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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2018

Highly Efficient Carbon Dots with Reversibly Switchable Green–Red Emissions for Trichromatic White Light-Emitting Diodes

Biao Yuan, Shanyue Guan, Xingming Sun, Xiaoming Li, Haibo Zeng, Zheng Xie, Ping Chen, Shuyun Zhou

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Highly Efficient Carbon Dots with Reversibly Switchable Green–Red Emissions for Trichromatic White Light-Emitting DiodesOriginalHighly efficient carbon dots and their nanohybrids for trichromatic white LEDs39Greener Luminescent Solar Concentrators with High Loading Contents Based on in Situ Cross-Linked Carbon Nanodots for Enhancing Solar Energy Harvesting and Resisting Concentration-Induced Quenching62Optimization of Illumination Performance of Trichromatic White Light-Emitting Diode and Characterization of Its Modulation Bandwidth for Communication Applications17Recognition of Latent Fingerprints and Ink-Free Printing Derived from Interfacial Segregation of Carbon Dots71White light emission by energy transfer from areca nut husk extract loaded with carbon dots synthesized from the same extract18Fingerprint identification of copper ions with absorption and emission dual-mode responses by N,S co-doped red carbon dots20A tailored molecular imprinting ratiometric fluorescent sensor based on red/blue carbon dots for ultrasensitive tetracycline detection772D MnO 2 nanosheets generated signal transduction with 0D carbon quantum dots: synthesis strategy, dual-mode behavior and glucose detection51An easy and smart way to explore the light-emitting responses of carbon dot and doxorubicin hydrochloride assembly: white light generation and pH-dependent reversible photoswitching36Fluorescent Self-Healing Carbon Dot/Polymer Gels183Synthesis and Applications of Red‐Emissive Carbon Dots79Energy transfer and luminescence properties of Dy3+/Eu3+ doped silicoaluminate phosphors46Refractive index dependent optical property of carbon dots integrated luminescent solar concentrators48Highly fluorescent near-infrared emitting carbon dots derived from lemon juice and its bioimaging application124Application advances of carbon quantum dots in optoelectronic devices6Multi-color fluorescent carbon dots with single wavelength excitation for white light-emitting diodes73Red carbon dots: Optical property regulations and applications321Simultaneous and Reversible Triggering of the Phase Transfer and Luminescence Change of Amidine-Modified Carbon Dots by CO29Water Dispersible Red Fluorescent Carbon Nanoparticles via Carbonization of Resorcinol29Carbon dots for energy conversion applications62Efficient Red/Near‐Infrared‐Emissive Carbon Nanodots with Multiphoton Excited Upconversion Fluorescence183The fluorescence mechanism of carbon dots, and methods for tuning their emission color: a review492pH-Responsive Mn-Doped Carbon Dots for White-Light-Emitting Diodes, Fingerprinting, and Bioimaging73Application of carbon dots in dye‐sensitized solar cells: A review135Optimization and performance of nitrogen-doped carbon dots as a color conversion layer for white-LED applications20Aphen-derived N-doped white-emitting carbon dots with room temperature phosphorescence for versatile applications43Multicolor emissive sulfur, nitrogen co-doped carbon dots and their application in ion detection and solid lighting28Multicolor carbon dots with concentration-tunable fluorescence and solvent-affected aggregation states for white light-emitting diodes174Bright tricolor ultrabroad-band emission carbon dots for white light-emitting diodes with a 96.5 high color rendering index68Rational synthesis of highly efficient ultra-narrow red-emitting carbon quantum dots for NIR-II two-photon bioimaging113Eco-friendly synthesis of tunable fluorescent carbon nanodots from Malus floribunda for sensors and multicolor bioimaging72A carbon dot-based tandem luminescent solar concentrator97A visible-light-excited afterglow achieved by carbon dots from rhodamine B fixed in boron oxide79An Efficient Synthesis and Photoelectric Properties of Green Carbon Quantum Dots with High Fluorescent Quantum Yield107Blue-emitting thermoreversible oligourethane gelators with aggregation-induced emission properties13Earth abundant colloidal carbon quantum dots for luminescent solar concentrators54Facile synthesis of red dual-emissive carbon dots for ratiometric fluorescence sensing and cellular imaging98Highly luminescent aggregate-induced emission from polyethylene glycol-coated carbon quantum dot clusters under blue light illumination34Highly luminescent N-doped carbon dots as a fluorescence detecting platform for Fe 3+ in solutions and living cells24Purple-emissive carbon dots enhance sensitivity of Si photodetectors to ultraviolet range64A solvent-governed surface state strategy for rational synthesis of N and S co-doped carbon dots with multicolour fluorescence6Rapid synthesis of B-N co-doped yellow emissive carbon quantum dots for cellular imaging54Green Synthesis of Fluorescent Nitrogen–Sulfur Co-Doped Carbon Dots from Scallion Leaves for Hemin Sensing52Scalable Synthesis of Green Fluorescent Carbon Dot Powders with Unprecedented Efficiency115Surface metal-ion-functionalized carbon dots and their application in pH sensing8Facile Preparation of Stable Solid-State Carbon Quantum Dots with Multi-Peak Emission39Green and Orange Emissive Carbon Dots with High Quantum Yields Dispersed in Matrices for Phosphor-Based White LEDs69Synthesis of multiple-color emissive carbon dots towards white-light emission9Orange-red, green, and blue fluorescence carbon dots for white light emitting diodes61Multi‐Color Fluorescent Carbon Dots: Graphitized sp 2 Conjugated Domains and Surface State Energy Level Co‐Modulate Band Gap Rather Than Size Effects134Facile Access to Solid-State Carbon Dots with High Luminescence Efficiency and Excellent Formability via Cellulose Derivative Coatings63Unraveling the Fluorescence Mechanism of Carbon Dots with Sub -Single-Particle Resolution217Great enhancement of red emitting carbon dots with B/Al/Ga doping for dual mode anti-counterfeiting65Self‐Quenching‐Resistant Red Emissive Carbon Dots with High Stability for Warm White Light‐Emitting Diodes with a High Color Rendering Index82Amphiphilic Carbon Dots with Excitation‐Independent Double‐Emissions17Carbon dots with red/near-infrared emissions and their intrinsic merits for biomedical applications255Fluorescent carbon dots in solid-state: From nanostructures to functional devices115Nitrogen and fluorine co-doped green fluorescence carbon dots as a label-free probe for determination of cytochrome c in serum and temperature sensing52State-of-the-Art on the Preparation, Modification, and Application of Biomass-Derived Carbon Quantum Dots185Highly Luminescent Solid‐State Carbon Dots Embedded in a Boric Acid Matrix28Tunable Carbon–CsPbI3 Quantum Dots for White LEDs28Autoencoder based blind source separation for photoacoustic resolution enhancement12Reaction kinetic acceleration induced by atomic-hybridized channels in carbon quantum dot/ReS2 composites for efficient Cr(VI) reduction21Inkjet printing based ultra-small MnO2 nanosheets synthesis for glutathione sensing10Carbon Nanodots With Nearly Unity Fluorescent Efficiency Realized via Localized Excitons2Facile synthesis of dual-emission fluorescent carbon nanodots for a multifunctional probe6White light employing luminescent engineered large (mega) Stokes shift molecules: a review100Carbon Dots: An Emerging Smart Material for Analytical Applications100Ultra-narrow-bandwidth graphene quantum dots for superresolved spectral and spatial sensing48Preparation and photocatalytic activity of red light-emitting carbon dots/P25 heterojunction photocatalyst with ultra-wide absorption spectrum11Applications of Carbon Dots in Optoelectronics123Green preparation of carbon dots with different surface states simultaneously at room temperature and their sensing applications64Carbon Dots Detect Water-to-Ice Phase Transition and Act as Alcohol Sensors via Fluorescence Turn-Off/On Mechanism50Construction and Multifunctional Applications of Visible-Light-Excited Multicolor Long Afterglow Carbon Dots/Boron Oxide Composites121Carbon‐Dot‐Based White‐Light‐Emitting Diodes with Adjustable Correlated Color Temperature Guided by Machine Learning97Carbon‐Dot‐Based White‐Light‐Emitting Diodes with Adjustable Correlated Color Temperature Guided by Machine Learning41A novel and highly stable dual-emission carbon dots-based phosphor20Dual-channel fluorescent signal readout strategy for cysteine sensing12Multicolor carbon dots: Induced by sp2-sp3 hybridized domains and their application in ion detection and WLED24Green-emissive carbon quantum dots with high fluorescence quantum yield: Preparation and cell imaging46Photoluminescent Carbon Quantum Dots: Synthetic Approaches and Photophysical Properties75CdTe‐Based Solar Cells with Variations in Mg Concentration in the MgZnO Emitter19Influence of sulfur doping on the molecular fluorophore and synergistic effect for citric acid carbon dots*4Multi-color carbon dots from cis-butenedioic acid and urea and highly luminescent carbon dots@Ca(OH)2 hybrid phosphors with excellent thermal stability for white light-emitting diodes18Multifunctional N-Doped Carbon Dots for Bimodal Detection of Bilirubin and Vitamin B12, Living Cell Imaging, and Fluorescent Ink71Excellent color rendering index single system white light emitting carbon dots for next generation lighting devices53Synthesizing Red Fluorescent Carbon Dots from Rigid Polycyclic Conjugated Molecules: Dual‐Mode Sensing and Bioimaging in Biochemical Applications13Lifetime-tunable green room temperature phosphorescence of carbon dots by the multi-step modification9Recent advances in the rational synthesis of red-emissive carbon dots for nanomedicine applications: A review44Black phosphorus nanosheet-based new drug delivery system for the anticancer agents: A review6Towards Red Emissive Systems Based on Carbon Dots0Synthesis and modulation of multicolor fluorescent carbon dots from p-phenylenediamine and dansyl derivative for white light emitting diodes16Transparent Hard Coatings with SiON-Encapsulated N-Doped Carbon Dots for Complete UV Blocking and White Light Emission24N-Doped Carbon Dots for Visual Recognition of 4-Nitroaniline and Use in Fluorescent Inks29Self-quenching-resistant solid-state carbon dots for mechanism and applications32Na-doped carbon nanodots: shed light on the concentration modulated photoluminescence and two-photon absorption performance8Crystalline-Induced Luminescence of Carbon Dots for the WLED and Fingerprint Recognition7Self-carbonization synthesis of highly-bright red/near-infrared carbon dots by solvent-free method61Surface state modulation of blue-emitting carbon dots with high quantum yield and high product yield38Synthesis, optical properties and applications of red/near-infrared carbon dots69The light of carbon dots: From mechanism to applications974Tunable multimodal printable up-/down-conversion nanomaterials for gradient information encryption19Highly Emissive Carbon Dots/Organosilicon Composites for Efficient and Stable Luminescent Solar Concentrators40Ionic Liquid‐Assisted Fast Synthesis of Carbon Dots with Strong Fluorescence and Their Tunable Multicolor Emission141Dual Fluorescence in Glutathione-Derived Carbon Dots Revisited28An Investigation on CCT and Ra Optimization for Trichromatic White LEDs Using a Dual-Weight-Coefficient-Based Algorithm5Yellow‐Emissive Carbon Dots with High Solid‐State Photoluminescence231Tuning the photoluminescence by engineering surface states/size of S, N co-doped carbon dots for cellular imaging applications13Seeking eye protection from biomass: Carbon dot-based optical blocking films with adjustable levels of blue light blocking46Perspectives of different colour‐emissive nanomaterials in fluorescent ink, LEDs, cell imaging, and sensing of various analytes22Trivalent rare-earth-codoped silicate phosphor materials (Ba1.3Ca0.7−x−y SiO4: xDy3+/yEu3+) for solid-state lighting3Preparation and luminescent modulation of yellow carbon dots for electroluminescent device13Carbon Dots for Carbon Dummies: The Quantum and The Molecular Questions Among Some Others58Green, sustainable, and economical synthesis of fluorescent nitrogen-doped carbon quantum dots for applications in optical displays and light-emitting diodes38Mixed-Metal and Mixed-Ligand Lanthanide Metal–Organic Frameworks Based on 2,6-Naphthalenedicarboxylate: Thermally Activated Sensitization and White-Light Emission25Color Conversion Light-Emitting Diodes Based on Carbon Dots: A Review32Microwave irradiation and color converting film application of carbon dots originated from wasted toner powder10Carbon Nanodots with Nearly Unity Fluorescent Efficiency Realized via Localized Excitons62Ultra‐Broadband Random Laser and White‐Light Emissive Carbon Dots/Crystal In‐Situ Hybrids31Solid-state fluorescence based on nitrogen and calcium co-doped carbon quantum dots @ bioplastic composites for applications in optical displays and light-emitting diodes40“One stone, five birds”: Ultrabright and multifaceted carbon dots for precise cell imaging and glutathione detection40Carbon dots (C-dots): fluorescence processes and bioimaging7Development of graphitic-N-based carbon dots using solid-state synthesis for fingerprinting, LEDs, and anticounterfeiting14Liquid and solid-state tunable fluorescent carbon dots for trace water detection24Open system synthesis of narrow-bandwidth red-fluorescent carbon quantum dots with a function of multi-metal ion sensing7Recent progress of emitting long-wavelength carbon dots and their merits for visualization tracking, target delivery and theranostics33Color integration in biomass-derived carbon dots to realize one-step white light14Carbon dots preserve strong blue emission in both aqueous and solid states and their application in intracellular temperature sensing and white light-emitting diodes10Diethylenetriamine-β-CD-modified carbon quantum dots for selective fluorescence sensing of Hg2+ and Fe3+ and cellular imaging49The Formation Process and Mechanism of Carbon Dots Prepared from Aromatic Compounds as Precursors: A Review156Bright and multicolor emissive carbon dots/organosilicon composite for highly efficient tandem luminescent solar concentrators61Advances in Fluorescent Sensing Carbon Dots: An Account of Food Analysis80Carbon dots based on targeting unit inheritance strategy for Golgi apparatus-targeting imaging5Turn on fluorescence detection of curcumin in food matrices by the novel fluorescence sensitizer14Mechanistic regulation of gram-scale synthesis of triple emission cyanobacteria-based carbon dots and visual ratiometric sensing applications23Paper-Fiber-Activated Triplet Excitons of Carbon Nanodots for Time-Resolved Anti-counterfeiting Signature with Artificial Intelligence Authentication13Synthesis of matrix-free carbon dots for information encryption, fingerprinting, and antibacterial activity15Recent developments of Red/NIR carbon dots in biosensing, bioimaging, and tumor theranostics105Easy-to-perform organic-solvent-free synthesis of carbon dots with strong green photoluminescence17Innovations in the Solid‐State Fluorescence of Carbon Dots: Strategies, Optical Manipulations, and Applications140Carbon Quantum Dots: The Role of Surface Functional Groups and Proposed Mechanisms for Metal Ion Sensing225Long wavelength emission multicolor fluorescent carbon quantum dots for the detection of pH, amino acids, and metal ions12Multifunctional Carbon Nanodot‐Based Advanced Diagnostics and Therapeutics11Organosilicon‐Based Carbon Dots and Their Versatile Applications32Multicolor Carbon Dots for Warm White Light-Emitting Diodes with a High Color Rendering Index of 93.226Lasing of carbon dots: Chemical design, mechanisms, and bright future148Recent advances in solid-state fluorescent of red carbon dots: A comprehensive review27Gram-scale synthesis of aggregation-caused quenching-resistant red-emissive carbon dots for potential applications9Highly fluorescent fish scale-derived carbon dots for quercetin sensing5Two birds with one stone: An innovative fluorescent cellulose polyacrylamide-hydrogel modified by born/nitrogen-doped carbon dots with sensitive visual sensing and superior extraction capacity toward Ag+8

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