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RESEARCH PAPER · Chemistry of Materials · 2002

A Stoichiometric Model for Sillenites

Matjaž Valant, Danilo Suvorov

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A Stoichiometric Model for SillenitesOriginalMechanochemical synthesis of γ-Bi2O331Isomorphic A‐Site Substitution on Sillenite‐Type Compounds6Dielectric Characteristics of Bismuth Oxide Solid Solutions with a Fluorite‐Like Crystal Structure24Synthesis and characterisation of bismuth phosphate-based sillenites8Equilibrium phases in the Bi2O3-rich region of the ZnO–Bi2O3 system23A Tetrameric Neodymium Silanolate: [Nd(OSiMe3)3]411Grain Boundary Defects Induced Switching in Zn- Bi- Mo Ceramic6From molecules to bismuth oxide-based materials: Potential homo- and heterometallic precursors and model compounds293Estudio termodinámico de la región rica en Bi2O3 del sistema Bi2O3-ZnO8Tunable Synthesis of Bismuth Ferrites with Various Morphologies295Photocatalytic activity of Bi24Ga2O39 for degrading methylene blue46Structures and Oxide Mobility in Bi−Ln−O Materials: Heritage of Bi2O3268Dopedγ-Bi2O3: synthesis of microcrystalline samples and crystal chemical analysis of structural data10Evidence of improvement in gas sensing properties of nanostructured bismuth cobaltite prepared by solution-polymerization method16Photocatalytic activity of a sillenite-type material Bi25GaO3938Tuning the Morphology of Bismuth Ferrite Nano‐ and Microcrystals: From Sheets to Fibers51Alkali Metal Ions‐Assisted Controllable Synthesis of Bismuth Ferrites by a Hydrothermal Method57Defects in Inorganic Photorefractive Materials and Their Investigations15Characterization of photorefractive undoped and doped sillenite crystals using holographic and photoconductivity techniques18Vanadium-doped photorefractive titanosillenite crystal13Hydrothermal synthesis and photo-catalytic Property of Bi25FeO40 powders14MOCVD of crystalline Bi2O3 thin films using a single-source bismuth alkoxide precursor and their use in photodegradation of water62Hydrothermal Synthesis of Bi12TiO20 Nanostrucutures Using Anodized TiO2 Nanotubes and Its Application in Photovoltaics37The effects of solvents on the formation of sol–gel-derived Bi12SiO20 thin films18Formation and photocatalytic properties of bismuth ferrite submicrocrystals with tunable morphologies52Microwave Hydrothermal Synthesis, Structural Characterization, and Visible‐Light Photocatalytic Activities of Single‐Crystalline Bismuth Ferric Nanocrystals89Carbon dioxide sensing properties of bismuth cobaltite12Synthesis and characterization of Bi2Fe4O9 powders69Microwave-hydrothermal synthesis of perovskite bismuth ferrite nanoparticles86Structural, electronic, optical, and magneto-optical properties of Bi12MO20 (M = Ti, Ge, Si) sillenite crystals from first principles calculations53Hydrothermal growths, optical features and first-principles calculations of sillenite-type crystals comprising discrete MO 4 tetrahedra32Sillenite-type Bismuth Ferric Nanocrystals: Microwave Hydrothermal Synthesis, Structural Characterization, and Visible-Light Photocatalytic Properties17Improved structural model of Pb-doped γ -Bi 2 O 3 : (Bi 23.68 Pb 0.32 )(Bi 1.28 Pb 0.72 )O 38.483Humidity sensing properties of bismuth phosphates43Microscopical and physical characterization of microwave and microwave-hydrothermal synthesis products80Microstructure Engineering to Drastically Reduce the Leakage Currents of High Voltage ZnO Varistor Ceramics9Dielectric Properties of Sol–Gel‐Derived Bi 12 SiO 20 Thin Films0Raman spectroscopy evidence of inhomogeneous disorder in the bismuth-oxygen framework of Bi 25 InO 39 and other sillenites21Preparation, structural and linear optical properties of zinc sillenite (Bi12.66Zn0.33O19.33) nanocrystals7Relaxor-like Dielectric Behavior in Stoichiometric Sillenite Bi12SiO2030Controllable Synthesis of Different Bismuth Ferrites by a PVA Modified Hydrothermal Method and Photocatalytic Characterization1Morphology and optical absorption of Bi2Fe4O9 crystals via mineralizer-assisted hydrothermal synthesis40Controllable preparation of BiFeO3@carbon core/shell nanofibers with enhanced visible photocatalytic activity43Phase diagram of the pseudobinary system Bi–Co–O26Coexistence of several sillenite-like phases in pseudo-binary and pseudo-ternary systems based on Bi2O35First-principles study of the BiMO4antisite defect in the Bi12MO20(M=Si, Ge, Ti) sillenite compounds13Dielectric and Magnetic Properties of NiFe2-xBixO4 Nanoparticles at Microwave Frequencies Prepared via co-precipitation Method10Room temperature synthesis of Bi 25 FeO 39 and hydrothermal kinetic relations between sillenite- and distorted perovskite-type bismuth ferrites32Surfactant-free solvothermal synthesis and optical characterization of Bi2Fe4O9 in mixed H2O/EtOH solvent38Electron diffraction study of the sillenites Bi12SiO20, Bi25FeO39 and Bi25InO39: Evidence of short-range ordering of oxygen-vacancies in the trivalent sillenites16Preparation and magnetic properties of Bi2Fe4O9/CoFe2O4 composite powders8Controllable phase evolution of bismuth ferrite oxides by an organic additive modified hydrothermal method18First-principles study of the phonon modes in bismuth sillenites7Appearance of [110] orientated growth layer on (100) face and exposure of (111) faces of cubic bismuth phosphate crystal7Heat capacity, entropy, oxygen non-stoichiometry and magnetic properties of cobalt sillenite Bi24Co2O39−7Shape-controlled synthesis and facet-dependent performance of single-crystal Bi 25 GaO 39 photocatalysts12Influence of femtosecond pulsed laser irradiation on bismuth germanium oxide single crystal properties5Novel Molten Oxide Membrane for Ultrahigh Purity Oxygen Separation from Air33Influence of nitrogen flow during sintering of bismuth manganite ceramics on grain morphology and surface disorder13Electric relaxation and Mn3+/Mn4+ charge transfer in Fe-doped Bi12MnO20–BiMn2O5 structural self-composite32Nonlinear photovoltaic effect in Sillenite photorefractive crystals10Synthesis of carbon nanotube ( CNT )‐BiFeO 3 and ( CNT )‐Bi 2 Fe 4 O 9 nanocomposites and its enhanced photocatalytic properties18Influence of Thickness on Structural and Magnetic Properties of Co-rich Bi10Co16O38 Sillenite Thin Films3An Operando Study of the Initial Discharge of Bi and Bi/Cu Modified MnO 231Synthesis and characterization of electrical features of bismuth manganite and bismuth ferrite: effects of doping in cationic and anionic sublattice: Materials for applications21Stabilization of the δ-Bi2O3-like structure down to room temperature by thermal nanocrystallization of bismuth oxide-based glasses25γ-Bi2O3 – To Be or Not To Be? Comparison of the Sillenite γ-Bi2O3 and Isomorphous Sillenite-Type Bi12SiO2044A comparative investigation of structural and optical properties of annealing modified mullite bismuth ferrite14Hierarchical manganese sillenite Bi12MnO20 microparticles assembled by nanocubes with microwave absorption enhancement10The effect of graphene oxide on structural, opto-electrical and thermal properties of manganese sillenite (Bi12MnO20) nano-powders6Bi25feo40 polycrystalline ceramic as highly efficient photocatalyst synthesised via economical chemical route14Bibliography0Structural and vibrational spectroscopic studies of new phases with sillenite type in the system Bi2O3- In2O3 –MgO2Effect of Composition on the Optical and Photocatalytic Properties of Visible Light Responsive Materials Bi26–xMgxO4012Thermal, magnetic and photoelectrical behaviors of sillenite Bi25FeO39 microcrystals13Controlled synthesis of photoactive gallium based sillenite single crystal and its application in environmental remediation6Optical, electrical, and catalytic (photo-and sono-) properties of indium doped γ-Bi2O3 with Sillenite structure7Facile and reproducible method of stabilizing $\hbox {Bi}_2\hbox {O}_3$ phases confined in nanocrystallites embedded in amorphous matrix16Caracterização de materiais fotorrefrativos0Comments on the paper on the double doped BiFeO3 crystal by Nitin Kumar et al., and published in J. Alloy. Compd. 688, (2016) 8581Comments on the paper on the multiferroic Bi(Cd0.5Ti0.5)O3-BiFeO3 solid solution written by N. Kumar et al. and published in J. Alloys Compd. 747, 895 (2018)3Discovery of a new type of sillenite structure. Comments on the papers by Nitin Kumar et al. On the BiFeO3 crystal co-doped by Co/Ti and Ni/Ti ions and published in Ceramics International 45, 822 (2019) and 47, 22147 (2021)1Comment on “Structural, electrical, and multiferroic characteristics of lead-free multiferroic: Bi(Co 0.5 Ti 0.5 )O 3 –BiFeO 3 solid solution” by N. Kumar, A. Shukla, N. Kumar, R. Choudhary and A. Kumar, RSC Adv. , 2018, 8 , 36939”2Coupled Experimental Study and Thermodynamic Optimization on Bi2o3–Zno System0Magnetic dipolar correlations in sillenite-structure bismuth ferrite: magnetic and Mössbauer effect studies4Bi25FeO40/Bi2O2CO3 piezoelectric catalyst with built-in electric fields that was prepared via photochemical self-etching of Bi25FeO40 for 4-chlorophenol degradation43Bismuth Sillenite Crystals as Recent Photocatalysts for Water Treatment and Energy Generation: A Critical Review54Comment on “Structural, dielectric, and magnetic characteristics of Bi(Ni0.25Ti0.25Fe0.50)O3 ceramics” [J. Mater. Sci.: Mater. Electron. 27, 1209 (2016)]; “Structural and electrical characteristics of (Co, Ti)-modified BiFeO3” [J. Mater. Sci.: Mater. Electron. 27, 7115 (2016)]; “Structural, electrical, and magnetic characteristics of Ni/Ti-modified BiFeO3 lead-free multiferroic material” [J. Mater. Sci.: Mater. Electron. 28, 6673 (2017)]2Structural, optical, dielectric, and magnetic properties of iron-sillenite Bi25FeO4054Thermodynamics properties of Bi 38 ZnO 58 and phase equilibria of Bi 2 O 3 –ZnO system6Indium containing sillenite semiconductor: Synthesis, structural, spectroscopic, and thermogravimetric analysis3Bismuth and Cobalt Multiphasic System: Synthesis and Application as Microstrip Patch Antenna Substrate4Effect of Conditions of Mannitol-Nitrate Synthesis on Photocatalytic Properties of φ-Bi8Pb5O170Effect of Conditions of Mannitol-Nitrate Synthesis on Photocatalytic Properties of φ-Bi8Pb5O171Electrocatalytic OER behavior of the Bi–Fe–O system: an understanding from the perspective of the presence of oxygen vacancies15Recent advances in designing and developing efficient sillenite-based materials for photocatalytic applications31Phase relations in the Bi 2 O 3 –Mn 2 O 3 –M 2 O 3 (MFe, Al, and Ga) pseudoternary systems1Zn Makes a Difference: Cubic ZnBi38O60 as a Durable and High-Rate Anode for Rechargeable Na-Ion Batteries6A high-performance magnetically separable and reusable BiFeO 3 /Bi 25 FeO 40 nano-photocatalyst for purifying water under visible light irradiation4Lone pair electron-induced attrition of lanthanide ions from a sillenite-structured bismuth gallate host2Mn-doped Bi 25 FeO 40 sillenite: Solid state reaction synthesis, structural, morphological, magnetic and optical properties2Stoichiometric Ternary Metal Oxide, ZnBi38O60 - Reduced Graphene Oxide Composite for Stable and High-Rate Li-Ion Storage1Electrochemical Hydrogen Storage of Nanoflake‐Shaped Composites of Bi 25 FeO 40 /Zn 0.56 Al 0.44 (OH) 2 (CO 3 ) 0.22 .xH 2 O: Synthesis, Design, and Structural Characterization0Tunable multifunctionality in aliovalent substituted Bi12MnO20 sillenite for thermistor and other fascinating applications0Towards a deeper insight into the stabilisation mechanism of δ-Bi2O3-like phase to low temperature by confinement of nanograins in glassy matrix2Tunable multifunctionality in aliovalent substituted Bi12MnO20 sillenite for thermistor and other fascinating applications0Tailoring sillenite Bi25FeO39 microcrystals into tetrahedral and cubic series and exploring their electrical performance after sintering0Phase relationships, crystal structures, and the electrical, dielectric, and optical properties in the Bi2O3-In2O3-SnO2 system0Tunable multifunctionality in aliovalent substituted Bi12MnO20 sillenite for thermistor and other fascinating applications0

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  1. Mechanochemical synthesis of γ-Bi2O3

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  2. Isomorphic A‐Site Substitution on Sillenite‐Type Compounds

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  3. Dielectric Characteristics of Bismuth Oxide Solid Solutions with a Fluorite‐Like Crystal Structure

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  4. Synthesis and characterisation of bismuth phosphate-based sillenites

    Solid State Ionics · 2004-10-28

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  5. Equilibrium phases in the Bi2O3-rich region of the ZnO–Bi2O3 system

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  6. A Tetrameric Neodymium Silanolate: [Nd(OSiMe3)3]4

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  7. Grain Boundary Defects Induced Switching in Zn- Bi- Mo Ceramic

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  8. From molecules to bismuth oxide-based materials: Potential homo- and heterometallic precursors and model compounds

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  9. Estudio termodinámico de la región rica en Bi2O3 del sistema Bi2O3-ZnO

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  10. Tunable Synthesis of Bismuth Ferrites with Various Morphologies

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  11. Photocatalytic activity of Bi24Ga2O39 for degrading methylene blue

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  12. Structures and Oxide Mobility in Bi−Ln−O Materials: Heritage of Bi2O3

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  13. Dopedγ-Bi2O3: synthesis of microcrystalline samples and crystal chemical analysis of structural data

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  14. Evidence of improvement in gas sensing properties of nanostructured bismuth cobaltite prepared by solution-polymerization method

    Sensors and Actuators B Chemical · 2007-02-21

    Carlos Rafael Michel, Emilio Delgado, Alma Hortensia Martínez-Preciado

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  15. Photocatalytic activity of a sillenite-type material Bi25GaO39

    Catalysis Communications · 2007-02-27

    Xinping Lin, Fuqiang Huang, Wendeng Wang, Yujuan Xia, Yaoming Wang, Minling Liu, Jianlin Shi

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  16. Tuning the Morphology of Bismuth Ferrite Nano‐ and Microcrystals: From Sheets to Fibers

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  17. Alkali Metal Ions‐Assisted Controllable Synthesis of Bismuth Ferrites by a Hydrothermal Method

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  18. Defects in Inorganic Photorefractive Materials and Their Investigations

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  19. Characterization of photorefractive undoped and doped sillenite crystals using holographic and photoconductivity techniques

    Journal of Optics A Pure and Applied Optics · 2008-08-27

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  20. Vanadium-doped photorefractive titanosillenite crystal

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  22. MOCVD of crystalline Bi2O3 thin films using a single-source bismuth alkoxide precursor and their use in photodegradation of water

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  23. Hydrothermal Synthesis of Bi12TiO20 Nanostrucutures Using Anodized TiO2 Nanotubes and Its Application in Photovoltaics

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  24. The effects of solvents on the formation of sol–gel-derived Bi12SiO20 thin films

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  25. Formation and photocatalytic properties of bismuth ferrite submicrocrystals with tunable morphologies

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  26. Microwave Hydrothermal Synthesis, Structural Characterization, and Visible‐Light Photocatalytic Activities of Single‐Crystalline Bismuth Ferric Nanocrystals

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  27. Carbon dioxide sensing properties of bismuth cobaltite

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  28. Synthesis and characterization of Bi2Fe4O9 powders

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  30. Structural, electronic, optical, and magneto-optical properties of Bi12MO20 (M = Ti, Ge, Si) sillenite crystals from first principles calculations

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  31. Hydrothermal growths, optical features and first-principles calculations of sillenite-type crystals comprising discrete MO 4 tetrahedra

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  33. Improved structural model of Pb-doped γ -Bi 2 O 3 : (Bi 23.68 Pb 0.32 )(Bi 1.28 Pb 0.72 )O 38.48

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  34. Humidity sensing properties of bismuth phosphates

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  36. Microstructure Engineering to Drastically Reduce the Leakage Currents of High Voltage ZnO Varistor Ceramics

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  37. Dielectric Properties of Sol–Gel‐Derived Bi 12 SiO 20 Thin Films

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  38. Raman spectroscopy evidence of inhomogeneous disorder in the bismuth-oxygen framework of Bi 25 InO 39 and other sillenites

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  39. Preparation, structural and linear optical properties of zinc sillenite (Bi12.66Zn0.33O19.33) nanocrystals

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  40. Relaxor-like Dielectric Behavior in Stoichiometric Sillenite Bi12SiO20

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  41. Controllable Synthesis of Different Bismuth Ferrites by a PVA Modified Hydrothermal Method and Photocatalytic Characterization

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  42. Morphology and optical absorption of Bi2Fe4O9 crystals via mineralizer-assisted hydrothermal synthesis

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  43. Controllable preparation of BiFeO3@carbon core/shell nanofibers with enhanced visible photocatalytic activity

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  44. Phase diagram of the pseudobinary system Bi–Co–O

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  45. Coexistence of several sillenite-like phases in pseudo-binary and pseudo-ternary systems based on Bi2O3

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  46. First-principles study of the BiMO4antisite defect in the Bi12MO20(M=Si, Ge, Ti) sillenite compounds

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  47. Dielectric and Magnetic Properties of NiFe2-xBixO4 Nanoparticles at Microwave Frequencies Prepared via co-precipitation Method

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  48. Room temperature synthesis of Bi 25 FeO 39 and hydrothermal kinetic relations between sillenite- and distorted perovskite-type bismuth ferrites

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  49. Surfactant-free solvothermal synthesis and optical characterization of Bi2Fe4O9 in mixed H2O/EtOH solvent

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  50. Electron diffraction study of the sillenites Bi12SiO20, Bi25FeO39 and Bi25InO39: Evidence of short-range ordering of oxygen-vacancies in the trivalent sillenites

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