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RESEARCH PAPER · Angewandte Chemie International Edition · 2017

Macroscopic Polarization Enhancement Promoting Photo‐ and Piezoelectric‐Induced Charge Separation and Molecular Oxygen Activation

Hongwei Huang, Shuchen Tu, Chao Liu Zeng, Tierui Zhang, A.H. Reshak, Yihe Zhang

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Macroscopic Polarization Enhancement Promoting Photo‐ and Piezoelectric‐Induced Charge Separation and Molecular Oxygen ActivationOriginalTemplate-free precursor-surface-etching route to porous, thin g-C 3 N 4 nanosheets for enhancing photocatalytic reduction and oxidation activity374Intercalation Effect of Attapulgite in g-C3N4 Modified with Fe3O4 Quantum Dots To Enhance Photocatalytic Activity for Removing 2-Mercaptobenzothiazole under Visible Light126Liquid-Phase Exfoliation into Monolayered BiOBr Nanosheets for Photocatalytic Oxidation and Reduction181Novel Z-scheme BiOBr/reduced graphene oxide/protonated g-C3N4 photocatalyst: Synthesis, characterization, visible light photocatalytic activity and mechanism173ZnWO 4 nanocrystals: synthesis, morphology, photoluminescence and photocatalytic properties162Multifunctional Bi2O2(OH)(NO3) Nanosheets with {001} Active Exposing Facets: Efficient Photocatalysis, Dye-Sensitization, and Piezoelectric-Catalysis139A core–satellite structured Z-scheme catalyst Cd 0.5 Zn 0.5 S/BiVO 4 for highly efficient and stable photocatalytic water splitting183Positive effects of phosphotungstic acid on the in-situ solid-state polymerization and visible light photocatalytic activity of polyimide-based photocatalyst148Black Phosphorus and Polymeric Carbon Nitride Heterostructure for Photoinduced Molecular Oxygen Activation462Oxygen Reduction Reaction for Generating H 2 O 2 through a Piezo‐Catalytic Process over Bismuth Oxychloride125Band structure engineering and efficient charge transport in oxygen substituted g-C3N4 for superior photocatalytic hydrogen evolution192Facile construction of novel direct solid-state Z-scheme AgI/BiOBr photocatalysts for highly effective removal of ciprofloxacin under visible light exposure: Mineralization efficiency and mechanisms239Activation of amorphous Bi2WO6 with synchronous Bi metal and Bi2O3 coupling: Photocatalysis mechanism and reaction pathway230CaB5O7F3: A Beryllium-Free Alkaline-Earth Fluorooxoborate Exhibiting Excellent Nonlinear Optical Performances192Efficient construction of bismuth vanadate-based Z-scheme photocatalyst for simultaneous Cr(VI) reduction and ciprofloxacin oxidation under visible light: Kinetics, degradation pathways and mechanism276In situfabrication of hierarchically porous g-C3N4 and understanding on its enhanced photocatalytic activity based on energy absorption126Facile Hydrothermal Synthesis of Z-Scheme Bi2Fe4O9/Bi2WO6 Heterojunction Photocatalyst with Enhanced Visible Light Photocatalytic Activity483FeOOH quantum dots coupled g-C3N4 for visible light driving photo- Fenton degradation of organic pollutants327N-CQDs accelerating surface charge transfer of Bi4O5I2 hollow nanotubes with broad spectrum photocatalytic activity144Fabrication of Z-scheme Bi3O4Cl/g-C3N4 2D/2D heterojunctions with enhanced interfacial charge separation and photocatalytic degradation various organic pollutants activity248Construction of 2D/2D BiVO4/g-C3N4 nanosheet heterostructures with improved photocatalytic activity161The facile fabrication of novel visible-light-driven Z-scheme CuInS2/Bi2WO6 heterojunction with intimate interface contact by in situ hydrothermal growth strategy for extraordinary photocatalytic performance213Piezoelectric materials for catalytic/photocatalytic removal of pollutants: Recent advances and outlook689Thickness‐Dependent Facet Junction Control of Layered BiOIO3 Single Crystals for Highly Efficient CO2 Photoreduction441Facile synthesis of In2S3/UiO-66 composite with enhanced adsorption performance and photocatalytic activity for the removal of tetracycline under visible light irradiation155Two-dimensional g-C3N4/TiO2 nanocomposites as vertical Z-scheme heterojunction for improved photocatalytic water disinfection130Ultrathin Bi4O5Br2 nanosheets for selective photocatalytic CO2 conversion into CO171Ferroelectric polarization promoted bulk charge separation for highly efficient CO2 photoreduction of SrBi4Ti4O15204Enabling PIEZOpotential in PIEZOelectric Semiconductors for Enhanced Catalytic Activities366Promoting charge separation of biochar-based Zn-TiO2/pBC in the presence of ZnO for efficient sulfamethoxazole photodegradation under visible light irradiation130Efficient piezo-catalytic hydrogen peroxide production from water and oxygen over graphitic carbon nitride185Graphitic carbon nitride synthesized by simple pyrolysis: role of precursor in photocatalytic hydrogen production208Photocatalytic activity of ZrO 2 composites with graphitic carbon nitride for hydrogen production under visible light150Rational nanostructure design of graphitic carbon nitride for photocatalytic applications230Visible-light photocatalysis by carbon-nano-onion-functionalized ZnO tetrapods: degradation of 2,4-dinitrophenol and a plant-model-based ecological assessment169The Role of Polarization in Photocatalysis930Enhanced Visible-Light-Induced Photoactivity of Type-II CeO 2 /g-C 3 N 4 Nanosheet toward Organic Pollutants Degradation213Defect-mediated Z-scheme BiO2-x/Bi2O2.75 photocatalyst for full spectrum solar-driven organic dyes degradation212The pivotal effects of oxygen vacancy on Bi2MoO6: Promoted visible light photocatalytic activity and reaction mechanism144Surface‐Halogenation‐Induced Atomic‐Site Activation and Local Charge Separation for Superb CO2 Photoreduction434Unprecedented Eighteen‐Faceted BiOCl with a Ternary Facet Junction Boosting Cascade Charge Flow and Photo‐redox314Bismuth‐Based Photocatalysts for Solar Photocatalytic Carbon Dioxide Conversion190In situ preparation of g-C3N4/Bi4O5I2 complex and its elevated photoactivity in Methyl Orange degradation under visible light277Alkali-assisted synthesis of direct Z-scheme based Bi2O3/Bi2MoO6 photocatalyst for highly efficient photocatalytic degradation of phenol and hydrogen evolution reaction139Suppressing Photoinduced Charge Recombination via the Lorentz Force in a Photocatalytic System217Degradation of p-nitrophenol using a ferrous-tripolyphosphate complex in the presence of oxygen: The key role of superoxide radicals172Remarkably Enhanced Hydrogen Generation of Organolead Halide Perovskites via Piezocatalysis and Photocatalysis205Oxygen vacancy rich Bi2O4-Bi4O7-BiO2-x composites for UV–vis-NIR activated high efficient photocatalytic degradation of bisphenol A172Bi4NbO8Cl {001} nanosheets coupled with g-C3N4 as 2D/2D heterojunction for photocatalytic degradation and CO2 reduction164Few-layer transition metal dichalcogenides (MoS2, WS2, and WSe2) for water splitting and degradation of organic pollutants: Understanding the piezocatalytic effect320An Efficient Strategy for Boosting Photogenerated Charge Separation by Using Porphyrins as Interfacial Charge Mediators126One pot synthesis of CdS/BiOBr/Bi2O2CO3: A novel ternary double Z-scheme heterostructure photocatalyst for efficient degradation of atrazine272High piezo–catalytic activity of ZnO/Al2O3 nanosheets utilizing ultrasonic energy for wastewater treatment138Piezophototronic effect in enhancing charge carrier separation and transfer in ZnO/BaTiO3 heterostructures for high-efficiency catalytic oxidation283A photo-switch for peroxydisulfate non-radical/radical activation over layered CuFe oxide: Rational degradation pathway choice for pollutants145Inter-plane heterojunctions within 2D/2D FeSe2/g-C3N4 nanosheet semiconductors for photocatalytic hydrogen generation274Enhanced photoactivity and oxidizing ability simultaneously via internal electric field and valence band position by crystal structure of bismuth oxyiodide219Enhanced piezoelectric-induced catalysis of SrTiO3 nanocrystal with well-defined facets under ultrasonic vibration164Efficient BiVO4 Photoanodes by Postsynthetic Treatment: Remarkable Improvements in Photoelectrochemical Performance from Facile Borate Modification1712D Hybrid Perovskite Ferroelectric Enables Highly Sensitive X‐Ray Detection with Low Driving Voltage199Internal electric field engineering for steering photogenerated charge separation and enhancing photoactivity260Unravelling the Synergy between Oxygen Vacancies and Oxygen Substitution in BiO 2− x for Efficient Molecular‐Oxygen Activation280Kinetics and mechanisms of enhanced degradation of ibuprofen by piezo-catalytic activation of persulfate149Coupling Piezocatalysis and Photocatalysis in Bi4NbO8X (X = Cl, Br) Polar Single Crystals367Surface Engineering of g‐C3N4 by Stacked BiOBr Sheets Rich in Oxygen Vacancies for Boosting Photocatalytic Performance421Insights into the enhanced adsorption/photocatalysis mechanism of a Bi4O5Br2/g-C3N4 nanosheet142Enhanced PEC performance of hematite photoanode coupled with bimetallic oxyhydroxide NiFeOOH through a simple electroless method222Exclusive enhancement of catalytic activity in Bi 0.5 Na 0.5 TiO 3 nanostructures: new insights into the design of efficient piezocatalysts and piezo-photocatalysts159Ferroelectric polarization and thin-layered structure synergistically promoting CO 2 photoreduction of Bi 2 MoO 6164Highly selective aerobic oxidation of methane to methanol over gold decorated zinc oxide via photocatalysis125Integrating 2D/2D CdS/α-Fe2O3 ultrathin bilayer Z-scheme heterojunction with metallic β-NiS nanosheet-based ohmic-junction for efficient photocatalytic H2 evolution265Structure-property relationship in nonlinear optical materials with π-conjugated CO3 triangles146Preparation of heterometallic CoNi-MOFs-modified BiVO4: a steady photoanode for improved performance in photoelectrochemical water splitting298Unravelling the interfacial charge migration pathway at atomic level in 2D/2D interfacial Schottky heterojunction for visible-light-driven molecular oxygen activation225Recent Advances of Ferro-, Piezo-, and Pyroelectric Nanomaterials for Catalytic Applications332Piezopotential augmented photo- and photoelectro-catalysis with a built-in electric field143Construction of Hierarchical Hollow Co 9 S 8 /ZnIn 2 S 4 Tubular Heterostructures for Highly Efficient Solar Energy Conversion and Environmental Remediation345Facet-charge-induced coupling dependent interfacial photocharge separation: A case of BiOI/g-C3N4 p-n junction291Macroscopic Spontaneous Polarization and Surface Oxygen Vacancies Collaboratively Boosting CO 2 Photoreduction on BiOIO 3 Single Crystals591An Unprecedented Antimony(III) Borate with Strong Linear and Nonlinear Optical Responses224The critical role of furfural alcohol in photocatalytic H2O2 production on TiO2168Cooperation of oxygen vacancies and 2D ultrathin structure promoting CO2 photoreduction performance of Bi4Ti3O12224Fabrication of direct Z-scheme Co3O4/BiOI for ibuprofen and trimethoprim degradation under visible light irradiation149Visible light responsive CuS/ protonated g-C3N4 heterostructure for rapid sterilization173Preparation and characterization of Vanadium pentoxide (V2O5) for photocatalytic degradation of monoazo and diazo dyes176Thin‐Layered Photocatalysts175Oxygen vacancies engineering in TiO2 homojunction/ZnFe-LDH for enhanced photoelectrochemical water oxidation260In situ self-growing 3D hierarchical BiOBr/BiOIO3 Z-scheme heterojunction with rich oxygen vacancies and iodine ions as carriers transfer dual-channels for enhanced photocatalytic activity274Designing 3D‐MoS2Sponge as Excellent Cocatalysts in Advanced Oxidation Processes for Pollutant Control496Remarkable Piezophoto Coupling Catalysis Behavior of BiOX/BaTiO 3 (X = Cl, Br, Cl 0.166 Br 0.834 ) Piezoelectric Composites209Piezopotential-driven simulated electrocatalytic nanosystem of ultrasmall MoC quantum dots encapsulated in ultrathin N-doped graphene vesicles for superhigh H2 production from pure water178Construction of 2D/2D Bi2Se3/g-C3N4 nanocomposite with High interfacial charge separation and photo-heat conversion efficiency for selective photocatalytic CO2 reduction205Atomically thin ZnS nanosheets: Facile synthesis and superior piezocatalytic H2 production from pure H2O221Tuning piezoelectric field for optimizing the coupling effect of piezo-photocatalysis186Impact of oxygen vacancy occupancy on piezo-catalytic activity of BaTiO3 nanobelt416Vibration catalysis of eco-friendly Na0.5K0.5NbO3-based piezoelectric: An efficient phase boundary catalyst226Photocatalysis Enhanced by External Fields460Piezocatalysis and Piezo‐Photocatalysis: Catalysts Classification and Modification Strategy, Reaction Mechanism, and Practical Application986Pyroelectric catalysis157Plasmonic Hot Electrons from Oxygen Vacancies for Infrared Light‐Driven Catalytic CO 2 Reduction on Bi 2 O 3− x284Inside‐and‐Out Semiconductor Engineering for CO 2 Photoreduction: From Recent Advances to New Trends411Photocatalysis‐Assisted Co3O4/g‐C3N4 p–n Junction All‐Solid‐State Supercapacitors: A Bridge between Energy Storage and Photocatalysis153Promoted Photocharge Separation in 2D Lateral Epitaxial Heterostructure for Visible‐Light‐Driven CO2 Photoreduction129Strong piezocatalysis in barium titanate/carbon hybrid nanocomposites for dye wastewater decomposition141Construction of piezoelectric BaTiO3/MoS2 heterojunction for boosting piezo-activation of peroxymonosulfate208Novel strategy for efficient water splitting through pyro-electric and pyro-photo-electric catalysis of BaTiO3 by using thermal resource and solar energy136Surface defect engineering of Fe-doped Bi7O9I3 microflowers for ameliorating charge-carrier separation and molecular oxygen activation201Single Pd Atoms Synergistically Manipulating Charge Polarization and Active Sites for Simultaneously Photocatalytic Hydrogen Production and Oxidation of Benzylamine148Atomic‐Level Charge Separation Strategies in Semiconductor‐Based Photocatalysts505Recent advances on water disinfection using bismuth based modified photocatalysts: Strategies and challenges220Cocatalyst Engineering in Piezocatalysis: A Promising Strategy for Boosting Hydrogen Evolution133Oxygen Vacant Semiconductor Photocatalysts579Efficient piezocatalytic removal of BPA and Cr(VI) with SnS2/CNFs membrane by harvesting vibration energy169Role of transition metal oxides in g-C3N4-based heterojunctions for photocatalysis and supercapacitors230Synergistic Polarization Engineering on Bulk and Surface for Boosting CO 2 Photoreduction306Construction of K+ Ion Gradient in Crystalline Carbon Nitride to Accelerate Exciton Dissociation and Charge Separation for Visible Light H2 Production213Ultrasonic activation of inert poly(tetrafluoroethylene) enables piezocatalytic generation of reactive oxygen species385Diffusion‐Controlled Z‐Scheme‐Steered Charge Separation across PDI/BiOI Heterointerface for Ultraviolet, Visible, and Infrared Light‐Driven Photocatalysis144Emerging Trends in Nanomaterials for Antibacterial Applications197Polarization-enhanced photocatalytic activity in non-centrosymmetric materials based photocatalysis: A review132In situ construction of Sn-doped structurally compatible heterojunction with enhanced interfacial electric field for photocatalytic pollutants removal and CO2 reduction135The Mechanism of Piezocatalysis: Energy Band Theory or Screening Charge Effect?321The Mechanism of Piezocatalysis: Energy Band Theory or Screening Charge Effect?206Enhancing the macroscopic polarization of CdS for piezo-photocatalytic water splitting154Photocatalytic H2O Overall Splitting into H2 Bubbles by Single Atomic Sulfur Vacancy CdS with Spin Polarization Electric Field192Piezo-photoelectronic coupling effect of BaTiO3@TiO2 nanowires for highly concentrated dye degradation216Internal Electric Field on Steering Charge Migration: Modulations, Determinations and Energy‐Related Applications274Utilizing electrostatic effect in fibrous filters for efficient airborne particles removal: Principles, fabrication, and material properties138Chemically Bonded α‐Fe2O3/Bi4MO8Cl Dot‐on‐Plate Z‐Scheme Junction with Strong Internal Electric Field for Selective Photo‐oxidation of Aromatic Alcohols156Layered bismuth-based photocatalysts300Unlocking bimetallic active sites via a desalination strategy for photocatalytic reduction of atmospheric carbon dioxide131Construction of a novel S-scheme heterojunction piezoelectric photocatalyst V-BiOIO3/FTCN and immobilization with floatability for tetracycline degradation165Recent Advances on Single‐Atom Catalysts for CO 2 Reduction129Piezocatalytic Techniques in Environmental Remediation227Biomimetic electrodynamic nanoparticles comprising ginger-derived extracellular vesicles for synergistic anti-infective therapy140Design strategies and effect comparisons toward efficient piezocatalytic system157Tribocatalysis mechanisms: electron transfer and transition126Achieving Fast Charge Separation by Ferroelectric Ultrasonic Interfacial Engineering for Rapid Sonotherapy of Bacteria‐Infected Osteomyelitis125Piezocatalytic Medicine: An Emerging Frontier using Piezoelectric Materials for Biomedical Applications363Tunable Bi-bridge S-scheme Bi2S3/BiOBr heterojunction with oxygen vacancy and SPR effect for efficient photocatalytic reduction of Cr(VI) and industrial electroplating wastewater treatment127Efficient ciprofloxacin removal over Z-scheme ZIF-67/V-BiOIO3 heterojunctions: Insight into synergistic effect between adsorption and photocatalysis158Band Position‐Independent Piezo‐Electrocatalysis for Ultrahigh CO 2 Conversion129Oxygen‐Vacancy‐Rich Piezoelectric BiO2−x Nanosheets for Augmented Piezocatalytic, Sonothermal, and Enzymatic Therapies1532D MXenes polar catalysts for multi-renewable energy harvesting applications128Increasing the Photocatalytic Hydrogen Generation Activity of CdS Nanorods by Introducing Interfacial and Polarization Electric Fields140High-efficiency V-Mediated Bi2MoO6 photocatalyst for PMS activation: Modulation of energy band structure and enhancement of surface reaction139A contact-electro-catalytic cathode recycling method for spent lithium-ion batteries293Piezoelectricity, Pyroelectricity, and Ferroelectricity in Biomaterials and Biomedical Applications198Dynamic defects boost in-situ H 2 O 2 piezocatalysis for water cleanup139Piezocatalysts and Piezo‐Photocatalysts: From Material Design to Diverse Applications221

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    Sami Dursun, İsmail Cihan Kaya, Volkan Kalem, Hasan Akyıldız

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  39. Hydrothermally synthesized Na2Ti3O7 nanotube–V2O5 heterostructures with improved visible photocatalytic degradation and hydrogen evolution - Its photocorrosion suppression

    Journal of Alloys and Compounds · 2018-01-03

    S.V. Prabhakar Vattikuti, Police Anil Kumar Reddy, Patnamsetty Chidanandha Nagajyothi, Jaesool Shim, Chan Byon

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  40. Positive effects of phosphotungstic acid on the in-situ solid-state polymerization and visible light photocatalytic activity of polyimide-based photocatalyst

    Applied Catalysis B: Environmental · 2018-01-03

    Pengcheng Meng, Huimin Heng, Yanhong Sun, Junhao Huang, Jinpeng Yang, Xia Liu

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  41. Black Phosphorus and Polymeric Carbon Nitride Heterostructure for Photoinduced Molecular Oxygen Activation

    Advanced Functional Materials · 2018-01-08

    Yun Zheng, Zihao Yu, Honghui Ou, Abdullah Mohamed Asiri, Yilin Chen, Xinchen Wang

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  42. Nature-Derived Approach to Oxygen and Chlorine Dual-Vacancies for Efficient Photocatalysis and Photoelectrochemistry

    ACS Sustainable Chemistry & Engineering · 2018-01-09

    Min Li, Yihe Zhang, Xiaowei Li, Yonggang Wang, Fan Dong, Liqun Ye, Shixin Yu, Hongwei Huang

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  43. Oxygen Reduction Reaction for Generating H 2 O 2 through a Piezo‐Catalytic Process over Bismuth Oxychloride

    ChemSusChem · 2018-01-10

    Dengkui Shao, Ling Zhang, Songmei Sun, Wenzhong Wang

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  44. Visible-Light-Responsive Sillén-Structured Mixed-Cationic CdBiO2Br Nanosheets: Layer Structure Design Promoting Charge Separation and Oxygen Activation Reactions

    The Journal of Physical Chemistry C · 2018-01-20

    Hongwei Huang, A.H. Reshak, S. Auluck, Shifeng Jin, Na Tian, Yuxi Guo, Yihe Zhang

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  45. Bi 2 WO 6 /ZnO:一种在可见光下具有优良光催化性能的花状新型复合材料

    CHINESE JOURNAL OF CATALYSIS (CHINESE VERSION) · 2018-01-24

    程娟, 沈奕, 陈宽, 汪曦, 郭永福, 周晓吉, Renbi Bai

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  46. A novel photocatalytic water splitting solar-to-hydrogen energy conversion: Non-centro-symmetric borate CsZn2B3O7 photocatalyst

    Journal of Alloys and Compounds · 2018-01-31

    A.H. Reshak

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  47. Facile synthesis of Ni-doping Bi2WO6 nano-sheets with enhanced adsorptive and visible-light photocatalytic performances

    Journal of Materials Science · 2018-02-01

    Xiang Lei, Lei Chen, Ce-Hui Mo, Lianming Zheng, Zhong-Xiong Yu, Yanwen Li, Quan-Ying Cai, Hui Li, Wei-Dong Yang, Dongmei Zhou, Ming Hung Wong

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  48. Congruent melt terbium-rich borate Na2Tb2B2O7: Synthesis, crystal structure, optical and magnetic properties

    Journal of Alloys and Compounds · 2018-02-05

    Zhen Jia, Mingjun Xia

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  49. Single-crystal TiO2 nanorods assembly for efficient and stable cocatalyst-free photocatalytic hydrogen evolution

    Applied Catalysis B: Environmental · 2018-02-05

    Yong Jiang, Hongyan Ning, Chungui Tian, Baojiang Jiang, Qi Li, Haijing Yan, Xuliang Zhang, Jian‐Qiang Wang, Liqiang Jing, Honggang Fu

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  50. Au@TiO2 yolk-shell nanostructures for enhanced performance in both photoelectric and photocatalytic solar conversion

    Applied Surface Science · 2018-02-07

    Qinrong He, Hang Sun, Yinxing Shang, Yanan Tang, Ping She, Shan Zeng, Kongliang Xu, Guolong Lu, Song Miao Liang, Shengyan Yin, Zhenning Liu

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