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RESEARCH PAPER · Journal of Materials Chemistry A · 2016

Ionic liquid-based electrolytes for “beyond lithium” battery technologies

Guinevere A. Giffin

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Ionic liquid-based electrolytes for “beyond lithium” battery technologiesOriginalPrimary Sjogren's syndrome: rarity in India.20A lipophilic ionic liquid based on formamidinium cations and TFSI: the electric response and the effect of CO 2 on the conductivity mechanism2A sodium–aluminum hybrid battery37Development of novel inorganic electrolytes for room temperature rechargeable sodium metal batteries81Graphene-Coated Activated Carbon Fiber Cloth Positive Electrodes for Aluminum Rechargeable Batteries with a Chloroaluminate Room-Temperature Ionic Liquid15Ionic Liquid as an Effective Additive for Rechargeable Magnesium Batteries25Formation of Gd coordination polymer with 1D chains mediated by Bronsted acidic ionic liquids5Effect of Cl− and TFSI− anions on dual electrolyte systems in a hybrid Mg/Li4Ti5O12 battery18Odyssey of Multivalent Cathode Materials: Open Questions and Future Challenges1158Lyotropic Lamellar Structures of a Long-Chain Imidazolium and Their Application as Nanoreactors for X-ray-Initiated Polymerization4First examples of organosilica-based ionogels: synthesis and electrochemical behavior17Electrochemical cycling of Mg in Mg[TFSI] 2 /tetraglyme electrolytes96Magnesium Anode Pretreatment Using a Titanium Complex for Magnesium Battery26Electrochemical Device Applications1Fundamentals of Ionic Liquids197Stretchable Ionic-Liquid-Based Gel Polymer Electrolytes for Lithium-Ion Batteries47Ion pair and solvation dynamics of [Bmim][BF4] + water system26Bifunctional electrocatalysts for Zn–air batteries242Physicochemical Characterization of AlCl3–1-Ethyl-3-methylimidazolium Chloride Ionic Liquid Electrolytes for Aluminum Rechargeable Batteries135Transport and Association of Ions in Lithium Battery Electrolytes Based on Glycol Ether Mixed with Halogen-Free Orthoborate Ionic Liquid45Challenges, mitigation strategies and perspectives in development of zinc-electrode materials and fabrication for rechargeable zinc–air batteries434Impedance Characterization of the Transport Properties of Electrolytes Contained within Porous Electrodes and Separators Useful for Li-S Batteries50Strategic combination of Grignard reagents and allyl-functionalized ionic liquids as an advanced electrolyte for rechargeable magnesium batteries27Electrolytes, SEI Formation, and Binders: A Review of Nonelectrode Factors for Sodium‐Ion Battery Anodes358Anodic Stability of New Sulfone‐Based Electrolytes for Lithium‐Ion Batteries27Ionic liquids in electrochemical energy storage87High-capacity FeTiO3/C negative electrode for sodium-ion batteries with ultralong cycle life23Na 3 V 2 (PO 4 ) 3 /C Positive Electrodes with High Energy and Power Densities for Sodium Secondary Batteries with Ionic Liquid Electrolytes That Operate across Wide Temperature Ranges61Sodium metal anodes for room-temperature sodium-ion batteries: Applications, challenges and solutions321New Strategies for Probing Energy Systems with In Situ Liquid-Phase Transmission Electron Microscopy48Organosilicon‐group‐derived silica‐ionogel electrolyte for lithium ion batteries19Methyl quantum tunneling in ionic liquid [DMIm][TFSI] facilitated by Bis(trifluoromethane)sulfonimide lithium salt6Insights into the Structure and Transport of the Lithium, Sodium, Magnesium, and Zinc Bis(trifluoromethansulfonyl)imide Salts in Ionic Liquids105Ion Dynamics in Ionic‐Liquid‐Based Li‐Ion Electrolytes Investigated by Neutron Scattering and Dielectric Spectroscopy32Tetra-butyl ammonium fluoride – An advanced activator of aluminum surfaces in organic electrolytes for aluminum-air batteries37Solvate Ionic Liquids for Li, Na, K, and Mg Batteries71Separators and electrolytes for rechargeable batteries: Fundamentals and perspectives9Immobilized cation functional gel polymer electrolytes with high lithium transference number for lithium ion batteries81O2 reduction on a Au film electrode in an ionic liquid in the absence and presence of Mg2+ ions: Product formation and adlayer dynamics11A sub-100 ° C aluminum ion battery based on a ternary inorganic molten salt67Ionic liquid/ZnO(0001) single crystal and epitaxial film interfaces studied through a combination of electrochemical measurements and a pulsed laser deposition process under vacuum9Rechargeable aluminum batteries: effects of cations in ionic liquid electrolytes110Using CoS cathode materials with 3D hierarchical porosity and an ionic liquid (IL) as an electrolyte additive for high capacity rechargeable magnesium batteries46Critical Review of the Use of Reference Electrodes in Li-Ion Batteries: A Diagnostic Perspective166Mg Cathode Materials and Electrolytes for Rechargeable Mg Batteries: A Review146Caractérisation multi-échelle de la structure et du transport de cristaux liquides ioniques : vers des électrolytes solides innovants pour batteries lithium0Molecular relaxation and ionic conductivity of ionic liquids confined in a poly(vinylidene fluoride) polymer matrix: Influence of anion and cation type30Prototype rechargeable magnesium batteries using ionic liquid electrolytes64On the Beneficial Effect of MgCl2 as Electrolyte Additive to Improve the Electrochemical Performance of Li4Ti5O12 as Cathode in Mg Batteries12Effect of Li+ and Mg2+ on the Electrochemical Decomposition of the Ionic Liquid 1‐Butyl‐1‐ methylpyrrolidinium bis(trifluoromethanesulfonyl)imide and Related Electrolytes17Sodium Metal Anodes: Emerging Solutions to Dendrite Growth940Interactions in Sodium Bis(fluorosulfonyl)imide/1-Ethyl-3-methylimidazolium Bis(fluorosulfonyl)imide Electrolytes for Na-Ion Batteries: Insights from Molecular Dynamics Simulations18A new DMF-derived ionic liquid with ultra-high conductivity for high-capacitance electrolyte in electric double-layer capacitor26Recent advances on separator membranes for lithium-ion battery applications: From porous membranes to solid electrolytes369A safe and non-flammable sodium metal battery based on an ionic liquid electrolyte298The liquid ammoniate of sodium iodide as an alternative electrolyte for sodium ion batteries: The case of titanium dioxide nanotube electrodes10Recent advances in electrolytes and cathode materials for magnesium and hybrid-ion batteries172Polymer‐Based Separators for Lithium‐Ion Batteries4Exploring the use of EMImFSI ionic liquid as additive or co-solvent for room temperature sodium ion battery electrolytes26Stereolithography Provides Access to 3D Printed Ionogels with High Ionic Conductivity19Electroanalytical Investigation of the Electrode–Electrolyte Interface of Quaternary Ammonium Ionic Liquids: Impact of Alkyl Chain Length and Ether Functionality38Alkoxy-functionalized ionic liquid electrolytes: understanding ionic coordination of calcium ion speciation for the rational design of calcium electrolytes73Ionic Liquid Crystal Electrolytes based on Ether Functionalized Ionic Liquid for Lithium Batteries1Design strategies for nonaqueous multivalent-ion and monovalent-ion battery anodes437Anticipated Progress in the Near‐ to Mid‐Term Future of LIBs0High‐Safety and High‐Energy‐Density Lithium Metal Batteries in a Novel Ionic‐Liquid Electrolyte338Machine learning approach for solving inconsistency problems of Li‐ion batteries during the manufacturing stage12Vacuum Electrochemistry Approach to Investigate Electrical Double‐Layer Capacitances of Ionic Liquid for Epitaxial Thin‐Film Electrodes of TiO2 and SrO on Niobium‐Doped (001)SrTiO36Physicochemical characterization of AlCl3-urea ionic liquid analogs: Speciation, conductivity, and electrochemical stability45Reducing Capacity and Voltage Decay of Co‐Free Li1.2Ni0.2Mn0.6O2 as Positive Electrode Material for Lithium Batteries Employing an Ionic Liquid‐Based Electrolyte71Hydrogen sorption capacity as a tunable parameter in aprotic ionic liquids9Study of P(VDF-co-HFP)-ionic liquid based ionogels for designing flexible displays20Carbon coating of electrode materials for lithium-ion batteries57Self-arranged polythiophene on multi-walled carbon nanotube templated composites: Synthesis and application in rechargeable aluminium battery41Challenges of today for Na-based batteries of the future: From materials to cell metrics305Structural and Ion Dynamics in Fluorine-Free Oligoether Carboxylate Ionic Liquid-Based Electrolytes24Strategies towards the challenges of zinc metal anode in rechargeable aqueous zinc ion batteries359Approaching Electrochemical Limits of Mg x Cl y z+ Complex-Based Electrolytes for Mg Batteries by Tailoring the Solution Structure17Enabling Mg‐Based Ionic Liquid Electrolytes for Hybrid Dual‐Ion Capacitors24Manipulating Electrode/Electrolyte Interphases of Sodium-Ion Batteries: Strategies and Perspectives195Advanced electrode materials for nonaqueous calcium rechargeable batteries55Crystalline Ionic Liquid: New Type of Solid Electrolyte for High Na + Conductivity0Dendrite-free reversible Li plating/stripping in adiponitrile-based electrolytes for high-voltage Li metal batteries11High-voltage liquid electrolytes for Li batteries: progress and perspectives979Investigation of Cost-Effective AlCl3-Urea Ionic Liquid Analog for Al-Ion Batteries0Ionic Liquid-Based Electrolytes for Aluminum/Magnesium/Sodium-Ion Batteries198Recent progress in ‘water-in-salt’ and ‘water-in-salt’-hybrid-electrolyte-based high voltage rechargeable batteries54When graphene meets ionic liquids: a good match for the design of functional materials68Influence of Complexing Additives on the Reversible Deposition/Dissolution of Magnesium in an Ionic Liquid16An Ammonium Solvate Ionic Liquid4Insight into the Solid Electrolyte Interphase Formation in Bis(fluorosulfonyl)Imide Based Ionic Liquid Electrolytes58Benefits of the Mixtures of Ionic Liquid and Organic Electrolytes for Sodium-ion Batteries19Structure-Property Relationships of Silylamine-Type Reversible Ionic Liquids for Use as a Switchable Electrolyte1Galvanic Couples in Ionic Liquid‐Based Electrolyte Systems for Lithium Metal Batteries—An Overlooked Cause of Galvanic Corrosion?40Structural analysis of water in ionic liquid domains – A low pressure study18Application of Ionic Liquids for Batteries and Supercapacitors192Ionic Liquid-Based Electrospun Polymer Nanohybrid for Energy Harvesting21Synthesis and Characterization of a Novel Hydroquinone Sulfonate-Based Redox Active Ionic Liquid8The Critical Role of Ionic Liquid Crystal on Mg 2+ Ion Transport Properties in Magnesium Ion Batteries; Performance and Mechanism Approach12Enabling a Stable High-Power Lithium-Bromine Flow Battery Using Task-Specific Ionic Liquids14Electrodeposition of Zinc onto Au(111) and Au(100) from the Ionic Liquid [MPPip][TFSI]22Electrodeposition of Zinc onto Au(111) and Au(100) from the Ionic Liquid [MPPip][TFSI]2Electrolyte solutions design for lithium-sulfur batteries533Ionic Liquid Electrolytes for Electrochemical Energy Storage Devices78Opportunities and Limitations of Ionic Liquid‐ and Organic Carbonate Solvent‐Based Electrolytes for Mg‐Ion‐Based Dual‐Ion Batteries37Discovery of novel Li SSE and anode coatings using interpretable machine learning and high-throughput multi-property screening52Interfacial nanostructure and friction of a polymeric ionic liquid-ionic liquid mixture as a function of potential at Au(1 1 1) electrode interface19A Flexible Semi-Interpenetrating Network-Enhanced Ionogel Polymer Electrolyte for Highly Stable and Safe Lithium Metal Batteries25Cellulose ionogels, a perspective of the last decade: A review61High-Li+-fraction ether-side-chain pyrrolidinium–asymmetric imide ionic liquid electrolyte for high-energy-density Si//Ni-rich layered oxide Li-ion batteries30Safe, Flexible, and High-Performing Gel-Polymer Electrolyte for Rechargeable Lithium Metal Batteries180Effect of Solid Substrates on the Molecular Structure of Ionic Liquid Nanofilms10Solvation structure of phosphonium ionic liquid/ CH3SCN mixture as electrolytes for Li‐ion batteries: Infrared pump‐probe spectroscopic studies7Characterization of AlCl3-Urea Electrolyte for Speciation, Conductivity, and Electrochemical Stability and Its Application in Al-Ion Batteries1Electrolytes for lithium–sulfur batteries2MOF-supported crystalline ionic liquid: new type of solid electrolyte for enhanced and high ionic conductivity17Transport Properties of Alkali/Alkaline Earth Cations in Ionic-Liquid Based Electrolytes1Improved hydrogen sorption properties of Pd in protic and aprotic ionic liquids effected by superacid addition5Interaction of Mg with the ionic liquid 1-butyl-1-methylpyrrolidinium bis(trifluoromethylsulfonyl)imide—An experimental and computational model study of the electrode–electrolyte interface in post-lithium batteries10Unveiling the Cation Exchange Reaction between the NASICON Li 1.5 Al 0.5 Ge 1.5 (PO 4 ) 3 Solid Electrolyte and the pyr13TFSI Ionic Liquid38Eutectic Electrolytes Chemistry for Rechargeable Zn Batteries114A Kinetically Superior Rechargeable Zinc‐Air Battery Derived from Efficient Electroseparation of Zinc, Lead, and Copper in Concentrated Solutions11Advancement in field of Energy storage applications by using Ionic Liquids25Ionic Liquid Electrolytes for Next-generation Electrochemical Energy Devices93Smooth Modified Surfaces of Silicon for the Study of Ionic Liquid Interfaces by Neutron Reflectometry8Recent Achievements in Experimental and Computational Studies of Positive Electrode Materials for Nonaqueous Ca- and Al-Ion Batteries23Troubleshooting the Limited Zn2+ Storage Performance of the Ag2V4O11 Cathode in Zinc Sulfate Electrolytes via Favorable Synergism with Reduced Graphene Oxides25Recent development of ionic liquid-based electrolytes in lithium-ion batteries300A Nonaqueous Mg‐CO2 Battery with Low Overpotential50Initial Stages of Sodium Deposition onto Au(111) from [MPPip][TFSI]: An In‐Situ STM Study for Sodium‐Ion Battery Electrolytes10Inhibition of Aluminum Corrosion with the Addition of the Tris(pentafluoroethyl)trifluorophosphate Anion to a Sulfonylamide-Based Ionic Liquid for Sodium-Ion Batteries10An account on the deep eutectic solvents-based electrolytes for rechargeable batteries and supercapacitors69Transport properties of alkali/alkaline earth cations in ionic-liquid based electrolytes11Advances in electrolyte safety and stability of ion batteries under extreme conditions39Sulfur Dioxide and Sulfolane as Additives in Organic Electrolytes to Develop Room-Temperature Sodium Batteries5Machine learning accelerated carbon neutrality research using big data—from predictive models to interatomic potentials5Improving electrochemical stability and electromechanical efficiency of ipmcs: tuning ionic liquid concentration15An experimental and computational study of a low-temperature electrolyte design utilizing iodide-based ionic liquid and butyronitrile2Extremely slow dynamics of ionic liquid self-assembled nanostructures near a solid surface23Simulations of electric field gradient fluctuations and dynamics around sodium ions in ionic liquids8Unexplored Class of Eutectic Electrolytes for Rechargeable Magnesium Batteries20A comparison of the impact of cation chemistry in ionic liquid-based lithium battery electrolytes6Insights into structure–property relationships in ionic liquids using cyclic perfluoroalkylsulfonylimides15Ionic liquids as potential electrolytes for sodium-ion batteries: an overview41Reactive sputtering onto an ionic liquid, a new synthesis route for bismuth-based nanoparticles9Interface Engineering of Zinc Electrode for Rechargeable Alkaline Zinc‐Based Batteries43Mapping the Three‐Dimensional Nanostructure of the Ionic Liquid–Solid Interface Using Atomic Force Microscopy and Molecular Dynamics Simulations6(Localized) Highly Concentrated Electrolytes for Calcium Batteries13Reversible Zinc Electrodeposition at −60 °C Using a Deep Eutectic Electrolyte for Low-Temperature Zinc Metal Batteries22Imidazolium-based ionanofluid electrolytes with viscosity decoupled ion transport properties for lithium-ion batteries4

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  1. Primary Sjogren's syndrome: rarity in India.

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  2. A lipophilic ionic liquid based on formamidinium cations and TFSI: the electric response and the effect of CO 2 on the conductivity mechanism

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  3. A sodium–aluminum hybrid battery

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  4. Development of novel inorganic electrolytes for room temperature rechargeable sodium metal batteries

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  5. Graphene-Coated Activated Carbon Fiber Cloth Positive Electrodes for Aluminum Rechargeable Batteries with a Chloroaluminate Room-Temperature Ionic Liquid

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  6. Ionic Liquid as an Effective Additive for Rechargeable Magnesium Batteries

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  7. Formation of Gd coordination polymer with 1D chains mediated by Bronsted acidic ionic liquids

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  8. Effect of Cl− and TFSI− anions on dual electrolyte systems in a hybrid Mg/Li4Ti5O12 battery

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  10. Lyotropic Lamellar Structures of a Long-Chain Imidazolium and Their Application as Nanoreactors for X-ray-Initiated Polymerization

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  13. Magnesium Anode Pretreatment Using a Titanium Complex for Magnesium Battery

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  22. Impedance Characterization of the Transport Properties of Electrolytes Contained within Porous Electrodes and Separators Useful for Li-S Batteries

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  35. Tetra-butyl ammonium fluoride – An advanced activator of aluminum surfaces in organic electrolytes for aluminum-air batteries

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  36. Solvate Ionic Liquids for Li, Na, K, and Mg Batteries

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  38. Immobilized cation functional gel polymer electrolytes with high lithium transference number for lithium ion batteries

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  39. O2 reduction on a Au film electrode in an ionic liquid in the absence and presence of Mg2+ ions: Product formation and adlayer dynamics

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  43. Using CoS cathode materials with 3D hierarchical porosity and an ionic liquid (IL) as an electrolyte additive for high capacity rechargeable magnesium batteries

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  44. Critical Review of the Use of Reference Electrodes in Li-Ion Batteries: A Diagnostic Perspective

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  46. Caractérisation multi-échelle de la structure et du transport de cristaux liquides ioniques : vers des électrolytes solides innovants pour batteries lithium

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  47. Molecular relaxation and ionic conductivity of ionic liquids confined in a poly(vinylidene fluoride) polymer matrix: Influence of anion and cation type

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  48. Prototype rechargeable magnesium batteries using ionic liquid electrolytes

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  49. On the Beneficial Effect of MgCl2 as Electrolyte Additive to Improve the Electrochemical Performance of Li4Ti5O12 as Cathode in Mg Batteries

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