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RESEARCH PAPER · ACS Catalysis · 2017

Shape Effect Undermined by Surface Reconstruction: Ethanol Dehydrogenation over Shape-Controlled SrTiO3 Nanocrystals

Guo Shiou Foo, Zachary David Hood, Zili Wu

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Shape Effect Undermined by Surface Reconstruction: Ethanol Dehydrogenation over Shape-Controlled SrTiO3 NanocrystalsOriginalAcid–base catalysis over perovskites: a review144Understanding the Impact of Surface Reconstruction of Perovskite Catalysts on CH4 Activation and Combustion68Interstitial N-doped SrSnO 3 perovskite: structural design, modification and photocatalytic degradation of dyes17Impact of Surface Composition of SrTiO3 Catalysts for Oxidative Coupling of Methane54Surface Reconstructions of Metal Oxides and the Consequences on Catalytic Chemistry221Shape-Tunable SrTiO 3 Crystals Revealing Facet-Dependent Optical and Photocatalytic Properties93Enhancement of the SrTiO 3 Surface Reactivity by Exposure to Electric Fields26Unsupported and silica-supported perovskite-type lanthanum manganite and lanthanum ferrite in the conversion of ethanol19Surface Reconstruction under the Exposure of Electric Fields Enhances the Reactivity of Donor-Doped SrTiO 333Identification of an Active NiCu Catalyst for Nitrile Synthesis from Alcohol91Strong Effect of B-Site Substitution on the Reactivity of Layered Perovskite Oxides Probed via Isopropanol Conversion16NOx storage and reduction on Pt-supported BaTiO3 with alkali washing0β-SnWO4 with Morphology-Controlled Synthesis and Facet-Depending Photocatalysis25Capsule‐Structured Copper–Zinc Catalyst for Highly Efficient Hydrogenation of Carbon Dioxide to Methanol31Synthesis of SrTiO 3 submicron cubes with simultaneous and competitive photocatalytic activity for H 2 O splitting and CO 2 reduction29The interplay between surface facet and reconstruction on isopropanol conversion over SrTiO3 nanocrystals25Tuning the catalytic performance of Co/Mg-La system for ammonia synthesis via the active phase precursor introduction method27In Situ Exsolved Metal Nanoparticles: A Smart Approach for Optimization of Catalysts163Optimized Synthesis of Ag‐Modified Al‐Doped SrTiO 3 Photocatalyst for the Conversion of CO 2 Using H 2 O as an Electron Donor36A transient kinetic analysis of the evolution of a reducible metal oxide towards catalyzing nonoxidative alkanol dehydrogenation17Advances in catalytic dehydrogenation of ethanol to acetaldehyde121Defect engineering of oxide perovskites for catalysis and energy storage: synthesis of chemistry and materials science335Interfacial acidity on the strontium titanate surface: a scaling paradigm and the role of the hydrogen bond4The catalytic dehydrogenation of ethanol by heterogeneous catalysts79Stabilization of Size-Controlled BaTiO3 Nanocubes via Precise Solvothermal Crystal Growth and Their Anomalous Surface Compositional Reconstruction22Comparative Hybrid Hartree-Fock-DFT Calculations of WO2-Terminated Cubic WO3 as Well as SrTiO3, BaTiO3, PbTiO3 and CaTiO3 (001) Surfaces51Engineering the Surface of Fe3O4 Nanoparticles for Catalytic and Magnetic Applications0Zinc Oxide/Graphene Oxide as a Robust Active Catalyst for Direct Oxidative Synthesis of Nitriles from Alcohols in Water6Identifying Support Effects in Au-Catalyzed CO Oxidation6Orientation competition growth and mechanism of SrTiO3 film on CeO2 layer14The Effect of Water on the 2‐Propanol Oxidation Activity of Co‐Substituted LaFe1−xCoxO3 Perovskites13Atomically unraveling the dependence of surface microstructure on plasmon-induced hydrogen evolution on Au/SrTiO323Water Splitting on Multifaceted SrTiO3 Nanocrystals: Computational Study11Selectively triggering photoelectrons for CO 2 to CH 4 reduction over SrTiO 3 {110} facet with dual-metal sites8Scalable Synthesis of Pt/SrTiO3 Hydrogenolysis Catalysts in Pursuit of Manufacturing-Relevant Waste Plastic Solutions44Development of cobalt catalyst supported on MgO–Ln2O3 (Ln = La, Nd, Eu) mixed oxide systems for ammonia synthesis30Fundamental understanding of the synthesis of well-defined supported non-noble metal intermetallic compound nanoparticles9strong synergistic effect of the (110) and (100) facets of the SrTiO 3 perovskite micro/nanocrystal: decreasing the binding energy of exciton and superb photooxidation capability for Co 2+12Efficient Electron Transfer by Plasmonic Silver in SrTiO3 for Low-Concentration Photocatalytic NO Oxidation69Revealing the interplay between “intelligent behavior” and surface reconstruction of non-precious metal doped SrTiO3 catalysts during methane combustion9Water Splitting on Multifaceted SrTiO3 Nanocrystals: Calculations of Raman Vibrational Spectrum6Synergistic Effect of Sr‐O Divacancy and Exposing Facets in SrTiO3 Micro/Nano Particle: Accelerating Exciton Formation and Splitting, Highly Efficient Co2+ Photooxidation15Ni/SrTiO3 Nanoparticles for Photodegradation of Methylene Blue23Perovskite Micro-Nano Cage SrTiO 3 : Formation Mechanism, Vacancy Analysis, and Exciton Dynamics15CH4 Activation over Perovskite Catalysts: True Density and Reactivity of Active Sites22SrTiO3 catalysts prepared from topochemical conversion of Bi4Ti3O12 nanoplatelets: Surface characterizations and interactions with isopropanol18Synthesis of platinum nanoparticles on strontium titanate nanocuboids via surface organometallic grafting for the catalytic hydrogenolysis of plastic waste45Acid and Base Catalysis of Srtio3 Nanoparticles for C–C Bond-Forming Reactions8Case Study: Calorimetry1Recent advances in exsolved perovskite oxide construction: exsolution theory, modulation, challenges, and prospects86First Principles Calculations of Hydrogen Evolution Reaction and Proton Migration on Stepped Surfaces of SrTiO35Perovskite Catalysts for Biomass Valorization62Treasuring trash: Pt/SrTiO3 catalysts process plastic waste into high-value materials25A-site effects of titanate-perovskite (ATiO3)-based catalysts on dehydrogenation of N-heterocyclic molecules9Engineering strontium titanate-based photocatalysts for green hydrogen generation: Recent advances and achievements49Hydrogen-mediated polarity compensation on the (110) surface terminations of ABO3 perovskites1Recent Developments in Revealing the Impact of Complex Metal Oxide Reconstruction on Catalysis19Well Dispersed Small Lanthanum Oxide Nanoparticles on BAPDA Modified Graphene Oxide: A Robust Catalyst for the Direct Oxidative Synthesis of Nitriles from Alcohols and Aldehydes in Water0Synthesis and catalytic application of nanostructured metal oxides and phosphates25Tuning the Relative Binding Strengths of Reactants to Products on Shape-Controlled SrTiO3-Supported Palladium for an Enhanced Electrocatalytic Hydrodechlorination0Temperature-Induced Lattice Defects and Surface Reconstruction in BaTiO3 Nanocubes1Facet-dependent photocatalytic reduction of nitroaromatics using tailored SrTiO 3 crystals: mechanism and reactivity enhancement10Aligning the Facet-Oriented Electric Field via Facet-Selective Doping on Truncated SrTiO3 Nanoparticles for Photoinduced Carrier Migration and Hydrogen Evolution10Frequency-Resolved Modulation Excitation Spectroscopy Methodology for Identifying Surface Reaction Species in Ethanol Oxidation on Gold Catalysts2Effects of LaFeO3 Morphology on Oxygen Species and Chemical Looping Partial Oxidation of Methane17Amorphous ZnO as an active catalyst for hydrogen production from ethanol dehydrogenation3Significant Enhancement of the Basicity of SrTiO3 Nanoparticles by Alkali Metal Doping: Implication for the Knoevenagel Condensation7Perovskite nanostructures as effective bifunctional acid-base heterogenous catalysts for biodiesel production: A comprehensive review7Nanoengineering 2D ceria-perovskite monolayers on SrTiO 3 nanocubes: structure-redox property relationship1Structure–Reactivity Insights from Design of Experiments: Facet Orientation of SrTiO 3 Determines the Impact of Humidity and Light Intensity on the Photocatalytic Gas-Phase Oxidation of Acetone1

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  2. Understanding the Impact of Surface Reconstruction of Perovskite Catalysts on CH4 Activation and Combustion

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  3. Interstitial N-doped SrSnO 3 perovskite: structural design, modification and photocatalytic degradation of dyes

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  4. Impact of Surface Composition of SrTiO3 Catalysts for Oxidative Coupling of Methane

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  5. Surface Reconstructions of Metal Oxides and the Consequences on Catalytic Chemistry

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  6. Shape-Tunable SrTiO 3 Crystals Revealing Facet-Dependent Optical and Photocatalytic Properties

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  7. Enhancement of the SrTiO 3 Surface Reactivity by Exposure to Electric Fields

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  8. Unsupported and silica-supported perovskite-type lanthanum manganite and lanthanum ferrite in the conversion of ethanol

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  9. Surface Reconstruction under the Exposure of Electric Fields Enhances the Reactivity of Donor-Doped SrTiO 3

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  10. Identification of an Active NiCu Catalyst for Nitrile Synthesis from Alcohol

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  11. Strong Effect of B-Site Substitution on the Reactivity of Layered Perovskite Oxides Probed via Isopropanol Conversion

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  13. β-SnWO4 with Morphology-Controlled Synthesis and Facet-Depending Photocatalysis

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  15. Synthesis of SrTiO 3 submicron cubes with simultaneous and competitive photocatalytic activity for H 2 O splitting and CO 2 reduction

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