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RESEARCH PAPER · Dalton Transactions · 2014

A-site size effect in a family of unfilled ferroelectric tetragonal tungsten bronzes: Ba 4 R 0.67 Nb 10 O 30 (R = La, Nd, Sm, Gd, Dy and Y)

Jonathan Gardner, Finlay D. Morrison

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A-site size effect in a family of unfilled ferroelectric tetragonal tungsten bronzes: Ba 4 R 0.67 Nb 10 O 30 (R = La, Nd, Sm, Gd, Dy and Y)OriginalDielectric and ferroelectric properties of unfilled tungsten bronze KBa3RNb10O30 ceramics9Effect of local A-site strain on dipole stability in A 6 GaNb 9 O 30 (A = Ba, Sr, Ca) tetragonal tungsten bronze relaxor dielectrics25Effect of the cation size on the framework structures of magnesium tungstate, A 4 Mg(WO 4 ) 3 (A = Na, K), R 2 Mg 2 (WO 4 ) 3 (R = Rb, Cs)31Structure and oxide ion conductivity in tetragonal tungsten bronze BaBiNb 5 O 1521Vogel–Fulcher analysis of relaxor dielectrics with the tetragonal tungsten bronze structure: Ba6MNb9O30 (M = Ga, Sc, In)29A Crystal-Chemical Framework for Relaxor versus Normal Ferroelectric Behavior in Tetragonal Tungsten Bronzes195Electrical Characterization Induced by Structural Modulation in␣(Ca0.28Ba0.72)2.5–0.5x (Na0.5K0.5) x Nb5O15 Ceramics6Effect of cerium addition on the microstructure, electrical and relaxor behavior of Sr0.5Ba0.5Nb2O6 ceramics29Elastic and anelastic relaxations accompanying relaxor ferroelectric behaviour of Ba6GaNb9O30 tetragonal tungsten bronze from resonant ultrasound spectroscopy9Structural and relaxor-like dielectric properties of unfilled tungsten bronzes Ba5−5xSm5xTi5xNb10−5xO308Microstructural and high-temperature impedance spectroscopy study of Ba6MNb9O30 (M=Ga, Sc, In) relaxor dielectric ceramics with tetragonal tungsten bronze structure13Influence of erbium substitution on structural, electrical, and up-conversion photoluminescence properties of unfilled tungsten bronze oxides Ba3.75La0.833-xErxNb10O3020Relaxor-to-Ferroelectric Crossover and Disruption of Polar Order in “Empty” Tetragonal Tungsten Bronzes57Manipulation of polar order in the “empty” tetragonal tungsten bronzes: Ba4-xSrxDy0.67□1.33Nb10O30, x = 0, 0.25, 0.5, 1, 2, 328Large Magnetoelectric Coupling Near Room Temperature in Synthetic Melanostibite Mn2FeSbO629Large Magnetoelectric Coupling Near Room Temperature in Synthetic Melanostibite Mn2FeSbO67Dielectric properties of unfilled tetragonal tungsten bronze Ba4PrFe0.5Nb9.5O30 ceramics7Prospective crystal-chemistry : relaxors, ferroics and low temperature SPS0Sodium Cation Substitution in Sr2KTa5O15 toward Enhancement of Photocatalytic Conversion of CO2 Using H2O as an Electron Donor16Photocatalytic Conversion of Carbon Dioxide over A 2 BTa 5 O 15 (A = Sr, Ba; B = K, Na) Using Ammonia as an Efficient Sacrificial Reagent12Quantum critical points in ferroelectric relaxors: Stuffed tungsten bronze K3Li2Ta5O15 and lead pyrochlore ( Pb2Nb2O7 )5Effect of Lanthanide on Bi3.25Ln0.75Ti3O12 (Ln=La, Ce, Nd, Sm) Nanofibers for Humidity Sensing Properties4Preparation and dielectric properties of Ba4RFe0.5Nb9.5O30 (R = La, Nd, Eu, Gd) unfilled tungsten bronze ceramics21Structural, electrical and relaxor properties of Sc-In solid solution in tetragonal tungsten bronze ceramics5Preparation and dielectric properties of Ba4−xSm2Fe2−xNb8+xO30 tungsten bronze ceramics with an adjustable structure that changes from filled to unfilled4Effects of A-site cations on the electrical behaviors in (Sr1-Ca )2.1Na0.8Nb5O15 tungsten bronze ferroelectrics24Effect of rare earth on dielectric properties of Mn contained unfilled tungsten bronze ceramics6Structural and electrical effects of Ag substitution in tungsten bronze Sr2Ag Na1−Nb5O15 ceramics27Local Structure and Order–Disorder Transitions in “Empty” Ferroelectric Tetragonal Tungsten Bronzes13New high temperature dielectrics: Bi-free tungsten bronze ceramics with stable permittivity over a very wide temperature range20Antiferroelectricity and robust dielectric response owing to competing polar and antipolar instabilities in tetragonal tungsten bronze K 2 R Nb 5 O 15 ( R : rare-earth)16Relaxor Nature and Energy Storage Properties of Sr2– x M x NaNb5– x Ti x O15 (M = La3+ and Ho3+) Tungsten Bronze Ceramics61Relaxor regulation and improvement of energy storage properties of Sr2NaNb5O15-based tungsten bronze ceramics through B-site substitution86Tribocatalytic degradation of dyes by tungsten bronze ferroelectric Ba 2.5 Sr 2.5 Nb 8 Ta 2 O 30 submicron particles65Ferroelectric to relaxor crossover in Li solid solutions derived from Ba2Nd□2FeNb4O151Spontaneous polarization and DC resistivity investigations in Ba[1.6-(3x/2)]Sr2.4ErxNa1.4Li0.6Nb10O30 tungsten bronze structured nano-phased relaxor ferroelectrics0Relaxor nature and superior energy storage performance of Sr2Ag0.2Na0.8Nb5O15-based tungsten bronze ceramics through B-site substitution71Designing new polar materials1Enhanced energy storage properties and superior thermal stability in SNN-based tungsten bronze ceramics through substitution strategy49Active and passive defects in tetragonal tungsten bronze relaxor ferroelectrics5Enhancing Comprehensive Energy Storage Properties in Tungsten Bronze Sr 0.53 Ba 0.47 Nb 2 O 6 -Based Lead-free Ceramics by B-Site Doping and Relaxor Tuning64Role of coordination site in governing the structural, electronic and optical properties of Ca-doped strontium barium niobate5Cation Disorder in Ferroelectric Ba4M2Nb10O30 (M = Na, K, and Rb) Tetragonal Tungsten Bronzes11Remarkable energy storage performances of tungsten bronze Sr0.53Ba0.47Nb2O6-based lead-free relaxor ferroelectric for high-temperature capacitors application83Centrosymmetric Tetragonal Tungsten Bronzes A4Bi2Nb10O30 (A = Na, K, Rb) with a Bi 6s Lone Pair12Superior Energy Density Achieved in Unfilled Tungsten Bronze Ferroelectrics via Multiscale Regulation Strategy106Enhanced energy storage properties on calcium modified strontium barium niobate lead-free ferroelectric relaxor ceramics4A-Site Cation Disorder in SrxBa1–xNb2O6 (x = 0.25, 0.33, 0.50, 0.61) Studied by High-Resolution Resonant X-ray Powder Diffraction8Effect of sodium substitution by yttrium on the structural, dielectric and electrical properties of Ba2Na(1-3x)YxNb5O15 ceramics15Synthesis and characterization of (Ba (1.6-3/2X) Sr2.4Na2Nb10O30: xHo3+) ferroelectric nanomaterials by solid state reaction routes for device applications2Ultrahigh Energy Storage in Tungsten Bronze Dielectric Ceramics Through a Weakly Coupled Relaxor Design97The effect of cation size on structure and properties of Ba-based tetragonal tungsten bronzes Ba 4 M 2 Nb 10 O 30 (M = Na, K or Rb) and Ba 4 M 2 Nb 8 Ti 2 O 30 (M = Ca or Sr)8Tailoring Zr-doped tungsten bronze (Sr,Ba,Gd)Nb2O6 relaxor ferroelectric with high electrical insulation interface for dielectric capacitor36On the solubility of Bi in tetragonal tungsten bronzes7Polarization mechanism in filled tungsten bronze Ba4Sm2Ti4Nb6O30 with pinched P–E hysteresis loops1Structural and dielectric properties of CaSnO3-doped Sr2.1Na0.8Nb5O15 ceramics2Structural origins of dielectric anomalies in the filled tetragonal tungsten bronze Sr2NaNb5O1514Enhancing dielectric properties and thermal stability in microwave-synthesized Nd-modified barium titanate nanoceramics for possible MLCC applications16Structural and Dielectric Properties of RE3+, B3+ co-doped (RE3+=Sm3+, Dy3+) BaTa2O6 Tetragonal Tungsten Bronze-Type Ceramics4Influence of Boron Doping on the Dielectric Characteristics of Eu3+-Doped β-SrTa2O6 and Eu3+-Doped BaTa2O6 Tungsten Bronze-Type Ceramics10An investigation of structural, magnetic and electrical properties of Ca dominant A-site tungsten bronze ferroelectric ceramic2Impact of Ce Doping on the Relaxor Behavior and Electrical Properties of Sr0.4Ba0.6Nb2O6 Ferroelectric Ceramics2A study on the structural, morphological, spectral properties of BaTa2O6:RE3+, B3+ (RE = Sm, Dy) phosphors and the comparison of asymmetry ratios based on the hypersensitive transition of BaTa2O6:Eu3+, B3+ phosphor18Realizing Exceptional Energy Storage Performance in Tungsten Bronze-Based Ceramics via Weakly Coupled Relaxor and Grain Boundary Reinforcement Designs10Investigation of (Ba(1.6-3/2x) Sr2.4Na2Nb10O30:xHo3+) tungsten bronze structured ferroelectric nanomaterial for optoelectronic application0Quantifying Emptiness: On the Size of A-Site Vacancies in Tetragonal Tungsten Bronzes4Structural transitions and dielectric behavior of SrRTiNbO induced by rare-earth substitutions (R = Gd, Sm, Nd)1Tungsten bronze oxide ceramics for energy storage: Characterization, synthesis, and performance39Regulating relaxor behavior and microstructure evolution in (Sr,Ba)Nb2O6-based unfilled tungsten bronze ferroelectrics for enhanced energy storage at low electric fields0Correlating A and B site Co-doping effects on the crystallographic structure and dielectric properties of Sr2NaNb5O15 (SNN) tetragonal tungsten bronze (TTB)0A-site ionic gradient engineering for enhanced capacitive energy storage in bismuth-free relaxor ferroelectrics1The impact of dilute Gd and Mn co-doping in BaTiO₃: From crystal chemistry to morphological, magnetic, dielectric, and electric properties and in functional application0Enhanced energy-storage performance in lead-free tungsten bronze ceramics via A-site equimolar high-entropy design0Achieving 96.6% energy-storage efficiency in Nd-doped tungsten-bronze ceramics through A-site vacancy engineering1Bi doped (Ba,Ca)(Zr,Ti)O3 ceramics for simultaneously enhancing Curie temperature and piezoelectric performance0Wide temperature stability range of high-permittivity and low-loss Sr3-xNaxTi1-xNb4+xO15 tungsten bronze ceramics0

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  1. Dielectric and ferroelectric properties of unfilled tungsten bronze KBa3RNb10O30 ceramics

    Journal of Materials Science Materials in Electronics · 2014-10-27

    Changzheng Hu, Zhen Yu Sun, Qihua Zhu, Liang Fang, Laijun Liu

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  2. Effect of local A-site strain on dipole stability in A 6 GaNb 9 O 30 (A = Ba, Sr, Ca) tetragonal tungsten bronze relaxor dielectrics

    Dalton Transactions · 2015-01-01

    Andrew J. Miller, Andrei Rotaru, Donna C. Arnold, Finlay D. Morrison

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  3. Effect of the cation size on the framework structures of magnesium tungstate, A 4 Mg(WO 4 ) 3 (A = Na, K), R 2 Mg 2 (WO 4 ) 3 (R = Rb, Cs)

    Dalton Transactions · 2015-01-01

    Shujuan Han, Ying Wang, Qun Jing, Hongping Wu, Shilie Pan, Zhihua Yang

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  4. Structure and oxide ion conductivity in tetragonal tungsten bronze BaBiNb 5 O 15

    RSC Advances · 2015-01-01

    Hongqiang Ma, Kun Lin, Longlong Fan, Yangchun Rong, Jun Chen, Jinxia Nancy Deng, Laijun Liu, Shogo Kawaguchi, Kenichi Kato, Xianran Xing

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  5. Vogel–Fulcher analysis of relaxor dielectrics with the tetragonal tungsten bronze structure: Ba6MNb9O30 (M = Ga, Sc, In)

    Journal of Thermal Analysis and Calorimetry · 2015-01-30

    Andrei Rotaru, Finlay D. Morrison

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  6. A Crystal-Chemical Framework for Relaxor versus Normal Ferroelectric Behavior in Tetragonal Tungsten Bronzes

    Chemistry of Materials · 2015-04-09

    Xiao Li Zhu, Maosen Fu, Martin Christopher. Stennett, Paula Maria Vilarinho, Igor Levin, Clive A. Randall, Jonathan Gardner, Finlay D. Morrison, Ian Michael Reaney

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  7. Electrical Characterization Induced by Structural Modulation in␣(Ca0.28Ba0.72)2.5–0.5x (Na0.5K0.5) x Nb5O15 Ceramics

    Journal of Electronic Materials · 2015-11-30

    Bian Yang, Lingling Wei, Zhongming Wang, Shoucheng Kang, Xiaolian Chao, Zupei Yang

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  8. Effect of cerium addition on the microstructure, electrical and relaxor behavior of Sr0.5Ba0.5Nb2O6 ceramics

    Journal of Alloys and Compounds · 2016-01-02

    Thamil Selvi Velayutham, N.I.F. Salim, Wee Chen Gan, Wan Haliza Abd Majid

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  9. Elastic and anelastic relaxations accompanying relaxor ferroelectric behaviour of Ba6GaNb9O30 tetragonal tungsten bronze from resonant ultrasound spectroscopy

    Journal of Thermal Analysis and Calorimetry · 2016-01-06

    Andrei Rotaru, Jason Schiemer, Michael A. Carpenter

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  10. Structural and relaxor-like dielectric properties of unfilled tungsten bronzes Ba5−5xSm5xTi5xNb10−5xO30

    Journal of Applied Physics · 2016-03-28

    Tong Wei, Z. Dong, Chuan‐Zhen Zhao, Yipeng Guo, Qingjun Zhou, Z.P. Li

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  11. Microstructural and high-temperature impedance spectroscopy study of Ba6MNb9O30 (M=Ga, Sc, In) relaxor dielectric ceramics with tetragonal tungsten bronze structure

    Ceramics International · 2016-04-30

    Andrei Rotaru, Finlay D. Morrison

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  12. Influence of erbium substitution on structural, electrical, and up-conversion photoluminescence properties of unfilled tungsten bronze oxides Ba3.75La0.833-xErxNb10O30

    Journal of Alloys and Compounds · 2016-05-03

    Z. Dong, Tong Wei, Y.J. Ma, T.B. Zhang, Xiaoxue Lian, Yipeng Guo, Fengming Yang, Dongmin An

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  13. Relaxor-to-Ferroelectric Crossover and Disruption of Polar Order in “Empty” Tetragonal Tungsten Bronzes

    Chemistry of Materials · 2016-06-06

    Jonathan Gardner, Fengjiao Yu, Chiu Chung Tang, Winfried A. Kockelmann, Wuzong Zhou, Finlay D. Morrison

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  14. Manipulation of polar order in the “empty” tetragonal tungsten bronzes: Ba4-xSrxDy0.67□1.33Nb10O30, x = 0, 0.25, 0.5, 1, 2, 3

    Applied Physics Letters · 2016-08-15

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  15. Large Magnetoelectric Coupling Near Room Temperature in Synthetic Melanostibite Mn2FeSbO6

    Angewandte Chemie International Edition · 2017-03-23

    Antonio J. Dos santos‐García, Elena Solana‐Madruga, C. Ritter, Adrián Andrada‐Chacón, Javier Sánchez-Benítez, F. J. Mompeán, M. Garcı́a-Hernández, R. Sáez-Puche, Rainer Schmidt

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  16. Large Magnetoelectric Coupling Near Room Temperature in Synthetic Melanostibite Mn2FeSbO6

    Angewandte Chemie · 2017-03-23

    Antonio J. Dos santos‐García, Elena Solana‐Madruga, C. Ritter, Adrián Andrada‐Chacón, Javier Sánchez-Benítez, F. J. Mompeán, M. Garcı́a-Hernández, R. Sáez-Puche, Rainer Schmidt

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  17. Dielectric properties of unfilled tetragonal tungsten bronze Ba4PrFe0.5Nb9.5O30 ceramics

    Journal of Wuhan University of Technology-Mater Sci Ed · 2017-07-27

    Changzheng Hu, Qihua Zhu, Zhen Sun, Zhe Guo, Laijun Liu, Liang Fang

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  18. Prospective crystal-chemistry : relaxors, ferroics and low temperature SPS

    Unknown journal · 2017-09-26

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  19. Sodium Cation Substitution in Sr2KTa5O15 toward Enhancement of Photocatalytic Conversion of CO2 Using H2O as an Electron Donor

    ACS Omega · 2017-11-20

    Zeai Huang, Sumika Yoshizawa, Kentaro Teramura, Hiroyuki Asakura, Saburo Hosokawa, Tsunehiro Tanaka

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  20. Photocatalytic Conversion of Carbon Dioxide over A 2 BTa 5 O 15 (A = Sr, Ba; B = K, Na) Using Ammonia as an Efficient Sacrificial Reagent

    ACS Sustainable Chemistry & Engineering · 2018-05-15

    Zeai Huang, Sumika Yoshizawa, Kentaro Teramura, Hiroyuki Asakura, Saburo Hosokawa, Tsunehiro Tanaka

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  21. Quantum critical points in ferroelectric relaxors: Stuffed tungsten bronze K3Li2Ta5O15 and lead pyrochlore ( Pb2Nb2O7 )

    Physical Review Materials · 2018-08-22

    Rebecca M. Smith, Jonathan Gardner, Finlay D. Morrison, Stephen E. Rowley, Catarina Ferraz, M. A. Carpenter, Jiasheng Chen, Jack Hodkinson, Siân E. Dutton, J. F. Scott

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  22. Effect of Lanthanide on Bi3.25Ln0.75Ti3O12 (Ln=La, Ce, Nd, Sm) Nanofibers for Humidity Sensing Properties

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  23. Preparation and dielectric properties of Ba4RFe0.5Nb9.5O30 (R = La, Nd, Eu, Gd) unfilled tungsten bronze ceramics

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  24. Structural, electrical and relaxor properties of Sc-In solid solution in tetragonal tungsten bronze ceramics

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  25. Preparation and dielectric properties of Ba4−xSm2Fe2−xNb8+xO30 tungsten bronze ceramics with an adjustable structure that changes from filled to unfilled

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  26. Effects of A-site cations on the electrical behaviors in (Sr1-Ca )2.1Na0.8Nb5O15 tungsten bronze ferroelectrics

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  27. Effect of rare earth on dielectric properties of Mn contained unfilled tungsten bronze ceramics

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  28. Structural and electrical effects of Ag substitution in tungsten bronze Sr2Ag Na1−Nb5O15 ceramics

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  29. Local Structure and Order–Disorder Transitions in “Empty” Ferroelectric Tetragonal Tungsten Bronzes

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  30. New high temperature dielectrics: Bi-free tungsten bronze ceramics with stable permittivity over a very wide temperature range

    Journal of the European Ceramic Society · 2020-10-21

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  31. Antiferroelectricity and robust dielectric response owing to competing polar and antipolar instabilities in tetragonal tungsten bronze K 2 R Nb 5 O 15 ( R : rare-earth)

    Physical Review Materials · 2020-10-29

    Tomoki Murata, Hirofumi Akamatsu, Daisuke Hirai, Fumiyasu Oba, Sakyo Hirose

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  32. Relaxor Nature and Energy Storage Properties of Sr2– x M x NaNb5– x Ti x O15 (M = La3+ and Ho3+) Tungsten Bronze Ceramics

    ACS Sustainable Chemistry & Engineering · 2020-11-16

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  33. Relaxor regulation and improvement of energy storage properties of Sr2NaNb5O15-based tungsten bronze ceramics through B-site substitution

    Chemical Engineering Journal · 2020-11-25

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  34. Tribocatalytic degradation of dyes by tungsten bronze ferroelectric Ba 2.5 Sr 2.5 Nb 8 Ta 2 O 30 submicron particles

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  35. Ferroelectric to relaxor crossover in Li solid solutions derived from Ba2Nd□2FeNb4O15

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  36. Spontaneous polarization and DC resistivity investigations in Ba[1.6-(3x/2)]Sr2.4ErxNa1.4Li0.6Nb10O30 tungsten bronze structured nano-phased relaxor ferroelectrics

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  37. Relaxor nature and superior energy storage performance of Sr2Ag0.2Na0.8Nb5O15-based tungsten bronze ceramics through B-site substitution

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  38. Designing new polar materials

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  39. Enhanced energy storage properties and superior thermal stability in SNN-based tungsten bronze ceramics through substitution strategy

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  40. Active and passive defects in tetragonal tungsten bronze relaxor ferroelectrics

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  41. Enhancing Comprehensive Energy Storage Properties in Tungsten Bronze Sr 0.53 Ba 0.47 Nb 2 O 6 -Based Lead-free Ceramics by B-Site Doping and Relaxor Tuning

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  42. Role of coordination site in governing the structural, electronic and optical properties of Ca-doped strontium barium niobate

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  43. Cation Disorder in Ferroelectric Ba4M2Nb10O30 (M = Na, K, and Rb) Tetragonal Tungsten Bronzes

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  44. Remarkable energy storage performances of tungsten bronze Sr0.53Ba0.47Nb2O6-based lead-free relaxor ferroelectric for high-temperature capacitors application

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  45. Centrosymmetric Tetragonal Tungsten Bronzes A4Bi2Nb10O30 (A = Na, K, Rb) with a Bi 6s Lone Pair

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  46. Superior Energy Density Achieved in Unfilled Tungsten Bronze Ferroelectrics via Multiscale Regulation Strategy

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    Haonan Peng, Zhen Liu, Zhengqian Fu, Kai Dai, Zhongqian Lv, Shaobo Guo, Zhigao Hu, Fangfang Xu, Genshui Wang

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  47. Enhanced energy storage properties on calcium modified strontium barium niobate lead-free ferroelectric relaxor ceramics

    Journal of Materials Science Materials in Electronics · 2023-06-01

    Shaobo Guo, Zhen Liu, Chunhua Yao, Fei Cao, Genshui Wang

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  48. A-Site Cation Disorder in SrxBa1–xNb2O6 (x = 0.25, 0.33, 0.50, 0.61) Studied by High-Resolution Resonant X-ray Powder Diffraction

    ACS Omega · 2023-09-29

    Ola G. Grendal, Andrew Nicholas Fitch, Solveig Stubmo Aamlid

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  49. Effect of sodium substitution by yttrium on the structural, dielectric and electrical properties of Ba2Na(1-3x)YxNb5O15 ceramics

    Heliyon · 2023-10-17

    El Hassan Yahakoub, Amine Bendahhou, Ilyas Jalafi, Fatima Chaou, Soufian EL Barkany, Zahra Bahari, Mohamed Abou-Salama

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  50. Synthesis and characterization of (Ba (1.6-3/2X) Sr2.4Na2Nb10O30: xHo3+) ferroelectric nanomaterials by solid state reaction routes for device applications

    Solid State Sciences · 2023-10-31

    Solomon H. Didu, Menberu Mengesha Woldemariam, Shimelis A. Kitte, Shimelis L. Beshawured, S. Bheemeswara Rao, Nebiyu Gemechu Debelo

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