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RESEARCH PAPER · Journal of the American Chemical Society · 2010

Reversible Anion Exchange and Catalytic Properties of Two Cationic Metal−Organic Frameworks Based on Cu(I) and Ag(I)

Honghan Fei, David L. Rogow, Scott R. J. Oliver

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Reversible Anion Exchange and Catalytic Properties of Two Cationic Metal−Organic Frameworks Based on Cu(I) and Ag(I)OriginalTwo cationic metal–organic frameworks based on cadmium and α,ω-alkanedisulfonate anions and their photoluminescent properties15Solvent-Mediated Central Metals Transformation from a Tetranuclear NiII Cage to a Decanuclear CuII “Pocket”382D Cationic Metal-Organic Frameworks of Ag+ with Mixed Ligands (Semi-Rigid Dipyridyl, 3-pmpmd, and Diphosphine, dppe)5Metal‐Organic Frameworks: A Rapidly Growing Class of Versatile Nanoporous Materials1407Three-Dimensional Porous Cd(II) Coordination Polymer with Large One-Dimensional Hexagonal Channels: High Pressure CH 4 and H 2 Adsorption Studies74A mixed ligand route for the construction of tetrahedrally coordinated porous lithium frameworks22Controlling interpenetration in CuCN coordination polymers by size of the pendant substituents of terpyridine ligands21Dinuclear silver(i) complexes for the design of metal–ligand networks based on triazolopyrimidines45Macrocyclic receptor for pertechnetate and perrhenate anions25Recent progress in actinide borate chemistry94Self-assembled metallo-macrocycle based coordination polymers with unsymmetrical amide ligands20High-Throughput Study of the Cu(CH3COO)2·H2O−5-Nitroisophthalic Acid−Heterocyclic Ligand System: Synthesis, Structure, Magnetic, and Heterogeneous Catalytic Studies of Three Copper Nitroisophthalates31Rational Design of Zinc–Organic Coordination Polymers Directed by N‐Donor Co‐ligands62A New Paradigm for Anion Trapping in High Capacity and Selectivity: Crystal-to-Crystal Transformation of Cationic Materials279Thermal Transformation of a Layered Multifunctional Network into a Metal–Organic Framework Based on a Polymeric Organic Linker63Immobilization, Trapping, and Anion Exchange of Perrhenate Ion Using Copper-Based Tripodal Complexes56A trinuclear silver coordination polymer from a bipyridine bis-urea macrocyclic ligand and silver triflate22Control of Morphology and Catalytic Activity of a Cationic Layered Material4Three-Dimensional Phosphine Metal–Organic Frameworks Assembled from Cu(I) and Pyridyl Diphosphine66Single-Walled Polytetrazolate Metal–Organic Channels with High Density of Open Nitrogen-Donor Sites and Gas Uptake182Aza-heterocyclic ligand assisted assembly of new cobalt MOFs with pcu and graphite related structures35Design and construction of coordination polymers based on 2,2′-dinitro-4,4′-biphenyldicarboxylate and semi-rigid N-donor ligands: diverse structures and magnetic properties30Fast capture and separation of, and luminescent probe for, pollutant chromate using a multi-functional cationic heterometal-organic framework247Multi-functional metal–organic frameworks assembled from a tripodal organic linker52Solvothermal synthesis and characterization of two inorganic–organic hybrid materials based on barium8Surfactant-directed assembly of mesoporous metal–organic framework nanoplates in ionic liquids132Utilizing a copper MOF as a reagent in a solvent mediated reaction to form a topologically distinct MOF12Valence Force Field for Layered Double Hydroxide Materials Based on the Parameterization of Octahedrally Coordinated Metal Cations46Superbase Route to Supertetrahedral Chalcogenide Clusters86Development of Composite Inorganic Building Blocks for MOFs235Ion Exchange in Metal–Organic Framework for Water Purification: Insight from Molecular Simulation87Selectivity, Kinetics, and Efficiency of Reversible Anion Exchange with TcO4− in a Supertetrahedral Cationic Framework176Independent 1D Nanosized Metal–Organic Tube: Anion Exchange, Separation, and Anion-Responsive Luminescence64Synthesis, Structure, and Magnetic Properties of a New Eight-Connected Metal–Organic Framework (MOF) based on Co 4 Clusters52A sulfate-bridged CuII complex with 1-D helical-chain structure: Synthesis, structure and magnetic property6Solvothermal synthesis, structure and catalytic activity of a mixed-valence CuI/CuII complex with 1-D chain structure13Selective Metal Cation Capture by Soft Anionic Metal–Organic Frameworks via Drastic Single-Crystal-to-Single-Crystal Transformations128Anion Exchange of the Cationic Layered Material [Pb2F2]2+49Two Zeolite‐Type Frameworks in One Metal–Organic Framework with Zn 24 @Zn 104 Cube‐in‐Sodalite Architecture69Two Zeolite‐Type Frameworks in One Metal–Organic Framework with Zn 24 @Zn 104 Cube‐in‐Sodalite Architecture9A Cationic Antimonite Chain Templated by Sulfate: [Sb6O74+][(SO42–)2]9Coordination Polymers of Copper and Zinc Ions with a Linear Linker Having Imidazole at Each End and an Azo Moiety in the Middle: Pedal Motion, Gas Adsorption, and Emission Studies45Molecular Polyselenide Anions Sandwiched between Cationic Extended Metal Hydroxides: Synthesis and Structures of [Sr2Sn(OH)6(H2O)6]Se4and [Sr2Sn(OH)6(H2O)5]Se3·H2O4Unusual Coordination for Plutonium(IV), Cerium(IV), and Zirconium(IV) in the Cationic Layered Materials [M2Te4O11]X2 (M = Pu, Ce, Zr; X = Cl, Br)29Metal–Organic Frameworks and Self-Assembled Supramolecular Coordination Complexes: Comparing and Contrasting the Design, Synthesis, and Functionality of Metal–Organic Materials2950Synthesis and magnetic properties of a 3-D nickel hydroxide capped by succinate3Selective Adsorption Properties of Cationic Metal–Organic Frameworks Based on Imidazolic Linker56Construction of a series of coordination polymers from three imidazole-based multi-carboxylate ligands36Metal-organic frameworks displaying single crystal-to-single crystal transformation through postsynthetic uptake of metal clusters78Supramolecular isomerism, single-crystal to single-crystal transformation induced by release of in situ generated I2 between two supramolecular frameworks8Synthesis of a Cationic Inorganic Layered Material for Trapping Anionic Pharmaceutical Pollutants1Transmetalation: routes to metal exchange within metal–organic frameworks303A Cationic Metal–Organic Solid Solution Based on Co(II) and Zn(II) for Chromate Trapping144Series of 2D Heterometallic Coordination Polymers Based on Ruthenium(III) Oxalate Building Units: Synthesis, Structure, and Catalytic and Magnetic Properties23Fabrication of Supported Cuprous Sites at Low Temperatures: An Efficient, Controllable Strategy Using Vapor-Induced Reduction114Anion Exchange in Coordination‐Network Materials7Selective anion exchange with nanogated isoreticular positive metal-organic frameworks370Syntheses, structural diversity and photo-physical properties of copper(I) and silver(I) coordination polymers based on the pyridine-4-amidoxime ligand10The Chemistry and Applications of Metal-Organic Frameworks16945Photoluminescent Metal–Organic Frameworks – Rapid Preparation, Catalytic Activity, and Framework Relationships18Four Coordination Polymers Based on Identical Eight-Connected Heptanuclear Clusters: Spin Canting, Spin Glass, Antiferromagnetism, and Gas Adsorption46Syntheses, Structures, and Catalytic Activities of Copper(I) Complexes with the Ligand 2(4,5‐Diphenyl‐1H‐imidazol‐2‐yl)pyridine0Metal–Organic Frameworks Based on Previously Unknown Zr8/Hf8 Cubic Clusters233A Cationic Metal–Organic Framework Consisting of Nanoscale Cages: Capture, Separation, and Luminescent Probing of Cr2O72− through a Single‐Crystal to Single‐Crystal Process349A Cationic Metal–Organic Framework Consisting of Nanoscale Cages: Capture, Separation, and Luminescent Probing of Cr2O72− through a Single‐Crystal to Single‐Crystal Process53Perfect Statistical Symmetrization of a Heterofunctional Ligand Induced by Pseudo-Copper Trimer in an Expanded Matrix of HKUST-16Experimental Studies and Mechanism Analysis of High-Sensitivity Luminescent Sensing of Pollutional Small Molecules and Ions in Ln4O4 Cluster Based Microporous Metal–Organic Frameworks314Water molecule-driven reversible single-crystal to single-crystal transformation of a multi-metallic coordination polymer with controllable metal ion movement26A metal–organic framework assembled from Y(iii), Li(i), and terephthalate: hydrothermal synthesis, crystal structure, thermal decomposition and topological studies17Lanthanide ion exchange properties of a coordination polymer consisting of di(2-ethylhexyl) phosphoric acid and trivalent metal ions (Ce3+, Fe3+, or Al3+)23Substitution reactions in metal–organic frameworks and metal–organic polyhedra221Synthesis of a naphthalenediimide-based cyclophane for controlling anion–arene interactions10Metal–Organic Framework Threaded with Aminated Polymer Formed in Situ for Fast and Reversible Ion Exchange119Anion Stripping as a General Method to Create Cationic Porous Framework with Mobile Anions107A spin-canted Ni II 4 -based metal–organic framework with gas sorption properties and high adsorptive selectivity for light hydrocarbons29Versatile Mesoporous Dy III Coordination Framework for Highly Efficient Trapping of Diverse Pollutants34Dynamic structural transformations of coordination supramolecular systems upon exogenous stimulation113Anion-Directed Assemblies of Cationic Metal–Organic Frameworks Based on 4,4′-Bis(1,2,4-triazole): Syntheses, Structures, Luminescent and Anion Exchange Properties47A sulfonate-based Cu(I) metal-organic framework as a highly efficient and reusable catalyst for the synthesis of propargylamines under solvent-free conditions56A cage-based cationic body-centered tetragonal metal–organic framework: single-crystal to single-crystal transformation and selective uptake of organic dyes163A metal–organic framework as a highly efficient and reusable catalyst for the solvent-free 1,3-dipolar cycloaddition of organic azides to alkynes41Selective Anion Exchange and Tunable Luminescent Behaviors of Metal–Organic Framework Based Supramolecular Isomers60Water-Stable Metal–Organic Frameworks for Fast and High Dichromate Trapping via Single-Crystal-to-Single-Crystal Ion Exchange314A multifunctional microporous anionic metal–organic framework for column-chromatographic dye separation and selective detection and adsorption of Cr 3+126An In III -based anionic metal–organic framework: sensitization of lanthanide (III) ions and selective absorption and separation of cationic dyes136Combination effect of ionic liquid components on the structure and properties in 1,4-benzenedicarboxylate based zinc metal–organic frameworks32Diverse isostructural MOFs by postsynthetic metal node metathesis: anionic-to-cationic framework conversion, luminescence and separation of dyes72Metal–organic frameworks for applications in remediation of oxyanion/cation-contaminated water160Periodic tiling of triangular and square nanotubes in a cationic metal–organic framework for selective anion exchange78Stabilization of a highly porous metal–organic framework utilizing a carborane-based linker54Structural diversities in Cu( i ) and Ag( i ) sulfonate coordination polymers and their anion exchange properties11Template controlled synthesis of cluster-based porous coordination polymers: crystal structure, magnetism and adsorption16Triazole based Ag coordination clusters: synthesis, structural diversity and anion exchange properties24Tuned synthesis of two coordination polymers of Cd( ii ) using substituted bent 3-pyridyl linker and succinate: structures and their applications in anion exchange and sorption properties22CrIII and CuI complexes of 2,2′,2″-(1H-imidazole-2,4,5-triyl)-tripyridine: In situ generation of imidazole ring from the coupling of picolinaldehyde and ammonium acetate3Cation-Exchange Porosity Tuning in a Dynamic 4d–4f–3d Framework for NiII Ion-Selective Luminescent Probe40Polystyrenesulfonate Threaded in MIL-101Cr(III): A Cationic Polyelectrolyte Synthesized Directly into a Metal–Organic Framework62Cooperative Crystallization of Heterometallic Indium–Chromium Metal–Organic Polyhedra and Their Fast Proton Conductivity153Cooperative Crystallization of Heterometallic Indium–Chromium Metal–Organic Polyhedra and Their Fast Proton Conductivity28Applications of Supramolecular Anion Recognition1249Metal–organic frameworks assembled from lanthanide and 2,5-pyridinedicaboxylate with cubane-like [Ln4(OH)4] building units14Syntheses, structures and anion exchange properties of accommodative silver chains using a positively charged and flexible ligand14A new 3D Cd-triazolate framework obtained from in situ decarboxylication of 5-amino-3-carboxyl-1,2,4-triazole12Construction of porous cationic frameworks by crosslinking polyhedral oligomeric silsesquioxane units with N-heterocyclic linkers79A 3D chiral metal-organic framework based on left-handed helices containing 3-amino-1 H-1,2,4-triazole ligand9Perchlorate removal from aqueous solution with a novel cationic metal–organic frameworks based on amino sulfonic acid ligand linking with Cu-4,4′-bipyridyl chains40Two Series of Isostructural Coordination Polymers with Isomeric Benzenedicarboxylates and Different Azine Based N,N′-Donor Ligands: Syntheses, Characterization and Magnetic Properties38Computational characterization and prediction of metal–organic framework properties240Ionic metal-organic frameworks (iMOFs): Design principles and applications308Boosting Proton Conductivity in Highly Robust 3D Inorganic Cationic Extended Frameworks through Ion Exchange with Dihydrogen Phosphate Anions19Cation Exchange in Dynamic 3D Porous Magnets: Improvement of the Physical Properties21Two cadmium(II) coordination polymers constructed from dicarboxylate and bis(imidazole) ligands: Syntheses, crystal structures, luminescence and photocatalytic properties17A [Cu4I] cluster based metal-organic framework to detect F− ions26Creation of a new type of ion exchange material for rapid, high-capacity, reversible and selective ion exchange without swelling and entrainment103A Hexameric Cationic Copper(II) Metallacrown as a Pertechnetate and Perrhenate Scavenger12Structural transformations and solid-state reactivity involving nano lead(II) coordination polymers via thermal, mechanochemical and photochemical approaches49A durable luminescent ionic polymer for rapid detection and efficient removal of toxic Cr 2 O 7 2−61A unique multi-functional cationic luminescent metal–organic nanotube for highly sensitive detection of dichromate and selective high capacity adsorption of Congo red66Removal of TcO 4 − ions from solution: materials and future outlook321Selective removal of cesium and strontium using porous frameworks from high level nuclear waste183Synthesis, crystal structure and luminescence studies of zinc( ii ) and cadmium( ii ) complexes with 6-(1H-tetrazol-5-yl)-2-naphthoic acid15Two solvent-stable MOFs as a recyclable luminescent probe for detecting dichromate or chromate anions132A Water‐Stable Cationic Metal–Organic Framework as a Dual Adsorbent of Oxoanion Pollutants351A Water‐Stable Cationic Metal–Organic Framework as a Dual Adsorbent of Oxoanion Pollutants73Advancing Magnesium–Organic Porous Materials through New Magnesium Cluster Chemistry41Ionothermal synthesis, structures, properties of cobalt-1,4-benzenedicarboxylate metal–organic frameworks33First Cationic Uranyl–Organic Framework with Anion-Exchange Capabilities101Metal-organic frameworks as biosensors for luminescence-based detection and imaging174Azo Functionalized 5-Nitro-1,3-benzenedicarboxylate Based Coordination Polymers with Different Dimensionality and Functionality41Construction of Noninterpenetrating and Interpenetrating (4-Fold and 8-Fold) 3-D Cd(II) Networks with Tris(1,2,4-triazol-4-yl)phenyl)amine Modulated by Aromatic Dicarboxylate Coligands43Charge Control in Two Isostructural Anionic/Cationic CoII Coordination Frameworks for Enhanced Acetylene Capture33Cr(VI) removal via anion exchange on a silver-triazolate MOF308Two-Dimensional Frameworks Based on Ag(I)–N Bond Formation: Single Crystal to Single Molecular Sheet Transformation12Removal of Pertechnetate‐Related Oxyanions from Solution Using Functionalized Hierarchical Porous Frameworks137Microporous Hexanuclear Ln(III) Cluster-Based Metal–Organic Frameworks: Color Tunability for Barcode Application and Selective Removal of Methylene Blue153An unusual porous cationic metal–organic framework based on a tetranuclear hydroxyl-copper( ii ) cluster for fast and highly efficient dichromate trapping through a single-crystal to single-crystal process73Combination effect of ligands and ionic liquid components on the structure and properties of manganese metal–organic frameworks12Cu 2+ sorption from aqueous media by a recyclable Ca 2+ framework47Post-synthetic ion-exchange process in nanoporous metal–organic frameworks; an effective way for modulating their structures and properties170Smart polymer composite materials for water processing0Synthesis, structure, characterization, and multifunctional properties of a family of rare earth organic frameworks24Metal-organic frameworks: Challenges and opportunities for ion-exchange/sorption applications423Synthesis and Structural Studies of Three‐Dimensional Supramolecular Motifs Derived from Neutral and Cationic Zinc Alkanesulfonates14Direct extraction of U(VI) from alkaline solution and seawater via anion exchange by metal-organic framework175Tracking the Superefficient Anion Exchange of a Dynamic Porous Material Constructed by Ag(I) Nitrate and Tripyridyltriazole via Multistep Single-Crystal to Single-Crystal Transformations41Efficient and Selective Uptake of TcO 4 – by a Cationic Metal–Organic Framework Material with Open Ag + Sites415Hydrolytically Stable Luminescent Cationic Metal Organic Framework for Highly Sensitive and Selective Sensing of Chromate Anions in Natural Water Systems256Temperature Treatment of Highly Porous Zirconium-Containing Metal–Organic Frameworks Extends Drug Delivery Release332Highly efficient removal of perchlorate and phosphate by tailored cationic metal-organic frameworks based on sulfonic ligand linking with Cu-4,4′-bipyridyl chains33Selenium Sequestration in a Cationic Layered Rare Earth Hydroxide: A Combined Batch Experiments and EXAFS Investigation118

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  2. Solvent-Mediated Central Metals Transformation from a Tetranuclear NiII Cage to a Decanuclear CuII “Pocket”

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  37. Selective Metal Cation Capture by Soft Anionic Metal–Organic Frameworks via Drastic Single-Crystal-to-Single-Crystal Transformations

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  38. Anion Exchange of the Cationic Layered Material [Pb2F2]2+

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  39. Two Zeolite‐Type Frameworks in One Metal–Organic Framework with Zn 24 @Zn 104 Cube‐in‐Sodalite Architecture

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  40. Two Zeolite‐Type Frameworks in One Metal–Organic Framework with Zn 24 @Zn 104 Cube‐in‐Sodalite Architecture

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  41. A Cationic Antimonite Chain Templated by Sulfate: [Sb6O74+][(SO42–)2]

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  42. Coordination Polymers of Copper and Zinc Ions with a Linear Linker Having Imidazole at Each End and an Azo Moiety in the Middle: Pedal Motion, Gas Adsorption, and Emission Studies

    Crystal Growth & Design · 2012-08-27

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  43. Molecular Polyselenide Anions Sandwiched between Cationic Extended Metal Hydroxides: Synthesis and Structures of [Sr2Sn(OH)6(H2O)6]Se4and [Sr2Sn(OH)6(H2O)5]Se3·H2O

    Zeitschrift für anorganische und allgemeine Chemie · 2012-09-26

    Xiqu Wang, Haiyin H. Wang, Boris Makarenko, Allan J. Jacobson

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  44. Unusual Coordination for Plutonium(IV), Cerium(IV), and Zirconium(IV) in the Cationic Layered Materials [M2Te4O11]X2 (M = Pu, Ce, Zr; X = Cl, Br)

    Inorganic Chemistry · 2012-10-17

    Jian Hung Lin, Justin N. Cross, Juan Diwu, Matthew J. Polinski, Eric M. Villa, Thomas E. Albrecht‐Schmitt

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  45. Metal–Organic Frameworks and Self-Assembled Supramolecular Coordination Complexes: Comparing and Contrasting the Design, Synthesis, and Functionality of Metal–Organic Materials

    Chemical Reviews · 2012-11-02

    Timothy R. Cook, Yao‐Rong Zheng, Peter J. Stang

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  46. Synthesis and magnetic properties of a 3-D nickel hydroxide capped by succinate

    Journal of Materials Chemistry C · 2012-11-29

    Honghan Fei, Andrew D. LaForge, Onyango M. Tedmann, Jeremy C. Robins, Peter Y. Zavalij, Arthur P. Ramirez, Scott R. J. Oliver

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  47. Selective Adsorption Properties of Cationic Metal–Organic Frameworks Based on Imidazolic Linker

    Crystal Growth & Design · 2012-12-05

    Georg Nickerl, Andreas Notzon, Maja Heitbaum, Irena Senkovska, Frank Glorius, Stefan Kaskel

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  48. Construction of a series of coordination polymers from three imidazole-based multi-carboxylate ligands

    Dalton Transactions · 2013-01-01

    Beibei Guo, Li Li, Yang Wang, Yanyan Zhu, Gang Li

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  49. Metal-organic frameworks displaying single crystal-to-single crystal transformation through postsynthetic uptake of metal clusters

    Chemical Science · 2013-01-01

    Jia Li, Peng Huang, Xue-Ru Wu, Jun Tao, Rong‐Bin Huang, Lan‐Sun Zheng

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  50. Supramolecular isomerism, single-crystal to single-crystal transformation induced by release of in situ generated I2 between two supramolecular frameworks

    Dalton Transactions · 2013-01-01

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