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RESEARCH PAPER · MRS Bulletin · 2012

Control of octahedral connectivity in perovskite oxide heterostructures: An emerging route to multifunctional materials discovery

James M. Rondinelli, Steven J. May, J. W. Freeland

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Control of octahedral connectivity in perovskite oxide heterostructures: An emerging route to multifunctional materials discoveryOriginalTuning the ground state of La 0.67 Ca 0.33 MnO 3 films via coherent growth on orthorhombic NdGaO 3 substrates with different orientations51Atomic-resolution chemical imaging of oxygen local bonding environments by electron energy loss spectroscopy51Electronic Subband Reconfiguration in a d0 -Perovskite Induced by Strain-Driven Structural Transformations13Spin-assisted covalent bond mechanism in “charge-ordering” perovskite oxides32The impact of crystal symmetry on the electronic structure and functional properties of complex lanthanum chromium oxides55Misfit accommodation in oxide thin film heterostructures44Tunable conductivity at LaAlO3/SrxCa1−xTiO3 (0 ≤ x ≤ 1) heterointerfaces14Hybrid Improper Ferroelectricity in a Multiferroic and Magnetoelectric Metal‐Organic Framework338Structural origins of the properties of rare earth nickelate superlattices71X-ray photoelectron diffraction study of dopant effects in La0.7X0.3MnO3 (X = La, Sr, Ca, Ce) thin films10Interplay of Octahedral Tilts and Polar Order in BiFeO3 Films115Normal mode determination of perovskite crystal structures with octahedral rotations: theory and applications87Octahedral engineering of orbital polarizations in charge transfer oxides32Annealing assisted substrate coherency and high-temperature antiferromagnetic insulating transition in epitaxial La0.67Ca0.33MnO3/NdGaO3(001) films22Turning ABO3 Antiferroelectrics into Ferroelectrics: Design Rules for Practical Rotation‐Driven Ferroelectricity in Double Perovskites and A3B2O7 Ruddlesden‐Popper Compounds331Effect of growth oxygen pressure on anisotropic-strain-induced phase separation in epitaxial La0.67Ca0.33MnO3/NdGaO3(001) films8Symmetry Lowering in Extreme-Electron-Density Perovskite Quantum Wells56Surface Octahedral Distortions and Atomic Design of Perovskite Interfaces26Universal collaborative couplings between oxygen-octahedral rotations and antiferroelectric distortions in perovskites104Atomic level observation of octahedral distortions at the perovskite oxide heterointerface160Interplay of octahedral rotations and breathing distortions in charge-ordering perovskite oxides99Anisotropic resistivities in anisotropic-strain-controlled phase-separated La0.67Ca0.33MnO3/NdGaO3(100) films13Magnetism and local structure in low-dimensional Mott insulating GdTiO 324Double perovskites as a family of highly active catalysts for oxygen evolution in alkaline solution1629Neutron scattering—The key characterization tool for nanostructured magnetic materials38Untilting BiFeO3: The influence of substrate boundary conditions in ultra-thin BiFeO3 on SrTiO326Connecting bulk symmetry and orbital polarization in strained RNiO 3 ultrathin films46Critical thickness and strain relaxation in molecular beam epitaxy-grown SrTiO3 films46Quantum confinement in oxide quantum wells47Crystal-Chemistry Guidelines for Noncentrosymmetric A 2 BO 4 Ruddlesden−Popper Oxides88Size effects in epitaxial oxide thin films3Nucleation kinetics of SrTiO 3 3D islands and nanorings on Si substrates1Compressibility Systematics of Calcite-Type Borates: An Experimental and Theoretical Structural Study on ABO 3 (A = Al, Sc, Fe, and In)27Elastic strain engineering of ferroic oxides504Octahedral rotations in strained LaAlO3/SrTiO3 (001) heterostructures62Ferroelectric domain structure of NaNbO3 epitaxial thin films grown on (110) DyScO3 substrates13Correlation between metal-insulator transitions and structural distortions in high-electron-density SrTiO 3 quantum wells38Dynamics and Control in Complex Transition Metal Oxides172Magnetic Oxide Heterostructures231Effect of Interfacial Octahedral Behavior in Ultrathin Manganite Films141Octahedral Tilt Propagation Controlled by A-Site Cation Size at Perovskite Oxide Heterointerfaces51Control of Structural Distortions in Transition‐Metal Oxide Films through Oxygen Displacement at the Heterointerface49Effect of “symmetry mismatch” on the domain structure of rhombohedral BiFeO3 thin films78Unit-cell thick BaTiO3 blocks octahedral tilt propagation across oxide heterointerface17Electric field-induced magnetization switching in interface-coupled multiferroic heterostructures: a highly-dense, non-volatile, and ultra-low-energy computing paradigm9Ferroelectric domain structure of anisotropically strained NaNbO3 epitaxial thin films20Lattice distortions and octahedral rotations in epitaxially strained LaNiO3/LaAlO3 superlattices39Strain Effects in Narrow-Bandwidth Manganites: The Case of Epitaxial Eu0.7Sr0.3MnO3 Thin Films10Inductive crystal field control in layered metal oxides with correlated electrons14Correlating interfacial octahedral rotations with magnetism in (LaMnO3+δ)N/(SrTiO3)N superlattices122Quantum critical behaviour in confined SrTiO3 quantum wells embedded in antiferromagnetic SmTiO352Strain Accommodation by Facile WO6Octahedral Distortion and Tilting during WO3Heteroepitaxy on SrTiO3(001)40Dynamic layer rearrangement during growth of layered oxide films by molecular beam epitaxy155Interfaces and Nanostructures of Functional Oxide Octahedral Framework Structures2Nanoscale Resistive Switching in Amorphous Perovskite Oxide (a‐SrTiO3) Memristors140Covalent dependence of octahedral rotations in orthorhombic perovskite oxides82Microscopic origin of pressure-induced isosymmetric transitions in fluoromanganate cryolites5Symmetry and lattice mismatch induced strain accommodation near and away from correlated perovskite interfaces98Atomic-scale control of TiO6 octahedra through solution chemistry towards giant dielectric response94Colloquium : Emergent properties in plane view: Strong correlations at oxide interfaces272Nanostructure investigations of nonlinear differential conductance in NdNiO3 thin films9Strong Dependence of Oxygen Octahedral Distortions in SrRuO3 Films on Types of Substrate-Induced Epitaxial Strain27Atomically resolved EELS mapping of the interfacial structure of epitaxially strained LaNiO3/LaAlO3 superlattices39Enhancing the orthorhombicity and antiferromagnetic-insulating state in epitaxial La0.67Ca0.33MnO3/NdGaO3(001) films by inserting a SmFeO3 buffer layer4Dynamical systems study in single-phase multiferroic materials6Spatial control of functional properties via octahedral modulations in complex oxide superlattices84Mesoscale magnetism20Phase control of a perovskite transition-metal oxide through oxygen displacement at the heterointerface11The effects of strain on crystal structure and properties during epitaxial growth of oxides8Control of orbital reconstruction in (LaAlO3)M/(SrTiO3)N(001) quantum wells by strain and confinement35Manipulating oxygen sublattice in ultrathin cuprates: A new direction to engineer oxides12Cation ordering induced polarization enhancement for PbTiO3−SrTiO3 ferroelectric-dielectric superlattices9Intrinsic interfacial phenomena in manganite heterostructures37Phase transitions and octahedral rotations in epitaxial Ag(TaxNb1−x)O3 thin films under tensile strain7Enhancement of Ionic Transport in Complex Oxides through Soft Lattice Modes and Epitaxial Strain108Stoichiometry control of complex oxides by sequential pulsed-laser deposition from binary-oxide targets15Tailoring the electronic transitions of NdNiO3 films through (111)pc oriented interfaces80Local octahedral rotations and octahedral connectivity in epitaxially strained LaNiO3/LaGaO3 superlattices13Persistent semi-metal-like nature of epitaxial perovskite CaIrO3 thin films20Transition from Order to Configurational Disorder for Surface Reconstructions on SrTiO3 (111)41Dimensionality Controlled Octahedral Symmetry-Mismatch and Functionalities in Epitaxial LaCoO3/SrTiO3 Heterostructures86Anharmonic lattice interactions in improper ferroelectrics for multiferroic design72Mott Memory and Neuromorphic Devices371Towards 3D Mapping of BO6 Octahedron Rotations at Perovskite Heterointerfaces, Unit Cell by Unit Cell96Polar domain walls trigger magnetoelectric coupling30Oxygen Disorder, a Way to Accommodate Large Epitaxial Strains in Oxides21Capturing ultrafast photoinduced local structural distortions of BiFeO324Interfacial Control of Magnetic Properties at LaMnO3/LaNiO3 Interfaces111Tilt engineering of exchange coupling at G-type SrMnO3/(La,Sr)MnO3 interfaces18Crystal structure and electronic properties of bulk and thin film brownmillerite oxides100Evolution and control of the phase competition morphology in a manganite film56Static and Dynamic Optical Properties of La1–xSrxFeO3−δ: The Effects of A-Site and Oxygen Stoichiometry34Symmetry-Adapted Distortion Modes as Descriptors for Materials Informatics4Symmetry‐Driven Atomic Rearrangement at a Brownmillerite–Perovskite Interface26Effects of biaxial stress and layer thickness on octahedral tilts in LaNiO35Design of noncentrosymmetric perovskites from centric and acentric basic building units39Informatics-Based Approaches for Accelerated Discovery of Functional Materials2Lithiation-driven structural transition of VO 2 F into disordered rock-salt Li x VO 2 F26Physics of Ultrathin Films and Heterostructures of Rare-Earth Nickelates144Ferroelectric control of metal–insulator transition1Basic Research Needs Workshop on Quantum Materials for Energy Relevant Technology28Physical properties modulation of Fe 3 O 4 /Pb(ZrTi)O 3 heterostructure via Fe diffusion1Octahedral Rotation Preferences in Perovskite Iodides and Bromides145Ruddlesden–Popper perovskite sulfides A3B2S7: A new family of ferroelectric photovoltaic materials for the visible spectrum83Modulation of metal-insulator transitions by field-controlled strain in NdNiO3/SrTiO3/PMN-PT (001) heterostructures30Insulating phase at low temperature in ultrathin La0.8Sr0.2MnO3 films50Origin of thickness dependence of structural phase transition temperatures in highly strained BiFeO3 thin films10Controlled lateral anisotropy in correlated manganite heterostructures by interface-engineered oxygen octahedral coupling368Engineered Unique Elastic Modes at a BaTiO3/(2×1)−Ge(001) Interface21Tuning magnetic anisotropy by interfacially engineering the oxygen coordination environment in a transition metal oxide241Interplay between Cation and Charge Ordering in La1/3Sr2/3FeO3 Superlattices11Physics of Ultrathin Films and Heterostructures of Rare-Earth Nickelates307Polar metals by geometric design343An efficient ab-initio quasiharmonic approach for the thermodynamics of solids89Giant Enhancement of Magnetic Anisotropy in Ultrathin Manganite Films via Nanoscale 1D Periodic Depth Modulation54Cation ratio and ferroelectric properties of TbMnO3 epitaxial films grown by pulsed laser deposition10Directing Matter: Toward Atomic-Scale 3D Nanofabrication117Atomic-scale control of magnetic anisotropy via novel spin–orbit coupling effect in La 2/3 Sr 1/3 MnO 3 /SrIrO 3 superlattices145Materials design for new superconductors80Controlling Octahedral Rotations in a Perovskite via Strain Doping72Interfacial Octahedral Rotation Mismatch Control of the Symmetry and Properties of SrRuO 371Control of octahedral rotations via octahedral connectivity in an epitaxially strained [1 u.c.//4 u.c.] LaNiO3/LaGaO3 superlattice5Epitaxial-strain-induced polar-to-nonpolar transitions in layered oxides113Long‐Range Domain Structure and Symmetry Engineering by Interfacial Oxygen Octahedral Coupling at Heterostructure Interface30Coupling Between Strain and Oxygen Octahedral Distortions in Epitaxially Strained GdScO 3 /SrTiO 3 Heterostructure5Effect of Terraces at the Interface on the Structural and Physical Properties of La 0.8 Sr 0.2 MnO 3 Thin Films4Piezoelectricity and rotostriction through polar and non-polar coupled instabilities in bismuth-based piezoceramics24Octahedral rotation patterns in strained EuFeO3 and otherPbnmperovskite films: Implications for hybrid improper ferroelectricity31Cooperative photoinduced metastable phase control in strained manganite films170First-principles study of the cubic CaHfO3(001) surface6Interface-Driven Ferromagnetism within the Quantum Wells of a Rare Earth Titanate Superlattice16Magnetic structures and dynamics of multiferroic systems obtained with neutron scattering61Interfacial Symmetry Control of Emergent Ferromagnetism at the Nanoscale37Multiple strain-induced phase transitions in LaNiO3 thin films66Competing Interfacial Reconstruction Mechanisms in La 0.7 Sr 0.3 MnO 3 /SrTiO 3 Heterostructures28Ultra-Low-Energy Electric Field-Induced Magnetization Switching in Multiferroic Heterostructures11Evolution of electronic correlations across the rutile, perovskite, and Ruddelsden-Popper iridates with octahedral connectivity51Two-dimensional electron systems in functional oxides studied by photoemission spectroscopy0Interfacial Control of Ferromagnetism in Ultrathin La0.67Ca0.33MnO3 Sandwiched between CaRu1–xTixO3 (x = 0–0.8) Epilayers16Nanoscale self-templating for oxide epitaxy with large symmetry mismatch21Ruddlesden-Popper interface in correlated manganite heterostructures induces magnetic decoupling and dead layer reduction11Enhanced conductivity and metal–insulator transition of ultrathin CaRuO3in superlattices4Control of octahedral rotations via octahedral connectivity in an epitaxially strained [1 u.c. // 4 u.c. ] LaNiO3/LaGaO3 superlattice0Crystal engineering for novel functionalities with oxide thin film epitaxy35Informatics-Based Approaches for Accelerated Discovery of Functional Materials0Optimal Bandgap of Double Perovskite La-Substituted Bi 2 FeCrO 6 for Solar Cells: an ab initio GGA+ U Study16Electrically coupling complex oxides to semiconductors: A route to novel material functionalities15Structural refinement of Pbnm-type perovskite films from analysis of half-order diffraction peaks39Quantum-Matter Heterostructures74Non-spectroscopic composition measurements of SrTiO3-La0.7Sr0.3MnO3 multilayers using scanning convergent beam electron diffraction28

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  1. Tuning the ground state of La 0.67 Ca 0.33 MnO 3 films via coherent growth on orthorhombic NdGaO 3 substrates with different orientations

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  2. Atomic-resolution chemical imaging of oxygen local bonding environments by electron energy loss spectroscopy

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  3. Electronic Subband Reconfiguration in a d0 -Perovskite Induced by Strain-Driven Structural Transformations

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  4. Spin-assisted covalent bond mechanism in “charge-ordering” perovskite oxides

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  5. The impact of crystal symmetry on the electronic structure and functional properties of complex lanthanum chromium oxides

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  6. Misfit accommodation in oxide thin film heterostructures

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  7. Tunable conductivity at LaAlO3/SrxCa1−xTiO3 (0 ≤ x ≤ 1) heterointerfaces

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  8. Hybrid Improper Ferroelectricity in a Multiferroic and Magnetoelectric Metal‐Organic Framework

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  10. X-ray photoelectron diffraction study of dopant effects in La0.7X0.3MnO3 (X = La, Sr, Ca, Ce) thin films

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  11. Interplay of Octahedral Tilts and Polar Order in BiFeO3 Films

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  12. Normal mode determination of perovskite crystal structures with octahedral rotations: theory and applications

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  13. Octahedral engineering of orbital polarizations in charge transfer oxides

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  14. Annealing assisted substrate coherency and high-temperature antiferromagnetic insulating transition in epitaxial La0.67Ca0.33MnO3/NdGaO3(001) films

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  15. Turning ABO3 Antiferroelectrics into Ferroelectrics: Design Rules for Practical Rotation‐Driven Ferroelectricity in Double Perovskites and A3B2O7 Ruddlesden‐Popper Compounds

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  16. Effect of growth oxygen pressure on anisotropic-strain-induced phase separation in epitaxial La0.67Ca0.33MnO3/NdGaO3(001) films

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  17. Symmetry Lowering in Extreme-Electron-Density Perovskite Quantum Wells

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  18. Surface Octahedral Distortions and Atomic Design of Perovskite Interfaces

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  19. Universal collaborative couplings between oxygen-octahedral rotations and antiferroelectric distortions in perovskites

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  20. Atomic level observation of octahedral distortions at the perovskite oxide heterointerface

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  21. Interplay of octahedral rotations and breathing distortions in charge-ordering perovskite oxides

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  22. Anisotropic resistivities in anisotropic-strain-controlled phase-separated La0.67Ca0.33MnO3/NdGaO3(100) films

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  23. Magnetism and local structure in low-dimensional Mott insulating GdTiO 3

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  24. Double perovskites as a family of highly active catalysts for oxygen evolution in alkaline solution

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  26. Untilting BiFeO3: The influence of substrate boundary conditions in ultra-thin BiFeO3 on SrTiO3

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  28. Critical thickness and strain relaxation in molecular beam epitaxy-grown SrTiO3 films

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  29. Quantum confinement in oxide quantum wells

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  30. Crystal-Chemistry Guidelines for Noncentrosymmetric A 2 BO 4 Ruddlesden−Popper Oxides

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  31. Size effects in epitaxial oxide thin films

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  32. Nucleation kinetics of SrTiO 3 3D islands and nanorings on Si substrates

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  33. Compressibility Systematics of Calcite-Type Borates: An Experimental and Theoretical Structural Study on ABO 3 (A = Al, Sc, Fe, and In)

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  34. Elastic strain engineering of ferroic oxides

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  35. Octahedral rotations in strained LaAlO3/SrTiO3 (001) heterostructures

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  36. Ferroelectric domain structure of NaNbO3 epitaxial thin films grown on (110) DyScO3 substrates

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  37. Correlation between metal-insulator transitions and structural distortions in high-electron-density SrTiO 3 quantum wells

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  38. Dynamics and Control in Complex Transition Metal Oxides

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  39. Magnetic Oxide Heterostructures

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  40. Effect of Interfacial Octahedral Behavior in Ultrathin Manganite Films

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  41. Octahedral Tilt Propagation Controlled by A-Site Cation Size at Perovskite Oxide Heterointerfaces

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  42. Control of Structural Distortions in Transition‐Metal Oxide Films through Oxygen Displacement at the Heterointerface

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  43. Effect of “symmetry mismatch” on the domain structure of rhombohedral BiFeO3 thin films

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    Zuhuang Chen, Anoop Rama Damodaran, Ruijuan Xu, S. Lee, Lane W. Martin

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  44. Unit-cell thick BaTiO3 blocks octahedral tilt propagation across oxide heterointerface

    Journal of Applied Physics · 2014-05-12

    Daisuke Kan, Ryotaro Aso, Hiroki Kurata, Yuichi Shimakawa

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  45. Electric field-induced magnetization switching in interface-coupled multiferroic heterostructures: a highly-dense, non-volatile, and ultra-low-energy computing paradigm

    Journal of Physics D Applied Physics · 2014-05-23

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  46. Ferroelectric domain structure of anisotropically strained NaNbO3 epitaxial thin films

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  47. Lattice distortions and octahedral rotations in epitaxially strained LaNiO3/LaAlO3 superlattices

    Applied Physics Letters · 2014-06-02

    M. K. Kinyanjui, Yi Lu, Nicolas Gauquelin, Meng Qiang Wu, Alex Frañó, Peter Wochner, M. Reehuis, G. Christiani, Gennady Yu. Logvenov, H.‐U. Habermeier, Gianluigi A. Botton, Ute A. Kaiser, B. Keimer, E. Benckiser

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  48. Strain Effects in Narrow-Bandwidth Manganites: The Case of Epitaxial Eu0.7Sr0.3MnO3 Thin Films

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  49. Inductive crystal field control in layered metal oxides with correlated electrons

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  50. Correlating interfacial octahedral rotations with magnetism in (LaMnO3+δ)N/(SrTiO3)N superlattices

    Nature Communications · 2014-07-09

    Xiaofang Zhai, Long Cheng, Yang Liu, Christian Matthias Schlepütz, Shuai Dong, Hui Li, Xiaoqiang Zhang, Shengqi Chu, Lirong Zheng, Jing Zhang, Aidi Zhao, Hawoong Hong, Anand Bhattacharya, J. N. Eckstein, Changgan Zeng

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