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RESEARCH PAPER · Nano Research · 2017

Enhancing both selectivity and coking-resistance of a single-atom Pd1/C3N4 catalyst for acetylene hydrogenation

Xiaohui Huang, Yujia Xia, Yuanjie Cao, Xusheng Zheng, Haibin Pan, Junfa Zhu, Chao Ma, Hengwei Wang, Junjie Li, Rui You, Shiqiang Wei, Weixin Huang, Junling Lu

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Enhancing both selectivity and coking-resistance of a single-atom Pd1/C3N4 catalyst for acetylene hydrogenationOriginalPd@C core–shell nanoparticles on carbon nanotubes as highly stable and selective catalysts for hydrogenation of acetylene to ethylene46Potential of transition metal atoms embedded in buckled monolayer g-C 3 N 4 as single-atom catalysts101Tailoring the framework composition of carbon nitride to improve the catalytic efficiency of the stabilised palladium atoms109Atomically dispersed Pd catalysts in graphyne nanopore: formation and reactivity27All-solid-state Z-scheme 3,4-dihydroxybenzaldehyde-functionalized Ga2O3/graphitic carbon nitride photocatalyst with aromatic rings as electron mediators for visible-light photocatalytic nitrogen fixation184A systematic theoretical study on FeOx-supported single-atom catalysts: M1/FeOx for CO oxidation110In situ trapped high-density single metal atoms within graphene: Iron-containing hybrids as representatives for efficient oxygen reduction127Review Article: Catalysts design and synthesis via selective atomic layer deposition129Rational Design of Single Molybdenum Atoms Anchored on N‐Doped Carbon for Effective Hydrogen Evolution Reaction515Rational Design of Single Molybdenum Atoms Anchored on N‐Doped Carbon for Effective Hydrogen Evolution Reaction104Supported single-atom catalysts: synthesis, characterization, properties, and applications138Strategies for Stabilizing Atomically Dispersed Metal Catalysts377Single-atom catalysts and their applications in organic chemistry224Defect Effects on TiO 2 Nanosheets: Stabilizing Single Atomic Site Au and Promoting Catalytic Properties1035Designed Precursor for the Controlled Synthesis of Highly Active Atomic and Sub‐nanometric Platinum Catalysts on Mesoporous Silica17Revealing the Active Species for Aerobic Alcohol Oxidation by Using Uniform Supported Palladium Catalysts129Revealing the Active Species for Aerobic Alcohol Oxidation by Using Uniform Supported Palladium Catalysts41A Polymer Encapsulation Strategy to Synthesize Porous Nitrogen‐Doped Carbon‐Nanosphere‐Supported Metal Isolated‐Single‐Atomic‐Site Catalysts303Single-atom heterogeneous catalysts based on distinct carbon nitride scaffolds181Theoretical investigation of selective hydrogenation of 1,3-butadiene on Pt doping Cu nanoparticles16BNPd single-atom catalysts for selective hydrogenation of acetylene to ethylene: a density functional theory study7Kinetics of phenylacetylene selective hydrogenation to styrene over metal-free polymeric carbon nitrides17Single-atom catalyst: a rising star for green synthesis of fine chemicals386Nature of active palladium sites on nitrogen doped carbon nanofibers in selective hydrogenation of acetylene25Carbon‐Supported Single Atom Catalysts for Electrochemical Energy Conversion and Storage715The DFT Study of Single-Atom Pd1/g-C3N4 Catalyst for Selective Acetylene Hydrogenation Reaction30Highly Stable Single‐Atom Catalyst with Ionic Pd Active Sites Supported on N‐Doped Carbon Nanotubes for Formic Acid Decomposition119Toward Understanding of the Support Effect on Pd 1 Single-Atom-Catalyzed Hydrogenation Reactions88Single Atom Catalysts on Carbon‐Based Materials219Catalysis with Two-Dimensional Materials Confining Single Atoms: Concept, Design, and Applications1102Room-Temperature Tandem Condensation-Hydrogenation Catalyzed by Porous C3N4 Nanosheet-Supported Pd Nanoparticles17A flower-like Zn 3 V 2 O 8 /Ag composite with enhanced visible light driven photocatalytic activity: the triple-functional roles of Ag nanoparticles25Oxygen-assisted stabilization of single-atom Au during photocatalytic hydrogen evolution78Surface coordination chemistry on graphene and two-dimensional carbon materials for well-defined single atom supported catalysts46Enzymes Immobilized on Carbon Nitride (C3N4) Cooperating with Metal Nanoparticles for Cascade Catalysis33Recent Advances for MOF‐Derived Carbon‐Supported Single‐Atom Catalysts451Metal organic frameworks derived single atom catalysts for electrocatalytic energy conversion542Pd Single‐Atom Catalysts on Nitrogen‐Doped Graphene for the Highly Selective Photothermal Hydrogenation of Acetylene to Ethylene416Review of Metal Catalysts for Oxygen Reduction Reaction: From Nanoscale Engineering to Atomic Design876A General One‐Pot Methodology for the Preparation of Mono‐ and Bimetallic Nanoparticles Supported on Carbon Nanotubes: Application in the Semi‐hydrogenation of Alkynes and Acetylene35Gold nanoparticles supported on MgOx-Al2O3 composite oxide: An efficient catalyst for selective hydrogenation of acetylene40Supported Noble‐Metal Single Atoms for Heterogeneous Catalysis371Mesoporous Nitrogen‐Doped Carbon‐Nanosphere‐Supported Isolated Single‐Atom Pd Catalyst for Highly Efficient Semihydrogenation of Acetylene220Beneficial role of the nitrogen-doped carbon nanotubes in the synthesis of the active palladium supported catalyst12Atomic layer deposition: Catalytic preparation and modification technique for the next generation36Versatile Applications of Metal Single‐Atom @ 2D Material Nanoplatforms175Enhanced stability of Pd/SPS catalyst over the one-pot liquid-phase synthesis of methyl isobutyl ketone by adding GO6Selective Hydrogenation over Supported Metal Catalysts: From Nanoparticles to Single Atoms1609Anchoring Cu1 species over nanodiamond-graphene for semi-hydrogenation of acetylene333A Theory/Experience Description of Support Effects in Carbon-Supported Catalysts735Nitrogen Doped Carbon Nanotubes and Nanofibers for Green Hydrogen Production: Similarities in the Nature of Nitrogen Species, Metal–Nitrogen Interaction, and Catalytic Properties29Transforming Energy with Single-Atom Catalysts349Structure Sensitivity of Acetylene Semi-Hydrogenation on Pt Single Atoms and Subnanometer Clusters171Selectively catalytic hydrogenation of styrene-butadiene rubber over Pd/g-C3N4 catalyst27A DFT Study of Acetylene Hydrogenation Catalyzed by S-Doped Pd1/g-C3N411Reactive Metal–Biopolymer Interactions for Semihydrogenation of Acetylene46Adsorption and catalytic activation of N2 molecule on iron dimer supported by different two-dimensional carbon-based substrates: A computational study30Atomic-scale engineering of metal–oxide interfaces for advanced catalysis using atomic layer deposition46Dopamine polymer derived isolated single-atom site metals/N-doped porous carbon for benzene oxidation32Progress in the Selective Semi-hydrogenation of Alkynes by Nanocatalysis9Roles of Coordination Geometry in Single-Atom Catalysts5Structural Regulation with Atomic-Level Precision: From Single-Atomic Site to Diatomic and Atomic Interface Catalysis341Carbon-Based Single-Atom Catalysts for Advanced Applications747Selective Hydrogenation of Acetylene Catalysed by a B12N12 Cluster Doped with a Single Nickel Atom: A DFT Study11Isolated iron sites embedded in graphitic carbon nitride (g-C3N4) for efficient oxidative desulfurization131Carbon Nitride as a Ligand: Selective Hydrogenation of Terminal Alkenes Using [(η5‐C5Me5)IrCl(g‐C3N4‐κ2N,N’)]Cl15Superior Catalytic Performance of Atomically Dispersed Palladium on Graphene in CO Oxidation64Copper Catalysts in Semihydrogenation of Acetylene: From Single Atoms to Nanoparticles207Inherently Selective Atomic Layer Deposition and Applications121Adsorption Site Regulation to Guide Atomic Design of Ni–Ga Catalysts for Acetylene Semi‐Hydrogenation200Adsorption Site Regulation to Guide Atomic Design of Ni–Ga Catalysts for Acetylene Semi‐Hydrogenation35Selective continuous flow phenylacetylene hydrogenation over Pd-biogenic calcium carbonate11Single-atom catalysis enables long-life, high-energy lithium-sulfur batteries322Single Vanadium Atoms Anchored on Graphitic Carbon Nitride as a High-Performance Catalyst for Non-oxidative Propane Dehydrogenation102Enhancement of Alkyne Semi-Hydrogenation Selectivity by Electronic Modification of Platinum49A Review on Particle Size Effect in Metal‐Catalyzed Heterogeneous Reactions148Single‐Atom Catalysts for Electrocatalytic Applications741Atomically dispersed catalysts for hydrogen/oxygen evolution reactions and overall water splitting106A Promoted Charge Separation/Transfer System from Cu Single Atoms and C 3 N 4 Layers for Efficient Photocatalysis528Structural Regulation and Support Coupling Effect of Single‐Atom Catalysts for Heterogeneous Catalysis307Selective hydrogenation of acetylene on graphene-supported non-noble metal single-atom catalysts45Surface Coordination Chemistry of Atomically Dispersed Metal Catalysts596Synthesis of Zn doped g-C3N4 in KCl-ZnCl2 molten salts: The temperature window for promoting the photocatalytic activity28Recent advances and strategies in the stabilization of single‐atom catalysts for electrochemical applications68Supported Metal Clusters: Fabrication and Application in Heterogeneous Catalysis505Isolated Single Atoms Anchored on N-Doped Carbon Materials as a Highly Efficient Catalyst for Electrochemical and Organic Reactions143Making g-C3N4 ultra-thin nanosheets active for photocatalytic overall water splitting212Preparation of MoS2 nanosheets to support Pd species for selective steerable hydrogenation of acetylene12A Perspective on New Opportunities in Atom-by-Atom Synthesis of Heterogeneous Catalysts Using Atomic Layer Deposition51Magnetic selenium-doped graphitic carbon nitride nanocomposite as an effective catalyst support for stabilization of Cu NPs19Graphdiyne‐Supported Atomic Catalysts: Synthesis and Applications14Ligand Stabilized Ni1 Catalyst for Efficient CO Oxidation5C2H2 semi-hydrogenation on the PdxMy cluster/graphdiyne catalysts: Effects of cluster composition and size on the activity and selectivity19Single-Atom Catalysts across the Periodic Table1366Single-Atom Catalysts Based on the Metal–Oxide Interaction1085Recent Advances in Graphitic Carbon Nitride Supported Single‐Atom Catalysts for Energy Conversion79Single-Atom Catalysts for Thermal Heterogeneous Catalysis in Liquid: Recent Progress and Future Perspective20Ni catalyst supported on nitrogen-doped activated carbon for selective hydrogenation of acetylene with high concentration32Direct Synthesis of Atomically Dispersed Palladium Atoms Supported on Graphitic Carbon Nitride for Efficient Selective Hydrogenation Reactions54Synthesis of Quasi‐Bilayer Subnano Metal‐Oxide Interfacial Cluster Catalysts for Advanced Catalysis16Carbon-Based Materials for the Development of Highly Dispersed Metal Catalysts: Towards Highly Performant Catalysts for Fine Chemical Synthesis36A review of the hot spot analysis and the research status of single-atom catalysis based on the bibliometric analysis10Copper-based single-atom alloys for heterogeneous catalysis47Metal single-atom catalysts for selective hydrogenation of unsaturated bonds89Metal-doped carbon nitrides: synthesis, structure and applications50Noble-metal single-atoms in thermocatalysis, electrocatalysis, and photocatalysis388Regulating Pd/Al 2 O 3 catalyst by g-C 3 N 4 toward the enhanced selectivity of isoprene hydrogenation6Size-dependent strong metal–support interaction in Pd/ZnO catalysts for hydrogenation of CO 2 to methanol47Surface modification and functionalization of powder materials by atomic layer deposition: a review73Single Metal Atom Decorated Carbon Nitride for Efficient Photocatalysis: Synthesis, Structure, and Applications71Single copper sites dispersed on defective TiO2−x as a synergistic oxygen reduction reaction catalyst11Photochemical Solid-Phase In Situ Anchoring of Single Atoms Ag/g-C 3 N 4 for Enhanced Photocatalytic Activity7Adsorption Behavior and Electron Structure Engineering of Pd-IL Catalysts for Selective Hydrogenation of Acetylene21Pd Catalysts Supported on Bamboo-Like Nitrogen-Doped Carbon Nanotubes for Hydrogen Production21Recent Advancements of Porphyrin‐Like Single‐Atom Catalysts: Synthesis and Applications106Toward efficient single-atom catalysts for renewable fuels and chemicals production from biomass and CO2175Single atom catalysts by atomic diffusion strategy82Mechanistic insight into the hydrogenation of acetylene on the Pd2/g-C3N4 catalyst: effect of Pd clustering on the barrier energy and selectivity4Highly Selective Acetylene Semihydrogenation Catalyst with an Operation Window Exceeding 150 °C58Single noble metal atoms doped 2D materials for catalysis94Single-Atom Catalysts Designed and Prepared by the Atomic Layer Deposition Technique344Different catalytic behavior of Pd/Palygorskite catalysts for semi-hydrogenation of acetylene20Electrocatalytic Nitrogen Reduction by Transition Metal Single-Atom Catalysts on Polymeric Carbon Nitride40Synthesis of novel Ag-modified Pd-supported mesoporous carbon nitride for selective hydrogenation of acetylene with an excellence ethylene selectivity7Atomically dispersed Palladium-Ethylene Glycol- Bismuth oxybromide for photocatalytic nitrogen fixation: Insight of molecular bridge mechanism41Integration of Bimetallic Electronic Synergy with Oxide Site Isolation Improves the Selective Hydrogenation of Acetylene108Integration of Bimetallic Electronic Synergy with Oxide Site Isolation Improves the Selective Hydrogenation of Acetylene8N-containing silane coupling agent-assisted synthesis of highly dispersed and stable PdC phase for semi-hydrogenation of acetylene10Atomically dispersed Pd electrocatalyst for efficient aqueous phase dechlorination reaction44Synergizing metal–support interactions and spatial confinement boosts dynamics of atomic nickel for hydrogenations383Excellent stability of Pd/mpg-C3N4 in catalytic hydrodebenzylation of 2,4,6,8,10,12-Hexabenzyl-2,4,6,8,10,12- hexaazaisowurtzitane (HBIW)17Theoretical studies about C2H2 semi-hydrogenation on the carbon material supported metal cluster catalysts: Influences of support type and cluster size on the catalytic performance10Grafting nanometer metal/oxide interface towards enhanced low-temperature acetylene semi-hydrogenation100Factors Influencing the Performance of Copper-Bearing Catalysts in the CO 2 Reduction System103Toward Multicomponent Single-Atom Catalysis for Efficient Electrochemical Energy Conversion50Advanced Support Materials and Interactions for Atomically Dispersed Noble‐Metal Catalysts: From Support Effects to Design Strategies216Constructing Pd-N interactions in Pd/g-C3N4 to improve the charge dynamics for efficient photocatalytic hydrogen evolution39Recent progress in electrochemical reduction of carbon dioxide on metal single‐atom catalysts23Pd/Fe2O3 with Electronic Coupling Single-Site Pd–Fe Pair Sites for Low-Temperature Semihydrogenation of Alkynes176Fe 2 O 3 supported Pt single atom catalysts for the selective hydrogenation of cinnamaldehyde8Interfacing single-atom catalysis with continuous-flow organic electrosynthesis123Localized surface plasmon resonance effect enhanced Cu/TiO 2 core–shell catalyst for boosting CO 2 hydrogenation reaction36Single-atom site catalysts based on high specific surface area supports36Pyrolysis Temperature Tunes the Catalytic Properties of CuBTC-Derived Carbon-Embedded Copper Catalysts for Partial Hydrogenation24Recent progress on two-dimensional materials confining single atoms for CO2 photoreduction40Tuning selectivity in the gas phase hydrogenation of phenylacetylene over the platinum—mesoporous carbon nitride composites using organic modifiers2C2H2 semi-hydrogenation over Cu catalysts: Revealing the influence of Cu active site types on the catalytic performance7Construction of single-atom catalysts for electro-, photo- and photoelectro-catalytic applications: State-of-the-art, opportunities, and challenges66Distinct Crystal‐Facet‐Dependent Behaviors for Single‐Atom Palladium‐On‐Ceria Catalysts: Enhanced Stabilization and Catalytic Properties254Pt-O4 moiety induced electron localization toward In2O-Triggered acetylene Semi-Hydrogenation26

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  2. Potential of transition metal atoms embedded in buckled monolayer g-C 3 N 4 as single-atom catalysts

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  4. Atomically dispersed Pd catalysts in graphyne nanopore: formation and reactivity

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  19. Single-atom heterogeneous catalysts based on distinct carbon nitride scaffolds

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  41. Gold nanoparticles supported on MgOx-Al2O3 composite oxide: An efficient catalyst for selective hydrogenation of acetylene

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  43. Mesoporous Nitrogen‐Doped Carbon‐Nanosphere‐Supported Isolated Single‐Atom Pd Catalyst for Highly Efficient Semihydrogenation of Acetylene

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  44. Beneficial role of the nitrogen-doped carbon nanotubes in the synthesis of the active palladium supported catalyst

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  47. Enhanced stability of Pd/SPS catalyst over the one-pot liquid-phase synthesis of methyl isobutyl ketone by adding GO

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  48. Selective Hydrogenation over Supported Metal Catalysts: From Nanoparticles to Single Atoms

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  49. Anchoring Cu1 species over nanodiamond-graphene for semi-hydrogenation of acetylene

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