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RESEARCH PAPER · Journal of the American Chemical Society · 2009

Larger Spontaneous Polarization Ferroelectric Inorganic−Organic Hybrids: [PbI3]∞ Chains Directed Organic Cations Aggregation to Kagomé-Shaped Tubular Architecture

Hai-Rong Zhao, Dong-Ping Li, Xiao‐Ming Ren, You Song, Wanqin Jin

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Larger Spontaneous Polarization Ferroelectric Inorganic−Organic Hybrids: [PbI3]∞ Chains Directed Organic Cations Aggregation to Kagomé-Shaped Tubular ArchitectureOriginalA series of transition metal–azido extended complexes with various anionic and neutral co-ligands: synthesis, structure and their distinct magnetic behavior42A spontaneously resoluted zinc–organic framework with nonlinear optical and ferroelectric properties generated from tetrazolate-ethyl ester ligand33Ligand-Directed and pH-Controlled Assembly of Chiral 3d−3d Heterometallic Metal−Organic Frameworks138Iodine‐Induced Solvothermal Formation of Viologen Iodobismuthates70Ionothermal synthesis of a new (4,12)-connected heterometallic iodoplumbate with [Pb 4 (OH) 4 ] cubane as joint points of the helices28Anion- and auxiliary ligand-directed synthesis of cadmium( ii ) complexes with 3,5-di(1H-imidazol-1-yl)benzoate44Cyano-Bridged Homochiral Heterometallic Helical Complexes: Synthesis, Structures, Magnetic and Dielectric Properties38Inorganic–organic hybrid compounds based on face-sharing octahedral [PbI3]∞ chains: self-assemblies, crystal structures, and ferroelectric, photoluminescence properties41Nonlinear optical and ferroelectric materials based on 1-benzyl-2-phenyl-1H-benzimidazole salts8Toward design of multiple-property inorganic–organic hybrid compounds based on face-sharing octahedral iodoplumbate chains50Discovery of Ferroelectric Properties in Diammonium Hypodiphosphate (NH4)2H2P2O6 (ADhP)35Six New Metal−Organic Frameworks Based on Polycarboxylate Acids and V-shaped Imidazole-Based Synthon: Syntheses, Crystal Structures, and Properties90Multifunctional Polythreading Coordination Polymers: Spontaneous Resolution, Nonlinear‐Optic, and Ferroelectric Properties46Linear and Nonlinear Optical Properties of Ferroelectric Thin Films11Synthesis, Crystal Structures, and Spectral Properties of Three Complexes with a Tetrazole‐based Ligand6Homochiral ferroelectric three-dimensional cadmium(II) frameworks from racemic camphoric acid and 3,5-di(imidazol-1-yl)benzoic acid16catena-Poly[1-[(2-fluorobenzylidene)amino]quinolinium [plumbate(II)-tri-μ-iodido]]0Construction of coordination frameworks based on 4-imidazolyl tecton 1,4-di(1H-imidazol-4-yl)benzene and varied carboxylic acids74Countercation-directed chiral resolution of [Mo2O4(H2dtpa)]−, syntheses, crystal structures and CD spectra of (λ)-[NEt4][Mo2O4(H2dtpa)] and (δ)-Na[Mo2O4(H2dtpa)]6Multifunctional amino-decorated metal–organic frameworks: nonlinear-optic, ferroelectric, fluorescence sensing and photocatalytic properties149N-donor ligand mediated assembly of divalent zinc and cadmium coordination polymers based on 2,3,2′,3′-thiaphthalic acid: structures and properties26New homochiral ferroelectric supramolecular networks of complexes constructed by chiral S-naproxen ligand28Role of cooperative templates in the self-assembly process of microporous structures: syntheses and characterization of 12 new silver halide/thiocyanate supramolecular polymers67Two mono- and dinuclear Eu(iii) enantiomeric pairs based on chiral bis-bidentate bridging ligands: synthesis, structures, luminescent and ferroelectric properties37Syntheses, Structures Tuned by 4,4′-Bipyridine and Magnetic Properties of a Series of Transition Metal Compounds Containing o-Carboxylphenoxyacetate Acid40Structural Diversity in Coordination Self-Assembled Networks of a Multimodal Ligand Azacalix[4]pyrazine35Three iodometalate organic-inorganic hybrid materials based on methylene blue cation: Syntheses, structures, properties and DFT calculations28Haloplumbate hybrids with organically coordinated halometal complexes as templates and mixed halo atoms: Solvothermal syntheses, crystal structures, and optical properties27One-step synthesis of PANI/Mn3O4 nanocomposites and evaluation of their electrochemical properties7A green luminescent 1-D helical tubular dipyrazol-bridged cadmium(ii) complex: a coordination tube included in a supramolecular tube31A highly oriented hybrid microarray modified electrode fabricated by a template-free method for ultrasensitive electrochemical DNA recognition36A novel polymeric metal halide extended network lead(II)-bromido complex, [(2-amino-5-methylpyridinium) (PbBr 3 )] n2Cadmium(ii) and zinc(ii) complexes with rigid 1-(1H-imidazol-4-yl)-3-(4H-tetrazol-5-yl)benzene and varied carboxylate ligands39Reversible supra-channel effects: 3D kagome structure and catalysis via a molecular array of 1D coordination polymers20Solvothermal syntheses and crystal structures of one 1D and two 3D [PbxIy]-based coordination polymers19Inorganic–organic hybrid compound with face-sharing iodoplumbate chains showing novel dielectric relaxation13Ferroelectric Switchable Behavior through Fast Reversible De/adsorption of Water Spirals in a Chiral 3D Metal–Organic Framework133Semiconducting Tin and Lead Iodide Perovskites with Organic Cations: Phase Transitions, High Mobilities, and Near-Infrared Photoluminescent Properties5416Chiral and Noncentrosymmetric Metal–Organic Frameworks Featuring a 2D → 3D Parallel/Parallel Inclined Subpolycatenation27Three-Dimensional Hydrogen Bonding Framework in the Crystal Structure of a Zinc(II) Complex of Imidazole Multicarboxylic Acid1Two pairs of isomorphism and two 3D metal–organic frameworks based on a star-like ligand tri(4-pyridylphenyl)amine27A novel 3D 10-fold interpenetrated homochiral coordination polymer: large spontaneous polarization, dielectric loss and emission studies21Anion concentration control in the self-assembly of symmetrical α,α′,δ,δ′-tetramethyl-cucurbit[6]uril-based tubular architectures19Crystal structure and dielectric property of the first bromide/iodide heteroleptic haloplumbate-based lamellate inorganic–organic hybrid compound6Inorganic–organic hybrid with one-dimensional face-sharing iodoplumbate chain showing novel dielectric anomaly and semiconductor emission29A super water-stable europium–organic framework: guests inducing low-humidity proton conduction and sensing of metal ions191A Multifunctional 3D Chiral Porous Ferroelectric Metal–Organic Framework for Sensing Small Organic Molecules and Dye Uptake31Novel Barium–Organic Incorporated Iodometalates: Do They Have Template Properties for Constructing Rare Heterotrimetallic Hybrids?67Bulk crystal growth of hybrid perovskite material CH 3 NH 3 PbI 3590A comparison study of aliphatic and aromatic structure directing agents influencing the crystal and electronic structures, and properties of iodoplumbate hybrids: water induced structure conversion and visible light photocatalytic properties64A panchromatic hybrid crystal of iodoplumbate nanowires and J-aggregated naphthalene diimides with long-lived charge-separated states89Hierarchical symmetry transfer and flexible charge matching in five [M(phen) 3 ] 2+ directed iodoargentates with 1 to 3D frameworks57POMANI-Mn3O4 based thin film NTC thermistor and its linearization for overheating protection sensor7Symmetrically Related Construction and Optical Properties of Two Noncentrosymmetric 3D Iodides of d10 Cation (Cu+, Ag+) Based on the N-Benzylpyridinium and Its Supramolecular Interactions73Low-Dimensional Hybrid Cuprous Halides Directed by Transition Metal Complex: Syntheses, Crystal Structures, and Photocatalytic Properties77Diversity of Coordination Modes, Structures, and Properties of Chiral Metal–Organic Coordination Complexes of the Drug Voriconazole14Spontaneous chiral resolution and hierarchical directing effects of two-winged propeller-like SDAs on the construction of noncentrosymmetric iodoargentates/iodocuprates15Structural diversity in substituted-pyridinium iodo- and bromoplumbates: a matter of halide and temperature35Three iodocuprate hybrids symmetrically modulated by positional isomers and the chiral conformation of N-benzyl-methylpyridinium36Transition metal complex directed lead bromides with tunable structures and visible light driven photocatalytic properties54Two in one: switchable ion conductivity and white light emission integrated in an iodoplumbate-based twin chain hybrid crystal31Self-assembled Structure of Inorganic–Organic Hybrid Crystals Based on Keggin Polyoxometallates [SMo12O402–] and Supramolecular Cations17[AgPb2I3(OH)2]: An unprecedented quaternary heterometallic semiconducting framework synthesized under ionothermal condition2Syntheses, structures, surface photovoltage and luminescent properties of a novel lead(II) coordination polymer containing anthracene chromophore3Finding and Evaluating of Adequate Adsorbents for the Adsorption of CO2from Humid Gas Streams4A pair of 3D enantiotopic zinc( ii ) complexes based on two asymmetric achiral ligands12Comparison studies of hybrid lead halide [MPb 2 X 7 ] 2− (M = Cu, Ag; X = Br, I) chains: band structures and visible light driven photocatalytic properties41Do alkyl groups on aromatic or aliphatic structure directing agents affect water stabilities and properties of hybrid iodoargentates?29Enhanced single-ion magnetic and ferroelectric properties of mononuclear Dy( iii ) enantiomeric pairs through the coordination role of chiral ligands66Polymorphism of a chiral iron( ii ) complex: spin-crossover and ferroelectric properties22Charge density studies of an inorganic-organic hybrid p-phenylenediammonium tetrachlorocuprate8A pair of mononuclear Dy( iii ) enantiomers showing single-ion magnetic and ferroelectric properties30Extra thermo- and water-stable one-dimensional organic–inorganic hybrid perovskite [ N -methyldabconium]PbI 3 showing switchable dielectric behaviour, conductivity and bright yellow-green emission58The structures, water stabilities and photoluminescence properties of two types of iodocuprate( i )-based hybrids35Unravelling the origin of piezo/ferro-electric properties of metal-organic frameworks (MOFs) nanocrystals0Synthesis, structures and applications as fluorescence probes of novel Hg(II)/Ag(I) functional supramolecular compounds based on nitrogen heterocyclic cations5Synthesis, structure and optical properties of novel double penetration polypseudorotaxane compound templated by branched divalent cation template0Design of the Hybrid Metal–Organic Frameworks as Potential Supramolecular Piezo-/Ferroelectrics84Dielectric Relaxation and Beyond Limiting Behavior of Alternating‐Current Conductivity in a Supermolecular Ferroelectric2Two‐Step Structure Phase Transition, Dielectric Anomalies, and Thermochromic Luminescence Behavior in a Direct Band Gap 2D Corrugated Layer Lead Chloride Hybrid of [(CH3)4 N ]4Pb3Cl1022Synthesis, Structure, and Ferroelectricity of a Kaolinite-p--Aminobenzamide Intercalation Compound7An inorganic-organic hybrid compound with face-sharing bromoplumbate chain: Synthesis, crystal structure, Hirshfeld surface analysis, ferroelectric and dielectric properties10A Rotorlike Supramolecular Assembly, {[K(18-crown-6)]PbI3}∞, with a Reversible Breaking-Symmetry Phase Transition near Room Temperature15Recent progress in molecular ferroelectrics with perovskite structure16Chiral-perovskite optoelectronics909Broadband Emission Enhancement Induced by Self-Trapped Excited States in One-Dimensional EAPbI3 Perovskite under Pressure25Characterization of Catalysts by Advanced Scanning Probe Microscopy and Spectroscopy11Interatomic exchange‐correlation interaction energy from a measure of quantum theory of atoms in molecules topological bonding: A diatomic case22Electron-deficient naphthalene diimide directed metal halides with visible light driven photocatalytic properties16Spin selectivity in chiral metal–halide semiconductors40Supramolecular [Na(15-crown-5)] + cations anchored to face-sharing octahedral lead bromide chains featuring a rotor-like one-dimensional perovskite with a reversible isostructural phase transition near room temperature7Chiral halide perovskite crystals for optoelectronic applications238Harvesting mechanical energy for hydrogen generation by piezoelectric metal–organic frameworks95The first salicylaldehyde Schiff base organic–inorganic hybrid lead iodide perovskite ferroelectric14Advances in single crystals and thin films of chiral hybrid metal halides38Induced Chirality in Halide Perovskite Clusters through Surface Chemistry36Hybrid Organic Lead Iodides: Role of Organic Cation Structure in Obtaining 1D Chains of Face-Sharing Octahedra vs 2D Perovskites29Rationalizing the design and implementation of chiral hybrid perovskites129Regulating the crystal and electronic structures and optical properties of hybrid bromoplumbates with alkylated N, S- or P-containing aromatic cations2Dielectric relaxation and C-F…π (benzene ring) halo-bond interactions in a lead halide hybrid crystal with bromine/iodine heterogeneous double-chain layer2Toward Understanding the Composition–Structure Relationship of Hybrid Organic Lead Iodide Compounds: Impact from Secondary Structures of Organic Cations4Structurally Dimensional Engineering in Perovskite Photovoltaics103Molecular ferroelectrics and magnetoelectrics based on charge–transfer2Oxygen‐Induced Lattice Strain for High‐Performance Organic Transistors with Enhanced Stability21Efficient Self‐Sorting Behaviours of Metallacages with Subtle Structural Differences2Efficient Self‐Sorting Behaviours of Metallacages with Subtle Structural Differences13CPL-active hybrid copper(I) halides enabled by cation inclusion with chiral crown-ether11Chiral Methylbenzylpyridinium-Based Organic–Inorganic Lead Halides for Water-Resistant Photoluminescence Materials8Activating the Chiroptical Properties of High-Fold Axial Chiral Perovskite by a Chiral Induction Strategy11Dual‐Color Tunable Circularly Polarized Luminescence With Anti‐Thermal‐Quenching Enabled by Asymmetric Hydrogen‐Bonding Networks in Hybrid Manganese Halides3

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  4. Iodine‐Induced Solvothermal Formation of Viologen Iodobismuthates

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  5. Ionothermal synthesis of a new (4,12)-connected heterometallic iodoplumbate with [Pb 4 (OH) 4 ] cubane as joint points of the helices

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  6. Anion- and auxiliary ligand-directed synthesis of cadmium( ii ) complexes with 3,5-di(1H-imidazol-1-yl)benzoate

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  7. Cyano-Bridged Homochiral Heterometallic Helical Complexes: Synthesis, Structures, Magnetic and Dielectric Properties

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  8. Inorganic–organic hybrid compounds based on face-sharing octahedral [PbI3]∞ chains: self-assemblies, crystal structures, and ferroelectric, photoluminescence properties

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  9. Nonlinear optical and ferroelectric materials based on 1-benzyl-2-phenyl-1H-benzimidazole salts

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  10. Toward design of multiple-property inorganic–organic hybrid compounds based on face-sharing octahedral iodoplumbate chains

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  11. Discovery of Ferroelectric Properties in Diammonium Hypodiphosphate (NH4)2H2P2O6 (ADhP)

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  12. Six New Metal−Organic Frameworks Based on Polycarboxylate Acids and V-shaped Imidazole-Based Synthon: Syntheses, Crystal Structures, and Properties

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  13. Multifunctional Polythreading Coordination Polymers: Spontaneous Resolution, Nonlinear‐Optic, and Ferroelectric Properties

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  14. Linear and Nonlinear Optical Properties of Ferroelectric Thin Films

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  15. Synthesis, Crystal Structures, and Spectral Properties of Three Complexes with a Tetrazole‐based Ligand

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  16. Homochiral ferroelectric three-dimensional cadmium(II) frameworks from racemic camphoric acid and 3,5-di(imidazol-1-yl)benzoic acid

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  17. catena-Poly[1-[(2-fluorobenzylidene)amino]quinolinium [plumbate(II)-tri-μ-iodido]]

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  18. Construction of coordination frameworks based on 4-imidazolyl tecton 1,4-di(1H-imidazol-4-yl)benzene and varied carboxylic acids

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  19. Countercation-directed chiral resolution of [Mo2O4(H2dtpa)]−, syntheses, crystal structures and CD spectra of (λ)-[NEt4][Mo2O4(H2dtpa)] and (δ)-Na[Mo2O4(H2dtpa)]

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  20. Multifunctional amino-decorated metal–organic frameworks: nonlinear-optic, ferroelectric, fluorescence sensing and photocatalytic properties

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  21. N-donor ligand mediated assembly of divalent zinc and cadmium coordination polymers based on 2,3,2′,3′-thiaphthalic acid: structures and properties

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  22. New homochiral ferroelectric supramolecular networks of complexes constructed by chiral S-naproxen ligand

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  24. Two mono- and dinuclear Eu(iii) enantiomeric pairs based on chiral bis-bidentate bridging ligands: synthesis, structures, luminescent and ferroelectric properties

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  26. Structural Diversity in Coordination Self-Assembled Networks of a Multimodal Ligand Azacalix[4]pyrazine

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  30. A green luminescent 1-D helical tubular dipyrazol-bridged cadmium(ii) complex: a coordination tube included in a supramolecular tube

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  31. A highly oriented hybrid microarray modified electrode fabricated by a template-free method for ultrasensitive electrochemical DNA recognition

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  32. A novel polymeric metal halide extended network lead(II)-bromido complex, [(2-amino-5-methylpyridinium) (PbBr 3 )] n

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  33. Cadmium(ii) and zinc(ii) complexes with rigid 1-(1H-imidazol-4-yl)-3-(4H-tetrazol-5-yl)benzene and varied carboxylate ligands

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  34. Reversible supra-channel effects: 3D kagome structure and catalysis via a molecular array of 1D coordination polymers

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  35. Solvothermal syntheses and crystal structures of one 1D and two 3D [PbxIy]-based coordination polymers

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  36. Inorganic–organic hybrid compound with face-sharing iodoplumbate chains showing novel dielectric relaxation

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  37. Ferroelectric Switchable Behavior through Fast Reversible De/adsorption of Water Spirals in a Chiral 3D Metal–Organic Framework

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  40. Three-Dimensional Hydrogen Bonding Framework in the Crystal Structure of a Zinc(II) Complex of Imidazole Multicarboxylic Acid

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  41. Two pairs of isomorphism and two 3D metal–organic frameworks based on a star-like ligand tri(4-pyridylphenyl)amine

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  42. A novel 3D 10-fold interpenetrated homochiral coordination polymer: large spontaneous polarization, dielectric loss and emission studies

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  43. Anion concentration control in the self-assembly of symmetrical α,α′,δ,δ′-tetramethyl-cucurbit[6]uril-based tubular architectures

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  44. Crystal structure and dielectric property of the first bromide/iodide heteroleptic haloplumbate-based lamellate inorganic–organic hybrid compound

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  45. Inorganic–organic hybrid with one-dimensional face-sharing iodoplumbate chain showing novel dielectric anomaly and semiconductor emission

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  46. A super water-stable europium–organic framework: guests inducing low-humidity proton conduction and sensing of metal ions

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  47. A Multifunctional 3D Chiral Porous Ferroelectric Metal–Organic Framework for Sensing Small Organic Molecules and Dye Uptake

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  48. Novel Barium–Organic Incorporated Iodometalates: Do They Have Template Properties for Constructing Rare Heterotrimetallic Hybrids?

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  49. Bulk crystal growth of hybrid perovskite material CH 3 NH 3 PbI 3

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  50. A comparison study of aliphatic and aromatic structure directing agents influencing the crystal and electronic structures, and properties of iodoplumbate hybrids: water induced structure conversion and visible light photocatalytic properties

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