RESEARCH ARTICLE · Angewandte Chemie International Edition · 2017

Bridging the Gap between Industrial and Well‐Defined Supported Catalysts

Christophe Copéret, Florian Allouche, Ka Wing Chan, Matthew P. Conley, Murielle F. Delley, Alexey Fedorov, Ilia B. Moroz, Victor Mougel, Margherita Pucino, Keith Searles, Keishi Yamamoto, Pavel A. Zhizhko

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Abstract

Many industrial catalysts contain isolated metal sites on the surface of oxide supports. Although such catalysts have been used in a broad range of processes for more than 40 years, there is often a very limited understanding about the structure of the catalytically active sites. This Review discusses how surface organometallic chemistry (SOMC) engineers surface sites with well-defined structures and provides insight into the nature of the active sites of industrial catalysts; the Review focuses in particular on olefin production and conversion processes.

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