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RESEARCH PAPER · Dalton Transactions · 2011

The role of Zn–OR and Zn–OH nucleophiles and the influence of para-substituents in the reactions of binuclear phosphatase mimetics

Lena Josefine Daumann, Kristian E. Dalle, Gerhard Schenk, Ross P. McGeary, Paul V. Bernhardt, David L. Ollis, Lawrence R. Gahan

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The role of Zn–OR and Zn–OH nucleophiles and the influence of para-substituents in the reactions of binuclear phosphatase mimeticsOriginalEffect of intrathecal morphine on blood glucose, glucagon and tissue glycogen in rat: comparison with the effect of xanthan gum on blood glucose.9Ligand modifications modulate the mechanism of binuclear phosphatase biomimetics13Cadmium(II) Complexes: Mimics of Organophosphate Pesticide Degrading Enzymes and Metallo-β-lactamases25Spectroscopic Characterization of the Active FeIIIFeIII and FeIIIFeII Forms of a Purple Acid Phosphatase Model System48Asymmetric zinc(ii) complexes as functional and structural models for phosphoesterases21Synthesis, structure and spectral properties of O,N,N coordinating ligands and their neutral Zn(ii) complexes: a combined experimental and theoretical study30Synthesis, Magnetic Properties, and Phosphoesterase Activity of Dinuclear Cobalt(II) Complexes66Dinuclear Cobalt(II) Complexes as Metallo‐β‐lactamase Mimics11A Bis(μ‐phenoxo)‐Bridged Dizinc Complex with Hydrolytic Activity8Spectroscopic and mechanistic studies of dinuclear metallohydrolases and their biomimetic complexes78Mechanistic Studies of Cd(II) Complexes as Phosphoesterase and Metallo-β-lactamase Models0Catalytic hydrolysis of phosphodiesters by nucleophilic ions in gemini micellar media18Dinuclear Zinc(II) Complexes with Hydrogen Bond Donors as Structural and Functional Phosphatase Models86Selective H2PO4− anion sensing by two neutral Zn2+ complexes and combined theoretical and experimental studies of their structural and spectral properties17N, N coordinating schiff base ligand acting as a fluorescence sensor for zinc(II) and colorimetric sensor for copper(II), and zinc(II) in mixed aqueous media40Comparative DNA Binding Abilities and Phosphatase-Like Activities of Mono-, Di-, and Trinuclear Ni(II) Complexes: The Influence of Ligand Denticity, Metal–Metal Distance, and Coordinating Solvent/Anion on Kinetics Studies46Molecular Recognition and Scavenging of Arsenate from Aqueous Solution Using Dimetallic Receptors22A Highly Selective Two‐Photon Fluorescent Probe for Detection of Cadmium(II) Based on Intramolecular Electron Transfer and its Imaging in Living Cells43Synthesis, structure, magnetic properties and EPR spectroscopy of a copper( ii ) coordination polymer with a ditopic hydrazone ligand and acetate bridges55Photophysical property vs. medium: mononuclear, dinuclear and trinuclear Zn( ii ) complexes19Experimental and theoretical studies of hydrolysis of nerve agent sarin by binuclear zinc biomimetic catalysts9A Heterodinuclear FeIIIZnII Complex as a Mimic for Purple Acid Phosphatase with Site‐Specific ZnII Binding13A steroid-salen conjugate for zinc ion recognition and its applications in test-strips, living cells imaging, and cascade recognition for dihydrogen phosphate17An Approach to More Accurate Model Systems for Purple Acid Phosphatases (PAPs)41Cyclononanes: The extensive chemistry of fundamentally simple ligands16Bioinspired Activation of Oxygen with Pyrazole-Supported Dinuclear Copper Complexes3Comparative structure activity relationship for heterogeneous phosphatase-like catalytic activities of one-dimensional Cu( ii ) coordination polymers8Metallohydrolase biomimetics with catalytic and structural flexibility18Role of para-substitution in controlling phosphatase activity of dinuclear Ni II complexes of Mannich-base ligands: experimental and DFT studies9Investigation of the identity of the nucleophile initiating the hydrolysis of phosphate esters catalyzed by dinuclear mimics of metallohydrolases8Enhanced activity of trinuclear Zn( ii ) complexes towards phosphate ester bond cleavage by introducing three-metal cooperativity14Synthesis, Characterization and in vitro Cytotoxicity Studies of Pentadentate Ligand and its Copper(II) Complexes1Metal‐coordinated Hydroxide as a Nucleophile: a Brief History13Synthesis and characterization of phenoxo-bridged dinuclear zinc(II) halide complexes: Role of electron withdrawing group on phosphatase activity3Phosphatase-like Activity of Tetranuclear Iron(III) and Zinc(II) Complexes54Novel thiophene-based colorimetric and fluorescent turn-on sensor for highly sensitive and selective simultaneous detection of Al3+ and Zn2+ in water and food samples and its application in bioimaging109Dinuclear copper(II) complexes of “end-off” bicompartmental ligands: Alteration of the chelating arms on ligands to regulate the reactivity of the complexes towards DNA9Mechanistic Studies of Homo- and Heterodinuclear Zinc Phosphoesterase Mimics: What Has Been Learned?26A new coumarin-based fluorescence “turn-on” sensor for Al(III) ions and its bioimaging in cell19Zinc(II) complexes of a versatile heptadentate ligand as phosphohydrolase structural and functional mimics4Bimetallic Bis-anion Cascade Complexes of Magnesium in Nonaqueous Solution1Carbohydrate-Based Micro/Nanocapsules With Controlled External Surface for Medical Applications5Dual-Selective Catalysis in Dephosphorylation Tuned by Hf6‑Containing Metal–Organic Frameworks Mimicking Phosphatase47Synthesis, photophysical properties and theoretical studies of pyrrole-based azoaromatic Zn(II) complexes in mixed aqueous medium4Mono- and dinuclear zinc complexes bearing identical bis(thiosemicarbazone) ligand that exhibit alkaline phosphatase-like catalytic reactivity3A novel AIE-active camphor-based fluorescent probe for simultaneous detection of Al 3+ and Zn 2+ at dual channels in living cells and zebrafish18An ultrasensitive 4-(Diethylamino) salicylaldehyd-based fluorescence enhancement probe for the detection of Al3+ in aqueous solutions and its application in cells27Elucidating the Roles of Distinct Chemical Factors in the Hydrolytic Activities of Hetero- and Homonuclear Synthetic Analogues of Binuclear Metalloenzymes12A smart chemosensor with different response mechanisms to multi-analytes: Chromogenic and fluorogenic recognition of Cu2+, Fe3+, and Zn2+29Comparative DNA binding ability and phosphatase-like activity of mono and dinuclear Ni (II) complexes: a structure-activity correlation7Synthesis, characterization, and structures of mononuclear and phenoxo-/acetato-bridged trinuclear zinc(II) complexes from salan ligands: Study of their hydrolytic activity7A “turn-on” fluorescent probe based on coumarin imine for highly selective detection of Al3+ and Zn2+ in water samples and bioimaging of zebrafish10Protein degradation by a dinuclear zinc(II) complex featuring a symmetric phenol-based ligand with thioether moieties1

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  1. Effect of intrathecal morphine on blood glucose, glucagon and tissue glycogen in rat: comparison with the effect of xanthan gum on blood glucose.

    PubMed · 1996-12-05

    Ezzat S. El Daly

    Read original paper ↗ ·

  2. Ligand modifications modulate the mechanism of binuclear phosphatase biomimetics

    Polyhedron · 2012-06-15

    Kristian E. Dalle, Lena Josefine Daumann, Gerhard Schenk, Ross P. McGeary, Lyall R. Hanton, Lawrence R. Gahan

    Read original paper ↗ ·

  3. Cadmium(II) Complexes: Mimics of Organophosphate Pesticide Degrading Enzymes and Metallo-β-lactamases

    Inorganic Chemistry · 2012-07-03

    Lena Josefine Daumann, Lawrence R. Gahan, Peter Comba, Gerhard Schenk

    Read original paper ↗ ·

  4. Spectroscopic Characterization of the Active FeIIIFeIII and FeIIIFeII Forms of a Purple Acid Phosphatase Model System

    Inorganic Chemistry · 2012-10-30

    Peter Comba, Lawrence R. Gahan, Valeriu Mereacre, Graeme R. Hanson, Annie K. Powell, Gerhard Schenk, M. Zajaczkowski-Fischer

    Read original paper ↗ ·

  5. Asymmetric zinc(ii) complexes as functional and structural models for phosphoesterases

    Dalton Transactions · 2013-01-01

    Lena Josefine Daumann, Laurène Marty, Gerhard Schenk, Lawrence R. Gahan

    Read original paper ↗ ·

  6. Synthesis, structure and spectral properties of O,N,N coordinating ligands and their neutral Zn(ii) complexes: a combined experimental and theoretical study

    Dalton Transactions · 2013-01-01

    Amar Hens, Pallab Mondal, Kajal Krishna Rajak

    Read original paper ↗ ·

  7. Synthesis, Magnetic Properties, and Phosphoesterase Activity of Dinuclear Cobalt(II) Complexes

    Inorganic Chemistry · 2013-02-01

    Lena Josefine Daumann, Peter Comba, James A. Larrabee, Gerhard Schenk, Robert Stranger, Germán Cavigliasso, Lawrence R. Gahan

    Read original paper ↗ ·

  8. Dinuclear Cobalt(II) Complexes as Metallo‐β‐lactamase Mimics

    European Journal of Inorganic Chemistry · 2013-04-30

    Lena Josefine Daumann, James A. Larrabee, Peter Comba, Gerhard Schenk, Lawrence R. Gahan

    Read original paper ↗ ·

  9. A Bis(μ‐phenoxo)‐Bridged Dizinc Complex with Hydrolytic Activity

    Zeitschrift für anorganische und allgemeine Chemie · 2013-06-19

    Mainak Mitra, Reena Singh, Monika Pyrkosz‐Bulska, Matti Haukka, Elżbieta Gumienna‐Kontecka, Ebbe Nordlander

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  10. Spectroscopic and mechanistic studies of dinuclear metallohydrolases and their biomimetic complexes

    Dalton Transactions · 2013-10-18

    Lena Josefine Daumann, Gerhard Schenk, David L. Ollis, Lawrence R. Gahan

    Read original paper ↗ ·

  11. Mechanistic Studies of Cd(II) Complexes as Phosphoesterase and Metallo-β-lactamase Models

    Springer theses · 2014-01-01

    Lena Josefine Daumann

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  12. Catalytic hydrolysis of phosphodiesters by nucleophilic ions in gemini micellar media

    Journal of Physical Organic Chemistry · 2014-05-21

    Birendra Kumar, Deepti Tikariha, Manmohan Lal Satnami, Nadia Barbero, Pierluigi Quagliotto, Kallol Kumar Ghosh

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  13. Dinuclear Zinc(II) Complexes with Hydrogen Bond Donors as Structural and Functional Phosphatase Models

    Inorganic Chemistry · 2014-08-14

    Simone Bosch, Peter Comba, Lawrence R. Gahan, Gerhard Schenk

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  14. Selective H2PO4− anion sensing by two neutral Zn2+ complexes and combined theoretical and experimental studies of their structural and spectral properties

    Polyhedron · 2014-08-15

    Amar Hens, Pallab Mondal, Kajal Krishna Rajak

    Read original paper ↗ ·

  15. N, N coordinating schiff base ligand acting as a fluorescence sensor for zinc(II) and colorimetric sensor for copper(II), and zinc(II) in mixed aqueous media

    Inorganica Chimica Acta · 2014-09-02

    Amar Hens, Amit Ranjan Maity, Kajal Krishna Rajak

    Read original paper ↗ ·

  16. Comparative DNA Binding Abilities and Phosphatase-Like Activities of Mono-, Di-, and Trinuclear Ni(II) Complexes: The Influence of Ligand Denticity, Metal–Metal Distance, and Coordinating Solvent/Anion on Kinetics Studies

    Inorganic Chemistry · 2014-09-16

    Vimal Kumar Bhardwaj, Ajnesh Singh

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  17. Molecular Recognition and Scavenging of Arsenate from Aqueous Solution Using Dimetallic Receptors

    Chemistry - A European Journal · 2014-10-22

    Chris D. Moffat, Dominik Jakob Weiss, Arun Shivalingam, Andrew J. P. White, Pascal Salaün, Ramón Vilar

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  18. A Highly Selective Two‐Photon Fluorescent Probe for Detection of Cadmium(II) Based on Intramolecular Electron Transfer and its Imaging in Living Cells

    Chemistry - A European Journal · 2014-10-24

    Zhaohua Shi, Qingxin Han, Lizi Yang, Huan Yang, Xiaoliang Tang, Wei Dou, Zhiqi Li, Yange Zhang, Yongliang Shao, Liping Guan, Weisheng Liu

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  19. Synthesis, structure, magnetic properties and EPR spectroscopy of a copper( ii ) coordination polymer with a ditopic hydrazone ligand and acetate bridges

    Dalton Transactions · 2014-11-24

    Rahman Bikas, P. Aleshkevych, Hassan Hosseini‐Monfared, Joaquín Sanchiz, R. Szymczak, Tadeusz Lis

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  20. Photophysical property vs. medium: mononuclear, dinuclear and trinuclear Zn( ii ) complexes

    RSC Advances · 2014-11-28

    Amar Hens, Kajal Krishna Rajak

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  21. Experimental and theoretical studies of hydrolysis of nerve agent sarin by binuclear zinc biomimetic catalysts

    Chemical Physics · 2015-06-01

    Nan Guo, Jinyi Zhong, Shi‐Lu Chen, Jingquan Liu, Min Qi, Ruixue Shi

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  22. A Heterodinuclear FeIIIZnII Complex as a Mimic for Purple Acid Phosphatase with Site‐Specific ZnII Binding

    European Journal of Inorganic Chemistry · 2015-06-09

    Asha E. Roberts, Gerhard Schenk, Lawrence R. Gahan

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  23. A steroid-salen conjugate for zinc ion recognition and its applications in test-strips, living cells imaging, and cascade recognition for dihydrogen phosphate

    Sensors and Actuators B Chemical · 2015-07-04

    Jindan Wu, Xia Zhao, Yuxia Gao, Jun Hu, Yong Ju

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  24. An Approach to More Accurate Model Systems for Purple Acid Phosphatases (PAPs)

    Inorganic Chemistry · 2015-07-21

    Paul V. Bernhardt, Simone Bosch, Peter Comba, Lawrence R. Gahan, Graeme R. Hanson, Valeriu Mereacre, Christopher J. Noble, Annie K. Powell, Gerhard Schenk, Hubert Wadepohl

    Read original paper ↗ ·

  25. Cyclononanes: The extensive chemistry of fundamentally simple ligands

    Coordination Chemistry Reviews · 2015-12-29

    Lawrence R. Gahan

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  26. Bioinspired Activation of Oxygen with Pyrazole-Supported Dinuclear Copper Complexes

    Unknown journal · 2016-01-01

    Kristian E. Dalle

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  27. Comparative structure activity relationship for heterogeneous phosphatase-like catalytic activities of one-dimensional Cu( ii ) coordination polymers

    RSC Advances · 2016-01-01

    Navid Hussain, Pooja K. Joshi, Shah Raj Ali, Vimal Kumar Bhardwaj

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  28. Metallohydrolase biomimetics with catalytic and structural flexibility

    Dalton Transactions · 2016-01-01

    Luísa L. Mendes, Daniel Englert, Christiane Fernandes, Lawrence R. Gahan, Gerhard Schenk, Adolfo Horn

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  29. Role of para-substitution in controlling phosphatase activity of dinuclear Ni II complexes of Mannich-base ligands: experimental and DFT studies

    RSC Advances · 2016-01-01

    Ria Sanyal, Xuepeng Zhang, Prateeti Chakraborty, Franz Andreas Mautner, Cunyuan Zhao, Debasis Das

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  30. Investigation of the identity of the nucleophile initiating the hydrolysis of phosphate esters catalyzed by dinuclear mimics of metallohydrolases

    Journal of Inorganic Biochemistry · 2016-02-15

    Joshua J. Brown, Lawrence R. Gahan, Anne Schöffler, Elizabeth H. Krenske, Gerhard Schenk

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  31. Enhanced activity of trinuclear Zn( ii ) complexes towards phosphate ester bond cleavage by introducing three-metal cooperativity

    New Journal of Chemistry · 2017-12-27

    Pooja K. Joshi, Navid Hussain, Shah Raj Ali, Rishu Rishu, Vimal Kumar Bhardwaj

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  32. Synthesis, Characterization and in vitro Cytotoxicity Studies of Pentadentate Ligand and its Copper(II) Complexes

    Asian Journal of Chemistry · 2017-12-31

    Umapathy Chokkanathan, Kannappan Geetha

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  33. Metal‐coordinated Hydroxide as a Nucleophile: a Brief History

    Zeitschrift für anorganische und allgemeine Chemie · 2018-04-11

    Allan G. Blackman, Lawrence R. Gahan

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  34. Synthesis and characterization of phenoxo-bridged dinuclear zinc(II) halide complexes: Role of electron withdrawing group on phosphatase activity

    Journal of Chemical Sciences · 2018-07-27

    Monika Sheoran, Kishalay Bhar, Tanveer A. Khan, Anuj K. Sharma

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  35. Phosphatase-like Activity of Tetranuclear Iron(III) and Zinc(II) Complexes

    Inorganic Chemistry · 2018-08-21

    Nityananda Dutta, Shobhraj Haldar, Gonela Vijaykumar, Suvendu Paul, Asoke Prasun Chattopadhyay, Luca M. Carrella, Manindranath Bera

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  36. Novel thiophene-based colorimetric and fluorescent turn-on sensor for highly sensitive and selective simultaneous detection of Al3+ and Zn2+ in water and food samples and its application in bioimaging

    Analytica Chimica Acta · 2018-10-23

    Yang Li, Qingfen Niu, Tao Wei, Tianduo Li

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  37. Dinuclear copper(II) complexes of “end-off” bicompartmental ligands: Alteration of the chelating arms on ligands to regulate the reactivity of the complexes towards DNA

    Journal of Inorganic Biochemistry · 2018-12-29

    Shuhong Cao, Run Cheng, Dandan Wang, Yunfeng Zhao, Ruiren Tang, Xiu‐Li Yang, Jingwen Chen

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  38. Mechanistic Studies of Homo- and Heterodinuclear Zinc Phosphoesterase Mimics: What Has Been Learned?

    Frontiers in Chemistry · 2019-02-21

    Andrea Erxleben

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  39. A new coumarin-based fluorescence “turn-on” sensor for Al(III) ions and its bioimaging in cell

    Journal of Molecular Structure · 2019-07-11

    Lei Jin, Wenling Wang, Zheyu Shen, Jiahao Xu, Qingming Wang, Chengying Zhao

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  40. Zinc(II) complexes of a versatile heptadentate ligand as phosphohydrolase structural and functional mimics

    Inorganica Chimica Acta · 2019-08-19

    Steven H. Batha, Hadi D. Arman, Oleg V. Larionov, Ghezai T. Musie

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  41. Bimetallic Bis-anion Cascade Complexes of Magnesium in Nonaqueous Solution

    Inorganic Chemistry · 2020-04-17

    David Van Craen, Ian G. Flynn, Veronica Carta, Amar H. Flood

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  42. Carbohydrate-Based Micro/Nanocapsules With Controlled External Surface for Medical Applications

    Frontiers in Chemistry · 2020-06-26

    Roman Bielski, Zbigniew Janusz Witczak, John F. L. Newport

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  43. Dual-Selective Catalysis in Dephosphorylation Tuned by Hf6‑Containing Metal–Organic Frameworks Mimicking Phosphatase

    ACS Central Science · 2021-05-07

    Jie Dong, Hongde An, Ze-Kun Yue, Sheng‐Li Hou, Yao Chen, Zhenjie Zhang, Peng Cheng, Qian Peng, Bin Zhao

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  44. Synthesis, photophysical properties and theoretical studies of pyrrole-based azoaromatic Zn(II) complexes in mixed aqueous medium

    Inorganica Chimica Acta · 2021-08-22

    Tapas Ghorui, Amar Hens, Kausikisankar Pramanik

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  45. Mono- and dinuclear zinc complexes bearing identical bis(thiosemicarbazone) ligand that exhibit alkaline phosphatase-like catalytic reactivity

    JBIC Journal of Biological Inorganic Chemistry · 2021-10-29

    Hyeri Jeon, Hugo Vázquez‐Lima, Haewon Jeong, Kyung‐Bin Cho, Seungwoo Hong

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  46. A novel AIE-active camphor-based fluorescent probe for simultaneous detection of Al 3+ and Zn 2+ at dual channels in living cells and zebrafish

    The Analyst · 2021-11-11

    Shuai Gong, Yan Zhang, Ahui Qin, Mingxin Li, Yu Gao, Chenglong Zhang, Jie Song, Xu Xu, Zhonglong Wang, Shifa Wang

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  47. An ultrasensitive 4-(Diethylamino) salicylaldehyd-based fluorescence enhancement probe for the detection of Al3+ in aqueous solutions and its application in cells

    Journal of Photochemistry and Photobiology A Chemistry · 2022-02-09

    Xiaolan Lei, YingYi Zou, QingJian Liang, Weishao Xu, Shanshan Lao, Bin Yang, Ligui Li, Liting Yang, Liu Hong, Lijun Ma

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  48. Elucidating the Roles of Distinct Chemical Factors in the Hydrolytic Activities of Hetero- and Homonuclear Synthetic Analogues of Binuclear Metalloenzymes

    ACS Catalysis · 2023-02-16

    Vindi M. Jayasinghe‐Arachchige, Leonardo Farias Serafim, Qiaoyu Hu, Cihan Özen, Sreerag N. Moorkkannur, Gerhard Schenk, Rajeev S. Prabhakar

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  49. A smart chemosensor with different response mechanisms to multi-analytes: Chromogenic and fluorogenic recognition of Cu2+, Fe3+, and Zn2+

    Dyes and Pigments · 2023-02-21

    Da Li, Ailan Liu, Ailan Liu, Yifan Xing, Zhijun Li, Zhijun Li, Yang Luo, Shijie Zhao, Linlin Dong, Tianyou Xie, Kunpeng Guo, Jie Li

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  50. Comparative DNA binding ability and phosphatase-like activity of mono and dinuclear Ni (II) complexes: a structure-activity correlation

    Journal of Chemical Sciences · 2024-02-12

    Vaishali Yadav, Rohitash Kumar, Rishu Rishu, Vimal Kumar Bhardwaj

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