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RESEARCH PAPER · Journal of Materials Chemistry · 2006

Towards understanding, control and application of layered double hydroxide chemistry

Gareth R. Williams, Dermot M. O'Hare

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Towards understanding, control and application of layered double hydroxide chemistryOriginalInfluence of the Divalent Cation on the Thermal Activation and Reconstruction of Hydrotalcite-like Compounds69Selective Layer Reaction of Layer-by-Layer Assembled Layered Double-Hydroxide Nanocrystals79Catalysis by layered materials: A review397New Inorganic-Based Drug Delivery System of Indole-3-Acetic Acid-Layered Metal Hydroxide Nanohybrids with Controlled Release Rate244Molecular Dynamics Simulation of the Energetics and Structure of Layered Double Hydroxides Intercalated with Carboxylic Acids84Synthesis and anion exchange chemistry of new intercalation hosts containing lanthanide cations, Ln2(OH)5(NO3)·xH2O (Ln=Y, Gd–Lu)63Facile Synthesis and Catalytic Properties of Nickel-Based Mixed-Metal Oxides with Mesopore Networks from a Novel Hybrid Composite Precursor85Ln 2 (OH) 5 NO 3 · x H 2 O (Ln = Y, Gd−Lu): A Novel Family of Anion Exchange Intercalation Hosts215Three Dimensionally Ordered Macroporous Layered Double Hydroxides: Preparation by Templated Impregnation/Coprecipitation and Pattern Stability upon Calcination100Preparation of Ni2+−Fe3+ Layered Double Hydroxide Material with High Crystallinity and Well-Defined Hexagonal Shapes133Heterogeneous ultrathin films fabricated by alternate assembly of exfoliated layered double hydroxides and polyanion111Preparation and photophysical characterisation of Zn–Al layered double hydroxides intercalated by anionic pyrene derivatives71Direct Control of Drug Release Behavior from Layered Double Hydroxides through Particle Interactions81Corrosion Resistance of Superhydrophobic Layered Double Hydroxide Films on Aluminum527Corrosion Resistance of Superhydrophobic Layered Double Hydroxide Films on Aluminum73Fabrication of oriented layered double hydroxide films by spin coating and their use in corrosion protection139In situ growth of layered double hydroxide films on anodic aluminum oxide/aluminum and its catalytic feature in aldol condensation of acetone92Electrochemical Synthesis of Zn−Al Layered Double Hydroxide (LDH) Films122Multiple Effects of Dodecanesulfonate in the Crystal Growth Control and Morphosynthesis of Layered Double Hydroxides68Release studies of different NSAIDs encapsulated in Mg,Al,Fe-hydrotalcites90Theoretical study of the hexahydrated metal cations for the understanding of their template effects in the construction of layered double hydroxides74Intercalation of l -Dopa into Layered Double Hydroxides: Enhancement of Both Chemical and Stereochemical Stabilities of a Drug through Host−Guest Interactions120Role of Host Layer Flexibility in DNA Guest Intercalation Revealed by Computer Simulation of Layered Nanomaterials63Layered Double Hydroxides as Catalytic Materials: Recent Development167Synthesis and Crystal Structures of New Lanthanide Hydroxyhalide Anion Exchange Materials, Ln2(OH)5X·1.5H2O (X = Cl, Br; Ln = Y, Dy, Er, Yb)138Molecular models and simulations of layered materials284Alkyl sulfonate modified LDH: Effect of alkyl chain length on intercalation behavior, particle morphology and thermal stability68Precipitation synthesis of lanthanide hydroxynitrate anion exchange materials, Ln2(OH)5NO3·H2O (Ln=Y, Eu–Er)72Highly Efficient and Rapid Cs+ Uptake by the Layered Metal Sulfide K2xMnxSn3−xS6 (KMS-1)260One-Step Hydrothermal Crystallization of a Layered Double Hydroxide/Alumina Bilayer Film on Aluminum and Its Corrosion Resistance Properties191Polymer nanocomposites using zinc aluminum and magnesium aluminum oleate layered double hydroxides: Effects of LDH divalent metals on dispersion, thermal, mechanical and fire performance in various polymers139Layered double hydroxide nanoparticles in gene and drug delivery284Facile preparation of pure CaAl-layered double hydroxides and their application as a hardening accelerator in concrete126Facile synthesis and novel electrocatalytic performance of nanostructured Ni–Al layered double hydroxide/carbon nanotube composites162Hierarchical films of layered double hydroxides by using a sol–gel process and their high adaptability in water treatment133Layered double hydroxide films: synthesis, properties and applications461Morphology and thermal degradation behavior of highly exfoliated CoAl-layered double hydroxide/polycaprolactone nanocomposites prepared by simple solution intercalation84Facile Sodium Alginate Assisted Assembly of Ni−Al Layered Double Hydroxide Nanostructures68Erasable Nanoporous Antireflection Coatings Based on the Reconstruction Effect of Layered Double Hydroxides96Layer-by-Layer Ultrathin Films of Azobenzene-Containing Polymer/Layered Double Hydroxides with Reversible Photoresponsive Behavior88Antioxidant drugs intercalated into layered double hydroxide: Structure and in vitro release108The Effect of Trivalent Cations on the Performance of Mg‐M‐CO3 Layered Double Hydroxides for High‐Temperature CO2 Capture167Intercalation and release of antiinflammatory drug diclofenac into nanosized ZnAl hydrotalcite-like compound103Thermal decomposition, gas phase hydration and liquid phase reconstruction in the system Mg/Al hydrotalcite/mixed oxide: A comparative study95Optical pH Sensor with Rapid Response Based on a Fluorescein‐Intercalated Layered Double Hydroxide123CO2 capture by solid adsorbents and their applications: current status and new trends1609A novel approach towards solvent-free epoxidation of cyclohexene by Ti(IV)–Schiff base complex-intercalated LDH using H2O2 as oxidant78Fabrication and photocatalytic performance of a Zn Cd1−S solid solution prepared by sulfuration of a single layered double hydroxide precursor168Morphologies, Preparations and Applications of Layered Double Hydroxide Micro-/Nanostructures155Facile synthesis of NiAl-layered double hydroxide/graphene hybrid with enhanced electrochemical properties for detection of dopamine135Intercalation and grafting of benzene derivatives into zinc–aluminum and copper–chromium layered double hydroxide hosts: an XPS monitoring study92Self-assembly of layered double hydroxide nanosheets/Au nanoparticles ultrathin films for enzyme-free electrocatalysis of glucose102Synergistic catalysis by polyoxometalate-intercalated layered double hydroxides: oximation of aromatic aldehydes with large enhancement of selectivity77In situ growth of Mg–Al hydrotalcite conversion film on AZ31 magnesium alloy172A Family of Visible‐Light Responsive Photocatalysts Obtained by Dispersing CrO6 Octahedra into a Hydrotalcite Matrix107Synthesis of Highly Luminescent and Anion‐Exchangeable Cerium‐Doped Layered Yttrium Hydroxides for Sensing and Photofunctional Applications77Improvement of photocatalytic activity of TiO2 nanoparticles on selectively reconstructed layered double hydroxide96Adsorption of Methyl Orange from Aqueous Solution on Hydrothermal Synthesized Mg–Al Layered Double Hydroxide283Well-dispersed bi-component-active CoO/CoFe 2 O 4 nanocomposites with tunable performances as anode materials for lithium-ion batteries142Thermal, optical and dielectric properties of Zn–Al layered double hydroxide110Transformation Mechanism of Magnesium and Aluminum Precursor Solution into Crystallites of Layered Double Hydroxide140High pseudocapacitive cobalt carbonate hydroxide films derived from CoAl layered double hydroxides159Synthesis of graphene nanosheets with good control over the number of layers within the two-dimensional galleries of layered double hydroxides67Layered double hydroxides used as flame retardant for engineering plastic acrylonitrile–butadiene–styrene (ABS)97Modeling drug release from a layered double hydroxide–ibuprofen complex93Novel mesoporous Zn Cd1−S nanoparticles as highly efficient photocatalysts65Temperature-Controlled Electrochemical Switch Based on Layered Double Hydroxide/Poly(N-Isopropylacrylamide) Ultrathin Films Fabricated via Layer-by-Layer Assembly68Study of the in situ growth mechanism of Mg–Al hydrotalcite conversion film on AZ31 magnesium alloy164Study of the corrosion mechanism of the in situ grown Mg–Al–CO32− hydrotalcite film on AZ31 alloy102Highly Dispersed TiO6 Units in a Layered Double Hydroxide for Water Splitting150Facile fabrication of MWCNT-doped NiCoAl-layered double hydroxide nanosheets with enhanced electrochemical performances223A high performance oxygen storage material for chemical looping processes with CO 2 capture130Electrodepositing Ag nanodendrites on layered double hydroxides modified glassy carbon electrode: Novel hierarchical structure for hydrogen peroxide detection64Binary Cu–Co catalysts derived from hydrotalcites with excellent activity and recyclability towards NH3BH3 dehydrogenation66Catalytic conversion of syngas to mixed alcohols over CuFe-based catalysts derived from layered double hydroxides118Comprehensive investigation of CO2 adsorption on Mg–Al–CO3 LDH-derived mixed metal oxides210Layered double hydroxide (LDH)-based monolith with interconnected hierarchical channels: enhanced sorption affinity for anionic species67Layered double hydroxide-based catalysts: nanostructure design and catalytic performance333Effect of competing ligands on the sorption/desorption of arsenite on/from Mg–Fe layered double hydroxides (Mg–Fe-LDH)64Solvothermal One-Step Synthesis of Ni–Al Layered Double Hydroxide/Carbon Nanotube/Reduced Graphene Oxide Sheet Ternary Nanocomposite with Ultrahigh Capacitance for Supercapacitors272Polymer–inorganic supramolecular nanohybrids for red, white, green, and blue applications115Magnetic nanomaterial derived from graphene oxide/layered double hydroxide hybrid for efficient removal of methyl orange from aqueous solution147Transparent, Flexible Films Based on Layered Double Hydroxide/Cellulose Acetate with Excellent Oxygen Barrier Property127Ni–In Intermetallic Nanocrystals as Efficient Catalysts toward Unsaturated Aldehydes Hydrogenation149Visible-Light-Responsive Photocatalysts toward Water Oxidation Based on NiTi-Layered Double Hydroxide/Reduced Graphene Oxide Composite Materials165Nanohybrids from NiCoAl-LDH coupled with carbon for pseudocapacitors: understanding the role of nano-structured carbon202Supported nickel–iron nanocomposites as a bifunctional catalyst towards hydrogen generation from N2H4·H2O91In situ formation of LDH membranes of different microstructures with molecular sieve gas selectivity84Reactivity and applications of layered silicates and layered double hydroxides116Recent advances in solid sorbents for CO 2 capture and new development trends1168Recent advances in synthesis and applications of clay-based photocatalysts: a review193Nickel–Gallium Intermetallic Nanocrystal Catalysts in the Semihydrogenation of Phenylacetylene110Methotrexate intercalated layered double hydroxides with different particle sizes: Structural study and Controlled release properties69High‐Yield Preparation, Versatile Structural Modification, and Properties of Layered Cobalt Hydroxide Nanocones81pH sensitive nanocomposite hydrogel beads based on carboxymethyl cellulose/layered double hydroxide as drug delivery systems163Cr(VI) removal from aqueous solutions by hydrothermal synthetic layered double hydroxides: Adsorption performance, coexisting anions and regeneration studies154Layered Double Hydroxide-Based Nanocarriers for Drug Delivery249Electrochemical deposition and characterization of Zn-Al layered double hydroxides (LDHs) films on magnesium alloy111Recent advances for layered double hydroxides (LDHs) materials as catalysts applied in green aqueous media102Layered Double Hydroxide‐based Nanomaterials as Highly Efficient Catalysts and Adsorbents451Reverse Micelle Synthesis of Colloidal Nickel–Manganese Layered Double Hydroxide Nanosheets and Their Pseudocapacitive Properties79Core–shell Cu@(CuCo-alloy)/Al 2 O 3 catalysts for the synthesis of higher alcohols from syngas123Magnesium-based systems for carbon dioxide capture, storage and recycling: from leaves to synthetic nanostructured materials70One-step synthesis of zinc–cobalt layered double hydroxide (Zn–Co-LDH) nanosheets for high-efficiency oxygen evolution reaction222Remarkably Enhanced Gas Separation by Partial Self‐Conversion of a Laminated Membrane to Metal–Organic Frameworks151TiO 2 @Layered Double Hydroxide Core–Shell Nanospheres with Largely Enhanced Photocatalytic Activity Toward O 2 Generation263Trinary Layered Double Hydroxides as High‐Performance Bifunctional Materials for Oxygen Electrocatalysis387Corrosion of in-situ grown MgAl-LDH coating on aluminum alloy79New High- and Low-Temperature Phase Changes of ZIF-7: Elucidation and Prediction of the Thermodynamics of Transitions88Recent Progress in Cobalt‐Based Heterogeneous Catalysts for Electrochemical Water Splitting2443Layered Double Hydroxide Nanostructured Photocatalysts for Renewable Energy Production484Fabrication and Characterization of PO43−Intercalated Zn-Al- Layered Double Hydroxide Nanocontainer90In situ growth of ZIF-8 nanocrystals on layered double hydroxide nanosheets for enhanced CO 2 capture74Recent Advances in the Synthesis of Layered, Double‐Hydroxide‐Based Materials and Their Applications in Hydrogen and Oxygen Evolution117Influence of surface chemistry on the formation of crystalline hydroxide coatings on Mg alloys in liquid water and steam systems67Superior capability of MgAl2O4 for selenite removal from contaminated groundwater during its reconstruction of layered double hydroxides68Catalytic application of layered double hydroxide-derived catalysts for the conversion of biomass-derived molecules225Ordered assembly of hybrid room-temperature phosphorescence thin films showing polarized emission and the sensing of VOCs122Thermal decomposition and recovery properties of ZnAl–CO 3 layered double hydroxide for anionic dye adsorption: insight into the aggregative nucleation and growth mechanism of the LDH memory effect.143Phosphorus oxoanion-intercalated layered double hydroxides for high-performance oxygen evolution204Efficient removal of nitrobenzene by Fenton-like process with Co-Fe layered double hydroxide114Synthesis of hierarchical flower-like Mg2Al-Cl layered double hydroxide in a surfactant-free reverse microemulsion64A review of hydrotalcite based catalysts for hydrogen production systems201Wearable Fabrics with Self-Branched Bimetallic Layered Double Hydroxide Coaxial Nanostructures for Hybrid Supercapacitors308Tuning Electronic Structure of NiFe Layered Double Hydroxides with Vanadium Doping toward High Efficient Electrocatalytic Water Oxidation757Highly Efficient Separation of Magnesium and Lithium and High-Valued Utilization of Magnesium from Salt Lake Brine by a Reaction-Coupled Separation Technology82Functionalized layered double hydroxide with nitrogen and sulfur co-decorated carbondots for highly selective and efficient removal of soft Hg2+ and Ag+ ions95Enhancing DeNOx performance of CoMnAl mixed metal oxides in low-temperature NH3-SCR by optimizing layered double hydroxides (LDHs) precursor template105Electrochemiluminescence Resonance Energy Transfer System for Dual-Wavelength Ratiometric miRNA Detection117Design of high-performance heterogeneous catalysts using hydrotalcite for selective organic transformations79Nanocontainer-based self-healing coatings: current progress and future perspectives139Effect of Synthesis Conditions on the Controlled Growth of MgAl–LDH Corrosion Resistance Film: Structure and Corrosion Resistance Properties79Enhancement corrosion resistance of Mg Al layered double hydroxides films by anion-exchange mechanism on magnesium alloys99Separation and Remediation of 99TcO4– from Aqueous Solutions165Recent progress in preparation and agricultural application of microcapsules68Enlarged Interlayer Spacing in Cobalt–Manganese Layered Double Hydroxide Guiding Transformation to Layered Structure for High Supercapacitance131Why Do Carbonate Anions Have Extremely High Stability in the Interlayer Space of Layered Double Hydroxides? Case Study of Layered Double Hydroxide Consisting of Mg and Al (Mg/Al = 2)76Surface enhanced 3D rGO hybrids and porous rGO nano-networks as high performance supercapacitor electrodes for integrated energy storage devices76Effects of deformation processes on morphology, microstructure and corrosion resistance of LDHs films on magnesium alloy AZ3184Anion exchange behavior of M II Al layered double hydroxides: a molecular dynamics and DFT study103CO2 capturing, thermo-kinetic principles, synthesis and amine functionalization of covalent organic polymers for CO2 separation from natural gas: A review113Layered Double Hydroxide Protective Films Developed on Aluminum and Aluminum Alloys: Synthetic Methods and Anti-Corrosion Mechanisms68Recent advancement made in the field of reduced graphene oxide-based nanocomposites used in the energy storage devices: A review111Fundamentals, synthesis, characterization and environmental applications of layered double hydroxides: a review164Layered double hydroxide (LDH)-based materials: A mini-review on strategies to improve the performance for photocatalytic water splitting314Emerging two-dimensional nanostructured manganese-based materials for electrochemical energy storage: recent advances, mechanisms, challenges, and prospects105Advanced Two-Dimensional Materials for Green Hydrogen Generation: Strategies toward Corrosion Resistance Seawater Electrolysis─Review and Future Perspectives76A critical review on layered double hydroxide (LDH)-derived functional nanomaterials as potential and sustainable photocatalysts92Metal-organic frameworks-derived layered double hydroxides: From controllable synthesis to various electrochemical energy storage/conversion applications77A one-step regeneration method in-situ for deactivated aluminum-based lithium adsorbent used in high Mg2+/Li+ brines66

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  1. Towards Understanding, Control and Application of Layered Double Hydroxide Chemistry

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  2. Elaboration et caractérisation de matrices hydroxydes doubles lamellaires macroporeuses

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  4. Staging during anion-exchange intercalation into [LiAl2(OH)6]Cl·yH2O: structural and mechanistic insights

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  5. Influence of the Divalent Cation on the Thermal Activation and Reconstruction of Hydrotalcite-like Compounds

    The Journal of Physical Chemistry C · 2007-02-14

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  6. Selective Layer Reaction of Layer-by-Layer Assembled Layered Double-Hydroxide Nanocrystals

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  7. Catalysis by layered materials: A review

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  8. New Inorganic-Based Drug Delivery System of Indole-3-Acetic Acid-Layered Metal Hydroxide Nanohybrids with Controlled Release Rate

    Chemistry of Materials · 2007-04-20

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  9. Molecular Dynamics Simulation of the Energetics and Structure of Layered Double Hydroxides Intercalated with Carboxylic Acids

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  10. Preparation and wettability of Zn–Al layered double hydroxide film directly grown on highly porous anodic alumina oxide template

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  11. Influence of iron substitution on formation and structure of Cu-based mixed oxides derived from layered double hydroxides

    Journal of Physics and Chemistry of Solids · 2007-10-09

    L. H. Zhang, Xu Xiang, Lei Zhang, Fa‐tang Li, Jun Zhu, David G. Evans, Xinhui Duan

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  12. Stoichiometric synthesis of perovskite-like Ca2FexCo2−xO5 compounds from layered double hydroxide precursor

    Journal of Physics and Chemistry of Solids · 2007-12-01

    Zhouqing Gu, Xu Xiang, Fa‐tang Li, S.B. Liu, David G. Evans

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  13. Synthesis and anion exchange chemistry of new intercalation hosts containing lanthanide cations, Ln2(OH)5(NO3)·xH2O (Ln=Y, Gd–Lu)

    Journal of Physics and Chemistry of Solids · 2007-12-01

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  14. Facile Synthesis and Catalytic Properties of Nickel-Based Mixed-Metal Oxides with Mesopore Networks from a Novel Hybrid Composite Precursor

    Chemistry of Materials · 2007-12-05

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  15. Ln 2 (OH) 5 NO 3 · x H 2 O (Ln = Y, Gd−Lu): A Novel Family of Anion Exchange Intercalation Hosts

    Chemistry of Materials · 2007-12-05

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  16. Three Dimensionally Ordered Macroporous Layered Double Hydroxides: Preparation by Templated Impregnation/Coprecipitation and Pattern Stability upon Calcination

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  17. Preparation of Ni2+−Fe3+ Layered Double Hydroxide Material with High Crystallinity and Well-Defined Hexagonal Shapes

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  18. A kinetic study of the phase conversion of layered cobalt hydroxides

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  19. Heterogeneous ultrathin films fabricated by alternate assembly of exfoliated layered double hydroxides and polyanion

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  20. Preparation and photophysical characterisation of Zn–Al layered double hydroxides intercalated by anionic pyrene derivatives

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  22. Direct Control of Drug Release Behavior from Layered Double Hydroxides through Particle Interactions

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  23. Corrosion Resistance of Superhydrophobic Layered Double Hydroxide Films on Aluminum

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  24. Corrosion Resistance of Superhydrophobic Layered Double Hydroxide Films on Aluminum

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  25. Tailoring of Phase Composition and Photoresponsive Properties of Ti-Containing Nanocomposites from Layered Precursor

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  26. Fabrication of oriented layered double hydroxide films by spin coating and their use in corrosion protection

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  27. In situ growth of layered double hydroxide films on anodic aluminum oxide/aluminum and its catalytic feature in aldol condensation of acetone

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  29. Aluminium substitution in iron(II–III)-layered double hydroxides: Formation and cationic order

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  31. Electrochemical Synthesis of Zn−Al Layered Double Hydroxide (LDH) Films

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  32. Immobilization of anionic dyes by intercalation into hydrotalcite

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  33. Multiple Effects of Dodecanesulfonate in the Crystal Growth Control and Morphosynthesis of Layered Double Hydroxides

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  34. Release studies of different NSAIDs encapsulated in Mg,Al,Fe-hydrotalcites

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  35. Experimental investigation of sheet flexibility of layered double hydroxides: One-pot morphosynthesis of inorganic intercalates

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  36. Preparation of Layered Double Hydroxide Microspheres by Spray Drying

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    Yanchang Wang, Fazhi Zhang, Sailong Xu, Xiaoying Wang, David G. Evans, Xue Duan

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  37. One-step conversion of acetone to methyl isobutyl ketone over Pd-mixed oxide catalysts prepared from novel layered double hydroxides

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    Robert D. Hetterley, Richard Mackey, Jonathan A. Jones, Yaroslav Z. Khimyak, Andrew M. Fogg, I. V. Kozhevnikov

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  38. Theoretical study of the hexahydrated metal cations for the understanding of their template effects in the construction of layered double hydroxides

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  39. Facile Fabrication and Wettability of Nestlike Microstructure Maintained Mixed Metal Oxides Films from Layered Double Hydroxide Films Precursors

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  40. Intercalation of l -Dopa into Layered Double Hydroxides: Enhancement of Both Chemical and Stereochemical Stabilities of a Drug through Host−Guest Interactions

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    Min Wei, Min Pu, Jian Ting Guo, Jingbin Han, Feng Li, Jing He, David G. Evans, Xue Duan

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  41. Role of Host Layer Flexibility in DNA Guest Intercalation Revealed by Computer Simulation of Layered Nanomaterials

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  42. Investigation of Layered Double Hydroxides Intercalated by Oxomolybdenum Catecholate Complexes

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  43. Poly( L ‐lactide)/layered double hydroxides nanocomposites: Preparation and crystallization behavior

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  44. Nanostructured Materials Produced by Mixing and Restacking of Delaminated Layered Double Hydroxides

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    Rune E. Johnsen, Qinglan Wu, Anja Olafsen Sjåstad, Ørnulv B. Vistad, Frank Krumeich, Poul Norby

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  45. A comparativein situRietveld refinement study: thermal decomposition and transformation of CoAl and CoZnAl layered double hydroxides

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  46. Surface Selective Deposition of PMMA on Layered Double Hydroxide Nanocrystals Immobilized on Solid Substrates

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    Jong‐Hyeon Lee, Seog Woo Rhee, Hye Jin Nam, Duk‐Young Jung

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  47. Layered Double Hydroxides as Catalytic Materials: Recent Development

    Catalysis Surveys from Asia · 2008-11-14

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  48. Observation of Staging during Intercalation in Layered α-Cobalt Hydroxides: A Synthetic and Kinetic Study

    Inorganic Chemistry · 2008-11-14

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