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RESEARCH PAPER · Angewandte Chemie International Edition · 2014

A Displacive‐Type Metal Crown Ether Ferroelectric Compound: Ca(NO3)2(15‐crown‐5)

Heng‐Yun Ye, Yi Zhang, Da‐Wei Fu, Ren‐Gen Xiong

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A Displacive‐Type Metal Crown Ether Ferroelectric Compound: Ca(NO3)2(15‐crown‐5)OriginalPhase transitions and dielectric properties of a hexagonal ABX 3 perovskite-type organic–inorganic hybrid compound: [C 3 H 4 NS][CdBr 3 ]66Hydrogen-Bonded Displacive-Type Ferroelastic Phase Transition in a New Entangled Supramolecular Compound30A Resistance-Switchable and Ferroelectric Metal–Organic Framework119A high-temperature supramolecular-based switchable dielectric material with electrical bistability between high and low dielectric states17Crystal structures, phase transitions, and switchable dielectric behaviors: comparison of a series of N-heterocyclic ammonium perchlorates24Reversible Phase Transitions and Dielectric Properties in [(CH3)4P]2[Cr2O7] and [Et4P]2[Cr3O10]8Potentially Ferroelectric {CuIIL2} n Based Two-Dimensional Framework Exhibiting High Polarization and Guest-Assisted Dielectric Anomaly33Anomalous Dielectric Features and Structural Implications in Gallic Acid–Isoniazid Cocrystal Mediated by Lattice Water16Enhanced electrocaloric effect in displacive-type organic ferroelectrics3Phase transition metal–crown ether coordination compounds tuned by metal ions20A spiro-type ammonium based switchable dielectric material with two sequential reversible phase transitions above room temperature15Dibenzylammonium trichloroacetate: an above-room-temperature order–disorder switchable dielectric material16Polyether complexes of groups 13 and 1450Symmetry breaking in molecular ferroelectrics693Molecular Ferroelectric Pyridin-4-ylmethanaminium Perchlorate Undergoes Paraelectric–Ferroelectric and Ferroelectric–Ferroelectric Phase Transitions23New Molecular Ferroelectrics Accompanied by Ultrahigh Second-Harmonic Generation31Unusual Sequential Reversible Phase Transitions Containing Switchable Dielectric Behaviors in Cyclopentyl Ammonium 18-Crown-6 Perchlorate110Alcohol‐Mediated Resistance‐Switching Behavior in Metal–Organic Framework‐Based Electronic Devices92Alcohol‐Mediated Resistance‐Switching Behavior in Metal–Organic Framework‐Based Electronic Devices23Dynamic molecular crystals with switchable physical properties893Sequential Phase Transitions Near Room Temperature in a Metal–Crown Ether Compound SbBr 3 (15‐Crown‐5)7Optoelectronic Duple Bistable Switches: A Bulk Molecular Single Crystal and Unidirectional Ultraflexible Thin Film Based on Imidazolium Fluorochromate89Unusual Two–step Switchable Dielectric Behaviors and FerroelasticPhase Transition in a Simple 18‐Crown‐6 Clathrate18A semiconducting molecular ferroelectric with a bandgap much lower than that of BiFeO371Fast and slow integrated single-molecule dual dielectric switch based on a crystal/flexible thin film27Reversible structural phase transition, ferroelectric and switchable dielectric properties of an adduct molecule of hexamethylenetetramine ferrocene carboxylic acid23Tunable Dielectric Responses Triggered by Dimensionality Modification in Organic–Inorganic Hybrid Phase Transition Compounds (C5H6N)CdnCl2n+1 (n = 1 and 2)24Electrophilic Cyclization and Intermolecular Acetalation of 2-(4-Hydroxybut-1-yn-1-yl)benzaldehydes: Synthesis of Diiodinated Diepoxydibenzo[c,k][1,9]dioxacyclohexadecines8Structural phase transition-associated dielectric transition and ferroelectricity in coordination compounds166The Narrowest Band Gap Ever Observed in Molecular Ferroelectrics: Hexane‐1,6‐diammonium Pentaiodobismuth(III)118The Narrowest Band Gap Ever Observed in Molecular Ferroelectrics: Hexane‐1,6‐diammonium Pentaiodobismuth(III)78[(18‐Crown‐6)K][Fe(1)Cl(1)4]0.5[Fe(2)Cl(2)4]0.5: A Multifunctional Molecular Switch of Dielectric, Conductivity and Magnetic Properties11A Molecular Ferroelectric Showing Room‐Temperature Record‐Fast Switching of Spontaneous Polarization38A Molecular Ferroelectric Showing Room‐Temperature Record‐Fast Switching of Spontaneous Polarization15Monocycle‐like Molecular Rotor Induces a Dielectric Relaxation and Dielectric Phase Transformation in an Organic–Inorganic Hybrid Supermolecule4Metal-free three-dimensional perovskite ferroelectrics811Chiral to Chiral Phase Transition in a Novel Hydrogen Bond Type Molecular Ferroelectric7Ferroelectric Property, Switchable Dielectric, and Excellent Second Harmonic Generation Response in a Homochiral Organic Salt: l -Prolinammonium 1-Adamantane Carboxylate13High-temperature phase transitions, switchable dielectric behaviors and barocaloric effects in three new organic molecule-based crystals9Record-high thermal stability achieved in a novel single-component all-organic ferroelectric crystal exhibiting polymorphism18Insights on the Jahn–Teller distortion, hydrogen bonding and local-environment correlations in a promised multiferroic hybrid perovskite5An Above-Room-Temperature Molecular Ferroelectric: [Cyclopentylammonium]2CdBr461Enhancing switchable dielectric property for crystalline supramolecular rotor compounds by adding polar components7Structural Modulation of Electrically Conducting TCNQ Salts Using Na+(crown ether) Supramolecular Cations14Discovery of New Polymorphs of Gallium Oxides with Particle Swarm Optimization‐Based Structure Searches34Energy Harvesting and Pd(II) Sorption Based on Organic–Inorganic Hybrid Perovskites37A high- T c organic-ionic phase transition crystal obtained from a trivalent cation2Ten-Membered Rings or Larger With One or More Oxygen Atoms0Room-temperature dielectric switching in a host–guest crown ether inclusion complex27Record Enhancement of Curie Temperature in Host–Guest Inclusion Ferroelectrics104The First High‐Temperature Supramolecular Radical Ferroics58The First High‐Temperature Supramolecular Radical Ferroics4Effective Na+-Binding Ability and Molecular Assembly of an Alkylamide-Substituted Penta(ethylene)glycol Derivative0An Order–Disorder Type High‐Temperature Multiaxial Supramolecular Ferroelectric25Crown Ether Host‐Guest Molecular Ferroelectrics54A ferroelastic molecular rotator [(Me 2 N(CH 2 ) 2 NH 3 )(18-crown-6)]triflate with dual dielectric switches20A new crown-ether clathrate [15-crown-5][Y(NO 3 ) 2 (H 2 O) 5 ][NO 3 ] with switchable dielectric constant behaviour2Tetranitro- and tetraamino-dibenzo[18]crown-6-ether derivatives: complexes for alkali metal ions, redox potentials, crystal structures, molecular sorption, and proton conducting behaviours2Zero-Dimensional Molecular Ferroelectrics with Significant Nonlinear Effect and Giant Entropy33Fast switching of spontaneous polarization in a microporous molecular rotor ferroelectric3High temperature switchable dielectric properties in molecular crystal material 1,4,7-triazacyclononane trihydrochloride7Revealing the order–disorder type phase transition mechanism in two new supramolecular clathrates1Nonlinear Optical Switching Driven by the Lone Pair Electron Effect in a Hybrid Compound: (1S, 4S)‐(+)‐2‐Aza‐5‐oxabicyclo[2.2.1] heptane)2[SbCl5]2Crystal Sponge Behavior in a Two-Dimensional Rare-Earth Hybrid Coordinate Polymer14A Metal‐Free Molecular Ferroelectric [4‐Me‐cyclohexylamine]ClO4 Introduced by Boat and Chair Conformations of Cyclohexylamine5Multifunctional single-component organic molecular materials: ferroelectricity, negative thermal expansion, and polymorphism9Possible Perovskite Substitutes, Advances, and Future Prospects5The past 10 years of molecular ferroelectrics: structures, design, and properties173Order–disorder structural phase transition and dielectric–ferroelectric properties of a host-guest methionine–crown ether inclusion complex7Lead‐free halide perovskites for optoelectronic application: investigation of morphological, optical and electrical conductivity1Supramolecular Rotor Assembly for the Design of a Hybrid Ferroelectric‐Antiferromagnetic Multiferroic Semiconductor0Supramolecular Rotor Assembly for the Design of a Hybrid Ferroelectric‐Antiferromagnetic Multiferroic Semiconductor9The First Kleinman‐type Second‐Harmonic Generation Circular Dichroism On/Off Switchable Ferroelectrics28The First Kleinman‐type Second‐Harmonic Generation Circular Dichroism On/Off Switchable Ferroelectrics4A Lithium Complex Ferroelectric with High Curie Temperature: [Li(1,10-Phenanthroline)2]I1Synthesis and properties of L-arginine crown ether type supramolecular phase change materials0Tellurium‐Containing Crown Ether Nanozyme with Robust Redox Adaptability and Potent Glutathione Peroxidase‐Like Activity0Structural insights, dielectric behavior, and third-order nonlinear optical properties of a supramolecular cocrystal of [(3-acetyl-1-methylpyridinium)2 (18-crown-6)] diiodide0Asymmetric Coordination Designed Heterocrown Ether Host–Guest Ferroelectrics with Ultrahigh Tc10Water‐Triggered Domino‐Like Phase Transition in a Molecular Ferroelectric1

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  1. Phase transitions and dielectric properties of a hexagonal ABX 3 perovskite-type organic–inorganic hybrid compound: [C 3 H 4 NS][CdBr 3 ]

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  2. Hydrogen-Bonded Displacive-Type Ferroelastic Phase Transition in a New Entangled Supramolecular Compound

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  3. A Resistance-Switchable and Ferroelectric Metal–Organic Framework

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  4. A high-temperature supramolecular-based switchable dielectric material with electrical bistability between high and low dielectric states

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  5. Crystal structures, phase transitions, and switchable dielectric behaviors: comparison of a series of N-heterocyclic ammonium perchlorates

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  6. Reversible Phase Transitions and Dielectric Properties in [(CH3)4P]2[Cr2O7] and [Et4P]2[Cr3O10]

    European Journal of Inorganic Chemistry · 2015-06-25

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  7. Potentially Ferroelectric {CuIIL2} n Based Two-Dimensional Framework Exhibiting High Polarization and Guest-Assisted Dielectric Anomaly

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  8. Anomalous Dielectric Features and Structural Implications in Gallic Acid–Isoniazid Cocrystal Mediated by Lattice Water

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  9. Enhanced electrocaloric effect in displacive-type organic ferroelectrics

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  10. Phase transition metal–crown ether coordination compounds tuned by metal ions

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  11. A spiro-type ammonium based switchable dielectric material with two sequential reversible phase transitions above room temperature

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  12. Dibenzylammonium trichloroacetate: an above-room-temperature order–disorder switchable dielectric material

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  13. Polyether complexes of groups 13 and 14

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  15. Molecular Ferroelectric Pyridin-4-ylmethanaminium Perchlorate Undergoes Paraelectric–Ferroelectric and Ferroelectric–Ferroelectric Phase Transitions

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  16. New Molecular Ferroelectrics Accompanied by Ultrahigh Second-Harmonic Generation

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  17. Unusual Sequential Reversible Phase Transitions Containing Switchable Dielectric Behaviors in Cyclopentyl Ammonium 18-Crown-6 Perchlorate

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  18. Alcohol‐Mediated Resistance‐Switching Behavior in Metal–Organic Framework‐Based Electronic Devices

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  19. Alcohol‐Mediated Resistance‐Switching Behavior in Metal–Organic Framework‐Based Electronic Devices

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  20. Dynamic molecular crystals with switchable physical properties

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  21. Sequential Phase Transitions Near Room Temperature in a Metal–Crown Ether Compound SbBr 3 (15‐Crown‐5)

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  22. Optoelectronic Duple Bistable Switches: A Bulk Molecular Single Crystal and Unidirectional Ultraflexible Thin Film Based on Imidazolium Fluorochromate

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  23. Unusual Two–step Switchable Dielectric Behaviors and FerroelasticPhase Transition in a Simple 18‐Crown‐6 Clathrate

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  24. A semiconducting molecular ferroelectric with a bandgap much lower than that of BiFeO3

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  27. Tunable Dielectric Responses Triggered by Dimensionality Modification in Organic–Inorganic Hybrid Phase Transition Compounds (C5H6N)CdnCl2n+1 (n = 1 and 2)

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  30. The Narrowest Band Gap Ever Observed in Molecular Ferroelectrics: Hexane‐1,6‐diammonium Pentaiodobismuth(III)

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  32. [(18‐Crown‐6)K][Fe(1)Cl(1)4]0.5[Fe(2)Cl(2)4]0.5: A Multifunctional Molecular Switch of Dielectric, Conductivity and Magnetic Properties

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  34. A Molecular Ferroelectric Showing Room‐Temperature Record‐Fast Switching of Spontaneous Polarization

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  35. Monocycle‐like Molecular Rotor Induces a Dielectric Relaxation and Dielectric Phase Transformation in an Organic–Inorganic Hybrid Supermolecule

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  37. Chiral to Chiral Phase Transition in a Novel Hydrogen Bond Type Molecular Ferroelectric

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  40. Record-high thermal stability achieved in a novel single-component all-organic ferroelectric crystal exhibiting polymorphism

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  49. Room-temperature dielectric switching in a host–guest crown ether inclusion complex

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  50. Record Enhancement of Curie Temperature in Host–Guest Inclusion Ferroelectrics

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