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RESEARCH PAPER · ACS Catalysis · 2019

A Highly Active and Redox-Stable SrGdNi 0.2 Mn 0.8 O 4±δ Anode with in Situ Exsolution of Nanocatalysts

Kyeong Joon Kim, Manasa Kumar Rath, Hunho H. Kwak, Hyung Jun Kim, Jeong Woo Han, Seung‐Tae Hong, Kang Taek Lee

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A Highly Active and Redox-Stable SrGdNi 0.2 Mn 0.8 O 4±δ Anode with in Situ Exsolution of NanocatalystsOriginalHigh performance Mn 1.3 Co 1.3 Cu 0.4 O 4 spinel based composite cathodes for intermediate temperature solid oxide fuel cells51Phase transition of doped LaFeO3 anode in reducing atmosphere and their power generation property in intermediate temperature solid oxide fuel cell24Vanadium-Doped Strontium Molybdate with Exsolved Ni Nanoparticles as Anode Material for Solid Oxide Fuel Cells38Design of Ceria Catalysts for Low‐Temperature CO Oxidation129Novel anode current collector for hydrocarbon fuel solid oxide fuel cells14Symmetrical Exsolution of Rh Nanoparticles in Solid Oxide Cells for Efficient Syngas Production from Greenhouse Gases91In Situ Investigation of Reversible Exsolution/Dissolution of CoFe Alloy Nanoparticles in a Co‐Doped Sr 2 Fe 1.5 Mo 0.5 O 6− δ Cathode for CO 2 Electrolysis340Ruddlesden–Popper perovskites in electrocatalysis330A-site deficient perovskite with nano-socketed Ni-Fe alloy particles as highly active and durable catalyst for high-temperature CO2 electrolysis65Progress and Opportunities for Exsolution in Electrochemistry26In situ embedding of CoFe nanocatalysts into Sr3FeMoO7 matrix as high-performance anode materials for solid oxide fuel cells53Review on exsolution and its driving forces in perovskites138Exceptional Tunability over Size and Density of Spontaneously Formed Nanoparticles via Nucleation Dynamics38Computational approaches to the exsolution phenomenon in perovskite oxides with a view to design highly durable and active anodes for solid oxide fuel cells13Ultra-fast fabrication of anode-supported solid oxide fuel cells via microwave-assisted sintering technology7In-situ exsolved NiFe alloy nanoparticles on Pr0.8Sr1.2(NiFe)O4-δ for direct hydrocarbon fuel solid oxide fuel cells35A highly active and carbon-tolerant anode decorated with in situ grown cobalt nano-catalyst for intermediate-temperature solid oxide fuel cells88Efficient bifunctional electrocatalysts for solid oxide cells based on the structural evolution of perovskites with abundant defects and exsolved CoFe nanoparticles72Stability and activity controls of Cu nanoparticles for high-performance solid oxide fuel cells66Nanoparticle Ex-solution for Supported Catalysts: Materials Design, Mechanism and Future Perspectives181A highly active perovskite anode with an in situ exsolved nanoalloy catalyst for direct carbon solid oxide fuel cells12Promotion of oxygen reduction reaction on a double perovskite electrode by a water-induced surface modification132Physico-electrochemical properties and long-term stability of Mn1.45-0.5xCo1.45-0.5xCuxY0.1O4 spinel protective coatings on commercial metallic interconnects for solid oxide fuel cells14Nanoparticle exsolution in perovskite oxide and its sustainable electrochemical energy systems43The first observation of Ni nanoparticle exsolution from YSZ and its application for dry reforming of methane22Emergence and Future of Exsolved Materials214Enhancing Thermocatalytic Activities by Upshifting the d‐Band Center of Exsolved Co‐Ni‐Fe Ternary Alloy Nanoparticles for the Dry Reforming of Methane140Enhancing Thermocatalytic Activities by Upshifting the d‐Band Center of Exsolved Co‐Ni‐Fe Ternary Alloy Nanoparticles for the Dry Reforming of Methane22Improving the performance of Pr0.4Sr0.6Co0.2Fe0.7Nb0.1O3-δ-based single-component fuel cell and reversible single-component cells by manufacturing A-site deficiency38Degradation Mechanisms of Metal-Supported Solid Oxide Cells and Countermeasures: A Review67In-situ exsolution of Ni nanoparticles to achieve an active and stable solid oxide fuel cell anode catalyst on A-site deficient La0.4Sr0.4Ti0.94Ni0.06O3-δ42Electrochemical Performance of NiCo2O4 Spinel Cathodes for Intermediate Temperature Solid Oxide Fuel Cells14Synthesis of stimuli responsive nanoparticles for electrocatalysis0Co-improving the electrocatalytic performance and H 2 S tolerance of a Sr 2 Fe 1.5 Mo 0.5 O 6− δ based anode for solid oxide fuel cells23Phase transition with in situ exsolution nanoparticles in the reduced Pr 0.5 Ba 0.5 Fe 0.8 Ni 0.2 O 3− δ electrode for symmetric solid oxide cells55A Flexible Method to Fabricate Exsolution‐Based Nanoparticle‐Decorated Materials in Seconds33The metal/oxide heterointerface delivered by solid-based exsolution strategy: A review53Concurrent promotion of phase transition and bimetallic nanocatalyst exsolution in perovskite oxides driven by Pd doping to achieve highly active bifunctional fuel electrodes for reversible solid oxide electrochemical cells52Constructing highly active alloy-perovskite interfaces for efficient electrochemical CO2 reduction reaction51In Situ Exsolution of Core‐Shell Structured NiFe/FeO x Nanoparticles on Pr 0.4 Sr 1.6 (NiFe) 1.5 Mo 0.5 O 6‐δ for CO 2 Electrolysis128Dynamic Surface Evolution of Metal Oxides for Autonomous Adaptation to Catalytic Reaction Environments23Redox-manipulated RhOx nanoclusters uniformly anchored on Sr2Fe1.45Rh0.05Mo0.5O6–δ perovskite for CO2 electrolysis13Enhancing Bifunctional Electrocatalytic Activities of La 0.5 Sr 0.5 Co 0.2 Fe 0.8 O 3 in Reversible Single-Component Cells15Tunable Magnetism and Morphology of Ferromagnetic Nanocups in Perovskite Ferroelectric Films via Co Exsolution of Transition Metals2Synergistically Promoting Coking Resistance of a La0.4Sr0.4Ti0.85Ni0.15O3−δ Anode by Ru-Doping-Induced Active Twin Defects and Highly Dispersed Ni Nanoparticles18Metal exsolution engineering on perovskites for electrocatalysis: a perspective35Electrochemical Oxidation of Primary Alcohols Using a Co2NiO4 Catalyst: Effects of Alcohol Identity and Electrochemical Bias on Product Distribution30Tailoring dual redox pairs strategy on a defective spinel Mg0.4NixMn2.6−xO4+δ cathode for the boosting of SOFCs performance13Exsolution Modeling and Control to Improve the Catalytic Activity of Nanostructured Electrodes30Challenges in using perovskite-based anode materials for solid oxide fuel cells with various fuels: a review79Emerging Exsolution Materials for Diverse Energy Applications: Design, Mechanism, and Future Prospects45A robust direct-propane solid oxide fuel cell with hierarchically oriented full ceramic anode consisting with in-situ exsolved metallic nano-catalysts33Shifting Oxygen Evolution Reaction Pathway via Activating Lattice Oxygen in Layered Perovskite Oxide127Tuning exsolution of nanoparticles in defect engineered layered perovskite oxides for efficient CO2 electrolysis55Robust and efficient Fe/Mn bimetal doped Pr4/3Ba2/3Co2/3Fe2/3Mn2/3O5+δ double perovskite catalysts for direct CO2 electrolysis22Nanoparticle Exsolution on Perovskite Oxides: Insights into Mechanism, Characteristics and Novel Strategies102Nanotechnologies in ceramic electrochemical cells84Green hydrogen production by intermediate‐temperature protonic solid oxide electrolysis cells: Advances, challenges, and perspectives62A-site-deficiency range identified for in situ exsolution from (La 0.4 Sr 0.6 ) 1− α Ti 0.95 Ni 0.05 O 3± δ electrodes for SOFC and SOEC16Recent progress in oxygen electrodes for protonic ceramic electrochemical cells31Tuning the Product Selectivity of C 2 H 6 Electrolysis Using a Core–Shell-Structured Ni@NiO-Modified Anode in a Ceramic Electrochemical Reactor12Rapid Fabrication of Electrodes for Symmetrical Solid Oxide Cells by Extreme Heat Treatment6In Situ Exsolved CoFe Alloy Nanoparticles on Gd2SrCo0.8Fe1.2O7−δ for Direct Hydrocarbon Fuel Solid Oxide Fuel Cells10Enlarging the Three-Phase Boundary to Raise CO2/CH4 Conversions on Exsolved Ni–Fe Alloy Perovskite Catalysts by Minimal Rh Doping39A High-Performance and Durable Direct-Ammonia Symmetrical Solid Oxide Fuel Cell with Nano La0.6Sr0.4Fe0.7Ni0.2Mo0.1O3−δ-Decorated Doped Ceria Electrode25Electrocatalysis in Solid Oxide Fuel Cells and Electrolyzers141Unveiling optimal activity and mechanism of in situ Ni reduction Pr2Ni1-xZnxO4 anode for ammonia solid oxide fuel cells19An Efficient Tri‐Conductive Electrode for Ethane Direct Electrochemical Dehydrogenation on Proton Ceramic Electrolysis Cells6Reversible solid oxide electrochemical cells with regulated oxygen trapping nano-dots on Ni-Fe fuel electrode12High‐Performing Perovskite/Ruddlesden‐Popper Fuel Electrode for High‐Temperature Steam Electrolysis9Enhanced Sulfur-resistance for Solid Oxide Fuel Cells Anode via Doping Modification of NaYTiO41Design high-performance symmetrical electrode of stable double perovskite oxides with in situ exsolved nanoparticles for solid oxide cells3Tailoring oxide nanoparticle exsolution in La0.5Ba0.5-yCo1-xFexO3-δ2Research Progress in Epoxidation of Light Small-Molecule Olefins10In Situ Exsolved Bimetallic Nanoparticles on Double Perovskite for Efficient CO 2 Electrolysis and Synergistic Methane Reforming in SOEC8Exsolution‐enhanced performance for energy conversion and storage5Progress in sintering-free nanoscaled electrodes of solid oxide cells: A review4Perovskite oxide exsolution process and structure regulation strategy: a review2Nanofabrication technologies for low-temperature solid oxide cells: a comprehensive review of techniques, challenges, and future perspectives15Ruddlesden-popper Prn+1NinO3n+1 (n = 1, 2) oxides with in situ exsolved Ni nanoparticles as high-performance anodes for intermediated-temperature solid oxide fuel cells2Boosting the catalytic activity and redox kinetics of (Ba0.2Sr0.8)0.9Ni0.2Fe0.7Mo0.1O3 by A-site La substitution for reversible solid oxide cells2Nanoscale Interface Engineering of LaCrO 3 –CeO 2 Composite Fuel Electrode for High-Performance Multifunctional Solid Oxide Cells1Engineering Metal‐Metal Junctions from Layered Double Hydroxide Frameworks for High‐Rate Solid Oxide Cells1Anchored nanocatalysts enable efficient oxygen reduction in barium cobaltite cathodes1Strain‐Driven In Situ Epitaxial Fluorite Oxides as Multi‐Functional Fuel Electrodes for Solid Oxide Fuel Cells1Ruddlesden-popper symmetrical electrode enables efficient and robust symmetrical reversible solid oxide cells2Activation engineered Sr rich Ruddlesden–Popper oxides for robust SOFC and dry reforming catalysis1Processing‐Centric Innovative Strategies for Protonic Ceramic Electrochemical Cells1Exploring the potential of dynamic periodic operation on tackling challenging reactions under traditional steady state - a review0Proton-Conducting Solid Oxide Electrolysis Cells for Hydrogen Production: Coupled Challenges and Synergistic Breakthroughs in Materials, Interfaces, and Systems0

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  2. Phase transition of doped LaFeO3 anode in reducing atmosphere and their power generation property in intermediate temperature solid oxide fuel cell

    International Journal of Hydrogen Energy · 2019-05-29

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  3. Vanadium-Doped Strontium Molybdate with Exsolved Ni Nanoparticles as Anode Material for Solid Oxide Fuel Cells

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  4. Design of Ceria Catalysts for Low‐Temperature CO Oxidation

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  14. Computational approaches to the exsolution phenomenon in perovskite oxides with a view to design highly durable and active anodes for solid oxide fuel cells

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  15. Ultra-fast fabrication of anode-supported solid oxide fuel cells via microwave-assisted sintering technology

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  16. In-situ exsolved NiFe alloy nanoparticles on Pr0.8Sr1.2(NiFe)O4-δ for direct hydrocarbon fuel solid oxide fuel cells

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  17. A highly active and carbon-tolerant anode decorated with in situ grown cobalt nano-catalyst for intermediate-temperature solid oxide fuel cells

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  18. Efficient bifunctional electrocatalysts for solid oxide cells based on the structural evolution of perovskites with abundant defects and exsolved CoFe nanoparticles

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  45. Synergistically Promoting Coking Resistance of a La0.4Sr0.4Ti0.85Ni0.15O3−δ Anode by Ru-Doping-Induced Active Twin Defects and Highly Dispersed Ni Nanoparticles

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  46. Metal exsolution engineering on perovskites for electrocatalysis: a perspective

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  47. Electrochemical Oxidation of Primary Alcohols Using a Co2NiO4 Catalyst: Effects of Alcohol Identity and Electrochemical Bias on Product Distribution

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  48. Tailoring dual redox pairs strategy on a defective spinel Mg0.4NixMn2.6−xO4+δ cathode for the boosting of SOFCs performance

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  49. Exsolution Modeling and Control to Improve the Catalytic Activity of Nanostructured Electrodes

    Advanced Materials · 2023-01-24

    Yo Han Kim, Hyeongwon Jeong, Bo‐Ram Won, Jae‐ha Myung

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  50. Challenges in using perovskite-based anode materials for solid oxide fuel cells with various fuels: a review

    International Journal of Hydrogen Energy · 2023-03-17

    Ainaa Nadhirah Zainon, Mahendra Rao Somalu, Audi Majdan Kamarul Bahrain, Andanastuti Muchtar, Nurul Akidah Baharuddin, Muhammed Ali S.A, Nafisah Osman, Abdullah Abdul Samat, Абул Калам Азад, Nigel Peter Brandon

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