Imaging of Nanorod Adsorption and Assembly at Liquid Surfaces0Adaptive horizons in 4D printing: stimuli-responsive materials, computational intelligence, biomedical translation, and sustainable futures0

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  46. Layer‐by‐Layer Engineered All‐Liquid Microfluidic Chips for Enzyme Immobilization

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  49. Microfluidics-Enabled Soft Manufacture of Materials with Tailorable Wettability

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  50. The Assembly and Jamming of Nanoparticle Surfactants at Liquid–Liquid Interfaces

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