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RESEARCH PAPER · Journal of the American Chemical Society · 2011

White Light Emission and Second Harmonic Generation from Secondary Group Participation (SGP) in a Coordination Network

Jun Hui He, Mat­thias Zeller, Allen D. Hunter, Zhengtao Xu

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White Light Emission and Second Harmonic Generation from Secondary Group Participation (SGP) in a Coordination NetworkOriginalMulti-functional metal–organic frameworks assembled from a tripodal organic linker52Relativistic effects in triphenylbismuth and their influence on molecular structure and spectroscopic properties45Side chains chip in0Dual-Emission from a Single-Phase Eu–Ag Metal–Organic Framework: An Alternative Way to Get White-Light Phosphor244Luminescence and energy transfer of Eu3+ or/and Dy3+ co-doped in Sr3AlO4F phosphors with NUV excitation for WLEDs114Luminescent Color Conversion on Cyanostilbene‐Functionalized Quantum Dots via In‐situ Photo‐Tuning97A novel 3D porous cadmium(II) MOF based on conjugated ligand with potential application for sensing small linear conjugated molecule19Highly Thermostable One-Dimensional Lanthanide(III) Coordination Polymers Constructed from Benzimidazole-5,6-dicarboxylic Acid and 1,10-Phenanthroline: Synthesis, Structure, and Tunable White-Light Emission138Luminescence Tuning and White‐Light Emission of Co‐doped Ln–Cd–Organic Frameworks56A luminescent metal–organic framework for sensing methanol in ethanol solution61Carbon, silicon, germanium, tin and lead1Luminescent 2D bismuth–cadmium–organic frameworks with tunable and white light emission by doping different lanthanide ions37Syntheses, structures, and luminescence of four lanthanide metal–organic frameworks based on lanthanide-oxide chains with C2- or C3-symmetric trigonal-planar polycarboxylate ligands33Syntheses, structures, tunable emission and white light emitting Eu3+ and Tb3+ doped lanthanide metal–organic framework materials143White light emission based on a single component Sm( iii ) framework and a two component Eu( iii )-doped Gd( iii ) framework constructed from 2,2′-diphenyl dicarboxylate and 1 H -imidazo[4,5- f ][1,10]-phenanthroline108Luminescent Triarylboron-Functionalized Zinc Carboxylate Metal–Organic Framework53Structural Diversity and Luminescence Properties of Coordination Polymers Built With a Rigid Linear Dicarboxylate and Zn(II)/Pb(II) Ion73An investigation on photoluminescence and energy transfer of Eu3+/Sm3+ single-doped and co-doped Ca4YO(BO3)3 phosphors49Three-Dimensional {Co3+–Zn2+} and {Co3+–Cd2+} Networks Originated from Carboxylate-rich Building Blocks: Syntheses, Structures, and Heterogeneous Catalysis66Reversible and selective solvent adsorption in layered metal–organic frameworks by coordination control9Tailoring the Luminescence of Europium Ions in Mesoporous AlPO4 Monolithic Glass16Efficient and tunable white-light emission of metal–organic frameworks by iridium-complex encapsulation573Approaching White‐Light Emission from a Phosphorescent Trinuclear Gold(I) Cluster by Modulating Its Aggregation Behavior133Approaching White‐Light Emission from a Phosphorescent Trinuclear Gold(I) Cluster by Modulating Its Aggregation Behavior24A white-light-emitting LnMOF with color properties improved via Eu3+ doping: an alternative approach to a rational design for solid-state lighting72A magnesium MOF as a sensitive fluorescence sensor for CS 2 and nitroaromatic compounds130Controlling the energy transfer in lanthanide–organic frameworks for the production of white-light emitting materials58Delicate modulated assembly of a new kind of trinuclear copper( ii ) motif governed by N-containing agents11Lanthanide organic–inorganic hybrids based on functionalized metal–organic frameworks (MOFs) for a near-UV white LED92Pure white-light and yellow-to-blue emission tuning in single crystals of Dy( iii ) metal–organic frameworks158Syntheses, crystal structures and UV-visible absorption properties of five metal–organic frameworks constructed from terphenyl-2,5,2′,5′-tetracarboxylic acid and bis(imidazole) bridging ligands64Selective Ag(I) Binding, H 2 S Sensing, and White-Light Emission from an Easy-to-Make Porous Conjugated Polymer120Luminescence properties and energy transfer in the novel red emitting phosphors Ba2Ln(BO3)2Cl:Sm3+, Eu3+ (Ln=Y, Gd)19Synthesis and characterization of three novel 3D metal–organic frameworks constructed from semi-rigid V-shaped ligands6Hemi- and holo-directed lead( ii ) complexes in a soft ligand environment35Pd Uptake and H2S Sensing by an Amphoteric Metal–Organic Framework with a Soft Core and Rigid Side Arms98Pd Uptake and H2S Sensing by an Amphoteric Metal–Organic Framework with a Soft Core and Rigid Side Arms7Tunable photoluminescence and direct white-light emission in Mg-based coordination networks50A series of MOFs based on a triangular tri(4-pyridylphenyl)amine ligand combined with carboxylate or nitrate auxiliary ligands27A ketone functionalized luminescent terbium metal–organic framework for sensing of small molecules98Solution Processable MOF Yellow Phosphor with Exceptionally High Quantum Efficiency280Syntheses, crystal structures and properties of series of 4d–4f ln(III)–Ag(I) heterometallic coordination polymers10A new strategy for achieving white-light emission of lanthanide complexes: effective control of energy transfer from blue-emissive fluorophore to Eu( iii ) centres54Color tunable and near white-light emission of two solvent-induced 2D lead( ii ) coordination networks based on a rigid ligand 1-tetrazole-4-imidazole-benzene33Efficient and tunable multi-color and white light Ln-MOFs with high luminescence quantum yields42Lanthanide ions (Eu 3+ , Tb 3+ , Sm 3+ , Dy 3+ ) activated ZnO embedded zinc 2,5-pyridinedicarboxylic metal–organic frameworks for luminescence application43Lanthanides post-functionalized nanocrystalline metal–organic frameworks for tunable white-light emission and orthogonal multi-readout thermometry130Photoluminescence and white-light emission in two series of heteronuclear Pb( ii )–Ln( iii ) complexes23Ratiometric multiplexed barcodes based on luminescent metal–organic framework films41Semidirected versus holodirected coordination and single-component white light luminescence in Pb( ii ) complexes383D Microporous Lanthanide–Organic Frameworks Constructed from Left‐ and Right‐Handed Helical Chains: Synthesis, Crystal Structure, and Tunable Photoluminescence8Assembly of 1,3,5-tris(2-alkylthiol-pyrimidin-4-yl)benzene) (alkyl = Me, n-Pr) with copper(I) iodide: effect of alkyl side chain4Lanthanide Ion Codoped Emitters for Tailoring Emission Trajectory and Temperature Sensing292Stable Luminescent Metal–Organic Frameworks as Dual-Functional Materials To Encapsulate Ln 3+ Ions for White-Light Emission and To Detect Nitroaromatic Explosives207Multistimuli‐responsive White Luminescent Fluids Using Hybrid Lanthanide Metal–Coordinate Complex Probes38Structure and luminescent properties of complex compounds of tellurium(IV) with ammonium bases18Dye Encapsulated Metal‐Organic Framework for Warm‐White LED with High Color‐Rendering Index290A Boiling‐Water‐Stable, Tunable White‐Emitting Metal–Organic Framework from Soft‐Imprint Synthesis37A responsive MOF nanocomposite for decoding volatile organic compounds139Dual‐Emission Luminescence of Magnesium Coordination Polymers Based on Mixed Organic Ligands25A stable Alq3@MOF composite for white-light emission92A highly stable and white-light-emitting Eu( iii ) MOF29A lanthanide( iii ) metal–organic framework exhibiting ratiometric luminescent temperature sensing and tunable white light emission48A photochromic dual-functional Mg-CP exhibits white-emission after modification with CuI14Inorganic–organic hybrid white light phosphors107Synthesis and structure of color tunable and white-light emitting lanthanide metal–organic framework materials constructed from conjugated 1,1′-butadiynebenzene-3,3′,5,5′-tetracarboxylate ligand28Two-semiconductive-component hybrid coordination polymers with controllable photo-induced electron-transfer properties57Two second-order non-linear optical coordination polymers with noninterpenetrating honeycomb-like 2-D (6,3)-type networks6Luminescent and thermochromic properties of tellurium(IV) halide complexes with cesium50Synthesis and fluorescent pH sensing properties of nanoscale lanthanide metal-organic frameworks with silk fibroin powder as polymer ligands31An Azole-Based Metal–Organic Framework toward Direct White-Light Emissions by the Synergism of Ligand-Centered Charge Transfer and Interligand π–π Interactions47A Comparative Study on the Luminescence of the Cd2+ and Mn2+ Coordination Polymers Based on the Same Mixed Ligands7High-Performance Blue-Excitable Yellow Phosphor Obtained from an Activated Solvochromic Bismuth-Fluorophore Metal–Organic Framework59Emerging Multifunctional Metal–Organic Framework Materials1587Single Component Lanthanide Hybrids Based on Metal–Organic Framework for Near-Ultraviolet White Light LED119Structures of Metal–Organic Frameworks with Rod Secondary Building Units909Two blue-light excitable yellow-emitting LMOF phosphors constructed by triangular tri(4-pyridylphenyl)amine39Encapsulation of an iridium complex in a metal–organic framework to give a composite with efficient white light emission45Site-selective Eu( iii ) spectroscopy of highly efficient luminescent mixed-metal Pb( ii )/Eu( iii ) coordination polymers17Photoluminescence and Hydrothermal Stability Correlations via Isoreticular/Structural fcu Rare-Earth Organic Frameworks Platform12Luminescence of antimony(III) halogenides complexes with 2- and 4-benzylpyridine8Isomer dependent assembly of lead(II) compounds derived from 5-(n-pyridyl)tetrazole-2-isopropionic acid (n = 2,3)5Ligand-Driven Coordination Sphere-Induced Engineering of Hybride Materials Constructed from PbCl2 and Bis-Pyridyl Organic Linkers for Single-Component Light-Emitting Phosphors78Introduction of Red‐Green‐Blue Fluorescent Dyes into a Metal–Organic Framework for Tunable White Light Emission270Luminescent metal–organic frameworks and coordination polymers as alternative phosphors for energy efficient lighting devices218Facile preparation of a tetraphenylethylene-doped metal–organic framework for white light-emitting diodes28Photofunctional hybrids of TiO 2 and titanium metal–organic frameworks for dye degradation and lanthanide ion-tuned multi-color luminescence21Photonic functional metal–organic frameworks661Phosphors and Fluorescent Converters in Light Sources with Blue LED Crystals2Three Cd(II) MOFs with Different Functional Groups: Selective CO2 Capture and Metal Ions Detection97Two near white light emitting Pb(II) or Cd(II) complexes2Chiral Lead Halide Perovskite Nanowires for Second-Order Nonlinear Optics379Single-Phase White-Light-Emitting and Photoluminescent Color-Tuning Coordination Assemblies567Near-White Light Emission from Lead(II) Metal–Organic Frameworks48Photoluminescent, upconversion luminescent and nonlinear optical metal-organic frameworks: From fundamental photophysics to potential applications206Porous Organic Polymer from Aggregation-Induced Emission Macrocycle for White-Light Emission34An ultrastable metal–organic material emits efficient and broadband bluish white-light emission for luminescent thermometers26The First 2D Hybrid Perovskite Ferroelectric Showing Broadband White‐Light Emission with High Color Rendering Index178A stable luminescent zinc–organic framework as a dual-sensor toward Cu 2+ and Cr 2 O 7 2− , and excellent platform-encapsulated Ln 3+ for systematic color tuning and white-light emission13Rare earth-free composites of carbon dots/metal–organic frameworks as white light emitting phosphors86Second order nonlinear optical activity of amino acids, guanidines and pyridinium salts of inorganic anions0Crystals of Sb3+-coordination complexes exhibiting yellowish green emissions with outstanding lifetimes12Solid State Multicolor Emission in Substitutional Solid Solutions of Metal–Organic Frameworks113Sonochemical Synthesis of Carbon Dots/Lanthanoid MOFs Hybrids for White Light-Emitting Diodes with High Color Rendering88Color-Tuning and Near-Sunlight White Emission in Highly Stable Rod-Spacer MOFs with Defective Dicubane Based Lead(II)-Carboxyl Chains38Supramolecular architecture constructed from the hemidirected lead(II) complex with N'-(4-hydroxybenzylidene)isonicotinohydrazide49A moisture-stable organosulfonate-based metal–organic framework with intrinsic self-trapped white-light emission14Efficient detection of Cr 3+ and Cr 2 O 7 2− using a Zn( ii ) luminescent metal–organic framework9Highly stable 3D porous HMOF with enhanced catalysis and fine color regulation by the combination of d- and p-ions when compared with those of its monometallic MOFs70Lead( ii ) coordination polymers driven by pyridine-hydrazine donors: from anion-guided self-assembly to structural features35Люминесцентные и термохромные свойства комплексов галогенидов теллура(IV) с рубидием Rb-=SUB=-2-=/SUB=-TeHal-=SUB=-6-=/SUB=- (Hal = Cl, Br, I)2Hydrated proton conduction and luminescence of a carboxylate and sulfonate-included lead(II) coordination polymer8Synthesis and thermal behavior of two Sr(II) compounds derived from isomeric 5-(n-pyridyl)tetrazole-2-isopropionic acid (n = 2, 3)8Hybrid Inorganic‐Organic White Light Emitting Diodes16Second-Harmonic Generation and Photoluminescence Properties of Sn(II)- and Bi(III)-Based Lone Pair Cation–Pyridine Dicarboxylate Coordination Compounds17A robust stimuli responsive Eu3+ – Metalo organic hydrogel and xerogel emitting white light22Tetrel Bonding and Other Non-Covalent Interactions Assisted Supramolecular Aggregation in a New Pb(II) Complex of an Isonicotinohydrazide51The selective recognition and luminescence sensing demonstrated in yttrium - Organic framework10Tunable colors and white-light emissions by encapsulation of guest molecules or ions into a flexible metal–organic framework5Luminescence and Thermochromic Properties of Complexes of Tellurium(IV) Halides with Rubidium Rb2TeHal6 (Hal = Cl, Br, I)4A luminescent metal–organic framework with mixed-linker strategy for white-light-emitting by iridium-complex encapsulation11Two‐Dimensional Metal–Organic Frameworks‐Based Electrocatalysts for Oxygen Evolution and Oxygen Reduction Reactions53Люминесцентные свойства комплексов галогенидов теллура (IV) с пиридином (C-=SUB=-5-=/SUB=-H-=SUB=-5-=/SUB=-NH)-=SUB=-2-=/SUB=-TeHaI-=SUB=-6-=/SUB=- (где HaI=Cl, Br)0Tunable White Light Emission in a Zero‐Dimensional Organic–Inorganic Metal Halide Hybrid with Ultra‐High Color Rendering Index61Facile preparation of thioether/hydroxyl functionalized polyhedral oligomeric silsesquioxanes hybrid polymer for ultrahigh selective adsorption of silver(I) ions28Recent Advances on the Applications of Luminescent Pb2+-Containing Metal–Organic Frameworks in White-Light Emission and Sensing14Polymeric lead(II) phosphor featuring cubane [Pb4] and [Pb8] units: Organic vs inorganic binding competition, colour regulation and white luminescence2Luminescent Properties of Complexes of Tellurium(IV) Halides with Pyridine (C5H5NH)2TeHal6 (Hal = Cl, Br)1Heterobimetallic Cluster‐Based Coordination Polymers: Assembly, Structures and Third‐Order Nonlinear Optical Properties4White light emission phosphor modulation, nitrobenzene sensing property and barcode anti-counterfeiting via lanthanides post-functionalized metal-organic frameworks12Luminescent MOFs (LMOFs): recent advancement towards a greener WLED technology73Tin(IV) halide complexes with 5,7-dimethyl-8-quinolinol: structures, optical and thermal properties1Cluster‐Glass for Low‐Cost White‐Light Emission21Recent research progress in CDs@MOFs composites: fabrication, property modulation, and application29A synergetic model for implementing single-component white-light emission: a case study of zero-dimensional cadmium halides22Tetrel bonding stabilization of a new coordination polymer constructed from lead( ii ) azide and 1-(pyridin-2-yl)ethylidenepicolinohydrazide16Thiol and thioether-based metal–organic frameworks: synthesis, structure, and multifaceted applications42Tuning the rare-earth UiO-66 metal–organic framework platform for white light emission36Strategies, Synthesis, and Applications of Metal-Organic Framework Materials0Multicolor Fluorescent Lead‐MOFs for White‐Light‐Emitting and Anticounterfeiting Applications14Photoluminescence and third-order nonlinear optical limiting properties of Sn1-xNdxO2 thin films deposited via spray pyrolysis4Structure and Luminescent Properties of Tellurium(IV) Bromide Complex with p-Toluidinium (HPT)2TeBr6 · H2O0Structure and Luminescent Properties of Tellurium(IV) Bromide Complex with p-Toluidinium (HPT)2TeBr6·H2O2Assembly of two new self-interpenetrating metal-organic frameworks with tunable luminescent properties2A novel halide hybrid white light emitter with remarkable structural and emission stability1Blue- and white-light emitting 2D metal–organic frameworks of cis -5-norbornene- endo -2,3-dicarboxylic acid1Supramolecular lead(II) coordination polymers, obtained from polydonor N'-(amino(pyrazin-2-yl)methylene)thiosemicarbazide0Sulphur-enriched Metal-Organic Frameworks: Design, Manipulation, Strategies, Recent Advances and Perspectives10A supramolecular coordination polymer incorporating lead(II) perchlorate, amino(pyridin-2-yl)methylenepyridin-1-ium-4-carbohydrazonate and thiocyanate as an auxiliary ligand9Interaction of Lead(II) Perchlorate with N′-Isonicotinoylpicolinohydrazonamide and Its Sodium Salt in the Presence of Potassium Cyanide: Yellow Green Light Emitting Phosphors, Stabilized by Tetrel Bonds, and a System to Transform Methanol to Acetate10

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  4. Dual-Emission from a Single-Phase Eu–Ag Metal–Organic Framework: An Alternative Way to Get White-Light Phosphor

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  15. White light emission based on a single component Sm( iii ) framework and a two component Eu( iii )-doped Gd( iii ) framework constructed from 2,2′-diphenyl dicarboxylate and 1 H -imidazo[4,5- f ][1,10]-phenanthroline

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  33. Luminescence properties and energy transfer in the novel red emitting phosphors Ba2Ln(BO3)2Cl:Sm3+, Eu3+ (Ln=Y, Gd)

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  34. Synthesis and characterization of three novel 3D metal–organic frameworks constructed from semi-rigid V-shaped ligands

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  35. Hemi- and holo-directed lead( ii ) complexes in a soft ligand environment

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  37. Pd Uptake and H2S Sensing by an Amphoteric Metal–Organic Framework with a Soft Core and Rigid Side Arms

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  43. A new strategy for achieving white-light emission of lanthanide complexes: effective control of energy transfer from blue-emissive fluorophore to Eu( iii ) centres

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  44. Color tunable and near white-light emission of two solvent-induced 2D lead( ii ) coordination networks based on a rigid ligand 1-tetrazole-4-imidazole-benzene

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  45. Efficient and tunable multi-color and white light Ln-MOFs with high luminescence quantum yields

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  46. Lanthanide ions (Eu 3+ , Tb 3+ , Sm 3+ , Dy 3+ ) activated ZnO embedded zinc 2,5-pyridinedicarboxylic metal–organic frameworks for luminescence application

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  47. Lanthanides post-functionalized nanocrystalline metal–organic frameworks for tunable white-light emission and orthogonal multi-readout thermometry

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  48. Photoluminescence and white-light emission in two series of heteronuclear Pb( ii )–Ln( iii ) complexes

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  49. Ratiometric multiplexed barcodes based on luminescent metal–organic framework films

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  50. Semidirected versus holodirected coordination and single-component white light luminescence in Pb( ii ) complexes

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