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RESEARCH PAPER · Physical Review Letters · 2012

Surface Origin of High Conductivities in Undoped In 2 O 3 Thin Films

Stephan Lany, Andriy Zakutayev, T.O. Mason, John F. Wager, Kenneth Reinhard Poeppelmeier, John D. Perkins, Joseph J. Berry, David S. Ginley, Alex Zunger

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Surface Origin of High Conductivities in Undoped In 2 O 3 Thin FilmsOriginalBulk and surface characterization of In 2 O 3 (001) single crystals85Hydrogen in oxide semiconductors93Transport and angular resolved photoemission measurements of the electronic properties of In2O3 bulk single crystals78Novel lotus root slice-like self-assembled In2O3 microspheres: Synthesis and NO2-sensing properties68Transparent Conducting Oxides: Electronic Structure–Property Relationship from Photoelectron Spectroscopy with in situ Sample Preparation151Theory and Modeling of Oxide Semiconductors14Microscopic Origin of Electron Accumulation in In2O3119Quasi-reversible point defect relaxation in amorphous In-Ga-Zn-O thin films by in situ electrical measurements17Direct observation of the band gap shrinkage in amorphous In2O3–ZnO thin films26Orthorhombic In2O3: A Metastable Polymorph of Indium Sesquioxide56Orthorhombisches In2O3 – ein metastabiles Indiumsesquioxid‐ Polymorph3Epitaxial undoped indium oxide thin films: Structural and physical properties51Self-assembled homojunction In2O3transparent thin-film transistors9Enhancement of bias and illumination stability in thin-film transistors by doping InZnO with wide-band-gap Ta2O548The Effect of Solvent on the Morphology of Indium Oxide Deposited by Aerosol-assisted Chemical Vapour Deposition8In situhigh pressure high temperature experiments in multi-anvil assemblies with bixbyite-type In2O3and synthesis of corundum-type and orthorhombic In2O3polymorphs17Indium oxide thin-film homo-junctions: Morphology and electrical properties7First Combined Electron Paramagnetic Resonance and FT-IR Spectroscopic Evidence for Reversible O2Adsorption on In2O3–xNanoparticles33In situ Hall effect and conductivity measurements of ITO thin films24In‐gap states of In2O3 single crystals investigated by scanning tunneling spectroscopy15Non-equilibrium origin of high electrical conductivity in gallium zinc oxide thin films60Influence of polarity and hydroxyl termination on the band bending at ZnO surfaces113Effects of Solvent Treatment on the Characteristics of InGaZnO Thin-Film Transistors8Thermodynamics of native defects in In 2 O 3 crystals using a first-principles method15Effect of exposure to optical radiation and temperature on the electrical and optical properties of In2O3 films produced by autowave oxidation3Coloration and oxygen vacancies in wide band gap oxide semiconductors: Absorption at metallic nanoparticles induced by vacancy clustering—A case study on indium oxide35Schottky contacts to In2O371Effects of substrate and ambient gas on epitaxial growth indium oxide thin films27Oxygen Vacancies Confined in Ultrathin Indium Oxide Porous Sheets for Promoted Visible-Light Water Splitting1396Characterization and Modeling of a-IGZO TFTs22Nanostructured Transparent Conducting Oxides for Advanced Photovoltaic Applications3Electronic conduction properties of indium tin oxide: single-particle and many-body transport55Schottky contact by Ag on In2O3 (111) single crystals15Photoemission surface characterization of (001) In2O3 thin film through the interactions with oxygen, water and carbon monoxide: Comparison with (111) orientation21Study of electrical fatigue by defect engineering in organic light-emitting diodes28Phase Stability and Optoelectronic Properties of the Bixbyite Phase in the Gallium–Indium–Tin–Oxide System4Bias and Light-Induced Instabilities in a-IGZO Thin Film Transistors1Bias and Light-Induced Instabilities in a-IGZO Thin Film Transistors1Dopant and Defect Induced Electronic States at In2O3 Surfaces10Formation and local conduction of nanopits in BiFeO 3 epitaxial films13Theoretical Modeling of Oxygen and Water Adsorptionon Indium Oxide (111) Surface5Indium oxide—a transparent, wide-band gap semiconductor for (opto)electronic applications333Structural and optical properties of (In,Ga)2O3 thin films and characteristics of Schottky contacts thereon68Origin of the Accumulation Layer at the InN/a-In 2 O 3 Interface7Confirmation of the Dominant Defect Mechanism in Amorphous In–Zn–O Through the Application of In Situ Brouwer Analysis9Flexography‐Printed In2O3 Semiconductor Layers for High‐Mobility Thin‐Film Transistors on Flexible Plastic Substrate138Bias and Light-Induced Instabilities in a-IGZO Thin Film Transistors1Polaron character of the near-E F band of cleaved In 2 O 3 (111) single crystals5Research progress on oxide-based thin film transisitors12Photoexcited Surface Frustrated Lewis Pairs for Heterogeneous Photocatalytic CO2 Reduction289Electronic Reducibility Scales with Intergranular Interface Area in Consolidated In2O3 Nanoparticles Powders5Comparative study of the electronic structures of the In and Sn/In2O3 (111) interfaces16Silver oxide Schottky contacts and metal semiconductor field-effect transistors on SnO2 thin films35Simultaneous observation of small- and large-energy-transfer electron-electron scattering in three-dimensional indium oxide thick films3Understanding and control of bipolar self-doping in copper nitride43Spatial Separation of Charge Carriers in In2O3–x(OH)y Nanocrystal Superstructures for Enhanced Gas-Phase Photocatalytic Activity145Effect of Precursor Selection on the Photocatalytic Performance of Indium Oxide Nanomaterials for Gas-Phase CO2 Reduction61Observation of indium ion migration-induced resistive switching in Al/Mg0.5Ca0.5TiO3/ITO11Amorphous and crystalline In2O3-based transparent conducting films for photovoltaics43Device Physics Modeling of Surfaces and Interfaces from an Induced Gap State Perspective38Carrier dynamics and the role of surface defects: Designing a photocatalyst for gas-phase CO 2 reduction124Photoelectron spectroscopic study of electronic state and surface structure of In2O3 single crystals11Consequences of plasma oxidation and vacuum annealing on the chemical properties and electron accumulation of In2O3 surfaces22Low temperature, solution-processed ambipolar field-effect transistors based on polymer/self-assembled monolayer modified InOx hybrid structures for balanced hole and electron mobilities exceeding 1 cm2 V−1 s−17The variation of electrical transport properties with thickness for ultrathin indium oxide films3Creation of a Short-Range Ordered Two-Dimensional Electron Gas Channel in Al2O3/In2O3 Interfaces66Sustainable and scalable natural fiber welded palladium-indium catalysts for nitrate reduction57Direct visible light activation of a surface cysteine-engineered [NiFe]-hydrogenase by silver nanoclusters40Self-diffusion measurements in In2O3 isotopic heterostructures: Oxygen vacancy energetics4Deep vs shallow nature of oxygen vacancies and consequent n -type carrier concentrations in transparent conducting oxides155Degenerate and non-degenerate In2O3 thin films by pulsed electron beam deposition25Influence of hopping conduction on the thermopower of indium oxide thick films10Identification of Lone-Pair Surface States on Indium Oxide30Puzzling robust 2D metallic conductivity in undoped β-Ga2O3 thin films30Ultrafast growth rate and high mobility In2O3 films grown on c-sapphire via low pressure chemical vapor deposition16Threonine to Cysteine (T225C) variant of E coli hydrogenase-18The Itinerant 2D Electron Gas of the Indium Oxide (111) Surface: Implications for Carbon‐ and Energy‐Conversion Applications26Giant bulk photovoltaic effect in solar cell architectures with ultra-wide bandgap Ga2O3 transparent conducting electrodes42Nanostructures d’oxyde d’indium pour les mémoires résistives RRAM intégrées en CMOS Back-End-Of-Line0Advanced composite nanostructures as gas sensors0Recent progress on the electronic structure, defect, and doping properties of Ga2O3599Gas adsorption effects on electrical properties of amorphous In 2 O 3 thin-film transistors under various environments8Impact of hydrochloric acid on the epitaxial growth of In2O3 films on (0001)α-Al2O3 substrates by mist CVD11Aerobic Photocatalytic H2 Production by a [NiFe] Hydrogenase Engineered to Place a Silver Nanocluster in the Electron Relay45The role of water vapor during the synthesis of hydrogen doped In2O37A temperature sensor based on flexible substrate with ultra-high sensitivity for low temperature measurement65Optimizing the Electronic Structure of In 2 O 3 through Mg Doping for NiO/In 2 O 3 p–n Heterojunction Diodes28Mechanistic studies toward the rational design of oxide catalysts for carbon dioxide hydrogenation2Recent Development in Defects Engineered Photocatalysts: An Overview of the Experimental and Theoretical Strategies283Near ambient-pressure X-ray photoelectron spectroscopy study of CO2 activation and hydrogenation on indium/copper surface61Origin of simultaneous enhancement of work function and carrier concentration in In2O3 films by excimer-laser irradiation7Wide Bandgap Oxide Semiconductors: from Materials Physics to Optoelectronic Devices629Influence of Defects on the Schottky Barrier Height at BaTiO3/RuO2 Interfaces9Temporal Evolution of Microscopic Structure and Functionality during Crystallization of Amorphous Indium-Based Oxide Films23Influence of Surface Adsorption on the Electrical Transport Properties of Ultrathin Indium Tin Oxide Films1High CO2 resistance of indium-doped cobalt-free 60 wt.%Ce0.9Pr0.1O2-δ-40 wt.%Pr0.6Sr0.4Fe1-In O3-δ oxygen transport membranes18Atomistic Descriptions of Gas-Surface Interactions on Tin Dioxide18Do We Need “Ionosorbed” Oxygen Species? (Or, “A Surface Conductivity Model of Gas Sensitivity in Metal Oxides Based on Variable Surface Oxygen Vacancy Concentration”)62High-mobility hydrogenated polycrystalline In2O3 (In2O3:H) thin-film transistors247A Nonempirical Study of Oxygen Adsorption on the (011) In2O3 Surface5Perovskite–organic tandem solar cells with indium oxide interconnect423Impact of layer thickness on the operating characteristics of In2O3/ZnO heterojunction thin-film transistors33Modulating Oxygen Vacancies in Lead Chromate for Photoelectrocatalytic Water Splitting63On the CO2 photocatalytic reduction over indium tin oxide (ITO) ultra-thin films in water vapor: Experimental and theoretical study10The Fermi energy as common parameter to describe charge compensation mechanisms: A path to Fermi level engineering of oxide electroceramics67Oxygen Plasma Treatment to Enable Indium Oxide MESFET Devices8Tunable-performance all-oxide structure field-effect transistor based atomic layer deposited Hf-doped In2O3 thin films9Characteristics of Ultrathin Indium Oxide Thin‐Film Transistors with Diverse Channel Lengths Fabricated by Atomic Layer Deposition4Review—Extremely Thin Amorphous Indium Oxide Transistors107Effects of Doping Ratio and Thickness of Indium Tin Oxide Thin Films Prepared by Magnetron Sputtering at Room Temperature5High-performance nano-scale InSnO transistors1Effect of point defects on electrochemical performances of α-Ga2O3 microrods prepared with hydrothermal process for supercapacitor application6Unravelling the doping mechanism and origin of carrier limitation in Ti-doped In2O3 films8Realization of tunable-performance in atomic layer deposited Hf-doped In2O3 thin film transistor via oxygen vacancy modulation12Perovskite–organic tandem solar cells235Origin and quantification of the ultimate carrier concentration limits in In2O3 and Sn-doped In2O313On the mass action law and the power law response in tin dioxide gas sensors3Growth of high quality polycrystalline InGaO thin films by spray pyrolysis for coplanar thin-film transistors on polyimide substrate18Midgap states and energy alignment at interconnect are crucial for perovskite tandem solar cells5Mechanism of Reaction of H2 on the (011) In2O3 Surface with a Preadsorbed Oxygen Molecule0DFT modeling of reaction of H2 with O2 pre-adsorbed on In2O3(011) surface9Giant Decrease in Interfacial Energy of Liquid Metals by Native Oxides94Highly Stable, Crystalline InGaO Thin-Film Transistors by 7% Lanthanum Incorporation9High mobility In 2 O 3 thin films grown by atomic layer deposition using a microwave remote plasma source for field-effect transistor applications2In2O3: An Oxide Semiconductor for Thin-Film Transistors, a Short Review4Electron-Doped Semiconducting Rocksalt Al x Sc 1– x N: An Emerging Transparent Conducting Nitride0Suppression of Silver Interfacial Diffusion in Flexible Low‑E Membranes: Roles of Protective Layers and Doped In₂O₃ Dielectrics0Charge-state-driven structural evolution and aromaticity in the anionic and neutral In4O2 clusters revealed by joint experimental and theoretical investigation0High-Mobility Indium Native Oxide Transistors via Liquid-Metal Printing in Air0Reversible Thickness Engineering in Amorphous In 2 O 3 Transistors1Understanding the crystallization mechanism of atomic layer deposited InOx/GaOx nanolaminate structures0Overcoming the Surface Instability Bottleneck in High-Mobility Crystalline Indium Oxide Thin-Film Transistors by Yttrium Oxide Stabilization1Pump-light-induced carrier modulation and multimode optical absorption in dielectric-functionalized porous In 2 O 31Artificial Synaptic Device Based on Self‐Aligned c‐In 2 O 3 TFTs With an Ultrathin MgO Interlayer0Dual-Functional Modulation of Electronic Structure and Lattice Strain Toward Decoupled Thermoelectric Performance and Mechanical Enhancement in Na-Doped In2O3 Used for Welding Robot0

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  1. Bulk and surface characterization of In 2 O 3 (001) single crystals

    Physical Review B · 2012-03-28

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  2. Hydrogen in oxide semiconductors

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  3. Transport and angular resolved photoemission measurements of the electronic properties of In2O3 bulk single crystals

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  4. Novel lotus root slice-like self-assembled In2O3 microspheres: Synthesis and NO2-sensing properties

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  5. Transparent Conducting Oxides: Electronic Structure–Property Relationship from Photoelectron Spectroscopy with in situ Sample Preparation

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  6. Theory and Modeling of Oxide Semiconductors

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  7. Microscopic Origin of Electron Accumulation in In2O3

    Physical Review Letters · 2013-01-30

    K. H. L. Zhang, R.G. Egdell, F. Offi, Stefano Iacobucci, L. Petaccia, Sergey Gorovikov, P. D. C. King

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  8. Quasi-reversible point defect relaxation in amorphous In-Ga-Zn-O thin films by in situ electrical measurements

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    Alexander U. Adler, Ted C. Yeh, D. Bruce Buchholz, Robert P. H. Chang, Thomas O. Mason

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  9. Direct observation of the band gap shrinkage in amorphous In2O3–ZnO thin films

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  10. Orthorhombic In2O3: A Metastable Polymorph of Indium Sesquioxide

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  11. Orthorhombisches In2O3 – ein metastabiles Indiumsesquioxid‐ Polymorph

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  12. Epitaxial undoped indium oxide thin films: Structural and physical properties

    Solar Energy Materials and Solar Cells · 2013-05-07

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  13. Self-assembled homojunction In2O3transparent thin-film transistors

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  14. Enhancement of bias and illumination stability in thin-film transistors by doping InZnO with wide-band-gap Ta2O5

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  15. The Effect of Solvent on the Morphology of Indium Oxide Deposited by Aerosol-assisted Chemical Vapour Deposition

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  16. In situhigh pressure high temperature experiments in multi-anvil assemblies with bixbyite-type In2O3and synthesis of corundum-type and orthorhombic In2O3polymorphs

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  17. Indium oxide thin-film homo-junctions: Morphology and electrical properties

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  18. First Combined Electron Paramagnetic Resonance and FT-IR Spectroscopic Evidence for Reversible O2Adsorption on In2O3–xNanoparticles

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  19. In situ Hall effect and conductivity measurements of ITO thin films

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  20. In‐gap states of In2O3 single crystals investigated by scanning tunneling spectroscopy

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  21. Non-equilibrium origin of high electrical conductivity in gallium zinc oxide thin films

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  22. Influence of polarity and hydroxyl termination on the band bending at ZnO surfaces

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  23. Effects of Solvent Treatment on the Characteristics of InGaZnO Thin-Film Transistors

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  24. Thermodynamics of native defects in In 2 O 3 crystals using a first-principles method

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  25. Effect of exposure to optical radiation and temperature on the electrical and optical properties of In2O3 films produced by autowave oxidation

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  26. Coloration and oxygen vacancies in wide band gap oxide semiconductors: Absorption at metallic nanoparticles induced by vacancy clustering—A case study on indium oxide

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  27. Schottky contacts to In2O3

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  28. Effects of substrate and ambient gas on epitaxial growth indium oxide thin films

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  29. Oxygen Vacancies Confined in Ultrathin Indium Oxide Porous Sheets for Promoted Visible-Light Water Splitting

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  31. Nanostructured Transparent Conducting Oxides for Advanced Photovoltaic Applications

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  32. Electronic conduction properties of indium tin oxide: single-particle and many-body transport

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  33. Schottky contact by Ag on In2O3 (111) single crystals

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  34. Photoemission surface characterization of (001) In2O3 thin film through the interactions with oxygen, water and carbon monoxide: Comparison with (111) orientation

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  35. Study of electrical fatigue by defect engineering in organic light-emitting diodes

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  36. Phase Stability and Optoelectronic Properties of the Bixbyite Phase in the Gallium–Indium–Tin–Oxide System

    Journal of the American Ceramic Society · 2014-11-08

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  37. Bias and Light-Induced Instabilities in a-IGZO Thin Film Transistors

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  38. Bias and Light-Induced Instabilities in a-IGZO Thin Film Transistors

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  39. Dopant and Defect Induced Electronic States at In2O3 Surfaces

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  40. Formation and local conduction of nanopits in BiFeO 3 epitaxial films

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  41. Theoretical Modeling of Oxygen and Water Adsorptionon Indium Oxide (111) Surface

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  42. Indium oxide—a transparent, wide-band gap semiconductor for (opto)electronic applications

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  43. Structural and optical properties of (In,Ga)2O3 thin films and characteristics of Schottky contacts thereon

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  44. Origin of the Accumulation Layer at the InN/a-In 2 O 3 Interface

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  45. Confirmation of the Dominant Defect Mechanism in Amorphous In–Zn–O Through the Application of In Situ Brouwer Analysis

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  46. Flexography‐Printed In2O3 Semiconductor Layers for High‐Mobility Thin‐Film Transistors on Flexible Plastic Substrate

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  47. Bias and Light-Induced Instabilities in a-IGZO Thin Film Transistors

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  48. Polaron character of the near-E F band of cleaved In 2 O 3 (111) single crystals

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  49. Research progress on oxide-based thin film transisitors

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  50. Photoexcited Surface Frustrated Lewis Pairs for Heterogeneous Photocatalytic CO2 Reduction

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