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RESEARCH ARTICLE · Journal of the American Chemical Society · 1990

A well-defined rhenium(VII) olefin metathesis catalyst

Robert Toreki, Richard R. Schrock

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A well-defined rhenium(VII) olefin metathesis catalystOriginalChemInform Abstract: A Well‐Defined Rhenium(VII) Olefin Metathesis Catalyst.0Homogeneous Catalysis of Organic Reactions by Transition Metal Complexes5Recent Advances in the Chemistry of “ d 0 ” Alkylidene and Metallacyclobutane Complexes152Recent Advances in the Chemistry of Metal-Carbon Triple Bonds174Chemie Anorganische Chemie 19901Sterically Demanding Fluorinated Substituents and Metal Fluorides with Bulky Ligands28Transition metals in organic synthesis annual survey covering the year 199013Nitrido Complexes of Transition Metals225Nitrido‐Komplexe von Übergangsmetallen132Novel catalysts for the ring‐opening metathesis polymerization of norbornene‐type monomers27Organorhenium Chemistry32Ligand variation in alkylidene complexes of the type Mo(CHR)(NR′)(OR″)2222Homogeneous Catalysis of Organic Reactions by Transition Metal Complexes4Metathesis Polymerization: ROMPing towards new materials45Molecular heterogeneous metathesis catalysts: an attempted synthesis of surface-anchored alkylidenetungsten complexes39High-valent Organorhenium Compounds10New homogeneous rhenium-based metathesis catalysts as models of the rhenium on alumina heterogeneous catalyst25Transition Metals in Polymer Synthesis: Ring-opening Metathesis Polymerization and Other Transition Metal Polymerization Techniques16Living and stereoselective polymerization of [2.2]‐paracyclophan‐2‐ENE derivatives6The alkoxide ligand in olefin and acetylene metathesis reactions206Ring-Closing Metathesis and Related Processes in Organic Synthesis1051Synthesis and Reactions of Tungsten Oxo Vinylalkylidene Complexes: Reactions of WCl2(O)(PX3) (X = OMe, R) Precursors with 3,3-Diphenylcyclopropene61Rhenium(VII) Oxo−Alkyl Complexes: Reductive and α-Elimination Reactions35XANES studies on rhenium L absorption edges of Re2O7 graphite intercalation compounds and of other rhenium-oxygen compounds25Structure determination of a rhenium trimethylsilylmethyl acyl complex and hydrolysis of the carbon-silicon bond5Accessibility of 17-Electron Structures for Cyclopentadienylchromium(III) Compounds. 1. Experimental Studies on the Dichloride and Dimethyl Compounds24Bibliography0Bis[hydrazido(2−)] and related complexes of molybdenum(VI): towards alkene-metathesis catalysts based on hydrazido(2−) ligation10Ethylene Polymerization with Half-Sandwich Allyl Imido Complexes of Tantalum56Theoretical Studies on Alkene Addition to Molybdenum Alkylidenes72Block Copolymers by Transformation of Living Ring-Opening Metathesis Polymerization into Controlled/“Living” Atom Transfer Radical Polymerization152Alkene metathesis: new developments in catalyst design and application82Palladium carbonyl complexes67Ab Initio Study of Structures, Energetics, and Bonding in Formally High-Oxidation-State Copper Organometallics25Hydrogen Migration and HCl Elimination Promoted by Metal-Centered Nucleophilic Attack on Osmium Hydrido−Carbynes34Synthesis of cis- and trans-ReOMe2(bipy)Cl and related cationic oxorhenium(V) complexes14Organo transition metal initiated living polymerizations126Synthesis and properties of homogeneous models of the Re2O7/Al2O3 metathesis catalyst12A Highly Active Well-Defined Rhenium Heterogeneous Catalyst for Olefin Metathesis Prepared via Surface Organometallic Chemistry206High Oxidation State Multiple Metal−Carbon Bonds888Activation of the Re2O7/Al2O3 metathesis catalyst by aryloxyaluminium complexes9Synthesis of Molybdenum Carbene Complexes of Thiophene Derivatives26Metathesis – Homogeneous0Re‐Based Heterogeneous Catalysts for Olefin Metathesis Prepared by Surface Organometallic Chemistry: Reactivity and Selectivity93Ferrocene-based ligands in ruthenium alkylidene chemistry14Metallaoxetanes and Carbenes from Diolates in High‐Valent Rhenium Oxo Chemistry: The Importance of the Coordination Number52Metallaoxetanes and Carbenes from Diolates in High‐Valent Rhenium Oxo Chemistry: The Importance of the Coordination Number8ADMET Polymerization26The Discovery and Development of High Oxidation State Mo and W Imido Alkylidene Complexes for Alkene Metathesis38Heterogeneous well-defined catalysts for metathesis of inert and not so inert bonds45Mass Spectrometric Study of the Conversion of Rhenium Diolates to Metallaoxetanes and Carbenes. Coordination Number, Polar, and Steric Effects29Understanding Structural and Dynamic Properties of Well-Defined Rhenium-Based Olefin Metathesis Catalysts, Re(⋮CR)(CHR)(X)(Y), from DFT and QM/MM Calculations63Metathesereaktionen in der Totalsynthese334Metathesis Reactions in Total Synthesis1181d0 Re-Based Olefin Metathesis Catalysts, Re(⋮CR)(CHR)(X)(Y): The Key Role of X and Y Ligands for Efficient Active Sites162Surface versus Molecular Siloxy Ligands in Well‐Defined Olefin Metathesis Catalysts: [{(RO)3SiO}Mo(NAr)(CHtBu)(CH2tBu)]166Surface versus Molecular Siloxy Ligands in Well‐Defined Olefin Metathesis Catalysts: [{(RO)3SiO}Mo(NAr)(CHtBu)(CH2tBu)]42Unprecedented ROMP Activity of Low‐Valent Rhenium–Nitrosyl Complexes: Mechanistic Evaluation of an Electrophilic Olefin Metathesis System35Reactions of M(N-2,6-i-Pr2C6H3)(CHR)(CH2R‘)2 (M = Mo, W) Complexes with Alcohols To Give Olefin Metathesis Catalysts of the Type M(N-2,6-i-Pr2C6H3)(CHR)(CH2R‘)(OR‘ ‘)44Carbosilane dendrimers containing peripheral cyclopentadienyl niobium- and tantalum-imido complexes13Olefin metathesis for metal incorporation: Preparation of conjugated ruthenium-containing complexes and polymers12Mechanistic transformations involving living and controlled/living polymerization methods339Design and understanding of heterogeneous alkene metathesis catalysts83Strategies to Immobilize Well‐Defined Olefin Metathesis Catalysts: Supported Homogeneous Catalysis vs. Surface Organometallic Chemistry214Segmented Copolymers by Mechanistic Transformations9Strategies to Immobilize Well‐Defined Olefin Metathesis Catalysts: Supported Homogeneous Catalysis vs. Surface Organometallic Chemistry180The remarkable metal-catalysed olefin metathesis reaction1007Molecular understanding of Re-based heterogeneous olefin metathesis catalysts0Comparison of olefin metathesis by rhenium-containing γ-alumina or silica–aluminas and by some mesoporous analogues29Synthesis and reactivity of an unprecedented osmium(VIII) alkylidene5Functional end groups for polymers prepared using ring-opening metathesis polymerization228Olefin Metathesis Catalysts Containing Acyclic Diaminocarbenes73Rhenium Carbyne and η2-Vinyl Complexes from One-Pot Reactions of ReH5(PMe2Ph)3 with Terminal Alkynes30ADMET: Metathesis polycondensation109Alkene Metathesis0Well-Defined Block Copolymers12Hydrogen Shift Reactions of Rhenium Hydrido Carbyne Complexes18Block Copolymers by Multi‐Mode Polymerizations0Bipyridine Adducts of Molybdenum Imido Alkylidene and Imido Alkylidyne Complexes27Telechelic oligomers obtained by metathetic degradation of both polyisoprene and styrene–butadiene rubbers. Applications for recycling waste tyre rubber39Synthesis and Biological Activity of Anticoagulant Heparan Sulfate Glycopolymers0Ligand Development Directed Towards Applications in Late Metal Catalysis0Formation of diamonds and other carbon phases upon the destruction of palladium carbonyl clusters1Metathesis and Polymerization13Acyclic diene metathesis polymerization and precision polymers25ADMET Polymerization25Insights from Computational Studies on d 0 Metal‐Catalyzed Alkene and Alkyne Metathesis and Related Reactions4Polymeric Materials – Well Defined Block Copolymers5N–H cleavage as a route to new pincer complexes of high-valent rhenium12Bridging the Gap between Industrial and Well‐Defined Supported Catalysts253Eine Brücke zwischen industriellen und wohldefinierten Trägerkatalysatoren41Metathesis0Computational Design of an Iron Catalyst for Olefin Metathesis33ADMET polymers: synthesis, structure elucidation, and function48Preparation and activity of ruthenium catalyst based on β-cyclodextrin for ring-opening metathesis polymerization10Molybdenum0Olefin Metathesis by First‐Row Transition Metals34Diagonal Relationship among Organometallic Transition-Metal Complexes23Attempts at generating metathesis-active Fe(IV) and Co(IV) complexes via the reactions of (silox)2M(THF)2, [(silox)3M][Na(THF)2] (M = Fe, Co), and related species with propellanes and triphenylboron3Olefin Metathesis Catalyzed by a Hoveyda–Grubbs-like Complex Chelated to Bis(2-mercaptoimidazolyl) Methane: A Predictive DFT Study10On the ineffectiveness of grubbs-type iron olefin metathesis catalysts: Role of spin-state isomerism and cyclopropanation2Operando Spectroscopic Investigation of the Re2O7.2H2O Adduct obtained by Controlled Hydration of Re2O7.1Acyclic Diene Metathesis Polymerization Approach for Synthesis of Biobased Polyesters: Summary of Recent Reports4Recent advances in acyclic diene metathesis polymerization for the sustainable materials production0

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  1. ChemInform Abstract: A Well‐Defined Rhenium(VII) Olefin Metathesis Catalyst.

    ChemInform · 1990

    Robert Toreki, Richard R. Schrock

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  2. Homogeneous Catalysis of Organic Reactions by Transition Metal Complexes

    Springer eBooks · 1991

    MARTYN V. TWIGG

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  3. Recent Advances in the Chemistry of “ d 0 ” Alkylidene and Metallacyclobutane Complexes

    Progress in inorganic chemistry · 1991

    Jerald Feldman, Richard R. Schrock

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  4. Recent Advances in the Chemistry of Metal-Carbon Triple Bonds

    Advances in organometallic chemistry · 1991

    Andreas J. Mayr, Hans Martin Hoffmeister

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  5. Chemie Anorganische Chemie 1990

    Nachrichten aus Chemie Technik und Laboratorium · 1991

    Paul Binger, J. W. Richter

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  6. Sterically Demanding Fluorinated Substituents and Metal Fluorides with Bulky Ligands

    Progress in inorganic chemistry · 1992

    Michael Witt, Herbert W. Roesky

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  7. Transition metals in organic synthesis annual survey covering the year 1990

    Journal of Organometallic Chemistry · 1992

    Louis S. Hegedus

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  8. Nitrido Complexes of Transition Metals

    Angewandte Chemie International Edition in English · 1992

    Kurt Dehnicke, Joachim Strähle

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  9. Nitrido‐Komplexe von Übergangsmetallen

    Angewandte Chemie · 1992

    Kurt Dehnicke, Joachim Strähle

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  10. Novel catalysts for the ring‐opening metathesis polymerization of norbornene‐type monomers

    Journal of Applied Polymer Science · 1993

    BRIAN L. GOODALL, William J. Kroenke, Robert J. Minchak, Larry F. Rhodes

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  11. Organorhenium Chemistry

    Science · 1993

    Charles P. Casey

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  12. Ligand variation in alkylidene complexes of the type Mo(CHR)(NR′)(OR″)2

    Journal of Organometallic Chemistry · 1993

    John H. Oskam, Harold H. Fox, Kimo B. Yap, David H. McConville, Richard O'Dell, Bradley J. Lichtenstein, Richard R. Schrock

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  13. Homogeneous Catalysis of Organic Reactions by Transition Metal Complexes

    Springer eBooks · 1994

    MARTYN V. TWIGG

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  14. Metathesis Polymerization: ROMPing towards new materials

    Advanced Materials · 1994

    Vernon C. Gibson

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  15. Molecular heterogeneous metathesis catalysts: an attempted synthesis of surface-anchored alkylidenetungsten complexes

    Journal of the Chemical Society Dalton Transactions · 1994

    Regina Buffon, Michel Leconte, Agn�s Choplin, Jean‐Marie Basset

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  16. High-valent Organorhenium Compounds

    Elsevier eBooks · 1995

    David M. Hoffman

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  17. New homogeneous rhenium-based metathesis catalysts as models of the rhenium on alumina heterogeneous catalyst

    Journal of the Chemical Society Chemical Communications · 1995

    D. Commereuc

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  18. Transition Metals in Polymer Synthesis: Ring-opening Metathesis Polymerization and Other Transition Metal Polymerization Techniques

    Elsevier eBooks · 1995

    Jeffrey S. Moore

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  19. Living and stereoselective polymerization of [2.2]‐paracyclophan‐2‐ENE derivatives

    Macromolecular Symposia · 1995

    Yi‐Jun Miao, Benjamin J. Sun, Guillermo Carlos Bazan

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  20. The alkoxide ligand in olefin and acetylene metathesis reactions

    Polyhedron · 1995

    Richard R. Schrock

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  21. Ring-Closing Metathesis and Related Processes in Organic Synthesis

    Accounts of Chemical Research · 1995

    Robert Howard Grubbs, Scott J. Miller, Gregory C. Fu

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  22. Synthesis and Reactions of Tungsten Oxo Vinylalkylidene Complexes: Reactions of WCl2(O)(PX3) (X = OMe, R) Precursors with 3,3-Diphenylcyclopropene

    Organometallics · 1996

    F. Javier de la Mata, Robert Howard Grubbs

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  23. Rhenium(VII) Oxo−Alkyl Complexes: Reductive and α-Elimination Reactions

    Organometallics · 1996

    Shiang Cai, David M. Hoffman, Derk A. Wierda

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  24. XANES studies on rhenium L absorption edges of Re2O7 graphite intercalation compounds and of other rhenium-oxygen compounds

    Journal of Physics and Chemistry of Solids · 1996

    Michael Fröba, K. Lochte, Wolfgang Metz

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  25. Structure determination of a rhenium trimethylsilylmethyl acyl complex and hydrolysis of the carbon-silicon bond

    Polyhedron · 1996

    David M. Hoffman, Dimitrios Lappas, Derk A. Wierda

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  26. Accessibility of 17-Electron Structures for Cyclopentadienylchromium(III) Compounds. 1. Experimental Studies on the Dichloride and Dimethyl Compounds

    Organometallics · 1996

    James C. Fettinger, Sundeep P. Mattamana, Rinaldo Poli, Robin Don Rogers

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  27. Bibliography

    Elsevier eBooks · 1997

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  28. Bis[hydrazido(2−)] and related complexes of molybdenum(VI): towards alkene-metathesis catalysts based on hydrazido(2−) ligation

    Journal of the Chemical Society Dalton Transactions · 1997

    J.R. Dilworth, Vernon C. Gibson, Can‐Zhong Lu, John R. Miller, Carl Redshaw, Yifan Zheng

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  29. Ethylene Polymerization with Half-Sandwich Allyl Imido Complexes of Tantalum

    Organometallics · 1997

    David M. Antonelli, Ann E. Leins, Jeffrey M. Stryker

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  30. Theoretical Studies on Alkene Addition to Molybdenum Alkylidenes

    Journal of the American Chemical Society · 1997

    Yun‐Dong Wu, Zhi-Hui Peng

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  31. Block Copolymers by Transformation of Living Ring-Opening Metathesis Polymerization into Controlled/“Living” Atom Transfer Radical Polymerization

    Macromolecules · 1997

    Simion Coca, Hyun‐jong Paik, Krzysztof Aleksander Matyjaszewski

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  32. Alkene metathesis: new developments in catalyst design and application

    Coordination Chemistry Reviews · 1998

    C. Pariya, K. Narayanannair Jayaprakash, Amitabha Sarkar

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  33. Palladium carbonyl complexes

    Russian Chemical Reviews · 1998

    Tatiana A. Stromnova, Ilya I. Moiseev

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  34. Ab Initio Study of Structures, Energetics, and Bonding in Formally High-Oxidation-State Copper Organometallics

    Organometallics · 1998

    Jitendra K. Bera, Ashoka G. Samuelson, Jayaraman Chandrasekhar

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  35. Hydrogen Migration and HCl Elimination Promoted by Metal-Centered Nucleophilic Attack on Osmium Hydrido−Carbynes

    Organometallics · 1998

    Greg J. Spivak, Kenneth George Caulton

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  36. Synthesis of cis- and trans-ReOMe2(bipy)Cl and related cationic oxorhenium(V) complexes

    Journal of the Chemical Society Dalton Transactions · 1999

    June‐Ho Jung, Thomas A. Albright, David M. Hoffman, T. Randall Lee

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  37. Organo transition metal initiated living polymerizations

    Progress in Polymer Science · 2000

    Hajime Yasuda

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  38. Synthesis and properties of homogeneous models of the Re2O7/Al2O3 metathesis catalyst

    Journal of Molecular Catalysis A Chemical · 2000

    Gwenael Doledec, D. Commereuc

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  39. A Highly Active Well-Defined Rhenium Heterogeneous Catalyst for Olefin Metathesis Prepared via Surface Organometallic Chemistry

    Journal of the American Chemical Society · 2001

    Mathieu Chabanas, Anne Baudouin, Christophe Copéret, Jean‐Marie Basset

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  40. High Oxidation State Multiple Metal−Carbon Bonds

    Chemical Reviews · 2001

    Richard R. Schrock

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  41. Activation of the Re2O7/Al2O3 metathesis catalyst by aryloxyaluminium complexes

    Journal of Molecular Catalysis A Chemical · 2002

    D. Commereuc, Hélène Olivier‐Bourbigou, Virginie Kruger, Lucien Saussine

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  42. Synthesis of Molybdenum Carbene Complexes of Thiophene Derivatives

    Zeitschrift für anorganische und allgemeine Chemie · 2002

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  43. Metathesis – Homogeneous

    Encyclopedia of Catalysis · 2002

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  44. Re‐Based Heterogeneous Catalysts for Olefin Metathesis Prepared by Surface Organometallic Chemistry: Reactivity and Selectivity

    Chemistry - A European Journal · 2003

    Mathieu Chabanas, Christophe Copéret, Jean‐Marie Basset

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  45. Ferrocene-based ligands in ruthenium alkylidene chemistry

    Inorganic Chemistry Communications · 2003

    Ian R. Butler, Simon John Coles, Michael B. Hursthouse, Dilwyn J. Roberts, Naho Fujimoto

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  46. Metallaoxetanes and Carbenes from Diolates in High‐Valent Rhenium Oxo Chemistry: The Importance of the Coordination Number

    Angewandte Chemie International Edition · 2003

    Xueyi Chen, Xiangyang Zhang, Peter Chen

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  47. Metallaoxetanes and Carbenes from Diolates in High‐Valent Rhenium Oxo Chemistry: The Importance of the Coordination Number

    Angewandte Chemie · 2003

    Xueyi Chen, Xiangyang Zhang, Peter Chen

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  48. ADMET Polymerization

    Venue not supplied by source · 2003

    Stephen E. Lehman, Kenneth B. Wagener

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  49. The Discovery and Development of High Oxidation State Mo and W Imido Alkylidene Complexes for Alkene Metathesis

    Venue not supplied by source · 2003

    Richard R. Schrock

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  50. Heterogeneous well-defined catalysts for metathesis of inert and not so inert bonds

    Journal of Molecular Catalysis A Chemical · 2004

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