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RESEARCH PAPER · Chemical Reviews · 2011

Rational Synthesis of Noncentrosymmetric Metal–Organic Frameworks for Second-Order Nonlinear Optics

Cheng Wang, Teng Zhang, Wenbin Lin

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Rational Synthesis of Noncentrosymmetric Metal–Organic Frameworks for Second-Order Nonlinear OpticsOriginalA luminescent nanoscale metal–organic framework with controllable morphologies for spore detection152Functionalizing the pore wall of chiral porous metal–organic frameworks by distinct –H, –OH, –NH2, –NO2, –COOH shutters showing selective adsorption of CO2, tunable photoluminescence, and direct white-light emission149Metal–organic frameworks in mixed-matrix membranes for gas separation495Methane storage in advanced porous materials812Microporous metal–organic frameworks for storage and separation of small hydrocarbons322Metal‐Organic Framework Templated Synthesis of Fe2O3/TiO2 Nanocomposite for Hydrogen Production445Synthesis and Photophysical Investigation of a Series of Push–Pull Arylvinyldiazine Chromophores161NH 2 -MIL-53(Al): A High-Contrast Reversible Solid-State Nonlinear Optical Switch171Switching Kr/Xe Selectivity with Temperature in a Metal–Organic Framework202Selective Metal Cation Capture by Soft Anionic Metal–Organic Frameworks via Drastic Single-Crystal-to-Single-Crystal Transformations128Second‐Order Nonlinear Optical Activity Induced by Ordered Dipolar Chromophores Confined in the Pores of an Anionic Metal–Organic Framework299Control of Porosity by Using Isoreticular Zeolitic Imidazolate Frameworks (IRZIFs) as a Template for Porous Carbon Synthesis133Uranyl Bearing Hybrid Materials: Synthesis, Speciation, and Solid-State Structures418Crystal Engineering of a Microporous, Catalytically Active fcu Topology MOF Using a Custom‐Designed Metalloporphyrin Linker158A porous coordination framework for highly sensitive and selective solid-phase microextraction of non-polar volatile organic compounds200Metal–Organic Frameworks for Light Harvesting and Photocatalysis802Metal–Organic Frameworks and Self-Assembled Supramolecular Coordination Complexes: Comparing and Contrasting the Design, Synthesis, and Functionality of Metal–Organic Materials2950From metal–organic framework (MOF) to MOF–polymer composite membrane: enhancement of low-humidity proton conductivity379Structures, Sorption Characteristics, and Nonlinear Optical Properties of a New Series of Highly Stable Aluminum MOFs436Applications of magnetic metal–organic framework composites316CdS-decorated UiO–66(NH2) nanocomposites fabricated by a facile photodeposition process: an efficient and stable visible-light-driven photocatalyst for selective oxidation of alcohols300Highly porous and stable metal–organic frameworks for uranium extraction598Metal–organic frameworks as platforms for clean energy970Mineral neogenesis as an inspiration for mild, solvent-free synthesis of bulk microporous metal–organic frameworks from metal (Zn, Co) oxides149Multifunctional NH2-mediated zirconium metal–organic framework as an efficient visible-light-driven photocatalyst for selective oxidation of alcohols and reduction of aqueous Cr(vi)439Quantum chemical design of nonlinear optical materials by sp2-hybridized carbon nanomaterials: issues and opportunities176Water Sorption Cycle Measurements on Functionalized MIL-101Cr for Heat Transformation Application275Zr- and Hf-Based Metal–Organic Frameworks: Tracking Down the Polymorphism332Self‐Assembled Organic Microfibers for Nonlinear Optics146Reactivity of Surface Species in Heterogeneous Catalysts Probed by In Situ X-ray Absorption Techniques643Chiral Coordination Polymers with SHG-Active and Luminescence: An Unusual Homochiral 3D MOF Constructed from Achiral Components164Tracking the Formation of a Polynuclear Co 16 Complex and Its Elimination and Substitution Reactions by Mass Spectroscopy and Crystallography176Thermochemistry of Paddle Wheel MOFs: Cu-HKUST-1 and Zn-HKUST-1124Solid‐State Reversible Quadratic Nonlinear Optical Molecular Switch with an Exceptionally Large Contrast157Highly Selective Luminescent Sensing of Fluoride and Organic Small-Molecule Pollutants Based on Novel Lanthanide Metal–Organic Frameworks319Metal–Organic Frameworks as A Tunable Platform for Designing Functional Molecular Materials981Selective anion exchange with nanogated isoreticular positive metal-organic frameworks370Direct visualization of a guest-triggered crystal deformation based on a flexible ultramicroporous framework128Construction of Ultrastable Porphyrin Zr Metal–Organic Frameworks through Linker Elimination1126Metal–Organic Frameworks as Biomimetic Catalysts283A Highly Symmetric Metal–Organic Framework Based on a Propeller-Like Ru-Organic Metalloligand for Photocatalysis and Explosives Detection118Lanthanide Metal–Organic Frameworks Showing Luminescence in the Visible and Near‐Infrared Regions with Potential for Acetone Sensing137Phase Transitions, Prominent Dielectric Anomalies, and Negative Thermal Expansion in Three High Thermally Stable Ammonium Magnesium–Formate Frameworks143Growing Crystalline Zinc-1,3,5-benzenetricarboxylate Metal–Organic Frameworks in Different Surfactants165Luminescent metal–organic frameworks for chemical sensing and explosive detection4169From Hydrated Ni 3 (OH) 2 (C 8 H 4 O 4 ) 2 (H 2 O) 4 to Anhydrous Ni 2 (OH) 2 (C 8 H 4 O 4 ): Impact of Structural Transformations on Magnetic Properties297A malonitrile-functionalized metal-organic framework for hydrogen sulfide detection and selective amino acid molecular recognition117Microporous Metal–Organic Frameworks for Gas Separation197Beyond post-synthesis modification: evolution of metal–organic frameworks via building block replacement877Incorporating Polyoxometalates into a Porous MOF Greatly Improves Its Selective Adsorption of Cationic Dyes271Photoswitching CO 2 Capture and Release in a Photochromic Diarylethene Metal–Organic Framework272Photoswitching CO2 Capture and Release in a Photochromic Diarylethene Metal–Organic Framework222Coordination polymers with nucleobases: From structural aspects to potential applications119Biomimicry in metal–organic materials148Porous aromatic frameworks with anion-templated pore apertures serving as polymeric sieves155Unprecedented Second‐Timescale Blue/Green Emissions and Iodine‐Uptake‐Induced Single‐Crystal‐to‐Single‐Crystal Transformation in ZnII/CdII Metal–Organic Frameworks154Surfactant Media To Grow New Crystalline Cobalt 1,3,5-Benzenetricarboxylate Metal–Organic Frameworks159A Series of Highly Stable Mesoporous Metalloporphyrin Fe-MOFs452Porous Metal–Organic Frameworks for Gas Storage and Separation: What, How, and Why?636A Resistance-Switchable and Ferroelectric Metal–Organic Framework119Selective and Sensitive Aqueous‐Phase Detection of 2,4,6‐Trinitrophenol (TNP) by an Amine‐Functionalized Metal–Organic Framework334A Highly Stable Porphyrinic Zirconium Metal–Organic Framework with shp-a Topology431A new microporous anionic metal–organic framework as a platform for highly selective adsorption and separation of organic dyes192Water stabilization of Zr 6 -based metal–organic frameworks via solvent-assisted ligand incorporation131Recent advances on second-order NLO materials based on metal iodates328Bipyridine- and Phenanthroline-Based Metal–Organic Frameworks for Highly Efficient and Tandem Catalytic Organic Transformations via Directed C–H Activation289MOF Functionalization via Solvent-Assisted Ligand Incorporation: Phosphonates vs Carboxylates215Photosensitizing Metal–Organic Framework Enabling Visible-Light-Driven Proton Reduction by a Wells–Dawson-Type Polyoxometalate436Two-Photon Responsive Metal–Organic Framework205MOF based luminescence tuning and chemical/physical sensing337Porphyrinic metal-organic framework as electrochemical probe for DNA sensing via triple-helix molecular switch127Supramolecular-jack-like guest in ultramicroporous crystal for exceptional thermal expansion behaviour121Multifunctional Metal–Organic Frameworks for Photocatalysis615In Situ Construction of Three Anion-Dependent Cu(I) Coordination Networks as Promising Heterogeneous Catalysts for Azide–Alkyne “Click” Reactions125Inorganic nanocarriers for platinum drug delivery153Enhanced Photocatalytic Activity of MIL‐125 by Post‐Synthetic Modification with CrIII and Ag Nanoparticles118A Flexible Microporous Hydrogen-Bonded Organic Framework for Gas Sorption and Separation475Porphyrin-Metalation-Mediated Tuning of Photoredox Catalytic Properties in Metal–Organic Frameworks250Exploitation of Guest Accessible Aliphatic Amine Functionality of a Metal–Organic Framework for Selective Detection of 2,4,6-Trinitrophenol (TNP) in Water145Surfactants as Promising Media for the Preparation of Crystalline Inorganic Materials315Dual Exchange in PCN-333: A Facile Strategy to Chemically Robust Mesoporous Chromium Metal–Organic Framework with Functional Groups127High-energy metal–organic frameworks (HE-MOFs): Synthesis, structure and energetic performance336Robust, Chiral, and Porous BINAP-Based Metal–Organic Frameworks for Highly Enantioselective Cyclization Reactions161Crystal Facets Make a Profound Difference in Polyoxometalate-Containing Metal–Organic Frameworks as Catalysts for Biodiesel Production200Hybrid nanoparticles for combination therapy of cancer174One-Step Synthesis of Nanoscale Zeolitic Imidazolate Frameworks with High Curcumin Loading for Treatment of Cervical Cancer247Biomimetic Replication of Microscopic Metal–Organic Framework Patterns Using Printed Protein Patterns118A viologen-functionalized chiral Eu-MOF as a platform for multifunctional switchable material179Pyrazolate-Based Porphyrinic Metal–Organic Framework with Extraordinary Base-Resistance419Metal organic frameworks mimicking natural enzymes: a structural and functional analogy477Metal–organic frameworks as competitive materials for non-linear optics312Rational construction of functional molybdenum (tungsten)–copper–sulfur coordination oligomers and polymers from preformed cluster precursors127Sensing-functional luminescent metal–organic frameworks178Robust and Porous β-Diketiminate-Functionalized Metal–Organic Frameworks for Earth-Abundant-Metal-Catalyzed C–H Amination and Hydrogenation178Hierarchical Integration of Photosensitizing Metal–Organic Frameworks and Nickel‐Containing Polyoxometalates for Efficient Visible‐Light‐Driven Hydrogen Evolution276Azulene-based organic functional molecules for optoelectronics141Metal–Organic Framework Nodes Support Single-Site Magnesium–Alkyl Catalysts for Hydroboration and Hydroamination Reactions264Emerging Multifunctional Metal–Organic Framework Materials1587Optical Properties of Hybrid Organic‐Inorganic Materials and their Applications345Nonlinear Optical Materials for the Smart Filtering of Optical Radiation941Multifunctional Luminescent Eu(III)-Based Metal–Organic Framework for Sensing Methanol and Detection and Adsorption of Fe(III) Ions in Aqueous Solution225Centimetre-scale micropore alignment in oriented polycrystalline metal–organic framework films via heteroepitaxial growth363Nonlinear optical properties, upconversion and lasing in metal–organic frameworks683Retracted Article: Potential applications of functional porous organic polymer materials123Incorporation of Molecular Catalysts in Metal–Organic Frameworks for Highly Efficient Heterogeneous Catalysis353Visible-light reduction CO2 with dodecahedral zeolitic imidazolate framework ZIF-67 as an efficient co-catalyst637Ground-State versus Excited-State Interchromophoric Interaction: Topology Dependent Excimer Contribution in Metal–Organic Framework Photophysics159Significant Enhancement of C2H2/C2H4 Separation by a Photochromic Diarylethene Unit: A Temperature‐ and Light‐Responsive Separation Switch168Multivariate Metal–Organic Frameworks as Multifunctional Heterogeneous Asymmetric Catalysts for Sequential Reactions265The coordination chemistry of N-heterocyclic carboxylic acid: A comparison of the coordination polymers constructed by 4,5-imidazoledicarboxylic acid and 1H-1,2,3-triazole-4,5-dicarboxylic acid124Nanoscale metal–organic frameworks for phototherapy of cancer420Epitaxial growth and applications of oriented metal–organic framework thin films179Recent advances in gas storage and separation using metal–organic frameworks1571A mechanistic approach towards the photocatalytic organic transformations over functionalised metal organic frameworks: a review138Covalent Organic Frameworks and Cage Compounds: Design and Applications of Polymeric and Discrete Organic Scaffolds528New synthetic strategies to prepare metal–organic frameworks306Photonic functional metal–organic frameworks661Synthesis, functionalization, and applications of metal–organic frameworks in biomedicine242Towards high-efficiency sorptive capture of radionuclides in solution and gas149Designed fabrication of biomimetic metal–organic frameworks for catalytic applications172Enhanced Photodynamic Therapy by Reduced Levels of Intracellular Glutathione Obtained By Employing a Nano‐MOF with CuII as the Active Center328Green Approach To Synthesize Crystalline Nanoscale ZnII-Coordination Polymers: Cell Growth Inhibition and Immunofluorescence Study119Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals258Luminescent Lanthanide MOFs: A Unique Platform for Chemical Sensing235Nanoscale Metal–Organic Frameworks for Therapeutic, Imaging, and Sensing Applications692Excited-State Electronic Properties in Zr-Based Metal–Organic Frameworks as a Function of a Topological Network152Chiral Lead Halide Perovskite Nanowires for Second-Order Nonlinear Optics379Pore surface engineering of metal–organic frameworks for heterogeneous catalysis214Photoluminescent, upconversion luminescent and nonlinear optical metal-organic frameworks: From fundamental photophysics to potential applications206Ratiometric Monitoring of Thorium Contamination in Natural Water Using a Dual-Emission Luminescent Europium Organic Framework120Exceptional adsorption of arsenic by zirconium metal-organic frameworks: Engineering exploration and mechanism insight320Photofunctional MOF-based hybrid materials for the chemical sensing of biomarkers135Cancer-Cell-Activated Photodynamic Therapy Assisted by Cu(II)-Based Metal–Organic Framework248Bulk Photovoltaic Effect in a Pair of Chiral–Polar Layered Perovskite-Type Lead Iodides Altered by Chirality of Organic Cations193Tuning the Molecular and Cationic Affinity in a Series of Multifunctional Metal–Organic Frameworks Based on Dodecanuclear Zn(II) Carboxylate Wheels1202D organic‐inorganic hybrid perovskite materials for nonlinear optics131Recent Progress in 2D Metal‐Organic Frameworks for Optical Applications149Recent progress in lanthanide metal–organic frameworks and their derivatives in catalytic applications189Applications of nanoscale metal–organic frameworks as imaging agents in biology and medicine136Metal–organic frameworks as catalytic selectivity regulators for organic transformations254Stimuli-responsive metal–organic framework nanoparticles for controlled drug delivery and medical applications308Syntheses, design strategies, and photocatalytic charge dynamics of metal–organic frameworks (MOFs): a catalyzed photo-degradation approach towards organic dyes218Two-dimensional MOF and COF nanosheets for next-generation optoelectronic applications190Two-Dimensional Metal-Organic Framework Materials: Synthesis, Structures, Properties and Applications928Nonlinear Optical Properties and Applications of Fluorenone Molecular Materials161Third-Order Nonlinear Optical Behavior of an Amide-Tricarboxylate Zinc(II) Metal–Organic Framework with Two-Fold 3D+3D Interpenetration140Porous metal–organic frameworks for hydrogen storage179Chiral Metal–Organic Frameworks579Chiral metal–organic frameworks for photonics133Applications of macrocycle-based solid-state host–guest chemistry179

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