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RESEARCH PAPER · Dalton Transactions · 2008

Construction of different dimensional inorganic–organic hybrid materials based on polyoxometalates and metal–organic units via changing metal ions: from non-covalent interactions to covalent connections

Ya‐Qian Lan, Shun‐Li Li, Kui‐Zhan Shao, Xinlong Wang, Zhong‐Min Su

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Construction of different dimensional inorganic–organic hybrid materials based on polyoxometalates and metal–organic units via changing metal ions: from non-covalent interactions to covalent connectionsOriginalMPFs (Metal–Peptide Frameworks)0Synthesis and crystal structure of pseudo-sandwich-type heteropolytungstates functionalized by organometallic ruthenium(ii)26Stabilization and immobilization of polyoxometalates in porous coordination polymers through host–guest interactions247Construction of a series of 0D, 2D and 3D inorganic–organic hybrid coordination polymers based on octamolybdate and 2-(2-pyridyl)imidazole and its derivative19Recent advances in crystal engineering746Synthesis, crystal structures and properties of novel zinc(II) and cadmium(II) polymeric and cyclic bimetallic complexes with fluconazole and dicarboxylate co-ligands10Cations in control: crystal engineering polyoxometalate clusters using cation directed self-assembly146MOFs, MILs and more: concepts, properties and applications for porous coordination networks (PCNs)1185Unprecedented three-dimensional 10-connected bct nets based on trinuclear secondary building units and their magnetic behavior30Two new organic–inorganic supramolecular hybrids templated by the Wells–Dawson polyoxometalates9A new 2D 5-connected coordination polymer based on 3,4-bis(pyridin-4-ylmethoxy)benzoic acid ligand4Highly Connected Three-Dimensional Metal−Organic Frameworks Based on Polynuclear Secondary Building Units74A series of inorganic–organic hybrid compounds constructed from bis(undecatungstophosphate) lanthanates and copper-organic units22Construction of one- to two-dimensional POM-based compounds through adjusting the metal cations and polyanions2Two new organic–inorganic hybrid compounds based on metal–pyrazine coordination polymers and Keggin polyoxometalates: effect of metal ions on thestructure31Self-assembly of supramolecular networks based on biphosphopentamolybdate and copper–organic units4Coordination polymers based on the octamolybdate and flexible bis(triazole) ligands with different spacer lengths56Towards the computational modelling of polyoxoanions on metal surfaces: IR spectrum characterisation of [SiW12O40]4− on Ag(111)20Assembly of a New Cadmium(II)‐bis(Triazole) Coordination Polymer Templated by Keggin Polyoxometalate5Polyoxometalates containing late transition and noble metal atoms217Solvothermal Assembly of a Series of Organic–Inorganic Hybrid Materials Constructed from Keggin Polyoxometalate Clusters and Copper(I)–Organic Frameworks58A 3D POM-based framework: Synthesis and structure of [Cu2(bbtz)4(SiW12O40)]1Anion Effects on the Formation of Silver(I) Complexes with the Flexible Ligand 4,4′‐Bis(1,2,4‐triazol‐1‐ylmethyl)biphenyl8Discrete Covalent Organic–Inorganic Hybrids: Terpyridine Functionalized Polyoxometalates Obtained by a Modular Strategy and Their Metal Complexation93The Cu(II)-fluconazole complex revisited. Part I: Structural characteristics of the system15Assembly of a New 3D Octamolybdate‐based Compound: Using the Flexible Bis(triazole) ligand with a –(CH2)6– Spacer4A Series of 3D Rare‐Earth‐Metal–Organic Frameworks with Isolated Guest Keggin Silicotungstate Fragments as Anion Templates19Keggin polyanion and copper cluster based coordination polymer towards model for complex nanosystem13Novel 1-D double-chain organic–inorganic hybrid polyoxotungstates constructed from dimeric copper–lanthanide heterometallic silicotungstate units38Novel building units in the construction of materials of the oxomolybdate–organodiphosphonate/copper(II)–dipodal-organonitrogen ligand system: Structural influences of dipodal ligand tether length and flexibility11Two three-dimensional pillared metal–olsalazine complexes based on infinite rod-shaped secondary building units9Syntheses Study of Keggin POM Supporting MOFs System56Hydrothermal synthesis and structural characterization of a new inorganic–organic hybrid compound with photocatalytic activity based on Keggin-type polyanion and cadmium-1, 2, 4-triazolate units27Inserting -(CH2)n- (n = 2, 3, 4) Spacers into the Reactant Mercapto-methyltetrazole Ligand for Tuning the Multinuclear AgI Clusters in Keggin-Based Compounds81A Series of Highly Connected Metal–Organic Frameworks Based on Triangular Ligands and d10 Metals: Syntheses, Structures, Photoluminescence, and Photocatalysis260A host–guest hybrid framework with Anderson anions as template: synthesis, crystal structure and photocatalytic properties32Assembly of Polyoxometalate-Based Metal–Organic Frameworks with Silver(I)-Schiff Base Coordination Polymeric Chains as Building Blocks54A series of novel 1D coordination polymers constructed from metal–quinolone complex fragments linked by aromatic dicarboxylate ligands10Series of Inorganic–Organic Hybrid Materials Constructed From Octamolybdates and Metal–Organic Frameworks: Syntheses, Structures, and Physical Properties101Assembly of Cu/Ag-quinoxaline-polyoxotungstate hybrids: Influence of Keggin and Wells–Dawson polyanions on the structure101, 2,4, 5‐Benzenetetracarboxylate and Bis(pyridyl)‐1, 2,4‐triazolate as Co‐ligands in Zinc(II) Complexes: Synthesis, Crystal Structure, and Luminescence Properties6Two sinusoidal wavelike 2D coordination polymers with benzophenone-4,4′-dicarboxylate5Assembly of co-bimb-polyoxotungstate hybrids: from 1D chain to 3D framework influenced by the charge of Keggin anions25Synthesis, Structure and Properties of a 2D Cadmium(II) Coordination Polymer Based on Fluconazole and Isophthalate Ligands2Tuning the dimension of POM-based inorganic–organic hybrids from 3D self-penetrating framework to 1D poly-pendant chain via changing POM clusters and introducing secondary spacers34Metal–organic segment-induced dimensionality evolution in polyoxometalate-based hybrids3Recent advances in porous polyoxometalate-based metal–organic framework materials969Crystal structures and spectral properties of two polyoxometalate-based inorganic–organic compounds from silver–azine building blocks with bis-bidentate and tridentate ligands8Coordination site induced controllable assembly of metal–organic units in polyoxometalate-based hybrids6Synthesis, Crystal Structure and Fluorescence Properties of Three 1-D Coordination Polymers Based on Fluconazole3Synthesis, crystal structure, and properties of cobalt, zinc, and manganese coordination polymers based on fluconazole3Two new hybrid compounds assembled from Keggin phosphotungstates, cobalt/zinc cations and V-shaped imidazole ligands11Synthesis, Crystal Structure, and Properties of Two Zinc Tubular Coordination Polymers Based on Fluconazole1Tuning the topology structures of polymolybdate-based hybrids from interpenetrated framework to interdigitated architecture via changing polymolybdate clusters14Tuning the Optical Properties of 2‐Thienylpyridyl Iridium Complexes through Carboranes and Anions39Syntheses and electrochemical properties of three supramolecular architectures based on Keggin silicontungstates and different metal-organic units1Covalently-linked polyoxometalate–polymer hybrids: optimizing synthesis, appealing structures and prospective applications72POM species, temperature and counterions modulated the various dimensionalities of POM-based metal–organic frameworks34Two supramolecular complexes based on polyoxometalates and Co-EDTA units via covalent connection or non-covalent interaction13Synthesis of Three Novel Polyoxometalate–based Helical Hybrids from Simple to Complicated Helixes via Turing Metal Salt3Electrochemical and diffuse reflectance study on tetrahedral ε-Keggin-based metal–organic frameworks12Self-assembly of polyoxometalate-based hybrid aggregates: from a monomer to dimers by changing the pH value of reaction systems7Two hybrid polyoxometalates constructed from Preyssler P 5 W 30 clusters and Schiff base exhibiting interesting third-order NLO properties12A new inorganic 2D framework based on Bi-bismuth-capping Keggin polyoxometalate with photodegradation and selective absorption of organic dyes7A robust polyoxometalate-templated four-fold interpenetrating metal–organic framework showing efficient organic dye photodegradation in various pH aqueous solutions23Three hybrid tungstosilicates: Confinement of SiW12O404− anions in rigid concave surfaces with excellent nonlinear optical performance and interesting magnetic properties3Recent advances in transition-metal-containing Keggin-type polyoxometalate-based coordination polymers219A new Keggin-based organic-inorganic nanohybrid in the role of a dual-purpose catalyst7Self‐Assembly of ZnII/CdII/PbII Coordination Polymers with a Tripodal Ligand Derived from Aromatase Inhibitor Letrozole Derivative1Polyoxometalate-based metal–organic frameworks for heterogeneous catalysis163A 2D Cd-containing Keggin-type heteropolyoxometalate with electro-catalytic behaviors2Two bimetal-doped (Fe/Co, Mn) polyoxometalate-based hybrid compounds for visible-light-driven CO 2 reduction9Resurgence and Repurposing of Antifungal Azoles by Transition Metal Coordination for Drug Discovery13Noncovalent Interactions and Physicochemical Properties of an 8‐Hydroxyquinolinium‐Bromoferrate (III) Hybrid Material: Experimental and Computational Approaches2From coordination to hydrogen bonding: electronic and energetic insights into a morpholinium–chloridocadmate(II) hybrid0

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  3. Stabilization and immobilization of polyoxometalates in porous coordination polymers through host–guest interactions

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  4. Construction of a series of 0D, 2D and 3D inorganic–organic hybrid coordination polymers based on octamolybdate and 2-(2-pyridyl)imidazole and its derivative

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  5. Recent advances in crystal engineering

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  6. Synthesis, crystal structures and properties of novel zinc(II) and cadmium(II) polymeric and cyclic bimetallic complexes with fluconazole and dicarboxylate co-ligands

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  7. Cations in control: crystal engineering polyoxometalate clusters using cation directed self-assembly

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  8. MOFs, MILs and more: concepts, properties and applications for porous coordination networks (PCNs)

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  9. Unprecedented three-dimensional 10-connected bct nets based on trinuclear secondary building units and their magnetic behavior

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  10. Two new organic–inorganic supramolecular hybrids templated by the Wells–Dawson polyoxometalates

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  11. A new 2D 5-connected coordination polymer based on 3,4-bis(pyridin-4-ylmethoxy)benzoic acid ligand

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  12. Highly Connected Three-Dimensional Metal−Organic Frameworks Based on Polynuclear Secondary Building Units

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  13. A series of inorganic–organic hybrid compounds constructed from bis(undecatungstophosphate) lanthanates and copper-organic units

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  14. Construction of one- to two-dimensional POM-based compounds through adjusting the metal cations and polyanions

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  15. Two new organic–inorganic hybrid compounds based on metal–pyrazine coordination polymers and Keggin polyoxometalates: effect of metal ions on thestructure

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  16. Self-assembly of supramolecular networks based on biphosphopentamolybdate and copper–organic units

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  17. Coordination polymers based on the octamolybdate and flexible bis(triazole) ligands with different spacer lengths

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  18. Towards the computational modelling of polyoxoanions on metal surfaces: IR spectrum characterisation of [SiW12O40]4− on Ag(111)

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  19. Assembly of a New Cadmium(II)‐bis(Triazole) Coordination Polymer Templated by Keggin Polyoxometalate

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  20. Polyoxometalates containing late transition and noble metal atoms

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  21. Solvothermal Assembly of a Series of Organic–Inorganic Hybrid Materials Constructed from Keggin Polyoxometalate Clusters and Copper(I)–Organic Frameworks

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  22. A 3D POM-based framework: Synthesis and structure of [Cu2(bbtz)4(SiW12O40)]

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  23. Anion Effects on the Formation of Silver(I) Complexes with the Flexible Ligand 4,4′‐Bis(1,2,4‐triazol‐1‐ylmethyl)biphenyl

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  24. Discrete Covalent Organic–Inorganic Hybrids: Terpyridine Functionalized Polyoxometalates Obtained by a Modular Strategy and Their Metal Complexation

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  25. The Cu(II)-fluconazole complex revisited. Part I: Structural characteristics of the system

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  27. A Series of 3D Rare‐Earth‐Metal–Organic Frameworks with Isolated Guest Keggin Silicotungstate Fragments as Anion Templates

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  28. Keggin polyanion and copper cluster based coordination polymer towards model for complex nanosystem

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  31. Two three-dimensional pillared metal–olsalazine complexes based on infinite rod-shaped secondary building units

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  32. Syntheses Study of Keggin POM Supporting MOFs System

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  33. Hydrothermal synthesis and structural characterization of a new inorganic–organic hybrid compound with photocatalytic activity based on Keggin-type polyanion and cadmium-1, 2, 4-triazolate units

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  34. Inserting -(CH2)n- (n = 2, 3, 4) Spacers into the Reactant Mercapto-methyltetrazole Ligand for Tuning the Multinuclear AgI Clusters in Keggin-Based Compounds

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  35. A Series of Highly Connected Metal–Organic Frameworks Based on Triangular Ligands and d10 Metals: Syntheses, Structures, Photoluminescence, and Photocatalysis

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  36. A host–guest hybrid framework with Anderson anions as template: synthesis, crystal structure and photocatalytic properties

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  37. Assembly of Polyoxometalate-Based Metal–Organic Frameworks with Silver(I)-Schiff Base Coordination Polymeric Chains as Building Blocks

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  38. A series of novel 1D coordination polymers constructed from metal–quinolone complex fragments linked by aromatic dicarboxylate ligands

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  42. Two sinusoidal wavelike 2D coordination polymers with benzophenone-4,4′-dicarboxylate

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  45. Tuning the dimension of POM-based inorganic–organic hybrids from 3D self-penetrating framework to 1D poly-pendant chain via changing POM clusters and introducing secondary spacers

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  46. Metal–organic segment-induced dimensionality evolution in polyoxometalate-based hybrids

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  50. Synthesis, Crystal Structure and Fluorescence Properties of Three 1-D Coordination Polymers Based on Fluconazole

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