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RESEARCH PAPER · Advanced Materials · 2018

Incipient Metals: Functional Materials with a Unique Bonding Mechanism

Matthias Wuttig, Volker L. Deringer, Xavier Gonze, Christophe Bichara, Jean‐Yves Raty

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Incipient Metals: Functional Materials with a Unique Bonding MechanismOriginalDesign for quality: reconfigurable flat optics based on active metasurfaces126Atomic disordering processes in crystalline GeTe induced by ion irradiation6A Quantum‐Mechanical Map for Bonding and Properties in Solids305Local Structural Origin of the Crystallization Tendency of Pure and Alloyed Sb28Phase change thin films for non-volatile memory applications145Reducing structural change in the phase transition of Ge-doped Bi 0.5 Sb 1.5 Te 3 to enable high-speed and low-energy memory switching10Disorder Control in Crystalline GeSb2Te4 and its Impact on Characteristic Length Scales12Designing crystallization in phase-change materials for universal memory and neuro-inspired computing884Exploring Chemical Bonding in Phase‐Change Materials with Orbital‐Based Indicators32Thermoelectric GeTe with Diverse Degrees of Freedom Having Secured Superhigh Performance291Influence of substrate dimensionality on the growth mode of epitaxial 3D-bonded GeTe thin films: From 3D to 2D growth30Highly Confined and Switchable Mid-Infrared Surface Phonon Polariton Resonances of Planar Circular Cavities with a Phase Change Material62Pressure-Induced Phase Transitions in Germanium Telluride: Raman Signatures of Anharmonicity and Oxidation51Understanding the Crystallization Behavior of Surface-Oxidized GeTe Thin Films for Phase-Change Memory Application37Advanced Optical Programming of Individual Meta‐Atoms Beyond the Effective Medium Approach60Femtosecond x-ray diffraction reveals a liquid–liquid phase transition in phase-change materials168Impact of Bonding on the Stacking Defects in Layered Chalcogenides29Direct atomic insight into the role of dopants in phase-change materials81Switching between Crystallization from the Glassy and the Undercooled Liquid Phase in Phase Change Material Ge 2 Sb 2 Te 594Chalcogenide Thermoelectrics Empowered by an Unconventional Bonding Mechanism271The Origin of Optical Contrast in Sb2Te3‐Based Phase‐Change Materials18Phase-change materials: Empowered by an unconventional bonding mechanism23Phase-change materials: The view from the liquid phase and the metallicity parameter37Understanding the Structure and Properties of Sesqui‐Chalcogenides (i.e., V2VI3 or Pn2Ch3 (Pn = Pnictogen, Ch = Chalcogen) Compounds) from a Bonding Perspective160Surface Polariton‐Like s‐Polarized Waveguide Modes in Switchable Dielectric Thin Films on Polar Crystals21Preferred selenium incorporation and unexpected interlayer bonding in the layered structure of Sb2Te3− x Se x7Broadband transparent optical phase change materials for high-performance nonvolatile photonics726Cr-Triggered Local Structural Change in Cr2Ge2Te6 Phase Change Material37Persistence of spin memory in a crystalline, insulating phase-change material20Investigating Bond Rupture in Resonantly Bonded Solids by Field Evaporation of Carbon Nanotubes24Revealing nano-chemistry at lattice defects in thermoelectric materials using atom probe tomography111Ovonic Threshold Switching in Se‐Rich Ge x Se 1− x Glasses from an Atomistic Point of View: The Crucial Role of the Metavalent Bonding Mechanism16CHEMICAL EFFECTS OF NEUTRON IRRADIATION ON ARSENIC SULFIDES0Orpiment under compression: metavalent bonding at high pressure33Effect of vacancy disorder in phase-change materials2Phase change memory materials: Rationalizing the dominance of Ge/Sb/Te alloys40Uncovering β-relaxations in amorphous phase-change materials58Resistive switching materials for information processing1210Ovonic Threshold‐Switching Ge x Se y Chalcogenide Materials: Stoichiometry, Trap Nature, and Material Relaxation from First Principles86Evolution of Electronic States and Emergence of Superconductivity in the Polar Semiconductor GeTe by Doping Valence-Skipping Indium21Employing Interfaces with Metavalently Bonded Materials for Phonon Scattering and Control of the Thermal Conductivity in TAGS‐x Thermoelectric Materials67Toward ultimate nonvolatile resistive memories: The mechanism behind ovonic threshold switching revealed163The interplay between Peierls distortions and metavalent bonding in IV–VI compounds: comparing GeTe with related monochalcogenides76All‐Dielectric Programmable Huygens' Metasurfaces252Phase Change Materials for Nonvolatile, Solid‐State Reflective Displays: From New Structural Design Rules to Enhanced Color‐Changing Performance20Synergistically improving thermoelectric and mechanical properties of Ge0.94Bi0.06Te through dispersing nano-SiC38Chalcogenides by Design: Functionality through Metavalent Bonding and Confinement310Optical Properties of Amorphous and Crystalline GeTe Nanoparticle Thin Films: A Phase-Change Material for Tunable Photonics37Chemical Bonding in Chalcogenides: The Concept of Multicenter Hyperbonding110Local structure of [(GeTe) 2 /(Sb 2 Te 3 ) m ] n super-lattices by x-ray absorption spectroscopy13Violation of the Stokes–Einstein relation in Ge2Sb2Te5, GeTe, Ag4In3Sb67Te26, and Ge15Sb85, and its connection to fast crystallization24Structural Metastability in Chalcogenide Semiconductors: The Role of Chemical Bonding7Etude de matériaux chalcogénures amorphes et de leurs propriétés de commutation électrique pour la conception de dispositifs sélecteurs dédiés aux mémoires résistives0Changes of Structure and Bonding with Thickness in Chalcogenide Thin Films39Characterization and Decomposition of the Natural van der Waals SnSb2Te4 under Compression44Temperature dependence of dynamic dipole formation in PbTe24Nanocrystals of face-centred cubic carbon, i-carbon and diamond obtained by direct conversion of graphite at high temperatures and static ultra-high pressures10Exceptionally High Average Power Factor and Thermoelectric Figure of Merit in n-type PbSe by the Dual Incorporation of Cu and Te130Unveiling the structural origin to control resistance drift in phase-change memory materials185Metavalent bonding in crystalline solids: how does it collapse?3Efficient Training of Machine Learning Potentials by a Randomized Atomic-System Generator11High-Pressure Raman Study of Fe(IO3)3: Soft-Mode Behavior Driven by Coordination Changes of Iodine Atoms34Recent Advances on Neuromorphic Devices Based on Chalcogenide Phase‐Change Materials273Investigation of resistive memories for Storage Class Memory applications0Functional Monochalcogenides: Raman Evidence Linking Properties, Structure, and Metavalent Bonding30Revealing the Bonding Nature in an ALnZnTe3-Type Alkaline-Metal (A) Lanthanide (Ln) Zinc Telluride by Means of Experimental and Quantum-Chemical Techniques13Enhancing thermoelectric performance of Sb2Te3 through swapped bilayer defects58Tailoring the chemical bonding of GeTe-based alloys by MgB2 alloying to simultaneously enhance their mechanical and thermoelectric performance49Discovering Electron‐Transfer‐Driven Changes in Chemical Bonding in Lead Chalcogenides (PbX, where X = Te, Se, S, O)85Three distinct optical-switching states in phase-change materials containing impurities: From physical origin to material design9Overcoming the Thermal Stability Limit of Chalcogenide Phase‐Change Materials for High‐Temperature Applications in GeSe1−xTex Thin Films16Approaching the Glass Transition Temperature of GeTe by Crystallizing Ge15Te8522Microwave AC Resonance Induced Phase Change in Sb2Te3 Nanowires4Metavalent Bonding in Solids: Characteristic Representatives, Their Properties, and Design Options51Ingénierie aux échelles nanométriques de matériaux chalcogénures à changement de phase pour les mémoires à changement de phase du futur0Halide perovskites: third generation photovoltaic materials empowered by metavalent bonding5On the Chemical Bonding of Amorphous Sb2Te320Reduced phase space of heat-carrying acoustic phonons in single-crystalline InTe35METAVALENT CHEMICAL COMPOUNDS OF THE TYPE AIBVCVI2 (AI – Li, Na, K, Rb, Cs; BV – As, Sb, Bi; CVI – Se, Te)0Phase-change mechanism and role of each element in Ag-In-Sb-Te: Chemical bond evolution11Atypical phase-change alloy Ga 2 Te 3 : atomic structure, incipient nanotectonic nuclei, and multilevel writing15Bonding diversity in rock salt-type tellurides: examining the interdependence between chemical bonding and materials properties25Retarding Ostwald ripening through Gibbs adsorption and interfacial complexions leads to high-performance SnTe thermoelectrics131Multi‐Center Hyperbonding in Phase‐Change Materials30Materials Screening for Disorder‐Controlled Chalcogenide Crystals for Phase‐Change Memory Applications60In3SbTe2 as a programmable nanophotonics material platform for the infrared124Metavalent bonding induced abnormal phonon transport in diamondlike structures: Beyond conventional theory39Metavalent Bonding in GeSe Leads to High Thermoelectric Performance117Metavalent Bonding in GeSe Leads to High Thermoelectric Performance17Change in Structure of Amorphous Sb–Te Phase‐Change Materials as a Function of Stoichiometry22Vanishing‐Harmonicity and Phase‐Change Materials4Eu2CuSe3 Revisited by Means of Experimental and Quantum‐Chemical Techniques11Crystallization and Vitrification Kinetics by Design: The Role of Chemical Bonding1Thermoelectric materials for space applications38Universal memory based on phase-change materials: From phase-change random access memory to optoelectronic hybrid storage*38High‐Throughput Screening for Phase‐Change Memory Materials90Sulfide Perovskites for Thermoelectricity37Quantum signatures for screening metavalent solids15On the Molecular Mechanism of a Photo‐Responsive Phase Change Memory2Photocatalytic electrochemical sensor based on three-dimensional graphene nanocomposites for the ultrasensitive detection of CYFRA21-1 gene14Small Polarons in Two-Dimensional Pnictogens: A First-Principles Study11Unraveling the optical contrast in Sb2Te and AgInSbTe phase-change materials14Entropy engineering promotes thermoelectric performance in p-type chalcogenides259Alternative Lone‐Pair ns 2 ‐Cation‐Based Semiconductors beyond Lead Halide Perovskites for Optoelectronic Applications77Combining Switchable Phase‐Change Materials and Phase‐Transition Materials for Thermally Regulated Smart Mid‐Infrared Modulators45Glass transition of the phase change material AIST and its impact on crystallization16Full-color, multi-level transmittance modulators: From reflectivity/gradient absorption coupling mechanism to materials map5β−As2Te3 : Pressure-induced three-dimensional Dirac semimetal with ultralow room-pressure lattice thermal conductivity10Self-regulated growth of candidate topological superconducting parkerite by molecular beam epitaxy5Pipe-diffusion-enriched dislocations and interfaces in SnSe/PbSe heterostructures10Thermodynamics and kinetics of glassy and liquid phase-change materials29Long‐Range Forces in Rock‐Salt‐Type Tellurides and How they Mirror the Underlying Chemical Bonding61Pressure-Driven Symmetry-Preserving Phase Transitions in Co(IO3)223Boron Strengthened GeTe‐Based Alloys for Robust Thermoelectric Devices with High Output Power Density91Metavalent Bonding in Crystalline Solids: How Does It Collapse?149Disorder-induced Anderson-like localization for bidimensional thermoelectrics optimization35Longitudinal acoustic and higher-energy excitations in the liquid phase-change material Ge2Sb2Te53The potential of chemical bonding to design crystallization and vitrification kinetics57How to Identify Lone Pairs, Van der Waals Gaps, and Metavalent Bonding Using Charge and Pair Density Methods: From Elemental Chalcogens to Lead Chalcogenides and Phase‐Change Materials40Sub‐Picosecond Non‐Equilibrium States in the Amorphous Phase of GeTe Phase‐Change Material Thin Films17Multilevel Switching in Phase‐Change Photonic Memory Devices13Thermoelectric materials and transport physics214Superconducting Phase Induced by a Local Structure Transition in Amorphous Sb2Se3 under High Pressure27Exploring the frontier between polar intermetallics and Zintl phases for the examples of the prolific ALnTnTe3-type alkali metal (A) lanthanide (Ln) late transition metal (Tn) tellurides7Ultra‐Thin Switchable Absorbers Based on Lossy Phase‐Change Materials40Phonon transport anomaly in metavalent bonded materials: contradictory to the conventional theory19GeTe Nanosheets as Theranostic Agents for Multimodal Imaging and Therapy of Inflammatory Bowel Disease21Rb 3 Er 4 Cu 5 Te 10 : Exploring the Frontier between Polar Intermetallics and Zintl‐Phases via Experimental and Quantumchemical Approaches11Far-Infrared Near-Field Optical Imaging and Kelvin Probe Force Microscopy of Laser-Crystallized and -Amorphized Phase Change Material Ge3Sb2Te624Halide Perovskites: Advanced Photovoltaic Materials Empowered by a Unique Bonding Mechanism116Thermally Controlled Charge‐Carrier Transitions in Disordered PbSbTe Chalcogenides15Tailoring the Structural and Optical Properties of Germanium Telluride Phase-Change Materials by Indium Incorporation15Combined Experimental and Theoretical Studies: Lattice-Dynamical Studies at High Pressures with the Help of Ab Initio Calculations7Tailoring Crystallization Kinetics of Chalcogenides for Photonic Applications27Dynamically Tunable Terahertz Emission Enabled by Anomalous Optical Phonon Responses in Lead Telluride15Density dependent local structures in InTe phase-change materials5Mind the Mines: Lapieite Minerals with Ultralow Lattice Thermal Conductivity and High Power Factor for Thermoelectricity7Ultrafast dynamics in phase-change materials and chalcogenide glasses0Metavalent bonding in chalcogenides: DFT-chemical pressure approach8Phonon anharmonicity in binary chalcogenides for efficient energy harvesting19Thermodynamic and dynamic stability in a new potential Cs 2 AgAsCl 6 perovskite: insight from DFT study40Orbitale als Ausgangspunkt der Chemischen Bindung in Ge−Sb−Te‐Phasenwechselmaterialien**1The Orbital Origins of Chemical Bonding in Ge−Sb−Te Phase‐Change Materials**65Exceptionally low thermal conductivity realized in the chalcopyrite CuFeS2 via atomic-level lattice engineering49Designing Conductive‐Bridge Phase‐Change Memory to Enable Ultralow Programming Power72Thermoelectric Performance of the 2D Bi 2 Si 2 Te 6 Semiconductor70The formation of a one-dimensional van der Waals selenium crystal from the three-dimensional amorphous phase: A spectroscopic signature of van der Waals bonding4Bonding Nature and Optical Properties of As2Te3 Phase‐Change Material10The glass transition of water, insight from phase change materials21Observation of a Novel Lattice Instability in Ultrafast Photoexcited SnSe27

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  2. Atomic disordering processes in crystalline GeTe induced by ion irradiation

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  3. A Quantum‐Mechanical Map for Bonding and Properties in Solids

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  4. Local Structural Origin of the Crystallization Tendency of Pure and Alloyed Sb

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  5. Phase change thin films for non-volatile memory applications

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  6. Reducing structural change in the phase transition of Ge-doped Bi 0.5 Sb 1.5 Te 3 to enable high-speed and low-energy memory switching

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  7. Disorder Control in Crystalline GeSb2Te4 and its Impact on Characteristic Length Scales

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  8. Designing crystallization in phase-change materials for universal memory and neuro-inspired computing

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  9. Exploring Chemical Bonding in Phase‐Change Materials with Orbital‐Based Indicators

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  10. Thermoelectric GeTe with Diverse Degrees of Freedom Having Secured Superhigh Performance

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  11. Influence of substrate dimensionality on the growth mode of epitaxial 3D-bonded GeTe thin films: From 3D to 2D growth

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  12. Highly Confined and Switchable Mid-Infrared Surface Phonon Polariton Resonances of Planar Circular Cavities with a Phase Change Material

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  13. Pressure-Induced Phase Transitions in Germanium Telluride: Raman Signatures of Anharmonicity and Oxidation

    Physical Review Letters · 2019-04-09

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  14. Understanding the Crystallization Behavior of Surface-Oxidized GeTe Thin Films for Phase-Change Memory Application

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  15. Advanced Optical Programming of Individual Meta‐Atoms Beyond the Effective Medium Approach

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  16. Femtosecond x-ray diffraction reveals a liquid–liquid phase transition in phase-change materials

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  17. Impact of Bonding on the Stacking Defects in Layered Chalcogenides

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  18. Direct atomic insight into the role of dopants in phase-change materials

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  19. Switching between Crystallization from the Glassy and the Undercooled Liquid Phase in Phase Change Material Ge 2 Sb 2 Te 5

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  20. Chalcogenide Thermoelectrics Empowered by an Unconventional Bonding Mechanism

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  21. The Origin of Optical Contrast in Sb2Te3‐Based Phase‐Change Materials

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  22. Phase-change materials: Empowered by an unconventional bonding mechanism

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  25. Surface Polariton‐Like s‐Polarized Waveguide Modes in Switchable Dielectric Thin Films on Polar Crystals

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  29. Persistence of spin memory in a crystalline, insulating phase-change material

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  30. Investigating Bond Rupture in Resonantly Bonded Solids by Field Evaporation of Carbon Nanotubes

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  31. Revealing nano-chemistry at lattice defects in thermoelectric materials using atom probe tomography

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  32. Ovonic Threshold Switching in Se‐Rich Ge x Se 1− x Glasses from an Atomistic Point of View: The Crucial Role of the Metavalent Bonding Mechanism

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  33. CHEMICAL EFFECTS OF NEUTRON IRRADIATION ON ARSENIC SULFIDES

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  34. Orpiment under compression: metavalent bonding at high pressure

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  35. Effect of vacancy disorder in phase-change materials

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  36. Phase change memory materials: Rationalizing the dominance of Ge/Sb/Te alloys

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  37. Uncovering β-relaxations in amorphous phase-change materials

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  38. Resistive switching materials for information processing

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  39. Ovonic Threshold‐Switching Ge x Se y Chalcogenide Materials: Stoichiometry, Trap Nature, and Material Relaxation from First Principles

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  40. Evolution of Electronic States and Emergence of Superconductivity in the Polar Semiconductor GeTe by Doping Valence-Skipping Indium

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  41. Employing Interfaces with Metavalently Bonded Materials for Phonon Scattering and Control of the Thermal Conductivity in TAGS‐x Thermoelectric Materials

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  42. Toward ultimate nonvolatile resistive memories: The mechanism behind ovonic threshold switching revealed

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  43. The interplay between Peierls distortions and metavalent bonding in IV–VI compounds: comparing GeTe with related monochalcogenides

    Journal of Physics D Applied Physics · 2020-03-10

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  44. All‐Dielectric Programmable Huygens' Metasurfaces

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  45. Phase Change Materials for Nonvolatile, Solid‐State Reflective Displays: From New Structural Design Rules to Enhanced Color‐Changing Performance

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  46. Synergistically improving thermoelectric and mechanical properties of Ge0.94Bi0.06Te through dispersing nano-SiC

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  47. Chalcogenides by Design: Functionality through Metavalent Bonding and Confinement

    Advanced Materials · 2020-04-03

    Bart Jan Kooi, Matthias Wuttig

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  48. Optical Properties of Amorphous and Crystalline GeTe Nanoparticle Thin Films: A Phase-Change Material for Tunable Photonics

    ACS Applied Nano Materials · 2020-04-28

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  49. Chemical Bonding in Chalcogenides: The Concept of Multicenter Hyperbonding

    Advanced Materials · 2020-05-27

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  50. Local structure of [(GeTe) 2 /(Sb 2 Te 3 ) m ] n super-lattices by x-ray absorption spectroscopy

    Journal of Physics D Applied Physics · 2020-06-02

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