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RESEARCH PAPER · Chemistry of Materials · 2017

The Li3RuyNb1–yO4 (0 ≤ y ≤ 1) System: Structural Diversity and Li Insertion and Extraction Capabilities

Quentin Jacquet, Arnaud J. Perez, Dmitry Batuk, Gustaaf Van Tendeloo, Gwenaëlle Rousse, Jean‐Marie Tarascon

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The Li3RuyNb1–yO4 (0 ≤ y ≤ 1) System: Structural Diversity and Li Insertion and Extraction CapabilitiesOriginalApproaching the limits of cationic and anionic electrochemical activity with the Li-rich layered rocksalt Li3IrO4173Electrostatic Interactions versus Second Order Jahn–Teller Distortion as the Source of Structural Diversity in Li3MO4 Compounds (M = Ru, Nb, Sb and Ta)31Energy storage properties of iridium oxides : model materials for the study of anionic redox0A chemical redox reaction to generate rock salt-type materials: the case of Na 3 V 2 O 56Polyhedral perspectives on the capacity limit of cathode compounds for lithium-ion batteries: a case study for Li 6 CoO 420Polymorphism in Li4Zn(PO4)2 and Stabilization of its Structural Disorder to Improve Ionic Conductivity18Fundamental understanding and practical challenges of anionic redox activity in Li-ion batteries1588Chemical Activity of the Peroxide/Oxide Redox Couple: Case Study of Ba5Ru2O11 in Aqueous and Organic Solvents14Recent Advances in Transmission Electron Microscopy for Materials Science at the EMAT Lab of the University of Antwerp40Unexpectedly high energy density of a Li-Ion battery by oxygen redox in LiNiO2 cathode: First-principles study37Competition between Metal Dissolution and Gas Release in Li-Rich Li3RuyIr1–yO4 Model Compounds Showing Anionic Redox32Li-rich Li3MO4 model compounds for deciphering capacity and voltage aspects in anionic redox materials0Anionic redox for high-energy batteries. Fundamental understanding, practical challenges, and future outlook0Electronic Structure and Properties of Lithium-Rich Complex Oxides18Na 2 Ru 1−x Mn x O 3 as the cathode for sodium-ion batteries32Synthesis and Electrochemical Activity of Some Na(Li)‐Rich Ruthenium Oxides with the Feasibility to Stabilize Ru6+37Manganese‐Based Na‐Rich Materials Boost Anionic Redox in High‐Performance Layered Cathodes for Sodium‐Ion Batteries210High capacity Li/Ni rich Ni-Ti-Mo oxide cathode for Li-ion batteries7Quantification of Anionic Redox Chemistry in a Prototype Na-Rich Layered Oxide23Chimie du solide et énergie0Multiscale factors in designing alkali-ion (Li, Na, and K) transition metal inorganic compounds for next-generation rechargeable batteries144Two-dimensional, conductive niobium and molybdenum metal–organic frameworks20Exploration of ionic conductors and Li-rich sulfides for all-solid-state batteries0Definition of Redox Centers in Reactions of Lithium Intercalation in Li 3 RuO 4 Polymorphs15Design Rules for High-Valent Redox in Intercalation Electrodes148Anionic redox in Na-based layered oxide cathodes: a review with focus on mechanism studies77Mn4+-Substituted Li-Rich Li1.2Mn0.43+Mnx4+Ti0.4–xO2 Materials with High Energy Density25Fundamental understanding of high-capacity lithium-excess cathodes with disordered rock salt structure12Synthesis and characterization of new positive electrode materials for Li-ion high energy applications0Experimental considerations to study Li-excess disordered rock salt cathode materials40Evolution of Oxygen Ligands upon Large Redox Swings of Li 3 IrO 41High Energy Density Layered Oxide Cathodes for Sodium Ion Batteries0Importance of metal − oxygen bond for stable oxygen-redox reaction in Li-excess layered oxides18Revealing the Thermodynamics and Kinetics of In-Plane Disordered Li2MnO3 Structure in Li-Rich Cathodes81Synthesis, characterization and study of the properties of new exotic lithium ion intercalation compounds0X-Ray Absorption Spectroscopy Illustrates the Participation of Oxygen in the Electrochemical Cycling of Li4mn2o59Status of Li(Na)-based anionic redox materials for better batteries13Access to Ru(IV)–Ru(V) and Ru(V)–Ru(VI) Redox in Layered Li7RuO6 via Intercalation Reactions4Superior Multielectron‐Transferring Energy Storage by π‐d Conjugated Frameworks3Triggering Anionic Redox Activity in Li3NbS4 Through Cationic Disordering or Substitution11Fluorinated Rocksalt Cathode with Ultra‐high Active Li Content for Lithium‐ion Batteries24Fluorinated Rocksalt Cathode with Ultra‐high Active Li Content for Lithium‐ion Batteries0Machine Learning-based Comprehensive Survey on Lithium-rich Cathode Materials9Accessible Li Percolation and Extended Oxygen Oxidation Boundary in Rocksalt‐like Cathode Enabled by Initial Li‐deficient Nanostructure11Anionic Redox in Rechargeable Batteries: Mechanism, Materials, and Characterization39On the Active Components in Crystalline Li–Nb–O and Li–Ta–O Coatings from First Principles22Correlating concerted cations with oxygen redox in rechargeable batteries41Characteristics, materials, and performance of Ru-containing oxide cathode materials for rechargeable batteries44⁷Li NMR short-range ordering in hardened lithium sodium niobate1Phase Behavior and Ion Transport in Lithium–Niobium–Tantalum Oxide Alloys0

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  1. Approaching the limits of cationic and anionic electrochemical activity with the Li-rich layered rocksalt Li3IrO4

    Nature Energy · 2017-12-06

    Arnaud J. Perez, Quentin Jacquet, Dmitry Batuk, Antonella Iadecola, Matthieu Saubanère, Gwenaëlle Rousse, Dominique Larcher, Hervé Vezin, Marie‐Liesse Doublet, Jean‐Marie Tarascon

    Read original paper ↗ ·

  2. Electrostatic Interactions versus Second Order Jahn–Teller Distortion as the Source of Structural Diversity in Li3MO4 Compounds (M = Ru, Nb, Sb and Ta)

    Chemistry of Materials · 2017-12-07

    Quentin Jacquet, Gwenaëlle Rousse, Antonella Iadecola, Matthieu Saubanère, Marie‐Liesse Doublet, Jean‐Marie Tarascon

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  3. Energy storage properties of iridium oxides : model materials for the study of anionic redox

    Unknown journal · 2017-12-19

    Arnaud J. Perez

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  4. A chemical redox reaction to generate rock salt-type materials: the case of Na 3 V 2 O 5

    Dalton Transactions · 2017-12-22

    Evan Adamczyk, Emmanuel Anger, M. Freire, V. Pralong

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  5. Polyhedral perspectives on the capacity limit of cathode compounds for lithium-ion batteries: a case study for Li 6 CoO 4

    Physical Chemistry Chemical Physics · 2018-01-01

    Zhenlian Chen, Zhifeng Zhang, Jun Li

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  6. Polymorphism in Li4Zn(PO4)2 and Stabilization of its Structural Disorder to Improve Ionic Conductivity

    Chemistry of Materials · 2018-01-25

    Sujoy Saha, Gwenaëlle Rousse, Ignacio Blazquez Alcover, Matthieu Courty, Daniel Alves Dalla Corte, Jean‐Marie Tarascon

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  7. Fundamental understanding and practical challenges of anionic redox activity in Li-ion batteries

    Nature Energy · 2018-04-09

    Gaurav Assat, Jean‐Marie Tarascon

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  8. Chemical Activity of the Peroxide/Oxide Redox Couple: Case Study of Ba5Ru2O11 in Aqueous and Organic Solvents

    Chemistry of Materials · 2018-05-21

    Alexis Grimaud, Antonella Iadecola, Dmitry Batuk, Matthieu Saubanère, Artem M. Abakumov, J. W. Freeland, Jordi Cabana, Haifeng Li, Marie‐Liesse Doublet, Gwenaëlle Rousse, Jean‐Marie Tarascon

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  9. Recent Advances in Transmission Electron Microscopy for Materials Science at the EMAT Lab of the University of Antwerp

    Materials · 2018-07-28

    Giulio Guzzinati, Thomas Altantzis, Maria Batuk, Annick De Backer, Gunnar Lumbeeck, Vahid Samaee, Dmitry Batuk, Hosni Idrissi, Joke Hadermann, Sandra Van Aert, D. Schryvers, Johan Verbeeck, Sara Bals

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  10. Unexpectedly high energy density of a Li-Ion battery by oxygen redox in LiNiO2 cathode: First-principles study

    Electrochimica Acta · 2018-10-18

    Daehyeon Choi, Joonhee Kang, Byungchan Han

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  11. Competition between Metal Dissolution and Gas Release in Li-Rich Li3RuyIr1–yO4 Model Compounds Showing Anionic Redox

    Chemistry of Materials · 2018-10-19

    Quentin Jacquet, Antonella Iadecola, Matthieu Saubanère, Louis Lemarquis, Erik J. Berg, Daniel Alves Dalla Corte, Gwenaëlle Rousse, Marie‐Liesse Doublet, Jean‐Marie Tarascon

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  12. Li-rich Li3MO4 model compounds for deciphering capacity and voltage aspects in anionic redox materials

    Unknown journal · 2018-12-12

    Quentin Jacquet

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  13. Anionic redox for high-energy batteries. Fundamental understanding, practical challenges, and future outlook

    Unknown journal · 2018-12-14

    Gaurav Assat

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  14. Electronic Structure and Properties of Lithium-Rich Complex Oxides

    ACS Applied Electronic Materials · 2018-12-28

    Khang Hoang, Myungkeun Oh, Yongki Choi

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  15. Na 2 Ru 1−x Mn x O 3 as the cathode for sodium-ion batteries

    Journal of Materials Chemistry A · 2019-01-01

    Xiang Li, Shaohua Guo, Feilong Qiu, Linlin Wang, Masayoshi Ishida, Haoshen S. Zhou

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  16. Synthesis and Electrochemical Activity of Some Na(Li)‐Rich Ruthenium Oxides with the Feasibility to Stabilize Ru6+

    Advanced Energy Materials · 2019-02-27

    Misae Otoyama, Quentin Jacquet, Antonella Iadecola, Matthieu Saubanère, Gwenaëlle Rousse, Jean‐Marie Tarascon

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  17. Manganese‐Based Na‐Rich Materials Boost Anionic Redox in High‐Performance Layered Cathodes for Sodium‐Ion Batteries

    Advanced Materials · 2019-05-10

    Xiaoyu Zhang, Yu Qiao, Shaohua Guo, Kezhu Jiang, Sheng Ming Xu, Hang Xu, Peng Wang, Ping He, Haoshen S. Zhou

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  18. High capacity Li/Ni rich Ni-Ti-Mo oxide cathode for Li-ion batteries

    Solid State Ionics · 2019-12-06

    Jianan Xu, Ganguli Babu, Keiko Kato, Francisco Carlos Robles Hernandez, Anand B. Puthirath, Alexander Britz, Dennis L. Nordlund, Sami Sainio, Uwe Bergmann, Pulickel Madhavapanicker Ajayan

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  19. Quantification of Anionic Redox Chemistry in a Prototype Na-Rich Layered Oxide

    ACS Applied Materials & Interfaces · 2019-12-30

    Yue Hu, Tiefeng Liu, Chen Cheng, Yingying Yan, Manling Ding, Ting‐Shan Chan, Jinghua Guo, Liang Zhang

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  20. Chimie du solide et énergie

    L’annuaire du Collège de France · 2020-01-01

    Jean‐Marie Tarascon

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  21. Multiscale factors in designing alkali-ion (Li, Na, and K) transition metal inorganic compounds for next-generation rechargeable batteries

    Energy & Environmental Science · 2020-01-01

    Wontae Lee, Jaeyoung Kim, Soyeong Yun, Woosung Choi, Haegyeom Kim, Won‐Sub Yoon

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  22. Two-dimensional, conductive niobium and molybdenum metal–organic frameworks

    Chemical Science · 2020-01-01

    Michael E. Ziebel, Justin C. Ondry, Jeffrey R. Long

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  23. Exploration of ionic conductors and Li-rich sulfides for all-solid-state batteries

    Unknown journal · 2020-01-06

    Sujoy Saha

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  24. Definition of Redox Centers in Reactions of Lithium Intercalation in Li 3 RuO 4 Polymorphs

    Journal of the American Chemical Society · 2020-04-09

    Haifeng Li, Srinivasan Ramakrishnan, J. W. Freeland, Bryan D. McCloskey, Jordi Cabana

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  25. Design Rules for High-Valent Redox in Intercalation Electrodes

    Joule · 2020-06-11

    William E. Gent, Iwnetim Iwnetu Abate, Wanli Yang, Linda F. Nazar, William C. Chueh

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  26. Anionic redox in Na-based layered oxide cathodes: a review with focus on mechanism studies

    Materials Today Energy · 2020-07-07

    Chao Li, Fushan Geng, Bingwen Hu, Bingwen Hu, Bingwen Hu, Bingwen Hu

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  27. Mn4+-Substituted Li-Rich Li1.2Mn0.43+Mnx4+Ti0.4–xO2 Materials with High Energy Density

    ACS Applied Materials & Interfaces · 2020-08-07

    Shiyao Zheng, Ke Chao Zhou, Feng Zheng, Haodong Liu, Guiming Zhong, Wenhua Zuo, Ningbo Xu, Gang Zhao, Mingzeng Luo, Jue Wu, Chunyang Zhang, Zhongru Zhang, Shunqing Wu, Yong Yang

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  28. Fundamental understanding of high-capacity lithium-excess cathodes with disordered rock salt structure

    Journal of Material Science and Technology · 2020-09-28

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  29. Synthesis and characterization of new positive electrode materials for Li-ion high energy applications

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  30. Experimental considerations to study Li-excess disordered rock salt cathode materials

    Journal of Materials Chemistry A · 2020-12-15

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  31. Evolution of Oxygen Ligands upon Large Redox Swings of Li 3 IrO 4

    Journal of The Electrochemical Society · 2021-06-01

    Haifeng Li, Arnaud J. Perez, Beata Taudul, Teak D. Boyko, J. W. Freeland, Marie‐Liesse Doublet, Jean‐Marie Tarascon, Jordi Cabana

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  32. High Energy Density Layered Oxide Cathodes for Sodium Ion Batteries

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  33. Importance of metal − oxygen bond for stable oxygen-redox reaction in Li-excess layered oxides

    Energy storage materials · 2021-08-21

    Sojung Koo, Jaewoon Lee, Jinwoo Lee, Sangho Yoon, Duho Kim

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  34. Revealing the Thermodynamics and Kinetics of In-Plane Disordered Li2MnO3 Structure in Li-Rich Cathodes

    ACS Energy Letters · 2021-10-11

    Yunshan Jiang, Fu‐Da Yu, Lan‐Fang Que, Liang Deng, Yang Xia, Wang Ke, Yi Han, Zhen‐Bo Wang

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  35. Synthesis, characterization and study of the properties of new exotic lithium ion intercalation compounds

    Unknown journal · 2021-12-10

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  36. X-Ray Absorption Spectroscopy Illustrates the Participation of Oxygen in the Electrochemical Cycling of Li4mn2o5

    The Journal of Physical Chemistry C · 2022-01-01

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  37. Status of Li(Na)-based anionic redox materials for better batteries

    Elsevier eBooks · 2022-02-26

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  38. Access to Ru(IV)–Ru(V) and Ru(V)–Ru(VI) Redox in Layered Li7RuO6 via Intercalation Reactions

    Chemistry of Materials · 2022-04-15

    Haifeng Li, Beata Taudul, Grant C. B. Alexander, Jue Liu, J. W. Freeland, Marie‐Liesse Doublet, Jordi Cabana

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  39. Superior Multielectron‐Transferring Energy Storage by π‐d Conjugated Frameworks

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  40. Triggering Anionic Redox Activity in Li3NbS4 Through Cationic Disordering or Substitution

    Advanced Energy Materials · 2022-08-26

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  41. Fluorinated Rocksalt Cathode with Ultra‐high Active Li Content for Lithium‐ion Batteries

    Angewandte Chemie International Edition · 2022-10-20

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  42. Fluorinated Rocksalt Cathode with Ultra‐high Active Li Content for Lithium‐ion Batteries

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  43. Machine Learning-based Comprehensive Survey on Lithium-rich Cathode Materials

    Electrochemistry · 2023-02-27

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  44. Accessible Li Percolation and Extended Oxygen Oxidation Boundary in Rocksalt‐like Cathode Enabled by Initial Li‐deficient Nanostructure

    Advanced Functional Materials · 2023-04-27

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  45. Anionic Redox in Rechargeable Batteries: Mechanism, Materials, and Characterization

    Advanced Functional Materials · 2023-06-17

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  46. On the Active Components in Crystalline Li–Nb–O and Li–Ta–O Coatings from First Principles

    Chemistry of Materials · 2023-07-07

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  47. Correlating concerted cations with oxygen redox in rechargeable batteries

    Chemical Society Reviews · 2024-01-01

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  48. Characteristics, materials, and performance of Ru-containing oxide cathode materials for rechargeable batteries

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  49. ⁷Li NMR short-range ordering in hardened lithium sodium niobate

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  50. Phase Behavior and Ion Transport in Lithium–Niobium–Tantalum Oxide Alloys

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