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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2017

Highly Selective Separation of C2H2 from CO2 by a New Dichromate-Based Hybrid Ultramicroporous Material

Hayley S. Scott, Mohana Shivanna, Alankriti Bajpai, David Gerard Madden, Kai‐Jie Chen, Tony Pham, Katherine A. Forrest, Adam Hogan, Brian Space, John J. Perry, Michael John Zaworotko

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Highly Selective Separation of C2H2 from CO2 by a New Dichromate-Based Hybrid Ultramicroporous MaterialOriginalGas/vapour separation using ultra-microporous metal–organic frameworks: insights into the structure/separation relationship1324The effect of centred versus offset interpenetration on C 2 H 2 sorption in hybrid ultramicroporous materials59Enhanced Stability toward Humidity in a Family of Hybrid Ultramicroporous Materials Incorporating Cr2O72– Pillars16Simulations of hydrogen, carbon dioxide, and small hydrocarbon sorption in a nitrogen-rich rht -metal–organic framework17Crystal engineering of dichromate pillared hybrid ultramicroporous materials incorporating pyrazole-based ligands13Enhanced gas separation performance of an ultramicroporous pillared-layer framework induced by hanging bare Lewis basic pyridine groups35Theoretical study of the effect of halogen substitution in molecular porous materials for CO2 and C2H2 sorption4Upgrading gasoline to high octane numbers using a zeolite-like metal–organic framework molecular sieve with ana -topology28Efficient CO 2 Removal for Ultra ‐ Pure CO Production by Two Hybrid Ultramicroporous Materials18Efficient CO2 Removal for Ultra‐Pure CO Production by Two Hybrid Ultramicroporous Materials60Nanospace within metal–organic frameworks for gas storage and separation121Highly efficient separation of methane from nitrogen on a squarate‐based metal‐organic framework136A thermostable anion-pillared metal-organic framework for C2H2/C2H4 and C2H2/CO2 separations108Investigating C2H2 Sorption in α-[M3(O2CH)6] (M = Mg, Mn) Through Theoretical Studies2In Silico Screening of MOFs with open copper sites for C2H2/CO2 separation36Additive-Induced Supramolecular Isomerism and Enhancement of Robustness in Co(II)-Based MOFs for Efficiently Trapping Acetylene from Acetylene-Containing Mixtures90Achieving Superprotonic Conduction with a 2D Fluorinated Metal–Organic Framework136High Yield, Low-Waste Synthesis of a Family of Pyridyl and Imidazolyl-Substituted Schiff Base Linker Ligands17A calcium-based microporous metal-organic framework for efficient adsorption separation of light hydrocarbons90Inverse Adsorption Separation of CO 2 /C 2 H 2 Mixture in Cyclodextrin-Based Metal–Organic Frameworks202Metal-organic framework based carbon capture and purification technologies for clean environment43Reversing C 2 H 2 –CO 2 adsorption selectivity in an ultramicroporous metal–organic framework platform53Water-Stable Europium 1,3,6,8-Tetrakis(4-carboxylphenyl)pyrene Framework for Efficient C2H2/CO2 Separation91Investigating CO2 Sorption in SIFSIX-3-M (M = Fe, Co, Ni, Cu, Zn) through Computational Studies69Multipurpose Metal–Organic Framework for the Adsorption of Acetylene: Ethylene Purification and Carbon Dioxide Removal175MPMC and MCMD: Free High‐Performance Simulation Software for Atomistic Systems17A hydrostable cage-based MOF with open metal sites and Lewis basic sites immobilized in the pore surface for efficient separation and purification of natural gas and C 2 H 290An N -oxide-functionalized nanocage-based copper-tricarboxylate framework for the selective capture of C 2 H 233Crystal engineering of porous coordination networks to enable separation of C2 hydrocarbons184Inverse and highly selective separation of CO 2 /C 2 H 2 on a thulium–organic framework203Metal–organic frameworks for C 2 H 2 /CO 2 separation86Optimized nanospace of coordination isomers with selenium sites for acetylene separation13Two Co-based MOFs assembled from an amine-functionalized pyridinecarboxylate ligand: inorganic acid-directed structural variety and gas adsorption properties15Halogen–C2H2 Binding in Ultramicroporous Metal–Organic Frameworks (MOFs) for Benchmark C2H2/CO2 Separation Selectivity89Insights into the Gas Adsorption Mechanisms in Metal–Organic Frameworks from Classical Molecular Simulations37Mixed Metal–Organic Framework with Multiple Binding Sites for Efficient C 2 H 2 /CO 2 Separation439Mixed Metal–Organic Framework with Multiple Binding Sites for Efficient C2H2/CO2Separation50Selective Acetylene Adsorption within an Imino-Functionalized Nanocage-Based Metal–Organic Framework50Immobilization of Oxygen Atoms in the Pores of Microporous Metal–Organic Frameworks for C 2 H 2 Separation and Purification111RETRACTED ARTICLE: A porous Co(II)–MOF for selective C 2 H 2 /CO 2 separation and treatment activity on virus-induced COPD via reducing tlr3 gene expression1A Chemically Stable Hofmann‐Type Metal−Organic Framework with Sandwich‐Like Binding Sites for Benchmark Acetylene Capture385Rational Design of Microporous MOFs with Anionic Boron Cluster Functionality and Cooperative Dihydrogen Binding Sites for Highly Selective Capture of Acetylene184Rational Design of Microporous MOFs with Anionic Boron Cluster Functionality and Cooperative Dihydrogen Binding Sites for Highly Selective Capture of Acetylene40Gallate-Based Metal–Organic Frameworks for Highly Efficient Removal of Trace Propyne from Propylene26A chemically stable nanoporous coordination polymer with fixed and free Cu2+ ions for boosted C2H2/CO2 separation56Metrics for Evaluation and Screening of Metal–Organic Frameworks for Applications in Mixture Separations119Theoretical study of strain-controlled C2X (X = N, O) membrane for CO2/C2H2 separation15Excellent separation performance in a mesoporous MOF induced by 1D rhombic channels and bare nitrogen-donor sites5Rational design and synthesis of ultramicroporous metal-organic frameworks for gas separation218Two dimensional Ti-based metal-organic framework with polar oxygen atoms on the pore surface for efficient gas separation8Highly Robust Tetranuclear Cobalt-Based 3D Framework for Efficient C2H2/CO2 and C2H2/C2H4Separations14Thin film synthesis of hybrid ultramicroporous materials (HUMs)- a comparative approach7A square lattice topology coordination network that exhibits highly selective C2H2/CO2 separation performance12A new metal–organic framework based on rare [Zn 4 F 4 ] cores for efficient separation of C 2 H 215A window-space-directed assembly strategy for the construction of supertetrahedron-based zeolitic mesoporous metal–organic frameworks with ultramicroporous apertures for selective gas adsorption30Highly selective CO 2 separation from a CO 2 /C 2 H 2 mixture using a diamine-appended metal–organic framework49Molecular engineering in a family of pillared-layered metal–organic frameworks for tuning gas adsorption behavior6A MOF‐based Ultra‐Strong Acetylene Nano‐trap for Highly Efficient C2H2/CO2 Separation291A MOF‐based Ultra‐Strong Acetylene Nano‐trap for Highly Efficient C2H2/CO2 Separation74Selective capture of carbon dioxide from hydrocarbons using a metal-organic framework350Regulation on Topological Architectures and Gas Adsorption for Cadmium-Azolate-Carboxylate Frameworks by the Ligand Flexibility34Cage‐Like Porous Materials with Simultaneous High C2H2Storage and Excellent C2H2/CO2Separation Performance28Cage‐Like Porous Materials with Simultaneous High C2H2Storage and Excellent C2H2/CO2Separation Performance171An Isomeric Copper‐Diisophthalate Framework Platform for Storage and Purification of C 2 H 2 and Exploration of the Positional Effect of the Methyl Group7Modulation of Topological Structures and Adsorption Properties of Copper-Tricarboxylate Frameworks Enabled by the Effect of the Functional Group and Its Position9Efficient Capture of Trace Acetylene by an Ultramicroporous Metal–Organic Framework with Purine Binding Sites38Interpenetration Symmetry Control Within Ultramicroporous Robust Boron Cluster Hybrid MOFs for Benchmark Purification of Acetylene from Carbon Dioxide213Interpenetration Symmetry Control Within Ultramicroporous Robust Boron Cluster Hybrid MOFs for Benchmark Purification of Acetylene from Carbon Dioxide25Metal–Organic Frameworks Featuring 18-Connected Nonanuclear Rare-Earth Oxygen Clusters and Cavities for Efficient C2H2/CO2 Separation16Dense Packing of Acetylene in a Stable and Low‐Cost Metal–Organic Framework for Efficient C2H2/CO2 Separation207Dense Packing of Acetylene in a Stable and Low‐Cost Metal–Organic Framework for Efficient C2H2/CO2 Separation16Tuning the Selectivity between C2H2 and CO2 in Molecular Porous Materials15An ultra-stable Zr(IV)-MOF for highly efficient capture of SO2 from SO2/CO2 and SO2/CH4 mixtures70The First Sulfate‐Pillared Hybrid Ultramicroporous Material, SOFOUR‐1‐Zn, and Its Acetylene Capture Properties7The First Sulfate‐Pillared Hybrid Ultramicroporous Material, SOFOUR‐1‐Zn, and Its Acetylene Capture Properties66Metal–Organic Framework Based Hydrogen-Bonding Nanotrap for Efficient Acetylene Storage and Separation359A Review on Anion-Pillared Metal Organic Framework (Apmof) and its Composites with the Balance of Adsorption Capacity and Separation Selectivity for Efficient Gas Separation1An ato-topology metal–organic framework with large C 2 H 2 adsorption and C 2 H 2 /CO 2 separation capacity5Recent advances in microporous metal–organic frameworks as promising adsorbents for gas separation83Shell‐like Xenon Nano‐Traps within Angular Anion‐Pillared Layered Porous Materials for Boosting Xe/Kr Separation15Shell‐like Xenon Nano‐Traps within Angular Anion‐Pillared Layered Porous Materials for Boosting Xe/Kr Separation75Flexible molecular sieving of C2H2 from CO2 by a new cost-effective metal organic framework with intrinsic hydrogen bonds48A structural study into halogenated derivatives of mandelic acid as building blocks of chiral coordination polymers2Integrating tri-mural nanotraps into a microporous metal-organic framework for C2H2/CO2 and C2H2/C2H4 separation46A review on anion-pillared metal–organic frameworks (APMOFs) and their composites with the balance of adsorption capacity and separation selectivity for efficient gas separation102Efficient acetylene/carbon dioxide separation with excellent dynamic capacity and low regeneration energy by anion-pillared hybrid materials2Desolvation-Degree-Induced Structural Dynamics in a Rigid Cerium–Organic Framework Exhibiting Tandem Purification of Ethylene from Acetylene and Ethane18Optimization of Pore-Space-Partitioned Metal–Organic Frameworks Using the Bioisosteric Concept89Separating water isotopologues using diffusion-regulatory porous materials310A new perchlorate-based hybrid ultramicroporous material with rich bare oxygen atoms for high C2H2/CO2 separation39High-throughput computational screening of adsorbents and membrane materials for acetylene capture9CO2-Selective Capture from Light Hydrocarbon Mixtures by Metal-Organic Frameworks: A Review21A Stable Cd(Ii)-Mof for Efficient Separation of Trace So2 from So2/Co2/N2 Mixture0An ultramicroporous multi-walled metal–organic framework for efficient C 2 H 2 /CO 2 separation under humid conditions19Inverse CO 2 /C 2 H 2 separation assisted by coordinated water in a dysprosium( iii ) metal–organic framework14De‐Linker‐Enabled Exceptional Volumetric Acetylene Storage Capacity and Benchmark C2H2/C2H4and C2H2/CO2Separations in Metal–Organic Frameworks96De‐Linker‐Enabled Exceptional Volumetric Acetylene Storage Capacity and Benchmark C2H2/C2H4and C2H2/CO2Separations in Metal–Organic Frameworks2Strengthening Intraframework Interaction within Flexible MOFs Demonstrates Simultaneous Sieving Acetylene from Ethylene and Carbon Dioxide71Metal-organic frameworks for C2H2/CO2 separation: Recent development142Vertex Strategy in Layered 2D MOFs: Simultaneous Improvement of Thermodynamics and Kinetics for Record C 2 H 2 /CO 2 Separation Performance109Novel Pillared-Layer-like Metal–Organic Frameworks with Quadrilateral Channels for Efficient Separation of C2H2 from C2H2/CO2 and C2H2/C2H4 Mixtures6Consecutive Single‐Crystal‐to‐Single‐Crystal Isomerization of Novel Octamolybdate Anions within a Microporous Hybrid Framework with Robust Water Sorption Properties6Consecutive Single‐Crystal‐to‐Single‐Crystal Isomerization of Novel Octamolybdate Anions within a Microporous Hybrid Framework with Robust Water Sorption Properties13D Printing of Monoliths Using TIFSIX-Ni-Based Formulations for the Electric Swing Adsorption of CO216High-capacity dynamic exclusion for highly efficient dilute C2H2 separation from CO2 and multicomponent mixture in robust ultramicroporous MOF by topology regulation18A robust indium-organic framework with open tubular channels for efficient separation of acetylene19An In(III)-MOF based on pore engineering for efficient capture SF6 from SF6/N2 mixture33Interlayer Symmetry Control in Flexible-Robust Layered Metal–Organic Frameworks for Highly Efficient C 2 H 2 /CO 2 Separation101An anionic In(III)-MOF for efficient adsorption of CO2 from CO2/N2 mixture and dye removal15Construction and ReO4− adsorption of ionic covalent organic frameworks by solvothermal synthesis based on Zincke reaction26Separation of High-Purity C 2 H 2 from Binary C 2 H 2 /CO 2 Using Robust Al-Based MOFs Comprising Nitrogen-Containing Heterocyclic Dicarboxylate26A microporous Cd(II)-MOF for efficient separation of trace SO2 from SO2/CO2/N2 mixture30Crystal engineering of a new platform of hybrid ultramicroporous materials and their C 2 H 2 /CO 2 separation properties16Flexible–robust MOFs/HOFs for challenging gas separations137A stable Zr(IV)-MOF for efficient removal of trace SO2 from flue gas in dry and humid conditions17Recent Advances of Multidentate Ligand-Based Anion-Pillared MOFs for Enhanced Separation and Purification Processes44Metal-Organic Frameworks based on Newly Designed Polycarboxyaryl Linkers: Versatile Cooperative Non-Covalent Interactions and Applications on Small Hydrocarbon Separation and Carbon Capture0Installing Methyl Group Guards in a Metal–Organic Framework Featuring Multiple N/O Active Sites for Efficient C2H2/CO2 Separation under Moist Conditions13Multifunctional and Ultrastable Co-MOF Effectively Separates Various Different Component Gas Mixtures4One sulfate anion-bridged metal–organic framework for adsorptive separation of C2H2 from C2H4 and CO214Cooperative Immobilization of Transition-Metal Clusters into Kagome-Type Metal–Organic Framework for C2H2/CO2 Separation7Shifting C 2 H 2 /CO 2 Adsorption and Separation in Pillar‐Layered Metal–Organic Frameworks Finely‐Regulated by Molecular Rotation20Functional flexible adsorbents and their potential utility25Scalable copper-based coordination frameworks with tailored pore chemistry for energy-efficient C 2 H 2 /CO 2 separation6Two stable 2D indium(III)/zirconium(IV) metal-organic frameworks for highly efficient C2H2/CO2 separation0Selective separation of acetylene from ethylene using mixed matrix membranes with MIL-100(Fe) as a filler9Anion-Exchange Strategy for Ru/RuO2-Embedded N/S-Co-Doped Porous Carbon Composites for Electrochemical Nitrogen Fixation3Rapid Synthesis of Ultramicroporous Potassium-Pyrenetetracarboxylate Framework with Confined-Space-Charge-Driving CO2 Capture11New Viologen-Based Ionic Porous Organic Polymers for Efficient Removal of Anionic Dyes and Hexavalent Chromium (Cr (VI)) from Water11Review and analysis of porous adsorbents for effective CO2 capture70Zero- to One-Dimensional Transformation in a Highly Porous Metal–Organic Framework to Enhance Physicochemical Properties20Stannum-Doped Bismuth Nanocoral Catalysts for Highly Efficient Electrochemical CO2 Reduction to Formate1Borane cage hybrid supramolecular metal-organic frameworks (BSFs): Design, synthesis and gas separation performance1A Scalable and Cost-Effective Zeolite-Polymer Fiber Sorbent Enabled by Vapor-Induced Cu(I) Activation for Selective Acetylene Capture0Synthesis and structure of two 2D In(III)/Zr(IV)‑MOFs with highly efficient C2H2/CO2 separation0Crystal Engineering of Reticular Materials for Gas‐ and Liquid‐Phase Hydrocarbon Separation4Construction of Octadentate Carboxylate‐Based Metal–Organic Framework for Effective Acetylene Purification3Breathing Effect of Flexible Metal–Organic Frameworks Drives C 2 H 2 /CO 2 Separation0Scalable aqueous synthesis of NJU-Bai5 toward efficient C2H2/CO2 separation under humid conditions0Nanowire-like C2H2 assembly in a flow-channel crystal boosts C2H2/CO2 separation at 348 K0A novel cage-based Ni-MOF for efficient purification of C2H4 from C2H2/CO2/C2H4 mixtures0

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  1. Gas/vapour separation using ultra-microporous metal–organic frameworks: insights into the structure/separation relationship

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  2. The effect of centred versus offset interpenetration on C 2 H 2 sorption in hybrid ultramicroporous materials

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  3. Enhanced Stability toward Humidity in a Family of Hybrid Ultramicroporous Materials Incorporating Cr2O72– Pillars

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  4. Simulations of hydrogen, carbon dioxide, and small hydrocarbon sorption in a nitrogen-rich rht -metal–organic framework

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  5. Crystal engineering of dichromate pillared hybrid ultramicroporous materials incorporating pyrazole-based ligands

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  6. Enhanced gas separation performance of an ultramicroporous pillared-layer framework induced by hanging bare Lewis basic pyridine groups

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  7. Theoretical study of the effect of halogen substitution in molecular porous materials for CO2 and C2H2 sorption

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  8. Upgrading gasoline to high octane numbers using a zeolite-like metal–organic framework molecular sieve with ana -topology

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  9. Efficient CO 2 Removal for Ultra ‐ Pure CO Production by Two Hybrid Ultramicroporous Materials

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  10. Efficient CO2 Removal for Ultra‐Pure CO Production by Two Hybrid Ultramicroporous Materials

    Angewandte Chemie International Edition · 2018-01-29

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  11. Nanospace within metal–organic frameworks for gas storage and separation

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  12. Highly efficient separation of methane from nitrogen on a squarate‐based metal‐organic framework

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  13. A thermostable anion-pillared metal-organic framework for C2H2/C2H4 and C2H2/CO2 separations

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  14. Investigating C2H2 Sorption in α-[M3(O2CH)6] (M = Mg, Mn) Through Theoretical Studies

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  15. In Silico Screening of MOFs with open copper sites for C2H2/CO2 separation

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  16. Additive-Induced Supramolecular Isomerism and Enhancement of Robustness in Co(II)-Based MOFs for Efficiently Trapping Acetylene from Acetylene-Containing Mixtures

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  17. Achieving Superprotonic Conduction with a 2D Fluorinated Metal–Organic Framework

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  18. High Yield, Low-Waste Synthesis of a Family of Pyridyl and Imidazolyl-Substituted Schiff Base Linker Ligands

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  19. A calcium-based microporous metal-organic framework for efficient adsorption separation of light hydrocarbons

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  20. Inverse Adsorption Separation of CO 2 /C 2 H 2 Mixture in Cyclodextrin-Based Metal–Organic Frameworks

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  21. Metal-organic framework based carbon capture and purification technologies for clean environment

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  22. Reversing C 2 H 2 –CO 2 adsorption selectivity in an ultramicroporous metal–organic framework platform

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  23. Water-Stable Europium 1,3,6,8-Tetrakis(4-carboxylphenyl)pyrene Framework for Efficient C2H2/CO2 Separation

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  24. Investigating CO2 Sorption in SIFSIX-3-M (M = Fe, Co, Ni, Cu, Zn) through Computational Studies

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  25. Multipurpose Metal–Organic Framework for the Adsorption of Acetylene: Ethylene Purification and Carbon Dioxide Removal

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  27. A hydrostable cage-based MOF with open metal sites and Lewis basic sites immobilized in the pore surface for efficient separation and purification of natural gas and C 2 H 2

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  28. An N -oxide-functionalized nanocage-based copper-tricarboxylate framework for the selective capture of C 2 H 2

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  29. Crystal engineering of porous coordination networks to enable separation of C2 hydrocarbons

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  30. Inverse and highly selective separation of CO 2 /C 2 H 2 on a thulium–organic framework

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  31. Metal–organic frameworks for C 2 H 2 /CO 2 separation

    Dalton Transactions · 2020-01-01

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  32. Optimized nanospace of coordination isomers with selenium sites for acetylene separation

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    Huijie Wang, Nibedita Behera, Suna Wang, Qiubing Dong, Zhaoxu Wang, Baishu Zheng, Daqi Wang, Jingui Duan

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  33. Two Co-based MOFs assembled from an amine-functionalized pyridinecarboxylate ligand: inorganic acid-directed structural variety and gas adsorption properties

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  34. Halogen–C2H2 Binding in Ultramicroporous Metal–Organic Frameworks (MOFs) for Benchmark C2H2/CO2 Separation Selectivity

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  35. Insights into the Gas Adsorption Mechanisms in Metal–Organic Frameworks from Classical Molecular Simulations

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  36. Mixed Metal–Organic Framework with Multiple Binding Sites for Efficient C 2 H 2 /CO 2 Separation

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    Junkuo Gao, Xuefeng Qian, Rui‐Biao Lin, Rajamani Krishna, Hui Wu, Wei Zhou, Banglin Chen

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  37. Mixed Metal–Organic Framework with Multiple Binding Sites for Efficient C2H2/CO2Separation

    Angewandte Chemie · 2020-01-13

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  38. Selective Acetylene Adsorption within an Imino-Functionalized Nanocage-Based Metal–Organic Framework

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  39. Immobilization of Oxygen Atoms in the Pores of Microporous Metal–Organic Frameworks for C 2 H 2 Separation and Purification

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  40. RETRACTED ARTICLE: A porous Co(II)–MOF for selective C 2 H 2 /CO 2 separation and treatment activity on virus-induced COPD via reducing tlr3 gene expression

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  44. Gallate-Based Metal–Organic Frameworks for Highly Efficient Removal of Trace Propyne from Propylene

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  45. A chemically stable nanoporous coordination polymer with fixed and free Cu2+ ions for boosted C2H2/CO2 separation

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  46. Metrics for Evaluation and Screening of Metal–Organic Frameworks for Applications in Mixture Separations

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  47. Theoretical study of strain-controlled C2X (X = N, O) membrane for CO2/C2H2 separation

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  48. Excellent separation performance in a mesoporous MOF induced by 1D rhombic channels and bare nitrogen-donor sites

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  49. Rational design and synthesis of ultramicroporous metal-organic frameworks for gas separation

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