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RESEARCH PAPER · Angewandte Chemie International Edition · 2015

Direct Imaging of Octahedral Distortion in a Complex Molybdenum Vanadium Mixed Oxide

Thomas Lunkenbein, Frank Girgsdies, Anna Maria Wernbacher, Johannes Noack, Gudrun Auffermann, Akira Yasuhara, Achim Klein‐Hoffmann, Wataru Ueda, Maik Eichelbaum, Annette Trunschke, Robert Schlögl, Marc‐Georg Willinger

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Direct Imaging of Octahedral Distortion in a Complex Molybdenum Vanadium Mixed OxideOriginalElectron‐Irradiation‐Stimulated Atomic‐Scale Structural Dynamics of the Pentagonal Channel in a Complex MoVTeNbOx Catalyst3Microporous crystalline Mo–V mixed oxides for selective oxidations68Dioxidomolybdenum(VI) complexes of allyl N'-2-hydroxy-3-methoxybenzylidenecarbamohydrazonothioate: synthesis, spectral, and theoretical investigations10Small is Beautiful: Challenges and Perspectives of Nano/Meso/Microscience10Aberration-corrected scanning transmission electron microscopy for complex transition metal oxides7ADF-STEM Imaging of Nascent Phases and Extended Disorder Within the Mo–V–Nb–Te–O Catalyst System19Selective Oxidation: From a Still Immature Technology to the Roots of Catalysis Science59Local Information Powers Heterogeneous Catalysis Research: TEM Investigation of Industrial Relevant Cu/ZnO/Al2O3 Catalysts for Methanol Synthesis0Atomap: a new software tool for the automated analysis of atomic resolution images using two-dimensional Gaussian fitting301Structural Complexity in Heterogeneous Catalysis: Cataloging Local Nanostructures28How the distribution of reduced vanadium centers affects structure and stability of the MoVO x material12DFT Variants for Mixed-Metal Oxides. Benchmarks Using Multi-Center Cluster Models10A zeolitic vanadotungstate family with structural diversity and ultrahigh porosity for catalysis48Multi-dimensional Crystal Structuring of Complex Metal Oxide Catalysts of Group V and VI Elements by Unit-Assembling10Electronic and Dielectric Properties of MoV-Oxide (M1 Phase) under Alkane Oxidation Conditions28High dimensionally structured W-V oxides as highly effective catalysts for selective oxidation of toluene10Site specific and localized structural displacements in open structured multimetallic oxides12Compositional Decoupling of Bulk and Surface in Open-Structured Complex Mixed Oxides9Configurations of V4+ centers in the MoVO catalyst material. A systematic stability analysis of DFT results2Probing the Positions of TeO Moieties in the Channels of the MoVNbTeO M1 Catalyst: A Density Functional Theory Model Study7Nb−V Mixed Oxide with a Random Assembly of Pentagonal Units: A Catalyst for Oxidative Dehydrogenation of Ethane and Propane13Structural developments during the low-temperature oxidation of Nb7W10O473Mo-V-Based Crystalline Complex Metal Oxide Catalysts4Atomic and Electronic Structures of the Interfaces between Perovskite La0.75Sr0.25MnO3 and Brownmillerite SrCoO2.52Operando Electron Microscopy of Catalysts: The Missing Cornerstone in Heterogeneous Catalysis Research?127Oxidation Catalysis of Crystalline Mo3VOx for the Selective Oxidation of Ethane13Linking Bulk and Surface Structures in Complex Mixed Oxides7Fine-Tuning Microporosity of Crystalline Vanadomolybdate Frameworks for Selective Adsorptive Separation of Kr from Xe1

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  1. Electron‐Irradiation‐Stimulated Atomic‐Scale Structural Dynamics of the Pentagonal Channel in a Complex MoVTeNbOx Catalyst

    ChemCatChem · 2015-10-16

    Wei Zhang, Bingsen Zhang, Wei Zhang, Dang Sheng Su

    Read original paper ↗ ·

  2. Microporous crystalline Mo–V mixed oxides for selective oxidations

    Catalysis Science & Technology · 2015-11-09

    Satoshi Ishikawa, Wataru Ueda

    Read original paper ↗ ·

  3. Dioxidomolybdenum(VI) complexes of allyl N'-2-hydroxy-3-methoxybenzylidenecarbamohydrazonothioate: synthesis, spectral, and theoretical investigations

    Journal of Coordination Chemistry · 2016-01-21

    Reza Takjoo, Ponnadurai Ramasami, Joel T. Mague, Zohreh Hasani, Lydia Rhyman

    Read original paper ↗ ·

  4. Small is Beautiful: Challenges and Perspectives of Nano/Meso/Microscience

    Small · 2016-02-05

    Markus Antonietti

    Read original paper ↗ ·

  5. Aberration-corrected scanning transmission electron microscopy for complex transition metal oxides

    Chinese Physics B · 2016-06-01

    Qinghua Zhang, Dongdong Xiao, Lin Gu

    Read original paper ↗ ·

  6. ADF-STEM Imaging of Nascent Phases and Extended Disorder Within the Mo–V–Nb–Te–O Catalyst System

    Topics in Catalysis · 2016-08-15

    Thomas Vogt, Douglas A. Blom, Lewys Jones, Douglas J. Buttrey

    Read original paper ↗ ·

  7. Selective Oxidation: From a Still Immature Technology to the Roots of Catalysis Science

    Topics in Catalysis · 2016-08-18

    Robert Schlögl

    Read original paper ↗ ·

  8. Local Information Powers Heterogeneous Catalysis Research: TEM Investigation of Industrial Relevant Cu/ZnO/Al2O3 Catalysts for Methanol Synthesis

    European Microscopy Congress 2016: Proceedings · 2016-12-20

    Thomas Lunkenbein, Elias Frei, Julia Schumann, Malte Behrens, Marc‐Georg Willinger, Robert Schlögl

    Read original paper ↗ ·

  9. Atomap: a new software tool for the automated analysis of atomic resolution images using two-dimensional Gaussian fitting

    Advanced Structural and Chemical Imaging · 2017-02-13

    Magnus Nord, Per Erik Vullum, Ian MacLaren, Thomas Tybell, Randi Holmestad

    Read original paper ↗ ·

  10. Structural Complexity in Heterogeneous Catalysis: Cataloging Local Nanostructures

    The Journal of Physical Chemistry C · 2017-10-10

    Liudmyla Masliuk, Marc Heggen, Johannes Noack, Frank Girgsdies, Annette Trunschke, Klaus Hermann, Marc‐Georg Willinger, Robert Schlögl, Thomas Lunkenbein

    Read original paper ↗ ·

  11. How the distribution of reduced vanadium centers affects structure and stability of the MoVO x material

    Catalysis Science & Technology · 2018-01-01

    Wenqing Li, Torstein Fjermestad, Alexander Genest, Notker Rösch

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  12. DFT Variants for Mixed-Metal Oxides. Benchmarks Using Multi-Center Cluster Models

    The Journal of Physical Chemistry A · 2018-08-24

    Graham Rugg, Alexander Genest, Notker Rösch

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  13. A zeolitic vanadotungstate family with structural diversity and ultrahigh porosity for catalysis

    Nature Communications · 2018-09-11

    Zhenxin Zhang, Qianqian Zhu, Masahiro Sadakane, Toru Murayama, Norihito Hiyoshi, Akira Yamamoto, Shinichi Hata, Hisao Yoshida, Satoshi Ishikawa, Masahiko Hara, Wataru Ueda

    Read original paper ↗ ·

  14. Multi-dimensional Crystal Structuring of Complex Metal Oxide Catalysts of Group V and VI Elements by Unit-Assembling

    Topics in Catalysis · 2018-11-07

    Satoshi Ishikawa, Zhenxin Zhang, Toru Murayama, Norihito Hiyoshi, Masahiro Sadakane, Wataru Ueda

    Read original paper ↗ ·

  15. Electronic and Dielectric Properties of MoV-Oxide (M1 Phase) under Alkane Oxidation Conditions

    The Journal of Physical Chemistry C · 2019-04-29

    Anna Maria Wernbacher, Pierre Kube, Michael Hävecker, Robert Schlögl, Annette Trunschke

    Read original paper ↗ ·

  16. High dimensionally structured W-V oxides as highly effective catalysts for selective oxidation of toluene

    Catalysis Today · 2019-08-16

    Toru Murayama, Satoshi Ishikawa, Norihito Hiyoshi, Yoshinori Goto, Zhenxin Zhang, Takashi Toyao, Ken‐ichi Shimizu, Shutoku Lee, Wataru Ueda

    Read original paper ↗ ·

  17. Site specific and localized structural displacements in open structured multimetallic oxides

    Nanoscale · 2020-01-01

    Thomas Lunkenbein, Liudmyla Masliuk, Milivoj Plodinec, Gerardo Algara‐Siller, Sabrina Jung, Mateusz Jastak, Pierre Kube, Annette Trunschke, Robert Schlögl

    Read original paper ↗ ·

  18. Compositional Decoupling of Bulk and Surface in Open-Structured Complex Mixed Oxides

    The Journal of Physical Chemistry C · 2020-10-13

    Liudmyla Masliuk, Franz Schmidt, Walid Hetaba, Milivoj Plodinec, Gudrun Auffermann, Klaus Hermann, Detre Teschner, Frank Girgsdies, Annette Trunschke, Robert Schlögl, Thomas Lunkenbein

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  19. Configurations of V4+ centers in the MoVO catalyst material. A systematic stability analysis of DFT results

    SN Applied Sciences · 2020-10-28

    Torstein Fjermestad, Wenqing Li, Alexander Genest, Notker Rösch

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  20. Probing the Positions of TeO Moieties in the Channels of the MoVNbTeO M1 Catalyst: A Density Functional Theory Model Study

    Catalysis Letters · 2021-01-30

    Juan Manuel Arce-Ramos, Graham Rugg, Alexander Genest, Notker Rösch

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  21. Nb−V Mixed Oxide with a Random Assembly of Pentagonal Units: A Catalyst for Oxidative Dehydrogenation of Ethane and Propane

    ChemCatChem · 2021-04-15

    Kosuke Shimoda, Satoshi Ishikawa, Katsuya Matsumoto, Mai Miyasawa, Marino Takebe, Riku Matsumoto, Syutoku Lee, Wataru Ueda

    Read original paper ↗ ·

  22. Structural developments during the low-temperature oxidation of Nb7W10O47

    Journal of Solid State Chemistry · 2021-07-12

    Frank Krumeich, Michael Dieter Wörle

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  23. Mo-V-Based Crystalline Complex Metal Oxide Catalysts

    Springer eBooks · 2022-01-01

    Satoshi Ishikawa, Wataru Ueda

    Read original paper ↗ ·

  24. Atomic and Electronic Structures of the Interfaces between Perovskite La0.75Sr0.25MnO3 and Brownmillerite SrCoO2.5

    physica status solidi (b) · 2022-12-01

    Z.J. Wu, Wandong Xing, Yuanmin Zhu, Rong Yu

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  25. Operando Electron Microscopy of Catalysts: The Missing Cornerstone in Heterogeneous Catalysis Research?

    Chemical Reviews · 2023-11-15

    See Wee Chee, Thomas Lunkenbein, Robert Schlögl, Beatriz Roldán Cuenya

    Read original paper ↗ ·

  26. Oxidation Catalysis of Crystalline Mo3VOx for the Selective Oxidation of Ethane

    ACS Catalysis · 2023-11-17

    Satoshi Ishikawa, Kosuke Shimoda, Takashi Kamachi, Nagisa Aoki, Takeshi Hagiwara, Atsushi Urakawa, Wataru Ueda

    Read original paper ↗ ·

  27. Linking Bulk and Surface Structures in Complex Mixed Oxides

    ACS Catalysis · 2024-05-29

    Liudmyla Masliuk, Kyeonghyeon Nam, Maxwell W. Terban, Yonghyuk Lee, Pierre Kube, Daniel Delgado, Frank Girgsdies, Karsten Reuter, Robert Schlögl, Annette Trunschke, Christoph Scheurer, Mirijam Zobel, Thomas Lunkenbein

    Read original paper ↗ ·

  28. Fine-Tuning Microporosity of Crystalline Vanadomolybdate Frameworks for Selective Adsorptive Separation of Kr from Xe

    Langmuir · 2024-11-14

    Suchona Akter, Yong Li, Min‐Bum Kim, Md Omar Faruque, Zhonghua Peng, Praveen K. Thallapally, Mohammad R. Momeni

    Read original paper ↗ ·
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