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RESEARCH PAPER · Advanced Materials · 2017

A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal–Organic Frameworks

Raghavender Medishetty, Venkatram Nalla, Lydia Nemec, Sebastian Henke, David C. Mayer, Handong Sun, Karsten Reuter, Roland A. Fischer

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A New Class of Lasing Materials: Intrinsic Stimulated Emission from Nonlinear Optically Active Metal–Organic FrameworksOriginalNonlinear optical properties, upconversion and lasing in metal–organic frameworks683Multi‐Photon Absorption in Metal–Organic Frameworks110Multiphotonenabsorption in Metall‐organischen Gerüstverbindungen19Warm-White-Light-Emitting Diode Based on a Dye-Loaded Metal–Organic Framework for Fast White-Light Communication110A 3D metal-organic framework with a pcu net constructed from lead(II) and thiophene-2, 5-dicarboxylic acid: Synthesis, structure and ferroelectric property23A Two‐Photon Luminescent Dye‐Loaded Metal–Organic Framework for Physiological Temperature Sensing within Biological Windows18On the Existence of Excitonic Signatures in the Optical Response of Metal–Organic Frameworks: Comment on “van der Waals Metal–Organic Framework as an Excitonic Material for Advanced Photonics”1Fabrication of zinc-dicarboxylate- and zinc-pyrazolate-carboxylate-framework thin films through vapour–solid deposition19Multivariant synthesis, crystal structures and properties of four nickel coordination polymers based on flexible ligands16Photonic functional metal–organic frameworks661Wavelength dependent nonlinear optical response of tetraphenylethene aggregation-induced emission luminogens52Room-temperature sintered metal-organic framework nanocrystals: A new type of optical ceramics27Salts and Co-Crystalline Assemblies of Tetra(4-Pyridyl)Ethylene with Di-Carboxylic Acids1Luminescent Lanthanide MOFs: A Unique Platform for Chemical Sensing235Nonlinear-Optical Behaviors of a Chiral Metal–Organic Framework Comprised of an Unusual Multioriented Double-Helix Structure48Control of Aggregation-Induced Emission from a Tetraphenylethene Derivative through the Components in the Co-crystal32Ultrathin Metal–Organic Framework: An Emerging Broadband Nonlinear Optical Material for Ultrafast Photonics336Electronic Structure and Optical Response of Zn‐Based Metal–Organic Frameworks9Hypoxia-Triggered Nanoscale Metal–Organic Frameworks for Enhanced Anticancer Activity119Anionic Lanthanide Metal–Organic Frameworks: Selective Separation of Cationic Dyes, Solvatochromic Behavior, and Luminescent Sensing of Co(II) Ion110Nanometer scale metal-organic framework nanoparticles for optical application1Second harmonic generation from metal-organic framework derivatives2Albumin-Stabilized Metal–Organic Nanoparticles for Effective Delivery of Metal Complex Anticancer Drugs62Highly Porous Nanocrystalline UiO-66 Thin Films via Coordination Modulation Controlled Step-by-Step Liquid-Phase Growth25High quantum yield pure blue emission and fast proton conduction from an indium–metal–organic framework26Amino modified metal-organic frameworks as pH-responsive nanoplatforms for safe delivery of camptothecin60Cost-Effective Realization of Multimode Exciton–Polaritons in Single-Crystalline Microplates of a Layered Metal–Organic Framework13Cadmium‐Based Coordination Polymers from 1D to 3D: Synthesis, Structures, and Photoluminescent and Electrochemiluminescent Properties30Three-Photon Absorption of Coordination Polymer Transforms UV-to-VIS Thermometry into NIR-to-VIS Thermometry55Spatially defined molecular emitters coupled to plasmonic nanoparticle arrays30MOF‐Based Organic Microlasers52Controlling Multiphoton Absorption Efficiency by Chromophore Packing in Metal–Organic Frameworks86Metal–Organic Frameworks in Modern Physics: Highlights and Perspectives104All Roads Lead to Rome: Tuning the Luminescence of a Breathing Catenated Zr-MOF by Programmable Multiplexing Pathways52Pressure‐Induced Multiphoton Excited Fluorochromic Metal–Organic Frameworks for Improving MPEF Properties92Pressure‐Induced Multiphoton Excited Fluorochromic Metal–Organic Frameworks for Improving MPEF Properties19Recent advances in photofunctional polymorphs of molecular materials96Graphene Sandwich Stable Perovskite Quantum-Dot Light-Emissive Ultrasensitive and Ultrafast Broadband Vertical Phototransistors94Steric-Hindrance-Controlled Laser Switch Based on Pure Metal–Organic Framework Microcrystals95Auto-controlled fabrication of a metal-porphyrin framework thin film with tunable optical limiting effects105Organic solid-state lasers: a materials view and future development444Pure Metal–Organic Framework Microlasers with Controlled Cavity Shapes51Interpenetrated Metal–Organic Frameworks with ftw Topology and Versatile Functions34A new anionic metal–organic framework with suitable pore and PtS-type topology for selective adsorption and separation of cationic dyes4Postsynthetic Framework Contraction Enhances the Two-Photon Absorption Properties of Pillar-Layered Metal–Organic Frameworks40Coordination Polymers Based on Highly Emissive Ligands: Synthesis and Functional Properties112Tetraphenylethene-Based Luminescent Metal–Organic Framework for Effective Differentiation of cis/trans Isomers8Intrinsic Ultralow-Threshold Laser Action from Rationally Molecular Design of Metal–Organic Framework Materials24Photodynamical behaviour of MOFs and related composites: Relevance to emerging photon-based science and applications48Aggregation-Induced Emission-Responsive Metal–Organic Frameworks119Bismuth-MOF based on tetraphenylethylene derivative as a luminescent sensor with turn-off/on for application of Fe3+ detection in serum and bioimaging, as well as emissive spectra analysis by TRES77Let the light be a guide: Chromophore communication in metal-organic frameworks60Stimuli‐Responsive Luminescent Properties of Tetraphenylethene‐Based Strontium and Cobalt Metal–Organic Frameworks128Stimuli‐Responsive Luminescent Properties of Tetraphenylethene‐Based Strontium and Cobalt Metal–Organic Frameworks9Facile synthesis and structure elucidation of metal-organic frameworks with {ZnCa} and {Zn2Ca} metal cores23Construction of Hyaluronic Acid‐Covered Hierarchically Porous MIL‐nanoMOF for Loading and Controlled Release of Doxorubicin23A nitrophenyl-carbazole based push-pull linker as a building block for non-linear optical active coordination polymers: A structural and photophysical study11Environmental pollution analysis based on the luminescent metal organic frameworks: A review94Functional Scaffolds from AIE Building Blocks83Current advances in versatile metal-organic frameworks for cancer therapy29Controlled Shape Evolution of Pure‐MOF 1D Microcrystals towards Efficient Waveguide and Laser Applications22Design and Property Modulation of Metal–Organic Frameworks with Aggregation-Induced Emission148Lanthanide-doped metal-organic frameworks with multicolor mechanoluminescence25Metal–organic framework25Recent advances in luminescent metal–organic frameworks and their photonic applications57Aggregation-Induced Emission Properties in Fully π-Conjugated Polymers, Dendrimers, and Oligomers65Metal–Organic Layers with an Enhanced Two-Photon Absorption Cross-Section and Up-Converted Emission16Phosphor-Free Electrically Driven White Light Emission from Nanometer-Thick Barium–Organic Framework Films12Nonlinear Optical Properties of Emerging Nano‐ and Microcrystalline Materials100Structural Landscape of Zn(II) and Cd(II) Coordination Compounds with Two Isomeric Triimidazole Luminophores: Impact of Crystal Packing Patterns on Emission Properties15Hydrogen-Bonded Organic Framework Microlasers with Conformation-Induced Color-Tunable Output62Anisotropic Two-Photon Absorption and Second Harmonic Generation in Single Crystals of Silver(I) Coordination Complexes13Multi-photon absorption properties of semiconducting nanomaterials2Porous nickel oxide micron polyhedral particles for high-performance ultrafast photonics76Energy Transfer and Fabry-Perot Oscillation: A New Paradigm for Electrically Driven Laser in Quasi-2D Ruddlesden-Popper Perovskite Microplates Film0Framework-Shrinkage-Induced Wavelength-Switchable Lasing from a Single Hydrogen-Bonded Organic Framework Microcrystal38Novel Binary Ni-Based Mixed Metal–Organic Framework Nanosheets Materials and Their High Optical Power Limiting11Research progress in AIE-based crystalline porous materials for biomedical applications27Phenothiazine metal-organic framework materials with excellent third-order nonlinear properties15Progress in the Application of MOFs in the Field of Atmospheric Environment0Extremely Stable Thorium‐MOF Assembly of Tetraphenylethylene Derivative With Tunable AIE Property and Highly Selective Detection of Nitro Aromatic Compounds28Highly Luminescent Metal–Organic Frameworks Based on Binary Chromophoric Ligands Derived from Tetraphenylethylene9Electrically regulating nonlinear optical limiting of metal-organic framework film155Dual-Color 2D Lead–Organic Framework with Two-Fold Interlocking Structures for the Detection of Nitrofuran Antibiotics and 2,6-Dichloro-4-nitroaniline49Advancing metal–organic frameworks’ materials chemistry0Directional design of carboxylic acid coordination number fine-tuned space structure to improve the output performance of nanogenerators4Integrating a fluorinated photoactive chromophore into metal–organic frameworks for selective trifluoroethylation of styrenes8Ligand-regulated photoinduced electron transfer within metal–organic frameworks for efficient photocatalysis34Locking Effect in Metal@MOF with Superior Stability for Highly Chemoselective Catalysis174Fabry–Perot Oscillation and Resonance Energy Transfer: Mechanism for Ultralow-Threshold Optically and Electrically Driven Random Laser in Quasi-2D Ruddlesden–Popper Perovskites19Enhancement in Two-Photon Absorption and Photoluminescence in Single Crystals of Cd(II) Metal Organic Frameworks30Intra-cavity laser-assisted solar-energy conversion1Why Ligand Doping Increases the Fluorescence of an Anthracene-Based Metal–Organic Framework7Nonlinear Metal–Organic Framework Crystals for Efficient Multicolor Coherent Optical Emission39UiO-66 metal organic framework as stable platform for non-linear optical applications9Self‐Assembly of Hydrogen‐Bonded Organic Crystals on Arbitrary Surfaces for Efficient Amplified Spontaneous Emission22Tunable Nonlinear Optical Properties Based on Metal–Organic Framework Single Crystals26Adaptive Helical Chirality in Supramolecular Microcrystals for Circularly Polarized Lasing29Adaptive Helical Chirality in Supramolecular Microcrystals for Circularly Polarized Lasing0Metal–organic frameworks for nonlinear optics and lasing17Multiple Stimulus Response Material Based on Sr-tcbpe MOF for Mechanochromism, Visualization Labeling, and Etching Toward TNP21Topochemical Polymerization at Diacetylene Metal–Organic Framework Thin Films for Tuning Nonlinear Optics49Enhancing Two-Photon Excited Fluorescence of Metal–Organic Framework Single Crystals through Modulation of Inorganic Nodes6Emission Library and Applications of 2,1,3‐Benzothiadiazole and Its Derivative‐Based Luminescent Metal–Organic Frameworks24Emission Library and Applications of 2,1,3‐Benzothiadiazole and Its Derivative‐Based Luminescent Metal–Organic Frameworks0Development of colorimetric probe using robust zinc-MOF and its consistent melamine sponge composite: Instantaneous N3–, La3+ sensing and degradation applications29Multiphoton Excited Fluorescence Imaging over Metal‐Organic Frameworks2High performance core-shell Fe2O3@N-C anode materials derived from iron concentrate leachate for lithium ion batteries0Boosting One‐ and Two‐Photon Excited Fluorescence of Interpenetrated Tetraphenylethene‐Based Metal–Organic Frameworks (TPE‐MOFs) by Linker Installation20Boosting One‐ and Two‐Photon Excited Fluorescence of Interpenetrated Tetraphenylethene‐Based Metal–Organic Frameworks (TPE‐MOFs) by Linker Installation1Cavity Controlled Nonlinear Optical Filtering of Second Harmonic Signal in Metal Organic Framework Single Crystals4Synthesis, structural characterisation, luminescence properties and DFT calculations of a new 2D polymeric network of cadmium (II)3Metal-Metal Oxide, Metal-Organic Framework Nanocomposites for Energy Storage, Thermal Management, Radiation Shielding, and Magnetic Investigations with Quantum Computing2Layer-by-Layer Growth of an Oriented Tetraphenylethylene-Based MOF Thin Film for Fluorescence Sensing5Modulating Two‐Photon Absorption in a Pyrene‐Based MOF Series: An In‐Depth Investigation of Structure–Property Relationships4Comparative analysis of structural, optical, thermal, and nonlinear optical properties of imidazole L-tartrate and its derivatives for advanced optoelectronic applications0Design, synthesis, and applications of luminescent porous materials with aggregation-induced emission properties: a comprehensive review23Exploration of Two‐photon/Multi‐photon Excited Luminescence in Metal−Organic Frameworks ( MOFs ) †6Tailored synthetic strategies for tetraphenylethylene-based metal–organic frameworks: design, construction, and control7Metal–organic frameworks (MOFs) for nonlinear optical properties: design principles, DFT insights, and future directions for photonic applications1Organic micro-nanophotonics: Materials, devices and integrated circuits1Homochiral Metal–Organic Framework Microcrystals for Circularly Polarized Lasing4Two-photon luminescent MOFs/MOCs for biomedical applications0Molecular Geometry Modulation of Cd(II) Metal–Organic Frameworks for Enhanced Two-Photon Excited Fluorescence in Single Crystals0Intermolecular packing effects on the two-photon absorption of the H4TCPE linker0Heteronuclear MOF Heterostructures Based on Identical Auxiliary‐Ligand Bridging for Multi‐Function‐Integrated Photonic Devices4Dual–Wavelength Cascade Laser of Highly Emissive Lanthanide Organic Framework0Intrinsic Large‐Unit‐Cell Systems for Advanced Thermoelectrics and Thermal Management0Two-Photon Excited Fluorescence of Tetraphenylethylene-Based Metal–Organic Frameworks under Pressure with Different Ligand Arm Lengths0

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  3. Multiphotonenabsorption in Metall‐organischen Gerüstverbindungen

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  4. Warm-White-Light-Emitting Diode Based on a Dye-Loaded Metal–Organic Framework for Fast White-Light Communication

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  5. A 3D metal-organic framework with a pcu net constructed from lead(II) and thiophene-2, 5-dicarboxylic acid: Synthesis, structure and ferroelectric property

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  6. A Two‐Photon Luminescent Dye‐Loaded Metal–Organic Framework for Physiological Temperature Sensing within Biological Windows

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  7. On the Existence of Excitonic Signatures in the Optical Response of Metal–Organic Frameworks: Comment on “van der Waals Metal–Organic Framework as an Excitonic Material for Advanced Photonics”

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  8. Fabrication of zinc-dicarboxylate- and zinc-pyrazolate-carboxylate-framework thin films through vapour–solid deposition

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  9. Multivariant synthesis, crystal structures and properties of four nickel coordination polymers based on flexible ligands

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  13. Salts and Co-Crystalline Assemblies of Tetra(4-Pyridyl)Ethylene with Di-Carboxylic Acids

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  14. Luminescent Lanthanide MOFs: A Unique Platform for Chemical Sensing

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  15. Nonlinear-Optical Behaviors of a Chiral Metal–Organic Framework Comprised of an Unusual Multioriented Double-Helix Structure

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  16. Control of Aggregation-Induced Emission from a Tetraphenylethene Derivative through the Components in the Co-crystal

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  18. Electronic Structure and Optical Response of Zn‐Based Metal–Organic Frameworks

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  19. Hypoxia-Triggered Nanoscale Metal–Organic Frameworks for Enhanced Anticancer Activity

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  20. Anionic Lanthanide Metal–Organic Frameworks: Selective Separation of Cationic Dyes, Solvatochromic Behavior, and Luminescent Sensing of Co(II) Ion

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  22. Second harmonic generation from metal-organic framework derivatives

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  23. Albumin-Stabilized Metal–Organic Nanoparticles for Effective Delivery of Metal Complex Anticancer Drugs

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  24. Highly Porous Nanocrystalline UiO-66 Thin Films via Coordination Modulation Controlled Step-by-Step Liquid-Phase Growth

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  25. High quantum yield pure blue emission and fast proton conduction from an indium–metal–organic framework

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  30. Spatially defined molecular emitters coupled to plasmonic nanoparticle arrays

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  31. MOF‐Based Organic Microlasers

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  32. Controlling Multiphoton Absorption Efficiency by Chromophore Packing in Metal–Organic Frameworks

    Journal of the American Chemical Society · 2019-06-25

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  33. Metal–Organic Frameworks in Modern Physics: Highlights and Perspectives

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  34. All Roads Lead to Rome: Tuning the Luminescence of a Breathing Catenated Zr-MOF by Programmable Multiplexing Pathways

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  35. Pressure‐Induced Multiphoton Excited Fluorochromic Metal–Organic Frameworks for Improving MPEF Properties

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  36. Pressure‐Induced Multiphoton Excited Fluorochromic Metal–Organic Frameworks for Improving MPEF Properties

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  37. Recent advances in photofunctional polymorphs of molecular materials

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  38. Graphene Sandwich Stable Perovskite Quantum-Dot Light-Emissive Ultrasensitive and Ultrafast Broadband Vertical Phototransistors

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  39. Steric-Hindrance-Controlled Laser Switch Based on Pure Metal–Organic Framework Microcrystals

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  40. Auto-controlled fabrication of a metal-porphyrin framework thin film with tunable optical limiting effects

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  41. Organic solid-state lasers: a materials view and future development

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  42. Pure Metal–Organic Framework Microlasers with Controlled Cavity Shapes

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  43. Interpenetrated Metal–Organic Frameworks with ftw Topology and Versatile Functions

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  44. A new anionic metal–organic framework with suitable pore and PtS-type topology for selective adsorption and separation of cationic dyes

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  45. Postsynthetic Framework Contraction Enhances the Two-Photon Absorption Properties of Pillar-Layered Metal–Organic Frameworks

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  46. Coordination Polymers Based on Highly Emissive Ligands: Synthesis and Functional Properties

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  47. Tetraphenylethene-Based Luminescent Metal–Organic Framework for Effective Differentiation of cis/trans Isomers

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  48. Intrinsic Ultralow-Threshold Laser Action from Rationally Molecular Design of Metal–Organic Framework Materials

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    Krishna Prasad Bera, Saqib Kamal, Arif I. Inamdar, Batjargal Sainbileg, Hung‐I Lin, Yu‐Ming Liao, Rapti Ghosh, Ting-Jia Chang, Yen-Guang Lee, Hou Cheng-Fu, Yun‐Tzu Hsu, Michitoshi Hayashi, Chen‐Hsiung Hung, Tzuoo‐Tsair Luo, Kuang‐Lieh Lu, Yang‐Fang Chen

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