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RESEARCH PAPER · Chemical Society Reviews · 2007

Old materials with new tricks: multifunctional open-framework materials

Daniel Maspoch, Daniel Ruiz‐Molina, Jaume Veciana

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Old materials with new tricks: multifunctional open-framework materialsOriginalThe role of temperature on the structure and dimensionality of MOFs: an illustrative study of the formation of manganese oxy-bis(benzoate) structures120Low-Level Self-Assembly of Open Framework Based on Three Different Polyhedra: Metal-Organic Analogue of Face-Centered Cubic Dodecaboride129Mixed-ligand coordination polymers from 1,2-bis(1,2,4-triazol-4-yl)ethane and benzene-1,3,5-tricarboxylate: Trinuclear nickel or zinc secondary building units for three-dimensional networks with crystal-to-crystal transformation upon dehydration256MOFs as acid catalysts with shape selectivity properties149Rapid fabrication of metal organic framework thin films using microwave-induced thermal deposition231The use of aurophilic and other metal–metal interactions as crystal engineering design elements to increase structural dimensionality377A Luminescent and Magnetic Cyano-Bridged Tb3+−Mo5+ Coordination Polymer: toward Multifunctional Materials132Four 3D Porous Metal−Organic Frameworks with Various Layered and Pillared Motifs141Valence‐Tautomeric Metal–Organic Nanoparticles148Hybrid inorganic–organic materials: a new family in condensed matter physics327Single-Crystal to Single-Crystal Structural Transformation and Photomagnetic Properties of a Porous Iron(II) Spin-Crossover Framework232Metadynamics simulations of ice nucleation and growth172Open‐Framework Structures of Transition‐Metal Compounds380Copper-based metal-organic framework for the facile ring-opening of epoxides188Spin‐Crossover Nanocrystals with Magnetic, Optical, and Structural Bistability Near Room Temperature317Multifunctional Microporous MOFs Exhibiting Gas/Hydrocarbon Adsorption Selectivity, Separation Capability and Three‐Dimensional Magnetic Ordering170A Novel Metal−Organic Network with High Thermal Stability: Nonlinear Optical and Photoluminescent Properties111Predictions of effective physical properties of complex multiphase materials705Role of Temperature and Time in the Formation of Infinite −M−O−M− Linkages and Isolated Clusters in MOFs: A Few Illustrative Examples163Three‐Dimensional Chiral Microporous Germanium Antimony Sulfide with Ion‐Exchange Properties159A Bistable Porous Coordination Polymer with a Bond‐Switching Mechanism Showing Reversible Structural and Functional Transformations187Generation and O2 Adsorption Studies of the Microporous Magnets CsNi[Cr(CN)6] (TC = 75 K) and Cr3[Cr(CN)6]2·6H2O (TN = 219 K)120Magnetic and luminescence properties of Cu(II), Cu(II)4O4 core, and Cd(II) mixed-ligand metal–organic frameworks constructed from 1,2-bis(1,2,4-triazol-4-yl)ethane and benzene-1,3,5-tricarboxylate154The Kagomé Topology of the Gallium and Indium Metal-Organic Framework Types with a MIL-68 Structure: Synthesis, XRD, Solid-State NMR Characterizations, and Hydrogen Adsorption339Metal–Organic Spheres as Functional Systems for Guest Encapsulation211A porous 3D heterometal-organic framework containing both lanthanide and high-spin Fe(ii) ions146Crystal structures and solid-state CPMAS 13C NMR correlations in luminescent zinc(II) and cadmium(II) mixed-ligand coordination polymers constructed from 1,2-bis(1,2,4-triazol-4-yl)ethane and benzenedicarboxylate206Luminescent metal–organic frameworks4960Magnetic metal–organic frameworks2448Near-infrared emitting ytterbium metal–organic frameworks with tunable excitation properties145Selective gas adsorption and separation in metal–organic frameworks8932Synthesis of a metal–organic framework film by direct conversion technique for VOCs sensing124Thin films of metal–organic frameworks893A Luminescent Microporous Metal–Organic Framework for the Fast and Reversible Detection of High Explosives1237A Luminescent Microporous Metal–Organic Framework for the Fast and Reversible Detection of High Explosives191MOFs as Adsorbents for Low Temperature Heating and Cooling Applications438Adsorption and Separation of Noble Gases by IRMOF-1: Grand Canonical Monte Carlo Simulations158Bidirectional Chemo‐Switching of Spin State in a Microporous Framework548Bidirectional Chemo‐Switching of Spin State in a Microporous Framework127Fabrication of MOF-5 membranes using microwave-induced rapid seeding and solvothermal secondary growth332Luminescent and Magnetic Cyano-Bridged Coordination Polymers Containing 4d−4f Ions: Toward Multifunctional Materials136Comparative Study of Hydrogen Sulfide Adsorption in the MIL-53(Al, Cr, Fe), MIL-47(V), MIL-100(Cr), and MIL-101(Cr) Metal−Organic Frameworks at Room Temperature542ℝPM3: A Multifunctional Microporous MOF with Recyclable Framework and High H2 Binding Energy111Apical Ligand Substitution, Shape Recognition, Vapor-Adsorption Phenomenon, and Microcalorimetry for a Pillared Bilayer Porous Framework That Shrinks or Expands in Crystal-to-Crystal Manners upon Change in the Cobalt(II) Coordination Environment125Metal–Organic Frameworks: Opportunities for Catalysis1888Metall‐organische Gerüste für die Katalyse216Metal–Organic Perovskites: Synthesis, Structures, and Magnetic Properties of [C(NH2)3][MII(HCOO)3] (M=Mn, Fe, Co, Ni, Cu, and Zn; C(NH2)3= Guanidinium)267Zeolitic Polyoxometalate-Based Metal−Organic Frameworks (Z-POMOFs): Computational Evaluation of Hypothetical Polymorphs and the Successful Targeted Synthesis of the Redox-Active Z-POMOF1279Recent advances in crystal engineering746Soft porous crystals2436Thiacalix[4]arene-Supported Planar Ln4 (Ln = TbIII, DyIII) Clusters: Toward Luminescent and Magnetic Bifunctional Materials166Synthesis, Crystal Structure, and Photoluminescence of a Series of Zinc(II) Coordination Polymers with 1,4-Di(1H-imidazol-4-yl)benzene and Varied Carboxylate Ligands114Amino Acid Based MOFs: Synthesis, Structure, Single Crystal to Single Crystal Transformation, Magnetic and Related Studies in a Family of Cobalt and Nickel Aminoisophthales119Metal–organic framework (MOF): lanthanide(iii)-doped approach for luminescence modulation and luminescent sensing170Metal–organic frameworks as semiconductors498MOFs, MILs and more: concepts, properties and applications for porous coordination networks (PCNs)1185Solid-state transformation of [Co(NCS)2(pyridine)4] into [Co(NCS)2(pyridine)2]n: from Curie–Weiss paramagnetism to single chain magnetic behaviour110Hydrogen Storage in Metal–Organic Frameworks403Evaluation of synthetic methods for microporous metal–organic frameworks exemplified by the competitive formation of [Cu2(btc)3(H2O)3] and [Cu2(btc)(OH)(H2O)]305Supramolecular coordination chemistry of aromatic polyoxalamide ligands: A metallosupramolecular approach toward functional magnetic materials195Formate‐Based Magnetic Metal–Organic Frameworks Templated by Protonated Amines257Two Novel Metal−Organic Frameworks (MOFs) with (3,6)-Connected Net Topologies: Syntheses, Crystal Structures, Third-Order Nonlinear Optical and Luminescent Properties154Spin Crossover Phenomenon in Nanocrystals and Nanoparticles of [Fe(3-Fpy)2M(CN)4] (MII = Ni, Pd, Pt) Two-Dimensional Coordination Polymers149Nanoscale Metal–Organic Frameworks: Magnetic Resonance Imaging Contrast Agents and Beyond203Hybrid Organic−Inorganic Polyoxometalate Compounds: From Structural Diversity to Applications1755Metal–Organic Frameworks from Edible Natural Products781Catalysis of Transesterification by a Nonfunctionalized Metal−Organic Framework: Acido-Basicity at the External Surface of ZIF-8 Probed by FTIR and ab Initio Calculations586Exceptional Thermal Stability in a Supramolecular Organic Framework: Porosity and Gas Storage468Flexible Two-Dimensional Square-Grid Coordination Polymers: Structures and Functions135A Series of (6,6)-Connected Porous Lanthanide−Organic Framework Enantiomers with High Thermostability and Exposed Metal Sites: Scalable Syntheses, Structures, and Sorption Properties168Surface Chemistry of Metal–Organic Frameworks at the Liquid–Solid Interface318Framework-structured weak ferromagnets407Layered hydroxide hybrid nanostructures: a route to multifunctionality151Metal–biomolecule frameworks (MBioFs)426Microporous magnets524Role of solvents in coordination supramolecular systems665Single-Crystal Metal−Organic Framework Arrays114Solvothermal Synthesis, Structure, and Properties of Metal Organic Framework Isomers Derived from a Partially Fluorinated Link133Rapid Room‐Temperature Synthesis of Metal–Organic Framework HKUST‐1 Crystals in Bulk and as Oriented and Patterned Thin Films288Effect of Lanthanide Contraction on Crystal Structures of Three-Dimensional Lanthanide Based Metal–Organic Frameworks with Thiophene-2,5-Dicarboxylate and Oxalate110Precise Control and Consecutive Modulation of Spin Transition Temperature Using Chemical Migration in Porous Coordination Polymers223Luminescent Functional Metal–Organic Frameworks5697Polyoxometalate-Based Metal Organic Frameworks (POMOFs): Structural Trends, Energetics, and High Electrocatalytic Efficiency for Hydrogen Evolution Reaction545High Proton Conduction in a Chiral Ferromagnetic Metal–Organic Quartz-like Framework322Ligand design for functional metal–organic frameworks855Two Solvent-Dependent Zinc(II) Supramolecular Isomers: Rare kgd and Lonsdaleite Network Topologies Based on a Tripodal Flexible Ligand137Metal and metal oxidenanoparticle synthesis from metal organic frameworks (MOFs): finding the border of metal and metal oxides401Synergetic Effect of Host–Guest Chemistry and Spin Crossover in 3D Hofmann‐like Metal–Organic Frameworks [Fe(bpac)M(CN)4] (M=Pt, Pd, Ni)126A Multifunctional Organic–Inorganic Hybrid Structure Based on MnIII–Porphyrin and Polyoxometalate as a Highly Effective Dye Scavenger and Heterogenous Catalyst420Fluorinated Metal–Organic Frameworks: Advantageous for Higher H2 and CO2 Adsorption or Not?112Metal–Organic Frameworks in Biomedicine4168Combining Coordination Modulation with Acid–Base Adjustment for the Control over Size of Metal–Organic Frameworks286Attaching Persistent Organic Free Radicals to Surfaces: How and Why199Functional porphyrinic metal–organic frameworks: crystal engineering and applications127Highly biocompatible, hollow coordination polymer nanoparticles as cisplatin carriers for efficient intracellular drug delivery170In situ synthesis of Cu–BTC (HKUST-1) in macro-/mesoporous silica monoliths for continuous flow catalysis158Polyrotaxane metal–organic frameworks (PMOFs)170Patterning Techniques for Metal Organic Frameworks137Highly Selective Chemical Sensing in a Luminescent Nanoporous Magnet142Enhanced Hydrostability in Ni-Doped MOF-5263Homochiral Crystallization of Metal–Organic Silver Frameworks: Asymmetric [3+2] Cycloaddition of an Azomethine Ylide118Selective Gas and Vapor Sorption and Magnetic Sensing by an Isoreticular Mixed-Metal–Organic Framework118Dynamic magnetic MOFs618Design and construction of coordination polymers with mixed-ligand synthetic strategy774Highly Selective Sorption and Luminescent Sensing of Small Molecules Demonstrated in a Multifunctional Lanthanide Microporous Metal–Organic Framework Containing 1D Honeycomb‐Type Channels168Anchoring of Palladium onto Surface of Porous Metal–Organic Framework through Post-Synthesis Modification and Studies on Suzuki and Stille Coupling Reactions under Heterogeneous Condition113Spin state switching in iron coordination compounds755The controlled regulation of morphology and size of HKUST-1 by “coordination modulation method”180Highly Selective Luminescent Sensing of Fluoride and Organic Small-Molecule Pollutants Based on Novel Lanthanide Metal–Organic Frameworks319First-Principles Study of Microporous Magnets M-MOF-74 (M = Ni, Co, Fe, Mn): the Role of Metal Centers118Development of Structural Complexity by Liquid‐Crystal Self‐assembly631Selective, Sensitive, and Reversible Detection of Vapor-Phase High Explosives via Two-Dimensional Mapping: A New Strategy for MOF-Based Sensors113A Systematic Study of Fluorescence‐Based Detection of Nitroexplosives and Other Aromatics in the Vapor Phase by Microporous Metal–Organic Frameworks211Spin-Crossover Modification through Selective CO2 Sorption136A Highly Symmetric Metal–Organic Framework Based on a Propeller-Like Ru-Organic Metalloligand for Photocatalysis and Explosives Detection118Lanthanide Metal–Organic Frameworks Showing Luminescence in the Visible and Near‐Infrared Regions with Potential for Acetone Sensing137Luminescent metal–organic frameworks as explosive sensors371Oxamato-based coordination polymers: recent advances in multifunctional magnetic materials115A 3D Aluminoborate Open Framework Interpenetrated by 2D Zinc–Amine Coordination‐Polymer Networks in Its 11‐Ring Channels129A Robust Binary Supramolecular Organic Framework (SOF) with High CO2 Adsorption and Selectivity357Dynamic structural transformations of coordination supramolecular systems upon exogenous stimulation113Metal cluster-based functional porous coordination polymers281A “green” strategy to construct non-covalent, stable and bioactive coatings on porous MOF nanoparticles186Applications of ultrasound to the synthesis of nanoscale metal–organic coordination polymers229Multifunctional Radical-Doped Polyoxometalate-Based Host–Guest Material: Photochromism and Photocatalytic Activity145Postsynthetic Improvement of the Physical Properties in a Metal–Organic Framework through a Single Crystal to Single Crystal Transmetallation108A 2D Semiquinone Radical-Containing Microporous Magnet with Solvent-Induced Switching from Tc = 26 to 80 K209Guest-dependent single-ion magnet behaviour in a cobalt( ii ) metal–organic framework128Exploiting redox activity in metal–organic frameworks: concepts, trends and perspectives368Inorganic nanoparticles in porous coordination polymers265Controllable synthesis of dual-MOFs nanostructures for pH-responsive artemisinin delivery, magnetic resonance and optical dual-model imaging-guided chemo/photothermal combinational cancer therapy298Insights into the Dynamics of Grotthuss Mechanism in a Proton-Conducting Chiral bio MOF139Porous Organic Molecular Frameworks with Extrinsic Porosity: A Platform for Carbon Storage and Separation143Osteogenic activity and antibacterial effect of porous titanium modified with metal‐organic framework films150Facile synthesis of polypyrrole@metal–organic framework core–shell nanocomposites for dual-mode imaging and synergistic chemo-photothermal therapy of cancer cells126Luminescent Cd( ii )–organic frameworks with chelating NH 2 sites for selective detection of Fe( iii ) and antibiotics363Efficient removal of crystal violet and methylene blue from wastewater by ultrasound nanoparticles Cu-MOF in comparison with mechanosynthesis method153Porous Hydrogen-Bonded Organic Frameworks118Molecular magnetism, quo vadis? A historical perspective from a coordination chemist viewpoint☆348Rational Design of S-UiO-66@GO Hybrid Nanosheets for Proton Exchange Membranes with Significantly Enhanced Transport Performance155Coordination Polymers based on calixarene derivatives: Structures and properties151Fabrication of a hyaluronic acid conjugated metal organic framework for targeted drug delivery and magnetic resonance imaging118Photochemistry and photophysics of MOFs: steps towards MOF-based sensing enhancements656Photoluminescent metal–organic frameworks and their application for sensing biomolecules337Redox-active metal–organic frameworks for energy conversion and storage321Recent developments in luminescent coordination polymers: Designing strategies, sensing application and theoretical evidences508Metal–Organic Framework Magnets634Electrochemical Applications of Ferrocene‐Based Coordination Polymers119Two-birds-one-stone: multifunctional supercapacitors beyond traditional energy storage470Advanced Organic–Inorganic Hybrid Materials for Optoelectronic Applications222

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